arXiv subjects

Federico Capasso

Publications and source records attributed to Federico Capasso.

At least 55 records · Page 3Linked to original sources

arXiv2023

All-Optical tunability of metalenses infiltrated with liquid crystals

Metasurfaces have been extensively engineered to produce a wide range of optical phenomena, allowing unprecedented control over the propagation of light. However, they are generally designed as single-purpose devices without a modifiable post-fabrication optical response, which can be a limitation to real-world applications. In this work, we report a nanostructured planar fused silica metalens permeated with a nematic liquid crystal (NLC) and gold nanoparticle solution. The physical properties of embedded NLCs can be manipulated with the application of external stimuli, enabling reconfigurable optical metasurfaces. We report all-optical, dynamic control of the metalens optical response resulting from thermo-plasmonic induced changes of the NLC solution associated with the nematic-isotropic phase transition. A continuous and reversible tuning of the metalens focal length is experimentally demonstrated, with a variation of 80 um (0.16% of the 5 cm nominal focal length) along the optical axis. This is achieved without direct mechanical or electrical manipulation of the device. The reconfigurable properties are compared with corroborating numerical simulations of the focal length shift and exhibit close correspondence.

physics.optics↗

arXiv2022

Point singularity array with metasurfaces

Phase singularities are loci of darkness surrounded by monochromatic light in a scalar field, with applications in optical trapping, super-resolution imaging, and structured light-matter interactions. Although 1D singular structures, such as optical vortices, are the most common due to their robust topological properties, uncommon 0D (point) and 2D (sheet) singular structures can be generated by wavefront-shaping devices such as metasurfaces. Here, using the design flexibility of metasurfaces, we deterministically position ten identical point singularities in a cylindrically symmetric field generated by a single illumination source. The phasefront is inverse-designed using phase gradient maximization with an automatically-differentiable propagator. This process produces tight longitudinal intensity confinement. The singularity array is experimentally realized with a 1 mm diameter TiO2 metasurface. One possible application is blue-detuned neutral atom trap arrays, for which this light field would enforce 3D confinement and a potential depth around 0.22 mK per watt of incident trapping laser power. Metasurface-enabled point singularity engineering may significantly simplify and miniaturize the optical architecture required to produce super-resolution microscopes and dark traps.

physics.optics↗

arXiv2022

Roadmap on spatiotemporal light fields

Spatiotemporal sculpturing of light pulse with ultimately sophisticated structures represents the holy grail of the human everlasting pursue of ultrafast information transmission and processing as well as ultra-intense energy concentration and extraction. It also holds the key to unlock new extraordinary fundamental physical effects. Traditionally, spatiotemporal light pulses are always treated as spatiotemporally separable wave packet as solution of the Maxwell's equations. In the past decade, however, more generalized forms of spatiotemporally nonseparable solution started to emerge with growing importance for their striking physical effects. This roadmap intends to highlight the recent advances in the creation and control of increasingly complex spatiotemporally sculptured pulses, from spatiotemporally separable to complex nonseparable states, with diverse geometric and topological structures, presenting a bird's eye viewpoint on the zoology of spatiotemporal light fields and the outlook of future trends and open challenges.

physics.optics↗

arXiv2022

Topologically protected four-dimensional optical singularities

Optical singularities play a major role in modern optics and are frequently deployed in structured light, super-resolution microscopy, and holography. While phase singularities are uniquely defined as locations of undefined phase, polarization singularities studied thus far are either partial, i.e., bright points of well-defined polarization, or unstable for small field perturbations. We demonstrate for the first time a complete, topologically protected polarization singularity; it is located in the 4D space spanned by the three spatial dimensions and the wavelength and is created in the focus of a cascaded metasurface-lens system. The field Jacobian plays a key role in the design of such higher-dimensional singularities, which can be extended to multidimensional wave phenomena, and pave the way to novel applications in topological photonics and precision sensing.

physics.optics↗

arXiv2022

D-Flat: A Differentiable Flat-Optics Framework for End-to-End Metasurface Visual Sensor Design

Optical metasurfaces are planar substrates with custom-designed, nanoscale features that selectively modulate incident light with respect to direction, wavelength, and polarization. When coupled with photodetectors and appropriate post-capture processing, they provide a means to create computational imagers and sensors that are exceptionally small and have distinctive capabilities. We introduce D-Flat, a framework in TensorFlow that renders physically-accurate images induced by metasurface optical systems. This framework is fully differentiable with respect to metasurface shape and post-capture computational parameters and allows simultaneous optimization with respect to almost any measure of sensor performance. D-Flat enables simulation of millimeter to centimeter diameter metasurfaces on commodity computers, and it is modular in the sense of accommodating a variety of wave optics models for scattering at the metasurface and for propagation to photosensors. We validate D-Flat against symbolic calculations and previous experimental measurements, and we provide simulations that demonstrate its ability to discover novel computational sensor designs for two applications: single-shot depth sensing and single-shot spatial frequency filtering.

physics.optics↗

arXiv2022

Semiconductor ring laser frequency combs with active directional couplers

Rapid development of Fabry-Perot quantum cascade laser frequency combs has converted them from laboratory devices to key components of next-generation fast molecular spectrometers. Recently, free-running ring quantum cascade lasers allowed generation of new frequency comb states induced by phase turbulence. In absence of efficient light outcoupling, ring quantum cascade lasers are not suited for applications as they are limited in their power output to microwatt levels. Here we demonstrate electrically pumped ring quantum cascade lasers with integrated active directional couplers. These devices generate self-starting frequency combs and have output power above ten milliwatts at room temperature. We study the transmission of the ring-waveguide resonator system below the lasing threshold, which reveals the ability to individually control the mode indices in the coupled resonators, their quality factors, and the coupling coefficient. When the ring resonator is pumped above the lasing threshold, the intracavity unidirectional single-mode field parametrically amplifies an externally injected signal tuned into one of the ring resonances, generating an idler sideband via four-wave mixing. The ability to inject external optical signals into integrated laser cavities brings into reach coherent control of frequency comb states in ring semiconductor lasers. Furthermore, tunable coupled active resonators pumped below the lasing threshold enable a versatile platform for the studies of resonant electromagnetic effects, ranging from strong coupling to parity-time symmetry breaking.

physics.optics↗

arXiv2022

Resonators with tailored optical path by cascaded-mode conversions

Optical resonators enable the generation, manipulation, and storage of electromagnetic waves. They are widely used in technology and fundamental research, in telecommunications, lasers and nonlinear optics, ultra-sensitive measurements in cavity optomechanics, and the study of light-matter interactions in the context of cavity QED. The physics underlying their operation is determined by the constructive interference of electromagnetic waves at specific frequencies, giving rise to the resonance spectrum. This mechanism causes the limitations and trade-offs of resonator design, such as the difficulty of confining waves larger than the resonator and the fixed relationship between free spectral range, modal linewidth, and the resonator's refractive index and size. Here, we introduce a new class of optical resonators, generating resonances by designing the optical path through transverse mode coupling in a cascaded process created by mode-converting mirrors. The generalized round-trip phase condition leads to resonator characteristics that are markedly different from Fabry-Perot resonators and can be tailored over a wide range, such as the largest resonant wavelength, the free spectral range, the linewidth, and the quality factor. We confirm the existence of these modes experimentally in an integrated waveguide cavity with mode converters coupling two transverse modes into one supermode. The resonance signature of the cascaded-mode resonator is a spectrum resulting from the coherent superposition of the coupled transverse modes. We also demonstrate a transverse mode-independent transmission through the resonator and show that its engineered spectral properties agree with theoretical predictions. Cascaded-mode resonators introduce properties not found in traditional resonators and provide a mechanism to overcome the existing trade-offs in the design of resonators in various application areas.

physics.optics↗

arXiv2022

A quantum cascade laser-pumped molecular laser tunable over 1 THz

By introducing methyl fluoride (CH$_3$F) as a new gain medium for a quantum cascade laser-pumped molecular laser (QPML), we demonstrate continuous-wave lasing from more than 120 discrete transitions spanning the frequency range 0.25 to 1.3 THz. The unprecedented degree of spectral tuning achieved with CH$_3$F also confirms the universality of the QPML concept: for all polar gas molecules, lasing can be induced on any dipole-allowed rotational transition by sufficient pumping of a related roto-vibrational transition using a continuously tunable quantum cascade laser.

physics.optics↗

arXiv2022

Multi-line lasing in the broadly tunable ammonia quantum cascade laser pumped molecular laser

Gaseous ammonia has previously been demonstrated as a compelling gain medium for a quantum cascade laser pumped molecular laser (QPML), exhibiting good power efficiency but limited tunability. Here we explore the potential of the ammonia QPML to produce powerful, broadly tunable terahertz frequency lasing on rotational and pure inversion transitions. After theoretically predicting possible laser frequencies, pump thresholds, and efficiencies, we experimentally demonstrate unprecedented tunability -- from 0.762 to more than 4.5 THz -- by pumping Q- and R-branch infrared transitions with widely tunable quantum cascade lasers. We additionally demonstrate two types of multi-line lasing: simultaneous pure inversion and rotation-inversion transitions from the same pumped rotational state, and cascaded lasing involving transitions below the pumped rotational state. We report single frequency power levels as great as 0.33 mW from a low volume laser cavity.

physics.optics↗

arXiv2021

End-to-end metasurface inverse design for single-shot multi-channel imaging

We introduce end-to-end metaoptics inverse design for multi-channel imaging: reconstruction of depth, spectral and polarization channels from a single-shot monochrome image. The proposed technique integrates a single-layer metasurface frontend with an efficient Tikhonov reconstruction backend, without any additional optics except a grayscale sensor. Our method yields multi-channel imaging by spontaneous demultiplexing: the metaoptics front-end separates different channels into distinct spatial domains whose locations on the sensor are optimally discovered by the inverse-design algorithm. We present large-area metasurface designs, compatible with standard lithography, for multi-spectral imaging, depth-spectral imaging, and ``all-in-one'' spectro-polarimetric-depth imaging with robust reconstruction performance ($\lesssim 10\%$ error with 1\% detector noise). In contrast to neural networks, our framework is physically interpretable and does not require large training sets. It can be used to reconstruct arbitrary three-dimensional scenes with full multi-wavelength spectra and polarization textures.

physics.optics↗

arXiv2021

Gigahertz free-space electro-optic modulators based on Mie resonances

Electro-optic modulators from non-linear $χ^{(2)}$ materials are essential for sensing, metrology and telecommunications because they link the optical domain with the microwave domain. At present, most geometries are suited for fiber applications. In contrast, architectures that modulate directly free-space light at gigahertz (GHz) speeds have remained very challenging, despite their dire need for active free-space optics, in diffractive computing or for optoelectronic feedback to free-space emitters. They are typically bulky or suffer from much reduced interaction lengths. Here, we employ an ultrathin array of sub-wavelength Mie resonators that support quasi bound states in the continuum (BIC) as a key mechanism to demonstrate electro-optic modulation of free-space light with high efficiency at GHz speeds. Our geometry relies on hybrid silicon-organic nanostructures that feature low loss ($Q = $ 550 at $λ_{res} = 1594$ nm) while being integrated with GHz-compatible coplanar waveguides. We maximize the electro-optic effect by using high-performance electro-optic molecules (whose electro-optic tensor we engineer in-device to exploit $r_{33} = 100$ pm/V) and by nanoscale optimization of the optical modes. We demonstrate both DC tuning and high speed modulation up to 5~GHz ($f_{EO,-3 dB} =3$ GHz) and shift the resonant frequency of the quasi-BIC by $Δλ_{res}=$11 nm, surpassing its linewidth. We contrast the properties of quasi-BIC modulators by studying also guided mode resonances that we tune by $Δλ_{res}=$20 nm. Our approach showcases the potential for ultrathin GHz-speed free-space electro-optic modulators.

physics.optics↗

arXiv2021

Inverse design enables large-scale high-performance meta-optics reshaping virtual reality

Meta-optics has achieved major breakthroughs in the past decade; however, conventional forward design faces challenges as functionality complexity and device size scale up. Inverse design aims at optimizing meta-optics design but has been currently limited by expensive brute-force numerical solvers to small devices, which are also difficult to realize experimentally. Here, we present a general inverse design framework for aperiodic large-scale complex meta-optics in three dimensions, which alleviates computational cost for both simulation and optimization via a fast-approximate solver and an adjoint method, respectively. Our framework naturally accounts for fabrication constraints via a surrogate model. In experiments, we demonstrate, for the first time, aberration-corrected metalenses working in the visible with high numerical aperture, poly-chromatic focusing, and large diameter up to centimeter scale. Such large-scale meta-optics opens a new paradigm for applications, and we demonstrate its potential for future virtual-reality platforms by using a meta-eyepiece and a laser back-illuminated micro-Liquid Crystal Display.

physics.optics↗

arXiv2021

Spectrally resolved linewidth enhancement factor of a semiconductor frequency comb

The linewidth enhancement factor (LEF) has recently moved into the spotlight of research on frequency comb generation in semiconductor lasers. Here we present a novel modulation experiment, which enables the direct measurement of the spectrally resolved LEF in a laser frequency comb. By utilizing a phase-sensitive technique, we are able to extract the LEF for each comb mode. We first investigate and verify this universally applicable technique using Maxwell-Bloch simulations and then present the experimental demonstration on a quantum cascade laser frequency comb.

physics.optics↗

arXiv2021

Roadmap on multimode light shaping

Our ability to generate new distributions of light has been remarkably enhanced in recent years. At the most fundamental level, these light patterns are obtained by ingeniously combining different electromagnetic modes. Interestingly, the modal superposition occurs in the spatial, temporal as well as spatio-temporal domain. This generalized concept of structured light is being applied across the entire spectrum of optics: generating classical and quantum states of light, harnessing linear and nonlinear light-matter interactions, and advancing applications in microscopy, spectroscopy, holography, communication, and synchronization. This Roadmap highlights the common roots of these different techniques and thus establishes links between research areas that complement each other seamlessly. We provide an overview of all these areas, their backgrounds, current research, and future developments. We highlight the power of multimodal light manipulation and want to inspire new eclectic approaches in this vibrant research community.

physics.optics↗

arXiv2020

Jones matrix holography with metasurfaces

We propose a new class of computer generated holograms whose far fields possess designer-specified polarization response. We dub these Jones matrix holograms. We provide a simple procedure for their implementation using form-birefringent metasurfaces. Jones matrix holography generalizes a wide body of past work with a consistent mathematical framework, particularly in the field of metasurfaces, and suggests previously unrealized devices, examples of which are demonstrated here. In particular, we demonstrate holograms whose far-fields implement parallel polarization analysis and custom waveplate-like behavior.

physics.optics↗

arXiv2020

High quality factor polariton resonators using van der Waals materials

We present high quality factor optical nanoresonators operating in the mid-IR to far-IR based on phonon polaritons in van der Waals materials. The nanoresonators are disks patterned from isotopically pure hexagonal boron nitride (isotopes 10B and 11B) and α-molybdenum trioxide. We experimentally achieved quality factors of nearly 400, the highest ever observed in nano-resonators at these wavelengths. The excited modes are deeply subwavelength, and the resonators are 10 to 30 times smaller than the exciting wavelength. These results are very promising for the realization of nano-photonics devices such as optical bio-sensors and miniature optical components such as polarizers and filters.

physics.optics↗

arXiv2020

Response to Comment on Widely tunable compact terahertz gas lasers

We recently demonstrated a widely tunable THz molecular laser and reported mathematical formulas and a table for comparing how various molecules would perform as such lasers (Chevalier et al., Science, 15 November 2019, p. 856-860). Here we correct the value of a single parameter used to calculate the table (see Erratum for Chevalier et al.), thereby eliminating the concerns raised by Lampin and Barbieri (Lampin et al., arXiv:2004.04422). We also show that our simplified model for the output THz power is a better approximation than the alternative one proposed in the technical comment.

physics.app-ph↗

arXiv2020

Mode-locked ultrashort pulses from an 8 $μ$m wavelength semiconductor laser

Quantum cascade lasers (QCL) have revolutionized the generation of mid-infrared light. Yet, the ultrafast carrier transport in mid-infrared QCLs has so far constituted a seemingly insurmountable obstacle for the formation of ultrashort light pulses. Here, we demonstrate that careful quantum design of the gain medium and control over the intermode beat synchronization enable transform-limited picosecond pulses from QCL frequency combs. Both an interferometric radio-frequency technique and second-order autocorrelation shed light on the pulse dynamics and confirm that mode-locked operation is achieved from threshold to rollover current. Being electrically pumped and compact, mode-locked QCLs pave the way towards monolithically integrated non-linear photonics in the molecular fingerprint region beyond 6 $μ$m wavelength.

physics.optics↗