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Fabio Frassetto

Publications and source records attributed to Fabio Frassetto.

22 records · Page 2Linked to original sources

Polarization-control of absorption of virtual dressed-states in helium

The extreme ultraviolet absorption spectrum of an atom is strongly modified in the presence of a synchronized intense infrared field. In this work we demonstrate control of the absorption properties of helium atoms dressed by an infrared pulse by changing the relative polarization of the infrared and extreme ultraviolet fields. Light-induced features associated with the dressed $1s2s$, $1s3s$ and $1s3d$ states, referred to as $2s^{+}$, $3s^{\pm}$ and $3d^{\pm}$ light induced states, are shown to be strongly modified or even eliminated when the relative polarization is rotated. The experimental results agree well with calculations based on the solution of the time-dependent Schrödinger equation using a restricted excitation model that allows efficient treatment of the three dimensional problem. We also present an analysis of the light induced states based on Floquet theory, which allows for a simple explanation of their properties. Our results open a new route to creating controllable superpositions of dipole allowed and non-dipole allowed states in atoms and molecules.

physics.optics↗

Coherent diffractive imaging of single helium nanodroplets with a high harmonic generation source

Coherent diffractive imaging of individual free nanoparticles has opened novel routes for the in-situ analysis of their transient structural, optical, and electronic properties. So far, single-shot single-particle diffraction was assumed to be feasible only at extreme ultraviolet (XUV) and X-ray free-electron lasers, restricting this research field to large-scale facilities. Here we demonstrate single-shot imaging of isolated helium nanodroplets using XUV pulses from a femtosecond-laser driven high harmonic source. We obtain bright wide-angle scattering patterns, that allow us to uniquely identify hitherto unresolved prolate shapes of superfluid helium droplets. Our results mark the advent of single-shot gas-phase nanoscopy with lab-based short-wavelength pulses and pave the way to ultrafast coherent diffractive imaging with phase-controlled multicolor fields and attosecond pulses.

physics.atm-clus↗

Alignment and characterization of the two-stage time delay compensating XUV monochromator

We present the design, implementation and alignment procedure for a two-stage time delay compensating monochromator. The setup spectrally filters the radiation of a high-order harmonic generation source providing wavelength-selected XUV pulses with a bandwidth of 300 to 600~meV in the photon energy range of 3 to 50~eV. XUV pulses as short as $12\pm3$~fs are demonstrated. Transmission of the 400~nm (3.1~eV) light facilitates precise alignment of the monochromator. This alignment strategy together with the stable mechanical design of the motorized beamline components enables us to automatically scan the XUV photon energ in pump-probe experiments that require XUV beam pointing stability. The performance of the beamline is demonstrated by the generation of IR-assisted sidebands in XUV photoionization of argon atoms.

physics.ins-det↗

Momentum-dependent snapshots of a melting charge density wave

Charge density waves (CDWs) underpin the electronic properties of many complex materials. Near-equilibrium CDW order is linearly coupled to a periodic, atomic-structural distortion, and the dynamics is understood in terms of amplitude and phase modes. However, at the shortest timescales lattice and charge order may become de-coupled, highlighting the electronic nature of this many-body broken symmetry ground state. Using time and angle resolved photoemission spectroscopy with sub-30-fs XUV pulses, we have mapped the time- and momentum-dependent electronic structure in photo-stimulated 1T-TaS2, a prototypical two-dimensional charge density wave compound. We find that CDW order, observed as a splitting of the uppermost electronic bands at the Brillouin zone boundary, melts well before relaxation of the underlying structural distortion. Decoupled charge and lattice modulations challenge the view of Fermi Surface nesting as a driving force for charge density wave formation in 1T-TaS2.

cond-mat.str-el↗