arXiv subjects

Fa Wang

Publications and source records attributed to Fa Wang.

At least 55 records · Page 3Linked to original sources

arXiv2015

Computational Study of the Magnetic Structure of Na$_2$IrO$_3$

The magnetic structure of honeycomb iridate Na$_2$IrO$_3$ is of paramount importance to its exotic properties. The magnetic order is established experimentally to be zigzag antiferromagnetic. However, the previous assignment of ordered moment to the $\bm{a}$-axis is tentative. We examine the magnetic structure of Na$_{2}$IrO$_{3}$ using first-principles methods. Our calculations reveal that total energy is minimized when the zigzag antiferromagnetic order is magnetized along $\bm{g}\approx\bm{a}+\bm{c}$. Such a magnetic configuration is explained by adding anisotropic interactions to the nearest-neighbor Kitaev-Heisenberg model. Spin-wave spectrum is also calculated, where the calculated spin gap of $10.4$ meV can in principle be measured by future inelastic neutron scattering experiments. Finally we emphasize that our proposal is consistent with all known experimental evidence, including the most relevant resonant x-ray magnetic scattering measurements [X. Liu \emph{et al.} {Phys. Rev. B} \textbf{83}, 220403(R) (2011)].

cond-mat.mtrl-sci↗

arXiv2014

The edge engineering of topological Bi(111) bilayer

A topological insulator is a novel quantum state, characterized by symmetry-protected non-trivial edge/surface states. Our first-principle simulations show the significant effects of the chemical decoration on edge states of topological Bi(111) bilayer nanoribbon, which remove the trivial edge state and recover the Dirac linear dispersion of topological edge state. By comparing the edge states with and without chemical decoration, the Bi(111) bilayer nanoribbon offers a simple system for assessing conductance fluctuation of edge states. The chemical decoration can also modify the penetration depth and the spin texture of edge states. A low-energy effective model is proposed to explain the distinctive spin texture of Bi(111) bilayer nanoribbon, which breaks the spin-momentum orthogonality along the armchair edge.

cond-mat.mtrl-sci↗

arXiv2013

Detect Spinons via Spin Transport

Existence of spinons is the defining property of quantum spin liquids. These exotic excitations have (fractionalized) spin quantum number and no electric charge, and have been proposed to form Fermi surfaces in the recently discovered organic spin liquid candidates. However direct probes for them are still lacking. In this paper we propose to experimentally identify the spinons by measuring the spin current flowing through the spin liquid candidate materials, which would be a direct test for the existence of spin-carrying mobile excitations. By the nonequilibrium Green function technique we evaluate the spin current through the interface between a Mott insulator and a metal under a spin bias, and find that different kinds of Mott insulators, including quantum spin liquids, can be distinguished by different relations between the spin bias and spin current, In the end we will also discuss relations to experiments and estimate experimentally relevant parameters.

cond-mat.str-el↗

arXiv2013

Featureless and non-fractionalized Mott insulators on the honeycomb lattice at 1/2 site filling

Within the Landau paradigm, phases of matter are distinguished by spontaneous symmetry breaking. Implicit here is the assumption that a completely symmetric state exists: a paramagnet. At zero temperature such quantum featureless insulators may be forbidden, triggering either conventional order or topological order with fractionalized excitations. Such is the case for interacting particles when the particle number per unit cell, f, is not an integer. But, can lattice symmetries forbid featureless insulators even at integer f? An especially relevant case is the honeycomb (graphene) lattice --- where free spinless fermions at f=1 (the two sites per unit cell mean f=1 is half filling per site) are always metallic. Here we present wave functions for bosons, and a related spin-singlet wave function for spinful electrons, on the f=1 honeycomb, and demonstrate via quantum to classical mappings that they do form featureless Mott insulators. The construction generalizes to symmorphic lattices at integer f in any dimension. Our results explicitly demonstrate that in this case, despite the absence of a non-interacting insulator at the same filling, lack of order at zero temperature does not imply fractionalization.

cond-mat.str-el↗

arXiv2013

Emergent topological and half semimetallic Dirac Fermions at oxide interfaces

It is highly desirable to combine recent advances in the topological quantum phases with technologically relevant materials. Chromium dioxide (CrO2) is a half-metallic material, widely used in high-end data storage applications. Using first principles calculations, we show via interfacial orbital design that a novel class of half semi-metallic Dirac electronic phase emerges at the interface CrO2 with TiO2 in both thin film and superlattice configurations, with four spin-polarized Dirac points in momentum-space (k-space) band structure. When the spin and orbital degrees of freedom are allowed to couple, the CrO2/TiO2 superlattice becomes a Chern insulator without external fields or additional doping. With topological gaps equivalent to 43 Kelvin and a Chern number 2, the ensuing quantization of Hall conductance to 2e^2/h will enable potential development of these highly industrialized oxides for applications in topologically high fidelity data storage and energy-efficient electronic and spintronic devices.

cond-mat.mtrl-sci↗

arXiv2013

Longitudinal spin excitations and magnetic anisotropy in antiferromagnetically ordered BaFe2As2

We report on a spin-polarized inelastic neutron scattering study of spin waves in the antiferromagnetically ordered state of BaFe2As2. Three distinct excitation components are identified, with spins fluctuating along the c-axis, perpendicular to the ordering direction in the ab-plane, and parallel to the ordering direction. While the first two "transverse" components can be described by a linear spin-wave theory with magnetic anisotropy and inter-layer coupling, the third "longitudinal" component is generically incompatible with the local moment picture. It points towards a contribution of itinerant electrons to the magnetism already in the parent compound of this family of Fe-based superconductors.

cond-mat.supr-con↗

arXiv2013

Fermiology, Orbital Order, Orbital Fluctuation and Cooper Pairing in Iron-based Superconductors

We address two important issues that arise in recent studies of iron-based superconductivity. (1) Why are the T_c of A_xFe_{2-y}Se_2 and the single unit cell FeSe on SrTiO$_3$ so high despite both only have electron pockets? (2) What (if any) are the effects of orbital order and orbital fluctuation on the Cooper pairing. Our conclusions are summarized in the third paragraph of the paper.

cond-mat.supr-con↗

arXiv2013

Critical theories of phase transition between symmetry protected topological states and their relation to the gapless boundary theories

Symmetry protected topological states (SPTs) have the same symmetry and the phase transition between them are beyond Landau's symmetry breaking formalism. In this paper we study (1) the critical theory of phase transition between trivial and non-trivial SPTs, and (2) the relation between such critical theory and the gapless boundary theory of SPTs. Based on examples of SO(3) and SU(2) SPTs, we propose that under appropriate boundary condition the critical theory contains the delocalized version of the boundary excitations. In addition, we prove that the boundary theory is the critical theory spatially confined between two SPTs. We expect these conclusions to hold in general and, in particular, for discrete symmetry groups as well.

cond-mat.str-el↗

arXiv2012

The Topological Relation Between Bulk Gap Nodes and Surface Bound States : Application to Iron-based Superconductors

In the past few years materials with protected gapless surface (edge) states have risen to the central stage of condensed matter physics. Almost all discussions centered around topological insulators and superconductors, which possess full quasiparticle gaps in the bulk. In this paper we argue systems with topological stable bulk nodes offer another class of materials with robust gapless surface states. Moreover the location of the bulk nodes determines the Miller index of the surfaces that show (or not show) such states. Measuring the spectroscopic signature of these zero modes allows a phase-sensitive determination of the nodal structures of unconventional superconductors when other phase-sensitive techniques are not applicable. We apply this idea to gapless iron based superconductors and show how to distinguish accidental from symmetry dictated nodes. We shall argue the same idea leads to a method for detecting a class of the elusive spin liquids.

cond-mat.supr-con↗

arXiv2012

High $T_c$ superconductivity at the FeSe/SrTiO$_3$ Interface

In a recent experiment the superconducting gap of a single unit cell thick FeSe film on SrTiO$_3$ substrate is observed by scanning tunneling spectroscopy and angle-resolved photoemission spectroscopy. The value of the superconducting gap is much larger than that of the bulk FeSe under ambient pressure. In this paper we study the effects of screening due to the ferroelectric phonons on Cooper pairing. We conclude it can significantly enhance the energy scale of Cooper pairing and even change the pairing symmetry. Our results also raise some concerns on whether phonons can be completely ignored for bulk iron-based superconductors.

cond-mat.supr-con↗

arXiv2012

Nearly flat band with Chern number C=2 on the dice lattice

We point out the possibility of nearly flat band with Chern number C=2 on the dice lattice in a simple nearest-neighbor tightbinding model. This lattice can be naturally formed by three adjacent $(111)$ layers of cubic lattice, which may be realized in certain thin films or artificial heterostructures, such as SrTiO$_3$/SrIrO$_3$/SrTiO$_3$ trilayer heterostructure grown along $(111)$ direction. The flatness of two bands is protected by the bipartite nature of the lattice. Including the Rashba spin-orbit coupling on nearest-neighbor bonds separate the flat bands with others but maintains their flatness. Repulsive interaction will drive spontaneous ferromagnetism on the Kramer pair of flat bands and split them into two nearly flat bands with Chern number $C=\pm 2$. We thus propose that this may be a route to quantum anomalous Hall effect and further conjecture that partial filling of the C=2 band may realize exotic fractional quantum Hall effects.

cond-mat.str-el↗

arXiv2012

Functional renormalization group and variational Monte Carlo studies of the electronic instabilities in graphene near 1/4 doping

We study the electronic instabilities of near 1/4 electron doped graphene using the functional renormalization group (FRG) and variational Monte-Carlo method. A modified FRG implementation is utilized to improve the treatment of the von Hove singularity. At 1/4 doping the system is a chiral spin density wave state exhibiting the anomalous quantized Hall effect, or equivalently a Chern insulator. When the doping deviates from 1/4, the $d_{x^2-y^2}+i d_{xy}$ Cooper pairing becomes the leading instability. Our results suggest near 1/4 electron or hole doped graphene is a fertile playground for the search of Chern insulators and superconductors.

cond-mat.supr-con↗

arXiv2011

Anomalous isotope effect in phonon-dressed iron-based superconductor

The role of electron-phonon interactions in iron-based superconductor is currently under debate with conflicting experimental reports on the isotope effect. To address this important issue, we employ the renormalization-group method to investigate the competition between electron-electron and electron-phonon interactions in these materials. The renormalization-group analysis shows that the ground state is a phonon-dressed unconventional superconductor: the dominant electronic interactions account for pairing mechanism while electron-phonon interactions are subdominant. Because of the phonon dressing, the isotope effect of the critical temperature can be normal or reversed, depending on whether the retarded intra- or inter-band interactions are altered upon isotope substitutions. The connection between the anomalous isotope effect and the unconventional pairing symmetry is discussed at the end.

cond-mat.supr-con↗

arXiv2011

Two-orbital Schwinger Boson Representation of Spin-One: Application to a Non-abelian Spin Liquid with Quaternion Gauge Field

A non-abelian spin liquid in triangular lattice spin-1 systems was recently formulated in the form of continuum field theory [T. Grover, and T. Senthil, Phys. Rev. Lett. 107, 077203 (2011); Cenke Xu, A.W.W. Ludwig, arXiv:1012.5671]. It has spin-1/2 bosonic spinons coupled to emergent quaternion gauge fields, and can be obtained by quantum disordering a non-collinear spin nematic order hypothesized to describe NiGa_2S_4 [H. Tsunetsugu, and M. Arikawa, J. Phys. Soc. Jpn. 75, 083701 (2006)], However a microscopic lattice description, e.g. the lattice spinon (mean-field) Hamiltonian and the spin wavefunction, has been missing, and it has been noted that the standard Schwinger boson or bosonic triplon representations of spin-1 cannot describe this spin liquid. In this paper a two-orbital Schwinger boson representation for spin-1 systems is developed and used to construct a mean-field description of this quaternion spin liquid. Projecting the mean-field state produces a prototype wavefunction, which is a superposition of close-packed AKLT loop configurations with nontrivial amplitudes. This new formalism and related wavefunctions may be generalized to higher spin systems and can possibly produce spin liquid states with even richer emergent gauge structures.

cond-mat.str-el↗

arXiv2011

Spin Liquid Phases for Spin-1 systems on the Triangular lattice

Motivated by recent experiments on material Ba3NiSb2O9, we propose two novel spin liquid phases (A and B) for spin-1 systems on a triangular lattice. At the mean field level, both spin liquid phases have gapless fermionic spinon excitations with quadratic band touching, thus in both phases the spin susceptibility and C_v/T saturate to a constant at zero temperature, which are consistent with the experimental results on Ba3NiSb2O9. On the lattice scale, these spin liquid phases have Sp(4) ~ SO(5) gauge fluctuation; while in the long wavelength limit this Sp(4) gauge symmetry is broken down to U(1)xZ_2 in type A spin liquid phase, and broken down to Z_4 in type B phase. We also demonstrate that the $A$ phase is the parent state of the ferro-quadrupole state, nematic state, and the noncollinear spin density wave state.

cond-mat.str-el↗

arXiv2011

The electronic instabilities of the Iron-based superconductors: a variational Monte-Carlo study

We report the first variational Monte Carlo (VMC) study of the iron-based superconductors. We use realistic band structures, and the ordering instabilities/variational ansatzs are suggested by previous functional renormalization group calculations. We examine antiferromagnetism, superconducting pairing, normal state fermi surface distortion, and orbital order in the antiferromagnetic state.

cond-mat.str-el↗

arXiv2010

Twisted Hubbard Model for Sr2IrO4: Magnetism and Possible High Temperature Superconductivity

Sr2IrO4 has been suggested as a Mott insulator from a single J_eff=1/2 band, similar to the cuprates. However this picture is complicated by the measured large magnetic anisotropy and ferromagnetism. Based on a careful mapping to the J_eff=1/2 (pseudospin-1/2) space, we propose that the low energy electronic structure of Sr2IrO4 can indeed be described by a SU(2) invariant pseudospin-1/2 Hubbard model very similar to that of the cuprates, but with a "twisted" coupling to external magnetic field (a g-tensor with a staggered antisymmetric component). This perspective naturally explains the magnetic properties of Sr2IrO4. We also derive several simple facts based on this mapping and the known results about the Hubbard model and the cuprates, which may be tested in future experiments on Sr2IrO4. In particular we propose that (electron-)doping Sr2IrO4 can potentially realize high-temperature superconductivity.

cond-mat.str-el↗

arXiv2010

Nodes in the Gap Function of LaFePO, the Gap Function of the Fe(Se,Te) Systems, and the STM Signature of the s$_{\pm}$ Pairing

We reiterate, in more details, our previous proposal of using quasi-particle interference to determine the pairing form factor in iron-based superconductors. We also present our functional renormalization group(FRG) results on LaFePO and Fe(Se,Te) superconductors. In particular we found that the leading pairing channel in LaFePO is nodal s$_{\pm}$, with nodes on electron Fermi surfaces. For Fe(Se,Te) system we found fully gapped s$_{\pm}$ pairing, with substantial gap anisotropy on electron Fermi surfaces, and large gap is concentrated in regions with dominant $xy$ orbital character. We further fit the form factor obtained by FRG to real space orbital basis pairing picture, which shows more clearly the differences between different iron-based superconductors.

cond-mat.supr-con↗