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F. Sebastian Bergeret

Publications and source records attributed to F. Sebastian Bergeret.

At least 37 records · Page 2Linked to original sources

A universal phenomenology of charge-spin interconversion and dynamics in diffusive systems with spin-orbit coupling

We present an effective field theory for a unified description of transport in normal and superconducting metals in the presence of generic spin-orbit coupling (SOC). The structure of the quantum kinetic theory in the diffusive regime is determined by a set of fundamental constraints -- charge conjugation symmetry, the causality principle, and the crystal symmetry of a material. These symmetries uniquely fix the action of the Keldysh non-linear $σ$ model (NLSM), which at the saddle point yields the quantum kinetic Usadel-type equation. Our phenomenological approach is reminiscent of the Ginzburg-Landau theory, but is valid for superconductors in the whole temperature range, describes the diffusive transport in the normal state, and naturally captures the effects of superconducting fluctuations. As an application, we derive the NLSM and quantum transport equations which include all effects of spin-orbit coupling, allowed by the crystal symmetry, for example, the spin Hall, spin current swapping or spin-galvanic effects. Our approach can be extended to systems with broken time reversal symmetry, as well as to the description of hybrid interfaces, where the spin-charge interconversion can be enhanced due to strong interfacial SOC.

cond-mat.supr-con↗

Full counting statistics for unconventional superconductor junctions

Noise and current measurements are key tools for studying mesoscopic systems, revealing insights beyond conductance alone. For instance, noise measurements show that transport carriers in conventional superconductors have charge 2e. The noise power also depends on junction type, distinguishing different transport processes. Existing theories focus primarily on zero temperature shot noise in tunnel junctions with conventional superconductors, where transport is carried by quasiparticles and Cooper pairs. Here we develop a full counting statistics theory for unconventional superconductor / normal metal junctions of different types, incorporating the effect of thermal noise on the differential Fano factor, the ratio of differential noise power and conductance. In these junctions there is a third type of transport carrier, surface Andreev bound states. Our study reveals that junctions with dispersionless surface Andreev bound states exhibit negative differential Fano factor at finite temperatures. In contrast, in the presence of dispersive surface Andreev bound states, the noise power always increases with voltage, but there are local minima in the differential noise at those voltages corresponding to the extrema of the surface Andreev bound state spectrum. For normal metals and conventional superconductors the voltage dependence of the differential Fano factor is similar in all types of junctions, including tunnel junctions and diffusive barriers. However, significant differences arise with unconventional superconductors, making distinct junction types valuable tools for identifying pairing symmetries. Our results also highlight the importance of finite temperature effects in noise power measurements for potential unconventional superconductors, offering new means to determine pairing symmetries in topological superconductors.

cond-mat.supr-con↗

Diluted Yu-Shiba-Rusinov arrays on the $β$-Bi$_2$Pd anisotropic superconductor

Magnetic adatoms on s-wave superconductors induce bound states inside the superconducting gap, called Yu-Shiba-Rusinov states (YSR). The anisotropy of the Fermi surface determines the spatial extension of bound states in a quasi-two-dimensional superconductor. This is especially important in the diluted impurity limit since the orbital overlap determines the coupling of YSR states of neighboring atoms and the formation of the collective YSR system. Here, we build diluted arrays of Mn atoms with different dimensionalities on the surface of $β$-Bi$_2$Pd, and we measure the evolution of their YSR spectra with the structure. We detect the coupling as a split of YSR peaks in subgap spectra and find that the split size increases with the number of atoms. The orientation of the structures along different directions of the \bipd substrate modulates the split and particle-hole asymmetry of the YSR states due to the anisotropic character of the Fermi surface, captured by the Green function model. With the aid of the model, we found multiple YSR excitations in an extended 2D array of 25 Mn atoms, and we identified that their spatial distribution reflects a chiral LDOS.

cond-mat.supr-con↗

Large spin-charge interconversion induced by interfacial spin-orbit coupling in a highly conducting all-metallic system

Spin-charge interconversion in systems with spin-orbit coupling has provided a new route for the generation and detection of spin currents in functional devices for memory and logic such as spin-orbit torque switching in magnetic memories or magnetic state reading in spin-based logic. Disentangling the bulk (spin Hall effect) from the interfacial (inverse spin galvanic effect) contribution has been a common issue to properly quantify the spin-charge interconversion in these systems, being the case of Au paradigmatic. Here, we obtain a large spin-charge interconversion at a highly conducting Au/Cu interface which is experimentally shown to arise from the inverse spin galvanic effect of the interface and not from the spin Hall effect of bulk Au. We use two parameters independent of the microscopic details to properly quantify the spin-charge interconversion and the spin losses due to the interfacial spin-orbit coupling, providing an adequate benchmarking to compare with any spin-charge interconversion system. The good performance of this metallic interface, not based in Bi, opens the path to the use of much simpler light/heavy metal systems.

cond-mat.mes-hall↗

Superconducting diode effect in diffusive superconductors and Josephson junctions with Rashba spin-orbit coupling

We characterize the superconducting diode effect (SDE) in two-dimensional diffusive structures with Rashba spin-orbit coupling using the quasiclassical formalism. We consider both homogeneous superconductors and Josephson junctions. In the first case, the diode effect monotonically increases as the magnetic field is increased and the temperature is reduced, in contrast to the non-monotonic behavior found in clean structures. In Josephson junctions, SDE dramatically increases and changes its sign close to the $0-π$ transition of the junction, which occurs at specific junction lengths and strengths of the magnetic field. We show that the SDE is strongly suppressed in narrow junctions. Our results are relevant for understanding recent experiments that measure SDE in mesoscopic nanostructures, where significant disorder is unavoidable.

cond-mat.supr-con↗

Realisation of de Gennes$'$ Absolute Superconducting Switch with a Heavy Metal Interface

In 1966, Pierre-Gilles de Gennes proposed a non-volatile mechanism for switching superconductivity on and off in a magnetic device. This involved a superconductor (S) sandwiched between ferromagnetic (F) insulators in which the net magnetic exchange field could be controlled through the magnetisation-orientation of the F layers. Because superconducting switches are attractive for a range of applications, extensive studies have been carried out on $F/S/F$ structures. Although these have demonstrated a sensitivity of the superconducting critical temperature ($T_{c}$) to parallel (P) and antiparallel (AP) magnetisation-orientations of the F layers, corresponding shifts in $T_c$ (i.e., $ΔT_c = T_{c,AP} - T_{c,P}$) are lower than predicted with $ΔT_c$ only a small fraction of $T_{c,AP}$, precluding the development of applications. Here, we report $EuS/Au/Nb/EuS$ structures where EuS is an insulating ferromagnet, Nb is a superconductor and Au is a heavy metal. For P magnetisations, the superconducting state in this structure is quenched down to the lowest measured temperature of 20 mK meaning that $ΔT_c/T_{c,AP}$ is practically 1. The key to this so-called absolute switching effect is a sizable spin-mixing conductance at the $EuS/Au$ interface which ensures a robust magnetic proximity effect, unlocking the potential of $F/S/F$ switches for low power electronics.

cond-mat.supr-con↗

Probing Magnetic and Triplet Correlations in Spin-Split Superconductors with Magnetic Impurities

A superconductor (SC) in proximity to a ferromagnetic insulator (FMI) is predicted to exhibit mixed singlet and triplet pair correlations. The magnetic proximity effect of FMI spin-splits the energy of Bogoliubov excitations and leads to a spin polarization at the surface for superconducting films thinner than the superconducting coherence length. In this work, we study manifestations of these phenomena in the properties of a magnetic impurity coupled via Kondo coupling to this FMI/SC system. Using the numerical renormalization group (NRG) method, we compute the properties of the ground state and low-lying excited states of a model that incorporates the Kondo interaction and a Ruderman-Kittel-Kasuya-Yosida (RKKY)-like interaction with the surface spin polarization. Our main finding is an energy splitting of the lowest even fermion-parity states caused by the proximity to the FMI. As the Kondo coupling increases, the splitting grows and saturates to a universal value equal to twice the exchange field of the FMI. We introduce a two-site model that can be solved analytically and provides a qualitative understanding of this and other NRG results. In addition, using perturbation theory we demonstrate that the mechanism behind the splitting involves the RKKY field and the triplet correlations of the spin-split superconductor. A scaling analysis combined with NRG shows that the splitting can be written as a single-parameter scaling function of the ratio of the Kondo temperature and the superconducting gap, which is also numerically obtained.

cond-mat.mes-hall↗

Superconductivity Induced Ferromagnetism In The Presence of Spin-Orbit Coupling

We investigate the behavior of magnetic impurities placed on the surface of superconductor thin films with spin-orbit coupling. Our study reveals long-range interactions between the impurities, which decay according to a power law, mediated by the supercurrents. Importantly, these interactions possess a ferromagnetic component when considering the influence of the electromagnetic field, leading to the parallel alignment of the magnetic moments in the case of two impurities. In a Bravais lattice of magnetic impurities, superconductivity facilitates the establishment of ferromagnetic order within specific parameter ranges. These findings challenge the conventional understanding that ferromagnetism and superconductivity are mutually exclusive phenomena. Our theoretical framework provides a plausible explanation for the recently observed remanent flux in iron-based superconductors, particularly Fe(Se,Te).

cond-mat.supr-con↗

Theory of a Single Magnetic Impurity on a Thin Metal Film in Proximity to a Superconductor

We argue that the formation of Yu-Shiba-Rusinov excitations in proximitized thin films is largely mediated by a type of Andreev-bound state named after de Gennes and Saint James. This is shown by studying an experimentally motivated model and computing the overlap of the wave functions of these two subgap states. We find the overlap stays close to unity even as the system moves away from weak coupling across the parity-changing quantum phase transition. Based on this observation, we introduce a single-site model of the bound state coupled to a quantum spin. The adequacy of this description is assessed by reintroducing the coupling to the continuum as a weak perturbation and studying its scaling flow using Anderson's poor man's scaling.

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Ubiquitous Superconducting Diode Effect in Superconductor Thin Films

The macroscopic coherence in superconductors supports dissipationless supercurrents which could play a central role in emerging quantum technologies. Accomplishing unequal supercurrents in the forward and backward directions would enable unprecedented functionalities. This nonreciprocity of critical supercurrents is called superconducting (SC) diode effect. We demonstrate strong SC diode effect in conventional SC thin films, such as niobium and vanadium, employing external magnetic fields as small as 1 Oe. Interfacing the SC layer with a ferromagnetic semiconductor EuS, we further accomplish non-volatile SC diode effect reaching a giant efficiency of 65%. By careful control experiments and theoretical modeling, we demonstrate that the critical supercurrent nonreciprocity in SC thin films could be easily accomplished with asymmetrical vortex edge/surface barriers and the universal Meissner screening current governing the critical currents. Our engineering of the SC diode effect in simple systems opens door for novel technologies. Meanwhile, we reveal the ubiquity of Meissner screening effect induced SC diode effect in superconducting films, which should be eliminated with great care in the search of exotic superconducting states harboring finite-momentum Cooper pairing.

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Effects of the Spatial Extension of the Edge Channels on the Interference Pattern of a Helical Josephson Junction

Josephson junctions (JJs) in the presence of a magnetic field exhibit qualitatively different interference patterns depending on the spatial distribution of the supercurrent through the junction. In JJs based on two-dimensional topological insulators (2DTIs), the electrons/holes forming a Cooper pair (CP) can either propagate along the same edge or be split into the two edges. The former leads to a SQUID-like interference pattern, with the superconducting flux quantum $ϕ_0$ (where $ϕ_0=h/2e$) as a fundamental period. If CPs' splitting is additionally included, the resultant periodicity doubles. Since the edge states are typically considered to be strongly localized, the critical current does not decay as a function of the magnetic field. The present paper goes beyond this approach and inspects a topological JJ in the tunneling regime featuring extended edge states. It is here considered the possibility that the two electrons of a CP propagate and explore the junction independently over length scales comparable to the superconducting coherence length. As a consequence of the spatial extension, a decaying pattern with different possible periods is obtained. In particular, it is shown that, if crossed Andreev reflections (CARs) are dominant and the edge states overlap, the resulting interference pattern features oscillations whose periodicity approaches $2ϕ_0$.

cond-mat.supr-con↗

Reducing the frequency of the Higgs mode in a helical superconductor coupled to an LC-circuit

We show that the amplitude, or Higgs mode of a superconductor with strong spin-orbit coupling and an exchange field, couples linearly to the electromagnetic field. Furthermore, by coupling such a superconductor to an LC resonator, we demonstrate that the Higgs resonance becomes a regular mode at frequencies smaller than the quasiparticle energy threshold $2Δ$. We finally propose and discuss a possible experiment based on microwave spectroscopy for an unequivocal detection of the Higgs mode. Our approach may allow visualizing Higgs modes also in more complicated multiband superconductors with a coupling between the charge and other electronic degrees of freedom.

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Triplet odd-frequency superconductivity in hybrid superconductor-ferromagnet structures

We present an overview of the contributions made by Konstantin B. Efetov and the authors to the field of triplet odd-frequency superconductivity in hybrid ferromagnet-superconductor structures and the repercussions they had on experimental and theoretical research. Konstantin B. Efetov passed away in August 2021. We hope the present short review gives a faithful testimony of an important part of his scientific legacy.

cond-mat.supr-con↗

Emergence of large spin-charge interconversion at an oxidized Cu/W interface

Spin-orbitronic devices can integrate memory and logic by exploiting spin-charge interconversion (SCI), which is optimized by design and materials selection. In these devices, such as the magnetoelectric spin-orbit (MESO) logic, interfaces are crucial elements as they can prohibit or promote spin flow in a device as well as possess spin-orbit coupling resulting in interfacial SCI. Here, we study the origin of SCI in a Py/Cu/W lateral spin valve and quantify its efficiency. An exhaustive characterization of the interface between Cu and W electrodes uncovers the presence of an oxidized layer (WO$_x$). We determine that the SCI occurs at the Cu/WO$_x$ interface with a temperature-independent interfacial spin-loss conductance of $G_{||} \approx$ 20 $\times$ 10$^{13} Ω^{-1}m^{-2}$ and an interfacial spin-charge conductivity $σ_{SC}=-$1610 $Ω^{-1}cm^{-1}$ at 10 K ($-$830 $Ω^{-1}cm^{-1}$ at 300 K). This corresponds to an efficiency given by the inverse Edelstein length $λ_{IEE}=-$0.76 nm at 10 K ($-$0.4 nm at 300 K), which is remarkably larger than in metal/metal and metal/oxide interfaces and bulk heavy metals. The large SCI efficiency at such an oxidized interface is a promising candidate for the magnetic readout in MESO logic devices.

cond-mat.mes-hall↗

Pair excitations of a quantum spin on a proximitized superconductor

A magnetic impurity interacting with a superconductor develops a rich excitation spectrum formed by superposition of quasiparticles and spin states, which appear as Yu-Shiba-Rusinov and spin-flip excitations in tunneling spectra. Here, we show that tunneling electrons can also excite a superconducting pair-breaking transition in the presence of magnetic impurities, which is hidden for electrons on bare superconductors. Combining scanning tunneling spectroscopy with theoretical modeling, we map the excitation spectrum of a Fe-porphyrin molecule on the Au/V(100) proximitized surface into a manifold of many-body excitations and follow their behavior across a parity-changing transition. Pair excitations emerge in the tunneling spectra as peaks outside the gap in the strong interaction regime, scaling with the pair correlation. Our results unravel the quantum nature of magnetic impurities on superconductors and prove that pair excitations are parity detectors for magnetic impurities.

cond-mat.mes-hall↗

Yu-Shiba-Rusinov states in 2D superconductors with arbitrary Fermi contours

Magnetic impurities on a superconductor induce sub-gap Yu-Shiba-Rusinov (YSR) bound states, localized at the impurity site and fading away from it for distances up to several nanometers. In this article, we present a theoretical method to calculate the spatial distribution of the YSR spectrum of a two-dimensional superconductor with arbitrary Fermi contours (FCs) in the presence of magnetic impurities. Based on the Green's Function (GF) formalism, we obtain a general analytical expression by approximating an arbitrary contour shape to a regular polygon. This method allows us to show the connection between the spatial decay (and, hence, the extension) of YSR states and the shape of the FC of the host superconductor. We further apply this formalism to compute the evolution of YSR states in the presence of a nearby impurity atom, and compare the results with Scanning Tunneling Microscopy (STM) measurements on interacting manganese dimers on the $β$-Bi2Pd superconductor. The method can be easily extended to any arbitrary number of magnetically coupled impurities, thus, providing a useful tool for simulating the spectral properties of interacting YSR states in artificial atomic nanostructures.

cond-mat.mes-hall↗

Theory of the supercurrent diode effect in Rashba superconductors with arbitrary disorder

We calculate the non-reciprocal critical current and quantify the supercurrent diode effect in Rashba superconductors with arbitrary disorder, using the quasiclassical Eilenberger equation. The non-reciprocity is caused by the helical superconducting state, which appears when both inversion and time-reversal symmetries are broken. In the absence of disorder, we find a very strong diode effect, with the non-reciprocity exceeding 40% at optimal temperatures, magnetic fields and spin-orbit coupling. We establish that the effect persists even in the presence of strong disorder. We show that the sign of the diode effect changes as magnetic field and disorder are increased, reflecting the changes in the nature of the helical state.

cond-mat.supr-con↗

Ever-present Majorana bound state in a generic one-dimensional superconductor with odd number of Fermi surfaces

A quasi-1D superconductor with odd number of Fermi surfaces is expected to exhibit a nondegenerate Majorana bound state at the Fermi level at its boundary with an insulator (where the latter could be an actual insulator material or vacuum, for a terminated sample). Previous explicit theoretical demonstrations of this property were done for specific microscopic models of the bulk Hamiltonian and, most importantly, of the boundary. In this work, we theoretically demonstrate that this property holds for the whole class of systems, using the symmetry-based formalism of low-energy continuum models and general boundary conditions. We derive the general form of the Bogoliubov-de Gennes low-energy Hamiltonian that is subject only to charge-conjugation symmetry $\mathcal{C}_+$ of the type $\mathcal{C}_+^2=+1$ and a few minimal assumptions. Crucially, we also derive the most general form of the boundary conditions describing the boundary with an insulator, subject only to the fundamental principle of the probability-current conservation and $\mathcal{C}_+$ symmetry. Such {\em normal-reflection} boundary conditions do not contain scattering between electrons and holes. We find that for odd number of Fermi surfaces a Majorana bound state always exists as long as the bulk is in the gapped superconducting state, irrespective of the parameters of the bulk Hamiltonian and boundary conditions. Importantly, our general model includes a possible {\em Fermi-point mismatch}, when the two Fermi points are not at exactly opposite momenta, which disfavors superconductivity. We find that the Fermi-point mismatch does {\em not} have a direct destructive effect on the Majorana bound state, in the sense that once the bulk gap is opened the bound state is always present.

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