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F. Sebastian Bergeret

Publications and source records attributed to F. Sebastian Bergeret.

At least 19 recordsLinked to original sources

Stabilization of Interband Phase Solitons in Two-Band Noncentrosymmetric Superconducting Rings

Two-band superconductors maintain a relative interband phase which can carry winding soliton excitations in a superconducting ring, supported by independent winding numbers in the two bands. In rings of superconductors obeying the inversion symmetry the interband phase solitons are metastable states, separated from the uniform ground state by the energy of screening currents. In this work we find that, breaking the inversion symmetry strongly enough, one can make the soliton a true ground state. In that case, a magneto-electric coupling, absent in centrosymmetric materials, contributes critically above a certain threshold, a relevant, free-energy term, odd with respect to the winding number, which biases the energy balance in favor of a particular winding sign. Once the bias outweighs the energy cost that originally made the soliton metastable, a phase soliton with a finite winding number becomes the ground state, with chirality set by the applied field. In current--flux measurements performed in equilibrium states, the effect is demonstrated by field-odd soliton branches, that replace the metastable ones existing in mesoscopic rings, built by two-component superconductors, realizing a magneto-electric analog of the Little--Parks fluxoid-branch physics in the interband relative-phase sector.

cond-mat.supr-con

Direct demonstration of time-reversal-symmetry-breaking spin injection from a compensated magnet

The injection, propagation and detection of spin currents are essential physical processes in spintronics. So far, the separation of charge and spin currents was facilitated by the electrical spin injection from a ferromagnet (FM) or the injection by a relativistic spin Hall effect. The devices employed are lateral spin valves comprising spatially separated injection and detection electrodes, connected by a spin-propagation channel. The time-reversal symmetry (TRS) breaking FM spin injection is realized in a geometry with an electrical bias applied between the injection electrode and the channel and is modelled by a conserved spin-polarized drift current. In contrast, the spin injection by the T-symmetric relativistic spin Hall mechanism is driven by an electrical bias applied across the injection electrode alone, and is modelled by a non-conserved spin current transverse to the applied bias. In this work, we use a lateral spin valve with a Mn5Si3 injection electrode to directly demonstrate a TRS-breaking spin injection from a compensated magnet with a vanishing net magnetization. Specifically, the TRS-breaking is demonstrated by the fact that switching between time-reversed states of the compensated magnet changes the detected spin signal. Moreover, the TRS-breaking nature of the spin injection is observed in both experimental geometries with the different electrical biasing, while using the same detection electrode. We show that this unconventional spin-injection is consistent with different magnitudes and propagation angles of electrical currents in the spin-up and spin-down channel in a d-wave altermagnet. Here our symmetry analysis and first-principles calculations are based on the compensated collinear altermagnetic order which has provided a comprehensive microscopic interpretation of earlier structural, magnetic, and anomalous Hall and Nernst measurements in Mn5Si3 thin films.

cond-mat.mes-hall

Fluxoid solitons in superconducting tapered tubes and bottlenecks

A thin-walled tubular superconductor develops a quantized fluxoid in the presence of an axial magnetic field. The fluxoid corresponds to the number of phase windings of the superconducting order parameter and is topological in nature. When the tube has a radius variation along the axial direction, forming a bottleneck structure between sections with different radius, a fluxoid mismatch can appear depending on the applied magnetic field. The bottleneck then becomes a topological boundary and is host to topologically protected solutions for the order parameter, dubbed fluxoid solitons, that are free to move around bottlenecks with cylindrical symmetry. Fluxoid solitons are a new type of vortex with non-quantized flux, loosely related to Pearl vortices in thin superconducting films, and fluxons in Corbino Josephson junctions. We characterize their properties as a function of system parameters using the self-consistent quasiclassical theory of diffusive superconductors. We consider both short bottleneck structures and long tapered tubes, where multiple trapped fluxoid solitons adopt elaborate arrangements dictated by their mutual repulsion.

cond-mat.supr-con

Theory of Spin-splitter Magnetoresistance in Altermagnets

We develop a theory of angular-dependent magnetoresistance (ADMR) in metallic altermagnets coupled to ferromagnetic insulators and establish criteria that distinguish them from conventional compensated magnets with spin-orbit coupling. We show that, once its full set of angular dependencies is established, the spin-splitter magnetoresistance (SSMR)-- recently reported in the bilayer geometry of H. Chen et al. [Adv. Mater. 37, 2507764 (2025)] -- would constitute a smoking-gun signature of collinear d-wave altermagnetism in metallic systems. Although SSMR has been regarded as a close analogue of spin Hall magnetoresistance (SMR), we demonstrate that the two differ qualitatively in three key respects: SSMR depends solely on the relative orientation between the ferromagnetic magnetization and the altermagnetic Néel vector, yields a longitudinal ADMR response of opposite sign, and features a direct proportionality between longitudinal and transverse ADMR signals, absent in SMR. Building on these distinctions, we further show that the full angular dependence of the SSMR provides a practical recipe to extract the direction of the Néel vector from customary magnetoresistance measurements. These results provide a clear route to unambiguously identify altermagnets in transport.

cond-mat.mes-hall

Controlling magnetic domain walls with supercurrents

Establishing a versatile, fast and reliable magnetic memory technology is a giant bottleneck for cryogenic computing since present-day room-temperature solutions either cease to work or consume too much power. The long-term goal of superconducting spintronics has been to overcome this bottleneck by generating magnetic memories with equal-spin triplet supercurrent driven through them to control their magnetization direction. This path has been hampered by the short spin relaxation length and strong anisotropy in ferromagnets. Here we show how the supercurrent driven generation of spin accumulation in a superconductor/magnetic insulator bilayer, together with Gilbert damping of magnetization lead to a motion of magnetic domain walls. This manifests as a local voltage across the wall, which allows its position to be identified. Associated with this voltage and the current, there is Joule power which is dissipated via the Gilbert damping. The power required to maintain domain wall motion is orders of magnitude smaller than in the normal state, where most of the power is wasted in producing the current.

cond-mat.supr-con

Interplay between Superconductivity and Altermagnetism in Disordered Materials and Heterostructures

We study the interplay between superconductivity and altermagnetism in disordered systems using recently derived quantum kinetic transport equations. Starting from this framework, we derive the Ginzburg-Landau free energy and identify, in addition to the conventional pair-breaking term, a coupling between the spin and the spatial variation of the superconducting order parameter. Two distinct effects emerge from this coupling. The first is a nonlinear magnetoelectric effect, in which a supercurrent (i.e., a phase gradient) induces a spin texture; this contribution is quadratic in the phase gradient. The second effect arises when the magnitude, rather than the phase, of the superconducting order parameter varies in space, likewise leading to a finite magnetization. We show that these two contributions compete in the case of an Abrikosov vortex, where both the amplitude and phase of the order parameter vary spatially. The effect associated with amplitude variations also gives rise to a proximity-induced magnetization (PIM) in hybrid structures composed of a superconductor (S) and an altermagnet (AM). Using quasiclassical theory, we analyze the PIM in diffusive S/AM bilayers and S/AM/S Josephson junctions, and determine the induced magnetization profiles. In Josephson junctions, where both the PIM and the nonlinear magnetoelectric effect coexist, we further predict the occurrence of $0$-$π$ transitions.

cond-mat.supr-con

Signatures of time-reversal-symmetry breaking in multiband 2H-TaS2 revealed by zero-field Josephson nonreciprocity

Superconductors that spontaneously break time-reversal symmetry host complex order parameters and are widely regarded as a hallmark of unconventional superconductivity. Whether such symmetry breaking can also arise in superconductors with nominally isotropic spin-singlet pairing remains an open question. Here we report a zero-field Josephson diode effect in noncentrosymmetric 2H-TaS2/2H-NbSe2 van der Waals junctions. The diode efficiency shows no systematic correlation with supercurrent amplitude, TaS2 thickness, or normal-state resistance, arguing against simple extrinsic, purely interfacial, or transparency-driven mechanisms. Time-reversal-symmetric scenarios are further tested using symmetry-controlled and molecule-intercalated control devices, in which the nonreciprocal response is absent or strongly reduced. Normal-state Hall transport in TaS2 exhibits a nonlinear response consistent with multiband correlated electronic states. Within a Josephson framework, our modelling shows that interband scattering acts as a phase-locking mechanism generating an intrinsic anomalous phase difference and a nonsinusoidal asymmetric current-phase relation, leading to finite zero-field rectification. Together, zero-field Josephson nonreciprocity and nonlinear Hall transport provide complementary evidence for a multiband superconducting phase structure in 2H-TaS2, consistent with intrinsic time-reversal-symmetry breaking.

cond-mat.supr-con

Charge-tunable Cooper-pair diode

Superconducting diodes, devices that allow Cooper-pair currents to flow more easily in one direction than the other, are set to become key building blocks for dissipationless electronics. Existing realizations, however, rely on magnetic fields, ferromagnets, or complex heterostructures that hinder integration and scalability. Here we demonstrate a diode effect for Cooper-pairs that arises solely from electron-electron interactions in nanoscale superconducting lead islands. When these islands are driven into the Coulomb blockade regime, Cooper-pair transport occurs through resonant charge states. By tuning the island's electrostatic environment, we controllably break particle-hole symmetry and induce nonreciprocal supercurrents, thereby achieving a gate-switchable superconducting diode without any external magnetic field. Our approach enables robust rectification of superconducting currents and microwave photoresponse, providing a scalable strategy to superconducting logic devices.

cond-mat.mes-hall

Coherent subgap transport in spin-split Josephson junctions

We report the first experimental observation of subgap transport in ferromagnetic insulator/superconductor/insulator/superconductor junctions realized in EuS/Al/AlOx/Al vertical stacks. Differential conductance measurements reveal multiple Andreev reflection peaks, with odd-order peaks split by the spin-splitting induced in the superconductor adjacent to EuS, while even-order peaks remain unaffected. Combining experiments with quasiclassical transport modeling, we extract the spin-splitting and the distribution of transmission channels, finding that a significant fraction ($\sim 23\%$) of highly transparent channels ($τ\approx 0.9$) dominates transport. The observation of a Josephson current further confirms strong superconducting coupling through these channels. Our results demonstrate that a single spin-split superconductor is sufficient to observe the even-odd MAR effect. Our work establishes EuS/Al junctions as a versatile platform to study subgap transport, Josephson coupling, and spin-polarized superconducting phenomena.

cond-mat.supr-con

Nonequilibrium spin-splitter effect in altermagnet superconductor hybrids

We study the nonequilibrium spin-splitter effect in superconducting altermagnets and superconductor altermagnet hybrids by computing the alternating spin current and edge the spin density in the presence of an alternating electric field. We show that while in the normal state the effect is not sensitive to the field frequency, in the superconducting state, there is a strong effect for frequencies on the scale of $Δ_0$ or lower. We contrast the effect to the spin accumulation induced by the spin-Hall effect, by showing that for the altermagnet spin-splitter effect the out-of-phase spin density does not diverge in the adiabatic limit. This difference is attributed to the absence of any equilibrium spin-splitter effect in altermagnets. In fact, the out-of-phase component vanishes below the gap excitation frequency $2Δ_0$, because below this frequency the absence of dissipation and the behavior of the system under time-reversal directly determine the relative phase between the charge current, spin current, and spin accumulation. The nonequilibrium effect can be tuned by external parameters like temperature. In fact, it has a nonmonotonic temperature dependence, taking its largest value for temperatures around $0.8T_{c}$. The value at this temperature can be significantly larger than the normal state spin density or the low temperature spin density. Thus, besides using the nonequilibrium spin-splitter effect to identify altermagnets, its tunability makes it also suitable for applications.

cond-mat.supr-con

Weak-anti-localization-to-spin-dependent scattering at a proximity-magnetized heavy metal interface

A change in a materials electrical resistance with magnetic field (magnetoresistance) results from quantum interference effects and, or spin-dependent transport, depending on materials properties and dimensionality. In disordered conductors, electron interference leads to weak localization or anti-localization; in contrast, ferromagnetic conductors support spin-dependent scattering, leading to giant magnetoresistance (GMR). By varying the thickness of Au between 4 and 28 nm in a EuS/Au/EuS spin-switches, we observe a crossover from weak anti-localization to interfacial GMR. The crossover is related to a magnetic proximity effect in Au due to electron scattering at the insulating EuS interface. The proximity-induced exchange field in Au suppresses weak anti-localization, consistent with Maekawa-Fukuyama theory. With increasing Au thickness, GMR emerges along with spin Hall magnetoresistance. These findings demonstrate spin transport governed by interfacial exchange fields, building a framework for spintronic functionality without metallic magnetism.

cond-mat.mtrl-sci

Interfacial spin-orbit coupling in superconducting hybrid systems

We investigate the effects of interfacial spin-orbit coupling (ISOC) on superconductors, focusing on its impact on electronic transport and spin-charge conversion. Using a symmetry-based nonlinear sigma model, we derive effective boundary conditions for the Usadel and Maxwell equations that account for the spin-galvanic effect, spin relaxation, and spin precession. This approach allows for the analysis of various interfaces without relying on specific microscopic models. We apply these boundary conditions to derive ISOC-induced terms in the Ginzburg-Landau functional, which is then used to compute the critical temperature of superconducting films with ISOC subjected to an external magnetic field. Our findings show that, contrary to a recent prediction, the critical temperature of a film cannot be enhanced by an external magnetic field. Additionally, we demonstrate that the combination of ISOC and an external magnetic field leads to a superconducting diode effect. Its efficiency strongly depends on the interplay between the spin-galvanic and the spin relaxation terms. Our results provide a framework for understanding ISOC in superconducting systems and highlight the potential for optimizing diode efficiency through careful interface engineering.

cond-mat.supr-con

Local control of parity and charge in nanoscale superconducting lead islands

Small superconducting islands can exhibit charge quantization, where Coulomb interactions compete with Cooper pairing. Using scanning tunneling spectroscopy, we probe this interplay by measuring the charging energy ($E_C$) and the pairing energy ($Δ$) of individual nano-islands. Below a critical island size, where $E_C > Δ$, we observe a crossover between even and odd parity ground states. By applying controlled voltage pulses, we continuously tune the island's electrostatic potential and map the full charge-parity landscape. These results demonstrate tunable superconducting ground states, offering a potential platform for qubit design and control.

cond-mat.mes-hall

Quantum transport theory for unconventional magnets: Interplay of altermagnetism and p-wave magnetism with superconductivity

We present a quantum transport theory for generic magnetic metals, in which magnetism occurs predominantly due to exchange interactions, such as ferromagnets, antiferromagnets, altermagnets and p-wave magnets. Our theory is valid both for the normal and the superconducting state. We derive the effective low-energy action for each of these materials, where the spin space groups are used to determine the form of the tensor coefficients appearing in the action. The transport equations, which are obtained as the saddle point equations of this action, describe a wider range of phenomena than the usual quasiclassical equations. In ferromagnets, in addition to the usual exchange field and spin relaxation effects, we identify a spin-dependent renormalization of the diffusion coefficient, which provides a description of spinpolarized currents in both the normal and superconducting equal spin-triplet states. In the normal state, our equations provide a complete description of the spin-splitting effect in diffusive systems, recently predicted in ideal clean altermagnets. In the superconducting state, our equations predict a proximity induced magnetization, the appearance of a spontaneous magnetic moment in hybrid superconductor-altermagnet systems. The distribution and polarization direction of this magnetic moment depend on the symmetry of the structure, thus measurements of such polarization reveal the underlying microscopic symmetry of the altermagnet. Finally, for inversionsymmetry broken antiferromagnets, such as the p-wave magnet, we show that spin-galvanic effects which are distinguishable from the spin-galvanic effect induced by spin-orbit coupling only in the superconducting state. Besides these examples, our model applies to arbitrary magnetic systems, providing a complete theory for nonequilibrium transport in diffusive nonconventional magnets at arbitrary temperatures.

cond-mat.supr-con

Gate-tunable polarity inversions and three-fold rotation symmetry of the superconducting diode effect

The superconducting diode effect is an asymmetry in the critical current with respect to the supercurrent polarity. One impetus driving recent interest in the effect is its dependence on intrinsic or microscopic symmetry breaking mechanisms. Here, we study the superconducting diode effect in gated planar Josephson junctions fabricated on a superconductor--semiconductor heterostructure under an in-plane magnetic field. We observe two gate-driven inversions of the diode polarity in the vicinity of zero field, as well as a third-harmonic component in the dependence of the diode efficiency on the in-plane field angle. We analyze the Lifshitz invariant for an arbitrary spin--orbit coupling and show that multiple polarity inversions are possible in the presence of both linear and cubic Dresselhaus terms, where the Rashba parameter varies monotonically with gate voltage. Numerical calculations of the diode efficiency further reveal the presence of higher harmonics in its field-angle dependence in the presence of spin--orbit coupling.

cond-mat.mes-hall

From local to collective superconductivity in proximitized graphene

The superconducting proximity effect induces pairing correlations in metallic systems via Andreev scattering. This effect is particularly intriguing in graphene, as it enables two-dimensional superconductivity that is tunable through doping. Understanding how superconducting correlations propagate within the metal is crucial to unveiling the key factors behind this tunability. Here, we employ scanning tunneling microscopy to investigate the energy and length scales of the proximity effect induced by Pb islands on graphene. Using tip-induced manipulation, we assemble S/N/S junctions with tunable N-region spacing and explore the evolution of the proximitized state in the confined normal region. We find that different doping levels can lead to either localized or collective superconducting states. By combining our experimental results with quasiclassical theory, we demonstrate that interface conductance plays a key role in determining the strength and coherence length of pairing correlations and inter-island coupling. Our findings provide new insights into the design of novel superconducting states and the control of their properties.

cond-mat.mes-hall

Revealing inter-band electron pairing in a superconductor with spin-orbit coupling

Most superconducting mechanisms pair electrons within the same band, forming spin singlets. However, the discovery of multi-band superconductivity has opened new scenarios for pairing, particularly in systems with strong spin-orbit coupling. Here, we reveal inter-band pairing in the superconductor \bipd\ by mapping the amplitude of sub-gap Yu-Shiba-Rusinov (YSR) states around Vanadium adatoms deposited on its surface. The surface of \bipd\ is characterized by spin-helical-like bands near the Fermi level. Scanning tunneling spectroscopy reveals anisotropic YSR amplitude oscillations around the impurity, driven by spin-conserving Bogoliubov quasiparticle interference (BQPI). Analysis of the BQPI patterns at the YSR energy exposes inter-band pairing in this material. Interestingly, only a small subset of all possible inter-band scattering processes observed in the normal state contribute to the BQPI patterns. Combining experimental data and theory, we demonstrate that the observed band selectivity results from the hybridization of the band coupled with the impurity with other bands. Our findings reveal unconventional pairing mechanisms in \bipd\ and highlight the crucial role of spin-orbit interactions in their formation.

cond-mat.mes-hall

A universal phenomenology of charge-spin interconversion and dynamics in diffusive systems with spin-orbit coupling

We present an effective field theory for a unified description of transport in normal and superconducting metals in the presence of generic spin-orbit coupling (SOC). The structure of the quantum kinetic theory in the diffusive regime is determined by a set of fundamental constraints -- charge conjugation symmetry, the causality principle, and the crystal symmetry of a material. These symmetries uniquely fix the action of the Keldysh non-linear $σ$ model (NLSM), which at the saddle point yields the quantum kinetic Usadel-type equation. Our phenomenological approach is reminiscent of the Ginzburg-Landau theory, but is valid for superconductors in the whole temperature range, describes the diffusive transport in the normal state, and naturally captures the effects of superconducting fluctuations. As an application, we derive the NLSM and quantum transport equations which include all effects of spin-orbit coupling, allowed by the crystal symmetry, for example, the spin Hall, spin current swapping or spin-galvanic effects. Our approach can be extended to systems with broken time reversal symmetry, as well as to the description of hybrid interfaces, where the spin-charge interconversion can be enhanced due to strong interfacial SOC.

cond-mat.supr-con