arXiv subjects

F. M. Grosche

Publications and source records attributed to F. M. Grosche.

26 records · Page 2Linked to original sources

arXiv2011

Transport and Thermodynamic Evidence for a Marginal Fermi Liquid State in ZrZn$_2$

Measurements of low temperature transport and thermodynamic properties have been used to characterize the non-Fermi liquid state of the itinerant ferromagnet ZrZn$_2$. We observe a $T^{5/3}$ temperature dependence of the electrical resistivity at zero field, which becomes $T^2$ like in an applied field of 9 T. In zero field we also measured the thermal conductivity, and we see a novel linear in $T$ dependence of the difference between the thermal and electrical resistivities. Heat capacity measurements, also at zero field, reveal an upturn in the electronic contribution at low temperatures when the phonon term is subtracted. Taken together, we argue that these properties are consistent with a marginal Fermi liquid state which is predicted by a mean-field model of enhanced spin fluctuations on the border of ferromagnetism in three dimensions. We compare our data to quantitative predictions and establish this model as a compelling theoretical framework for understanding ZrZn$_2$.

cond-mat.str-el↗

arXiv2011

Enhancement of the Superconducting Transition Temperature under Pressure in Rare-Earth Doped Ca$_{1-x}$La$_x$Fe$_2$As$_2$ (x=0.27)

We report measurements of the pressure dependence of the superconducting transition temperature T_c in single crystal samples of the rare-earth doped superconductor Ca$_{0.73}$La$_{0.27}$Fe$_2$As$_2$. We track T_c with two techniques, via in-plane resistivity measurements and with a resonant tunnel diode oscillator circuit which is sensitive to the skin depth. We show that initially T_c rises steeply with pressure, forming a superconducting dome with a maximum T_c of ~44 K at 20 kbar. We discuss this observation in the context of other electron-doped iron pnictide superconductors, and conclude that the application of pressure offers an independent way to tune T_c in this system.

cond-mat.supr-con↗

arXiv2010

Doping driven magnetic instabilities and quantum criticality of NbFe$_{2}$

Using density functional theory we investigate the evolution of the magnetic ground state of NbFe$_{2}$ due to doping by Nb-excess and Fe-excess. We find that non-rigid-band effects, due to the contribution of Fe-\textit{d} states to the density of states at the Fermi level are crucial to the evolution of the magnetic phase diagram. Furthermore, the influence of disorder is important to the development of ferromagnetism upon Nb doping. These findings give a framework in which to understand the evolution of the magnetic ground state in the temperature-doping phase diagram. We investigate the magnetic instabilities in NbFe$_{2}$. We find that explicit calculation of the Lindhard function, $χ_{0}(\mathbf{q})$, indicates that the primary instability is to finite $\mathbf{q}$ antiferromagnetism driven by Fermi surface nesting. Total energy calculations indicate that $\mathbf{q}=0$ antiferromagnetism is the ground state. We discuss the influence of competing $\mathbf{q}=0$ and finite $\mathbf{q}$ instabilities on the presence of the non-Fermi liquid behavior in this material.

cond-mat.str-el↗

arXiv2009

High pressure study of BaFe2As2 - role of hydrostaticity and uniaxial stress

We investigate the evolution of the electrical resistivity of BaFe2As2 single crystals with pressure. The samples used were from the same batch grown from self flux and showed properties that were highly reproducible. Samples were pressurised using three different pressure media: pentane-isopentane (in a piston cylinder cell), Daphne oil (in an alumina anvil cell) and steatite (in a Bridgman cell). Each pressure medium has its own intrinsic level of hydrostaticity, which dramatically affects the phase diagram. An increasing uniaxial pressure component in this system quickly reduces spin density wave order and favours the appearance of superconductivity, similar to what is seen in SrFe2As2.

cond-mat.supr-con↗

arXiv2009

Magnetism in Nb(1-y)Fe(2+y) - composition and magnetic field dependence

We present a systematic study of transport and thermodynamic properties of the Laves phase system Nb$_{1-y}$Fe$_{2+y}$. Our measurements confirm that Fe-rich samples, as well as those rich in Nb (for $\mid y\mid\geq 0.02$), show bulk ferromagnetism at low temperature. For stoichiometric NbFe$_2$, on the other hand, magnetization, magnetic susceptibility and magnetoresistance results point towards spin-density wave (SDW) order, possibly helical, with a small ordering wavevector $Q \sim 0.05$ Å$^{-1}$. Our results suggest that on approaching the stoichiometric composition from the iron-rich side, ferromagnetism changes into long-wavelength SDW order. In this scenario, $Q$ changes continuously from 0 to small, finite values at a Lifshitz point in the phase diagram, which is located near $y=+0.02$. Further reducing the Fe content suppresses the SDW transition temperature, which extrapolates to zero at $y\approx -0.015$. Around this Fe content magnetic fluctuations dominate the temperature dependence of the resistivity and of the heat capacity which deviate from their conventional Fermi liquid forms, inferring the presence of a quantum critical point. Because the critical point is located between the SDW phase associated with stoichiometric NbFe$_2$ and the ferromagnetic order which reemerges for very Nb-rich NbFe$_2$, the observed temperature dependences could be attributed both to proximity to SDW order or to ferromagnetism.

cond-mat.str-el↗

arXiv2005

Non-Fermi liquid states in the pressurized $CeCu_2(Si_{1-x}Ge_x)_2$ system: two critical points

In the archetypal strongly correlated electron superconductor CeCu$_2$Si$_2$ and its Ge-substituted alloys CeCu$_2$(Si$_{1-x}$Ge$_{x}$)$_2$ two quantum phase transitions -- one magnetic and one of so far unknown origin -- can be crossed as a function of pressure \cite{Yuan 2003a}. We examine the associated anomalous normal state by detailed measurements of the low temperature resistivity ($ρ$) power law exponent $α$. At the lower critical point (at $p_{c1}$, $1\leqα\leq 1.5$) $α$ depends strongly on Ge concentration $x$ and thereby on disorder level, consistent with a Hlubina-Rice-Rosch scenario of critical scattering off antiferromagnetic fluctuations. By contrast, $α$ is independent of $x$ at the upper quantum phase transition (at $p_{c2}$, $α\simeq 1$), suggesting critical scattering from local or Q=0 modes, in agreement with a density/valence fluctuation approach.

cond-mat.str-el↗

arXiv2000

Superconductivity on the threshold of magnetism in CePd2Si2 and CeIn3

The magnetic ordering temperature of some rare earth based heavy fermion compounds is strongly pressure-dependent and can be completely suppressed at a critical pressure, p$_c$, making way for novel correlated electron states close to this quantum critical point. We have studied the clean heavy fermion antiferromagnets CePd$_2$Si$_2$ and CeIn$_3$ in a series of resistivity measurements at high pressures up to 3.2 GPa and down to temperatures in the mK region. In both materials, superconductivity appears in a small window of a few tenths of a GPa on either side of p$_c$. We present detailed measurements of the superconducting and magnetic temperature-pressure phase diagram, which indicate that superconductivity in these materials is enhanced, rather than suppressed, by the closeness to magnetic order.

cond-mat.str-el↗

arXiv1998

Anomalous Low Temperature States in CeNi2Ge2

Ambient pressure studies on high purity single crystals of the stoichiometric 4f-electron metal CeNi2Ge2 reveal anomalous low temperature forms of the resistivity which challenge our understanding of the metallic state. Comparisons are made with the isostructural and isoelectronic compound CePd2Si2 near the border of magnetism at high pressure, and possible reasons for this novel non-Fermi liquid form of the resistivity are discussed. Phase diagrams of further anomalies are presented, which involve a loss of resistance at low temperature in some samples of CeNi2Ge2 and unexpected high pressure phases.

cond-mat.str-el↗