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Farkhad G. Aliev

Publications and source records attributed to Farkhad G. Aliev.

At least 19 recordsLinked to original sources

Superconducting spintronics with electron symmetry filtering and interfacial spin-orbit coupling

Over the recent years, crossroads of magnetism and superconductivity led to the emerging field of superconducting spintronics. A cornerstone of this venture is the generation of equal-spin triplet Cooper pairs in superconductor-ferromagnet hybrids, enabling long-range spin-polarized supercurrents and magnetic control over superconducting quantum states for the development of energy-efficient cryogenic devices. Until now, nearly all superconducting spintronic devices have relied on direct interfaces between superconductors and ferromagnets, since it was believed that an insulating barrier would decouple spin and charge transport. This assumption, however, appears to be invalid when a thin spin- and orbit-filtering barrier couples epitaxial ferromagnet and the superconductor. Symmetry filtering plays a crucial role in enhancing giant tunneling magnetoresistance (TMR) by selectively allowing specific electronic states to tunnel through the barrier. Such a mechanism is key for high-performance spintronic devices like magnetic random access memories, magnetic sensors or spin-light emitting diodes. This manuscript provides a comprehensive review of superconducting spintronics driven by electron symmetry filtering and interfacial SOC. It emphasizes the critical role of a crystalline MgO barrier in selectively transmitting specific electronic states between V(100) and Fe(100). The manuscript also highlights how interfacial SOC enables symmetry mixing, allowing for the interaction between ferromagnetic and superconducting orderings though MgO(100). This mutual interaction, mediated by interfacial SOC, facilitates the conversion of spin-singlet to spin-triplet Cooper pairs. The work provides key insights into designing SOC based superconductor-ferromagnet hybrid structures for advanced superconducting spintronic functionalities.

cond-mat.supr-con

Giant shot noise in superconductor/ferromagnet junctions with orbital-symmetry-controlled spin-orbit coupling

By measuring the shot noise, a consequence of charge quantization, in superconductor/insulator/ferromagnet (V/MgO/Fe) junctions, we discover a giant increase, orders of magnitude larger than expected. The origin of this giant noise is a peculiar realization of a superconducting proximity effect, where a simple superconductor influences its neighbors. Our measurements reveal largely unexplored implications of orbital-symmetry-controlled proximity effects. The importance of orbital symmetries and the accompanying spin-orbit coupling is manifested by an unexpected emergence of another superconducting region strikingly different from the parent superconductor. Unlike vanadium's common spin-singlet superconductivity, the broken inversion symmetry in V/MgO/Fe junctions and the resulting interfacial spin-orbit coupling leads to the formation of spin-triplet superconductivity across the ferromagnetic iron. Here we show that the enhanced shot noise, known from Josephson junctions with two superconductors, is measured even in a single superconductor, this discovery motivates revisiting how the spin-orbit coupling and superconducting proximity effects can transform many materials.

cond-mat.supr-con

Large Tunable Thermoelectric Effects in Superconducting Spin Valves with Commercially Available Materials

Recent studies have revealed magnetically controllable thermoelectric effects in superconductor/ferromagnet (S/F) structures. A tunable cryogenic thermoelectric generator needs not only a high conversion factor between electricity and heat, but also a large change in the thermoelectric output when switching the magnetic state of the device. However, the reported modifications in thermoelectric power are either minimal, involve superconductors with relatively low critical temperatures (below 1 K), or do not utilize commercially available spintronic materials. Here, we experimentally measure and numerically model thermoelectric effects in fully epitaxial F/S/F junctions based on commercially available, easily grown materials, as well as their dependence on the magnetic configuration of the F electrodes. We observe sizeable Seebeck coefficients for the parallel alignment of the ferromagnetic electrodes, reaching values of about $100$~$μ$V/K. Importantly, we find a decrease of the thermoelectric signal of more than an order of magnitude when switching from a parallel to an antiparallel configuration, constituting a large thermoelectric spin-valve effect. Theoretical modeling based on a self-consistent non-equilibrium Keldysh-Usadel Green's function theory, combined with micromagnetic simulations, qualitatively reproduce the experimental findings. The thermoelectric effect is optimized when there is a large spin-dependent electron-hole asymmetry in the superconductor combined with spin-dependent transmission through the interfaces. These findings pave the way for the development of efficient and versatile cryogenic thermoelectric heat engines.

cond-mat.supr-con

Unraveling spin texture and spin-orbit coupling contributions in spin triplet superconductivity

Over the past decade, it has been proposed theoretically and confirmed experimentally that long-range spin triplet (LRT) superconductivity can be generated in ferromagnet-superconductor hybrids either by the presence of spin textures (ST-LRT) or thanks to spin-orbit coupling (SOC-LRT). Nevertheless, there has been no theoretical or experimental investigation to date suggesting that both contributions could simultaneously exist within an experimental system. To disentangle these contributions, we present a comprehensive study of superconducting quasiparticle interference effects taking place inside a ferromagnetic layer interfacing a superconductor, through the investigation of above-gap conductance anomalies (CAs) related to MacMillan-Rowell resonances. The bias dependence of the CAs has been studied under a wide range of in-plane (IP) and out-of-plane (OOP) magnetic fields in two types of epitaxial, V/MgO/Fe-based ferromagnet-superconductor junctions with interfacial spin-orbit coupling. We observe an anisotropy of the CAs amplitude under small IP and OOP magnetic fields while remaining weakly affected by high fields, and implement micromagnetic simulations to help us distinguish between the ST-LRT and SOC-LRT contributions. Our findings suggest that further exploration of Fabry-Pérot type interference effects in electron transport could yield valuable insights into the hybridization between superconductors and ferromagnets induced by spin-orbit coupling and spin textures.

cond-mat.supr-con

Standing spin waves in Permalloy-NiO bilayers as a probe of the interfacial exchange coupling

Ferromagnetic/Antiferromagnetic (FM/AFM) bilayers dynamics have been a recent topic of interest due to the interaction occurring at the interface, where the magnetic moments of the AFM can be imprinted into the FM, and the exchange bias field can affect these dynamics. Here, we investigate Permalloy (Py) and NiO (Py/NiO) hybrids and for comparison single Py films in the broad Py thickness range varied from few nm to 200 nm by using static (Kerr effect) and dynamic (spin waves) measurements along with micromagnetic simulations. We observe hybrid modes between uniform (ferromagnetic resonance FMR, n=0) and perpendicular standing spin waves (PSSWs, n=1, 2) and a clear enhancement of the PSSWs modes frequencies upon interfacing Py with NiO both from experiments and simulations. This enhancement becomes less pronounced as the thickness of the film increases, demonstrating its interfacial origin rooted in the exchange coupling between the FM and AFM layers. Besides, through micromagnetic simulations, we investigate and correlate changes in spatial profiles of the PSSWs with the interfacial exchange coupling. As the thickness is increased, we see that the n=1 and n=2 modes begin to couple with the fundamental FMR mode, resulting in asymmetric (with respect the Py layer center) modes. Our results suggest that PSSWs detection in a ferromagnet offers a means of probing the interfacial exchange coupling with the adjacent AFM layer. Furthermore, the controlled spatial symmetry breaking by the AFM layer enables engineering of PSSWs with different spatial profiles in the FM.

cond-mat.mes-hall

Observation of magnetic state dependent thermoelectricity in superconducting spin valves

Superconductor-ferromagnet tunnel junctions demonstrate giant thermoelectric effects which are being exploited to engineer ultra-sensitive terahertz radiation detectors. Here, we experimentally observe the recently predicted complete magnetic control over thermoelectric effects in a superconducting spin valve, including the dependence of its sign on the magnetic state of the spin valve. The description of the experimental results is improved by the introduction of an interfacial domain wall in the spin filter layer interfacing the superconductor. Surprisingly, the application of high in-plane magnetic fields induces a double sign inversion of the thermoelectric effect, which exhibits large values even at applied fields twice the superconducting critical field.

cond-mat.supr-con

Dynamics and reversible control of the vortex Bloch-point vortex domain wall in short cylindrical magnetic nanowires

Fast and efficient switching of nanomagnets is one of the main challenges in the development of future magnetic memories. We numerically investigate the evolution of the static and dynamic spin wave (SW) magnetization in short (50-400 nm length and 120 nm diameter) cylindrical ferromagnetic nanowires, where competing single vortex (SV) and vortex domain wall with a Bloch point (BP-DW) magnetization configurations could be formed. For a limited nanowire length range (between 150 and 300 nm) we demonstrate a reversible microwave field induced (forward) and opposite spin currents (backwards) transitions between the topologically different SV and BP-DW states. By tuning the nanowire length, excitation frequency, the microwave pulse duration and the spin current values we show that the optimum (low power) manipulation of the BP-DW could be reached by a microwave excitation tuned to the main SW mode and for nanowire lengths around 230-250 nm, where single vortex domain wall magnetization reversal via nucleation and propagation of SV-DW takes place. An analytical model for dynamics of the Bloch point provides an estimation of the gyrotropic mode frequency close the one obtained via micromagnetic simulations. A practical implementation of the method on a device has been proposed involving microwave excitation and the generation of the opposite spin currents via spin orbit torque. Our findings open a new pathway for the creation of unforeseen topological magnetic memories.

cond-mat.mes-hall

Complete magnetic control over the superconducting thermoelectric effect

Giant thermoelectric effects are known to arise at the interface between superconductors and strongly polarized ferromagnets, enabling the construction of efficient thermoelectric generators. We predict that the thermopower of such a generator can be completely controlled by a magnetic input signal: Not only can the thermopower be toggled on and off by rotating a magnet, but it can even be entirely reversed. This in situ control diverges from conventional thermoelectrics, where the thermopower is usually fixed by the device design.

cond-mat.supr-con

Edge spin wave transmission through a vertex domain wall in triangular dots

Spin waves (SWs), being usually reflected by domain walls, could also be channeled along them. Edge domain walls yield the interesting, and potentially applicable to real devices property of broadband spin waves confinement to the edges of the structure. Here we investigate through numerical simulations the propagation of quasi one-dimensional spin waves in triangle-shaped amorphous YIG ($Y_3Fe_5O_{12}$) micron sized ferromagnets as a function of the angle aperture. The edge spin waves (ESWs) have been propagated over the corner in triangles of 2 microns side with a fixed thickness of 85 nm. Parameters such as superior vertex angle (in the range of 40$^\circ$-75$^\circ$) and applied magnetic field have been optimized in order to obtain a higher transmission coefficient of the ESWs over the triangle vertex. We observed that for a certain aperture angle for which dominated ESW frequency coincides with one of the localised DW modes, the transmission is maximized near one and the phase shift drops to $π/2$ indicating resonant transmission of ESWs through the upper corner. We compare the obtained results with existing theoretical models. These results could contribute to the development of novel basic elements for spin wave computing.

cond-mat.other

Low-Frequency 1/f Noise Characteristics of Ultra-Thin AlO$_{x}$-Based Resistive Switching Memory Devices with Magneto-Resistive Responses

Low-frequency 1/f voltage noise has been employed to probe stochastic charge dynamics in AlO$_{x}$-based non-volatile resistive memory devices exhibiting both resistive switching (RS) and magneto-resistive (MR) effects. A 1/f$^γ$ noise power spectral density is observed in a wide range of applied voltage biases. By analyzing the experimental data within the framework of Hooge's empirical relation, we found that the Hooge's parameter $α$ and the exponent $γ$ exhibit a distinct variation upon the resistance transition from the low resistance state (LRS) to the high resistance state (HRS), providing strong evidence that the electron trapping/de-trapping process, along with the electric field-driven oxygen vacancy migration in the AlO$_x$ barrier, plays an essential role in the charge transport dynamics of AlO$_x$-based RS memory devices.

cond-mat.mes-hall

Boosting room temperature tunnel magnetoresistance in hybrid magnetic tunnel junctions under electric bias

Spin-resolved electron symmetry filtering is a key mechanism behind giant tunneling magnetoresistance (TMR) in Fe/MgO/Fe and similar magnetic tunnel junctions (MTJs), providing room temperature functionality in modern spin electronics. However, the core process of the electron symmetry filtering breaks down under applied bias, dramatically reducing the TMR above 0.5 V. This strongly hampers the application range of MTJs. To circumvent the problem, resonant tunneling between ferromagnetic electrodes through quantum well states in thin layers has been used so far. This mechanism, however, is mainly effective at low temperatures. Here, a fundamentally different approach is demonstrated, providing a strong TMR boost under applied bias in V/MgO/Fe/MgO/Fe/Co hybrids. This pathway uses spin orbit coupling (SOC) controlled interfacial states in vanadium, which contrary to the V(001) bulk states are allowed to tunnel to Fe(001) at low biases. The experimentally observed strong increase of TMR with bias is modelled using two nonlinear resistances in series, with the low bias conductance of the first (V/MgO/Fe) element being boosted by the SOC-controlled interfacial states, while the conductance of the second (Fe/MgO/Fe) junctions controlled by the relative alignment of the two ferromagnetic layers. These results pave a way to unexplored and fundamentally different spintronic device schemes, with tunneling magnetoresistance uplifted under applied electric bias.

cond-mat.mes-hall

Superconductivity assisted change of the perpendicular magnetic anisotropy in V/MgO/Fe junctions

Controlling the perpendicular magnetic anisotropy (PMA) in thin films has received considerable attention in recent years due to its technological importance. PMA based devices usually involve heavy-metal (oxide)/ferromagnetic-metal bilayers, where, thanks to interfacial spin-orbit coupling (SOC), the in-plane (IP) stability of the magnetization is broken. Here we show that in V/MgO/Fe(001) epitaxial junctions with competing in-plane and out-of-plane (OOP) magnetic anisotropies, the SOC mediated interaction between a ferromagnet (FM) and a superconductor (SC) enhances the effective PMA below the superconducting transition. This produces a partial magnetization reorientation without any applied field for all but the largest junctions, where the IP anisotropy is more robust; for the smallest junctions there is a reduction of the field required to induce a complete OOP transition ($H_\text{OOP}$) due to the stronger competition between the IP and OOP anisotropies. Our results suggest that the degree of effective PMA could be controlled by the junction lateral size in the presence of superconductivity and an applied electric field. We also discuss how the $H_\text{OOP}$ field could be affected by the interaction between magnetic stray fields and superconducting vortices. Our experimental findings, supported by numerical modelling of the ferromagnet-superconductor interaction, open pathways to active control of magnetic anisotropy in the emerging dissipation-free superconducting spin electronics.

cond-mat.supr-con

Superconductivity-induced change in magnetic anisotropy in epitaxial ferromagnet-superconductor hybrids with spin-orbit interaction

The interaction between superconductivity and ferromagnetism in thin film superconductor/ferromagnet heterostructures is usually reflected by a change in superconductivity of the S layer set by the magnetic state of the F layers. Here we report the converse effect: transformation of the magnetocrystalline anisotropy of a single Fe(001) layer, and thus its preferred magnetization orientation, driven by the superconductivity of an underlying V layer through a spin-orbit coupled MgO interface. We attribute this to an additional contribution to the free energy of the ferromagnet arising from the controlled generation of triplet Cooper pairs, which depends on the relative angle between the exchange field of the ferromagnet and the spin-orbit field. This is fundamentally different from the commonly observed magnetic domain modification by Meissner screening or domain wall-vortex interaction and offers the ability to fundamentally tune magnetic anisotropies using superconductivity - a key step in designing future cryogenic magnetic memories.

cond-mat.supr-con

Time-Dependent Ginzburg-Landau Simulations of Superconducting Vortices in Three Dimensions

Here we describe a development of computer algorithm to simulate the Time Dependent Ginzburg-Landau equation (TDGL) and its application to understand superconducting vortex dynamics in confined geometries. Our initial motivation to get involved in this task was trying to understand better our experimental measurements on dynamics of superconductors with vortices at high frequencies leading to microwave stimulated superconductivity due to presence of vortex (Lara, et al., Scientific Reports, 59187 (2015)).

cond-mat.supr-con

Interfacial Spin-Orbit Coupling: New Platform for Superconducting Spintronics

Spin-orbit coupling (SOC) is a key interaction in spintronics, allowing an electrical control of spin or magnetization and, vice versa, a magnetic control of electrical current. However, recent advances have revealed much broader implications of SOC that is also central to the design of topological states, including topological insulators, skyrmions, and Majorana fermions, or to overcome the exclusion of two-dimensional ferro-magnetism expected from the Mermin-Wagner theorem. SOC and the resulting emergent interfacial spin-orbit fields are simply realized in junctions through structural inversion asymmetry, while the anisotropy in magnetoresistance (MR) allows for their experimental detection. Surprisingly, we demonstrate that an all-epitaxial ferromagnet/MgO/metal junction with only a negligible MR anisotropy undergoes a remarkable transformation below the superconducting transition temperature of the metal. The superconducting junction has a three orders of magnitude higher MR anisotropy and supports the formation of spin-triplet superconductivity, crucial for superconducting spintronics, and topologically-protected quantum computing. Our findings call for revisiting the role of SOC in other systems which, even when it seems negligible in the normal state, could have a profound influence on the superconducting response.

cond-mat.supr-con

Magnetic-State Controlled Molecular Vibrational Dynamics at Buried Molecular-Metal Interfaces

Self-assembled molecular structures have been intensively used in molecular electronics and spintronics. However, detailed nature of the interfaces between molecular layers and extended metallic contacts used to bias the real devices remains unclear. Buried interfaces greatly restrict application of standard techniques such as Raman or scanning electron microscopies. Here we introduce low frequency noise spectroscopy as a tool to characterize buried molecular-metal interfaces. We take advantage of vibrational heating of the molecules with incomplete contacts to the interface. Electrons, being the main spin and charge carriers propagating through the interfaces involving self-assembled molecules, interact inelastically with charged atomic ions. Such interactions produce quantum molecular vibrations (phonons). Detailed investigation of both conductance and conductance fluctuations in magnetic tunnel junctions with few nm Perylenetetracarboxylic dianhydride (PTCDA) allows to map vibrational heating at specific biases taking place in 'hot spots' where self-assembled layers weaker contact the metallic electrodes. We follow this effect as a function of PTCDA thickness and find the best molecular-metal order for the lowest (3-5 monolayers) barriers. Moreover, we unveil interplay between spin and phonons at interface showing experimentally and by modelling spin-control over molecular vibrational heating. We find that vibrational heating related low frequency noise essentially depends on the relative alignment of the electrodes with noise changes well beyond expectations from fluctuation-dissipation theorem.

cond-mat.mes-hall

Symmetry broken spin reorientation transition in epitaxial MgO/Fe/MgO layers with competing anisotropies

The observation of perpendicular magnetic anisotropy (PMA) at MgO/Fe interfaces boosted the development of spintronic devices based on ultrathin ferromagnetic layers. Yet, magnetization reversal in the standard magnetic tunnel junctions (MTJs) with competing PMA and in-plane anisotropies remains unclear. Here we report on the field induced nonvolatile broken symmetry magnetization reorientation transition from the in-plane to the perpendicular (out of plane) state at temperatures below 50K. The samples were 10 nm thick Fe in MgO/Fe(100)/MgO as stacking components of V/MgO/Fe/MgO/Fe/Co double barrier MTJs. Micromagnetic simulations with PMA and different second order anisotropies at the opposite Fe/MgO interfaces qualitatively reproduce the observed broken symmetry spin reorientation transition. Our findings open the possibilities to develop multistate epitaxial spintronics based on competing magnetic anisotropies.

cond-mat.mes-hall

Thermally driven inhibition of superconducting vortex avalanches

Complex systems close to their critical state can exhibit abrupt transitions, avalanches, between their metastable states. It is a challenging task to understand the mechanism of the avalanches and control their behavior. Here we investigate microwave (mw) stimulation of avalanches in the so- called vortex matter of type II superconductors, a system of interacting Abrikosov vortices close to the critical (Bean) state. Our main finding is that the avalanche incubation strongly depends on the excitation frequency, a completely unexpected behavior observed close to the so-called depinning frequencies. Namely, the triggered vortex avalanches in Pb superconducting films become effectively inhibited approaching the critical temperature or critical magnetic field when the mw stimulus is close to the vortex depinning frequency. We suggest a simple model explaining the observed counter- intuitive behaviors as a manifestation of the strongly nonlinear dependence of the driven vortex core size on the mw excitation intensity. This paves the way to controlling avalanches in complex systems through their nonlinear response.

cond-mat.supr-con