arXiv subjects

F. M. Grosche

Publications and source records attributed to F. M. Grosche.

At least 19 recordsLinked to original sources

arXiv2025

Spin-density wave of ferrimagnetic building blocks masking the ferromagnetic quantum-critical point in NbFe2

In the metallic magnet NbFe2, the low temperature threshold of ferromagnetism can be investigated by varying the Fe concentration within a narrow homogeneity range. NbFe2 is one of a number of compounds where modulated order is found to mask the ferromagnetic quantum critical point. However, here we report the rare case where the masking modulated magnetic order has been fully refined. Spherical neutron polarimetry and high-intensity single-crystal neutron diffraction reveal the first case of a longitudinal spin-density wave masking the ferromagnetic quantum critical point. The spin-density wave is characterised by a large-wavelength incommensurate modulation of its low average moment. It is formed from ferrimagnetic building blocks with antiparallel ferromagnetic sheets. The existence of ferromagnetic sheets and cancellation of the magnetisation only over mesoscopic length scales show local similarity between the spin-density wave and the ferromagnetic parent phase and indicate the spin-density wave's unconventional nature as emerging from underlying ferromagnetic quantum criticality.

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arXiv2025

Strange metallicity encompasses high magnetic field-induced superconductivity in UTe2

A strange metallic state - characterized by an electrical resistivity that rises linearly in temperature $T$ at a rate governed by Planckian energetic dissipation - is present in a number of unconventional superconductors. Despite widespread investigative efforts, the microscopic properties of strange metallicity continue to defy elementary description. Here we investigate heavy fermion UTe$_2$, which hosts a suite of exotic spin-triplet superconducting phases, the most extreme of which resides in a narrow angular window of intense magnetic fields $>$ 40 T. Through angle-dependent magnetotransport measurements in pulsed magnetic fields, we find that this superconductive phase emerges from a strange metallic state with Planckian $T$-linear resistivity confined to a small region of phase space where the field-induced superconductivity is strongest, suggesting a shared underlying mechanism. These findings reveal a novel setting for strange metallicity - in contrast to the general case of singlet superconductivity emerging on the border of antiferromagnetism, here strange metallicity accompanies field-induced triplet superconductivity within a spin-polarized magnetic state. This result demonstrates the remarkable ubiquity of strange metallicity across diverse materials settings, and highlights UTe$_2$ as a unique platform for exploring the interplay between unconventional superconductivity and quantum criticality.

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arXiv2024

Pressure-enhanced $f$-electron orbital weighting in UTe2 mapped by quantum interferometry

The phase landscape of UTe$_2$ features a remarkable diversity of superconducting phases under applied pressure and magnetic field. Recent quantum oscillation studies at ambient pressure have revealed the quasi-2D Fermi surface of this material. However, the pressure-dependence of the Fermi surface remains an open question. Here we track the evolution of the UTe$_2$ Fermi surface as a function of pressure up to 19.5 kbar by measuring quantum interference oscillations. We find that in sufficient magnetic field to suppress both superconductivity at low pressures and incommensurate antiferromagnetism at higher pressures, the quasi-2D Fermi surface found at ambient pressure smoothly connects to that at 19.5 kbar, with no signs of a reconstruction over this pressure interval. We observe a smooth increase in oscillatory frequency with increasing pressure, indicating that the warping of the cylindrical Fermi sheets continuously increases with pressure. By computing a tight-binding model, we show that this enhanced warping indicates increased $f$-orbital contribution at the Fermi level - up to and beyond the critical pressure at which superconductivity is truncated. These findings highlight the value of high-pressure quantum interference measurements as a new probe of the electronic structure in heavy fermion materials.

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arXiv2024

A quantum critical line bounds the high field metamagnetic transition surface in UTe$_2$

Quantum critical phenomena are widely studied across various materials families, from high temperature superconductors to magnetic insulators. They occur when a thermodynamic phase transition is suppressed to zero temperature as a function of some tuning parameter such as pressure or magnetic field. This generally yields a point of instability - a so-called quantum critical point - at which the phase transition is driven exclusively by quantum fluctuations. Here we show that the heavy fermion metamagnet UTe$_2$ possesses a quantum phase transition at extreme magnetic field strengths of over 70 T. Rather than terminating at one singular point, we find that the phase boundary is sensitive to magnetic field components in each of the three Cartesian axes of magnetic field space. This results in the three-dimensional transition surface being bounded by a continuous ring of quantum critical points, the locus of which forms an extended line of quantum criticality - a novel form of quantum critical phase boundary. Within this quantum critical line sits a magnetic field-induced superconducting state in a toroidal shape, which persists to fields over 70~T. We model our data by a phenomenological free energy expansion, and show how a three-dimensional quantum critical phase boundary - rather than a more conventional singular point of instability - anchors the remarkable high magnetic field phase landscape of UTe$_2$.

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arXiv2023

Flat Bands at the Fermi Level in Unconventional Superconductor YFe2Ge2

We report heavy electron behavior in unconventional superconductor YFe$_2$Ge$_2$ ($T_C \,{=}\, 1.2$ K). We directly observe very heavy bands ($m_\mathrm{eff}\sim 25 m_e$) within $\sim$10 meV of the Fermi level $E_{F}$ using angle-resolved photoelectron spectroscopy (ARPES). The flat bands reside at the X points of the Brillouin zone and are composed principally of $d_{xz}$ and $d_{yz}$ orbitals. We utilize many-body perturbative theory, GW, to calculate the electronic structure of this material, obtaining excellent agreement with the ARPES data with relatively minor band renormalizations and band shifting required. We obtain further agreement at the Dynamical Mean Field Theory (DMFT) level, highlighting the emergence of the many-body physics at low energies (near $E_F$) and temperatures.

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arXiv2023

Quantum interference between quasi-2D Fermi surface sheets in UTe2

UTe$_2$ is a spin-triplet superconductor candidate for which high quality samples with long mean free paths have recently become available, enabling quantum oscillation measurements to probe its Fermi surface and effective carrier masses. It has recently been reported that UTe$_2$ possesses a 3D Fermi surface component [Phys. Rev. Lett. 131, 036501 (2023)]. The distinction between 2D and 3D Fermi surface sections in triplet superconductors can have important implications regarding the topological properties of the superconductivity. Here we report the observation of oscillatory components in the magnetoconductance of UTe$_2$ at high magnetic fields. We find that these oscillations are well described by quantum interference between quasiparticles traversing semiclassical trajectories spanning magnetic breakdown networks. Our observations are consistent with a quasi-2D model of this material's Fermi surface based on prior dHvA-effect measurements. Our results strongly indicate that UTe$_2$ -- which exhibits a multitude of complex physical phenomena -- possesses a remarkably simple Fermi surface consisting exclusively of two quasi-2D cylindrical sections.

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arXiv2023

Enhanced triplet superconductivity in next generation ultraclean UTe2

The unconventional superconductor UTe$_2$ exhibits numerous signatures of spin-triplet superconductivity -- a rare state of matter which could enable quantum computation protected against decoherence. UTe$_2$ possesses a complex phase landscape comprising two magnetic field-induced superconducting phases, a metamagnetic transition to a field-polarised state, along with pair- and charge-density wave orders. However, contradictory reports between studies performed on UTe$_2$ specimens of varying quality have severely impeded theoretical efforts to understand the microscopic origins of the exotic superconductivity. Here, we report a comprehensive suite of high magnetic field measurements on a new generation of pristine quality UTe$_2$ crystals. Our experiments reveal a significantly revised high magnetic field superconducting phase diagram in the ultraclean limit, showing a pronounced sensitivity of field-induced superconductivity to the presence of crystalline disorder. We employ a Ginzburg-Landau model that excellently captures this acute dependence on sample quality. Our results suggest that in close proximity to a field--induced metamagnetic transition the enhanced role of magnetic fluctuations -- that are strongly suppressed by disorder -- is likely responsible for tuning UTe$_2$ between two distinct spin-triplet superconducting phases.

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arXiv2023

Quasi-2D Fermi surface in the anomalous superconductor UTe2

The heavy fermion paramagnet UTe$_2$ exhibits numerous characteristics of spin-triplet superconductivity. Efforts to understand the microscopic details of this exotic superconductivity have been impeded by uncertainty regarding the underlying electronic structure. Here we directly probe the Fermi surface of UTe$_2$ by measuring magnetic quantum oscillations in pristine quality crystals. We find an angular profile of quantum oscillatory frequency and amplitude that is characteristic of a quasi-2D Fermi surface, which we find is well described by two cylindrical Fermi sheets of electron- and hole-type respectively. Additionally, we find that both cylindrical Fermi sheets possess considerable undulation but negligible small-scale corrugation, which may allow for their near-nesting and therefore promote magnetic fluctuations that enhance the triplet pairing mechanism. Importantly, we find no evidence for the presence of any 3D Fermi surface sections. Our results place strong constraints on the possible symmetry of the superconducting order parameter in UTe$_2$.

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arXiv2022

Muon spin rotation and relaxation study on Nb$_{1-y}$Fe$_{2+y}$

We present a detailed study of the magnetic properties of weakly ferromagnetic/quantum critical Nb$_{1-y}$Fe$_{2+y}$ using muon spin rotation and relaxation ($\mu$SR). By means of an angular dependent study of the muon spin rotation signal in applied magnetic fields on a single crystal in the paramagnetic state we establish the muon stopping site in the crystallographic lattice of NbFe$_2$. With this knowledge we develop models to describe the muon spin rotation and relaxation signals in the weakly ferromagnetic, spin density wave and quantum critical phases of Nb$_{1-y}$Fe$_{2+y}$ and fit the corresponding experimental data. In particular, we quantify the $\mu$SR response for quantum critical behavior in Nb$_{1.0117}$Fe$_{1.9883}$ and extract the influence of residual weak structural disorder. From our analysis, Nb$_{1-y}$Fe$_{2+y}$ emerges to be uniquely suited to study quantum criticality close to weak itinerant ferromagnetic order.

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arXiv2018

Evidence of a structural quantum critical point in (Ca$_{x}$Sr$_{1-x}$)$_3$Rh$_4$Sn$_{13}$ from a lattice dynamics study

Approaching a quantum critical point (QCP) has been an effective route to stabilize superconductivity. While the role of magnetic QCPs has been extensively discussed, similar exploration of a structural QCP is scarce due to the lack of suitable systems with a continuous structural transition that can be conveniently tuned to 0~K. Using inelastic X-ray scattering, we examine the phonon spectrum of the nonmagnetic quasi-skutterudite (Ca$_{x}$Sr$_{1-x}$)$_3$Rh$_4$Sn$_{13}$, which represents a precious system to explore the interplay between structural instabilities and superconductivity by tuning the Ca concentration $x$. We unambiguously detect the softening of phonon modes around the M point on cooling towards the structural transition. Intriguingly, at $x=0.85$, the soft mode energy squared at the M point extrapolates to zero at $(-5.7 \pm 7.7)$~K, providing the first compelling microscopic evidence of a structural QCP in (Ca$_{x}$Sr$_{1-x}$)$_3$Rh$_4$Sn$_{13}$. The enhanced phonon density-of-states at low energy provides the essential ingredient for realizing strong-coupling superconductivity near the structural QCP.

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arXiv2017

Ultra-small moment incommensurate spin density wave order masking a ferromagnetic quantum critical point in NbFe$_2$

In the metallic magnet Nb$_{1-y}$Fe$_{2+y}$, the low temperature threshold of ferromagnetism can be investigated by varying the Fe excess $y$ within a narrow homogeneity range. We use elastic neutron scattering to track the evolution of magnetic order from Fe-rich, ferromagnetic Nb$_{0.981}$Fe$_{2.019}$ to approximately stoichiometric NbFe$_2$, in which we can, for the first time, characterise a long-wavelength spin density wave state burying a ferromagnetic quantum critical point. The associated ordering wavevector $\mathbf{q}_{\rm SDW}=$(0,0,$l_{\rm SDW}$) is found to depend significantly on $y$ and $T$, staying finite but decreasing as the ferromagnetic state is approached. The phase diagram follows a two order-parameter Landau theory, for which all the coefficients can now be determined. Our findings suggest that the emergence of SDW order cannot be attributed to band structure effects alone. They indicate a common microscopic origin of both types of magnetic order and provide strong constraints on related theoretical scenarios based on, e.g., quantum order by disorder.

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arXiv2015

Metallic Quantum Ferromagnets

This review gives an overview of the quantum phase transition (QPT) problem in metallic ferromagnets, discussing both experimental and theoretical aspects. These QPTs can be classified with respect to the presence and strength of quenched disorder: Clean systems generically show a discontinuous, or first-order, QPT from the ferromagnetic state to a paramagnetic one as a function of some control parameter, as predicted by theory. Disordered systems are much more complicated, depending on the disorder strength and the distance from the QPT. In many disordered materials the QPT is continuous, or second order, and Griffiths-phase effects coexist with QPT singularities near the transition. In other systems the transition from the ferromagnetic state at low temperatures is to a different type of long-range order, such as an antiferromagnetic or a spin-density-wave state. In still other materials a transition to a state with glass-like spin dynamics is suspected. The review provides a comprehensive discussion of the current understanding of these various transitions, and of the relation between experimental and theoretical developments.

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arXiv2015

Large Fermi Surface of Heavy Electrons at the Border of Mott Insulating State in NiS2

One of the early triumphs of quantum physics is the explanation why some materials are metallic whereas others are insulating. While a treatment based on single electron states correctly predicts the character of most materials this approach can fail spectacularly, when the electrostatic repulsion between electrons causes strong correlations. Not only can these favor new and subtle forms of order in metals, such as magnetism or superconductivity, they can even cause the electrons in a half-filled energy band to lock into position altogether, producing a correlated, or Mott insulator. Arguably the most extreme manifestation of electronic correlations in dense electronic matter, the transition into the Mott insulating state raises a number of fundamental questions. Foremost among these is the fate of the electronic Fermi surface and the associated charge carrier mass, as the Mott transition is approached at low temperature, which have been particularly controversial in the high temperature superconducting cuprates. We report the first direct observation of the Fermi surface on the metallic side of a Mott insulating transition by high pressure quantum oscillatory measurements in NiS2. Our results point at a large Fermi surface consistent with Luttinger's theorem and a strongly enhanced carrier effective mass, suggesting that electron localization occurs via a diverging effective mass and concomitant slowing down of charge carriers as predicted theoretically.

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arXiv2015

Ambient Pressure Structural Quantum Critical Point in the Phase Diagram of (Ca$_x$Sr$_{1-x}$)$_3$Rh$_4$Sn$_{13}$

The quasi-skutterudite superconductor Sr$_3$Rh$_4$Sn$_{13}$ features a pronounced anomaly in electrical resistivity at $T^*\sim$138 K. We show that the anomaly is caused by a second-order structural transition, which can be tuned to 0 K by applying physical pressure and chemical pressure via the substitution of Ca for Sr. A broad superconducting dome is centred around the structural quantum critical point. Detailed analysis of the tuning parameter dependence of $T^*$ as well as insights from lattice dynamics calculations strongly support the existence of a structural quantum critical point at ambient pressure when the fraction of Ca is 0.9 (i.e., $x_c=0.9$). This establishes (Ca$_x$Sr$_{1-x}$)$_3$Rh$_4$Sn$_{13}$ series as an important system for exploring the physics of structural quantum criticality without the need of applying high pressures.

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arXiv2014

Anomalous Pressure Dependence of the Superconducting Transition Temperature in TlNi$_2$Se$_{2-x}$S$_x$

We report the pressure dependence of the superconducting transition temperature, $T_c$, in TlNi$_2$Se$_{2-x}$S$_x$ detected via the AC susceptibility method. The pressure-temperature phase diagram constructed for TlNi$_{2}$Se$_{2}$, TlNi$_{2}$S$_{2}$ and TlNi$_{2}$SeS exhibits two unexpected features: (a) a sudden collapse of the superconducting state at moderate pressure for all three compositions and (b) a dome-shaped pressure dependence of $T_c$ for TlNi$_{2}$SeS. These results point to the nontrivial role of S substitution and its subtle interplay with applied pressure, as well as novel superconducting properties of the TlNi$_2$Se$_{2-x}$S$_x$ system.

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arXiv2014

Fermi liquid breakdown and evidence for superconductivity in YFe$_2$Ge$_2$

In the d-electron system YFe$_2$Ge$_2$, an unusually high and temperature dependent Sommerfeld ratio of the specific heat capacity $C/T \sim 100~\mathrm{mJ/(molK^2)}$ and an anomalous power law temperature dependence of the electrical resistivity $ρ\simeq ρ_0 + AT^{3/2}$ signal Fermi liquid breakdown, probably connected to a close-by quantum critical point. Full resistive transitions, accompanied by DC diamagnetic screening fractions of up to 80\% suggest that pure samples of YFe$_2$Ge$_2$ superconduct below $1.8~\mathrm{K}$.

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arXiv2013

Separation of antiferromagnetism and high-temperature superconductivity in Ca$_{1-x}$La$_x$Fe$_2$As$_2$ under pressure

We report the effect of applied pressures on magnetic and superconducting order in single crystals of the aliovalent La-doped iron pnictide material Ca$_{1-x}$La$_{x}$Fe$_{2}$As$_{2}$. Using electrical transport, elastic neutron scattering and resonant tunnel diode oscillator measurements on samples under both quasi-hydrostatic and hydrostatic pressure conditions, we report a series of phase diagrams spanning the range of substitution concentrations for both antiferromagnetic and superconducting ground states that include pressure-tuning through the antiferromagnetic (AFM) quantum critical point. Our results indicate that the observed superconducting phase with maximum transition temperature of $T_{c}$=47 K is intrinsic to these materials, appearing only upon suppression of magnetic order by pressure tuning through the AFM critical point. In contrast to all other intermetallic iron-pnictide superconductors with the ThCr$_2$Si$_2$ structure, this superconducting phase appears to exist only exclusively from the antiferromagnetic phase in a manner similar to the oxygen- and fluorine-based iron-pnictide superconductors with the highest transition temperatures reported to date. The unusual dichotomy between lower-$T_{c}$ systems with coexistent superconductivity and magnetism and the tendency for the highest-$T_{c}$ systems to show non-coexistence provides an important insight into the distinct transition temperature limits in different members of the iron-based superconductor family.

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arXiv2011

Shubnikov-de Haas measurements on LuRh2Si2

We present Shubnikov-de Haas measurements on LuRh2Si2, the non-magnetic reference compound to the prototypical heavy-fermion system YbRh2Si2. We find an extensive set of orbits with clear angular dependences. Surprisingly, the agreement with non-correlated band structure calculations is limited. This may be related to an uncertainty in the calculations arising from a lack of knowledge about the exact Si atom position in the unit cell. The data on LuRh2Si2 provide an extensive basis for the interpretation of measurements on YbRh2Si2 indicative of discrepancies between the high-field Fermi surface of YbRh2Si2 and the "small" Fermi surface configuration.

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