arXiv subjects

Fedor Jelezko

Publications and source records attributed to Fedor Jelezko.

At least 37 records · Page 2Linked to original sources

arXiv2026

High-resolution wide-field magnetic imaging with sparse sampling using nitrogen-vacancy centers

Nitrogen-vacancy (NV) centers in diamond enable quantitative magnetic imaging, yet practical implementations must balance spatial resolution against acquisition time (and thus per-pixel sensitivity). Single-NV scanning magnetometry achieves genuine nanoscale resolution, nonetheless requires typically a slow pixel-by-pixel acquisition. Meanwhile, wide-field NV-ensemble microscopy provides parallel readout over a large field of view, however is jointly limited by the optical diffraction limit and the sensor-sample standoff. Here, we present a sparse-sampling strategy for reconstructing high-resolution wide-field images from only a small number of measurements. Using simulated NV-ensemble detection of ac magnetic fields, we show that a mean-adjusted Bayesian estimation (MABE) framework can reconstruct 10000-pixel images from only 25 sampling points, achieving SSIM values exceeding 0.999 for representative smooth field distributions, while optimized dynamical-decoupling pulse sequences yield an approximately twofold improvement in magnetic-field sensitivity. The method further clarifies how sampling patterns and sampling density affect reconstruction accuracy and suggests a route toward faster and more scalable magnetic-imaging architectures that may extend to point-scanning NV sensors and other magnetometry platforms, such as SQUIDs, Hall probes, and magnetic tunnel junctions.

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arXiv2025

Overcoming frequency resolution limits using a solid-state spin quantum sensor

The ability to determine precisely the separation of two frequencies is fundamental to spectroscopy, yet the resolution limit poses a critical challenge: distinguishing two incoherent signals becomes impossible when their frequencies are sufficiently close. Here, we demonstrate a simple and powerful approach, dubbed {\it superresolution quantum sensing}, which experimentally resolves two nearly identical incoherent signals using a solid-state spin quantum sensor. By carefully choosing interrogation times that satisfy the superresolution condition, we eliminate quantum projection noise, overcoming the vanishing distinguishability of signals with near-identical frequencies. This leads to improved resolution, which scales as $t^{-2}$ in comparison to the standard $t^{-1}$ scaling. Together with a greatly reduced classical readout noise assisted by a nuclear spin, we are able to achieve sub-kHz resolution with a signal detection time of 80 microseconds. Our results highlight the potential of quantum sensing to overcome conventional frequency resolution limitations, with broad implications for precision measurements.

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arXiv2025

Room-Temperature Electrical Readout of Spin Defects in van der Waals Materials

Negatively charged boron vacancy ($\mathrm{V_B^-}$) in hexagonal boron nitride (hBN) is the most extensively studied room-temperature quantum spin system in two-dimensional (2D) materials. Nevertheless, the current effective readout of $\mathrm{V_B^-}$ spin states is carried out by systematically optical methods. This limits their exploitation in compact and miniaturized quantum devices, which would otherwise hold substantial promise to address quantum sensing and quantum information tasks. In this study, we demonstrated a photoelectric spin readout technique for $\mathrm{V_B^-}$ spins in hBN. The observed photocurrent signals stem from the spin-dependent ionization dynamics of boron vacancies, mediated by spin-dependent non-radiative transitions to a metastable state. We further extend this electrical detection technique to enable the readout of dynamical decoupling sequences, including the Carr-Purcell-Meiboom-Gill (CPMG) protocols, and of nuclear spins via electron-nuclear double resonance. These results provide a pathway toward on-chip integration and real-field exploitation of quantum functionalities based on 2D material platforms.

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arXiv2025

Quantum Memory Enhanced Multipoint Correlation Spectroscopy for Statistically Polarized NMR

Nuclear magnetic resonance spectroscopy with solid-state spin sensors is a promising pathway for the detection of nuclear spins at the micro- and nanoscale. Although many nanoscale experiments rely on a single sensor spin for the detection of the signal, leveraging spin ensembles can enhance sensitivity, particularly in cases in which the signal merely originates from statistically polarized nuclear spins. In this work, we introduce multipoint correlation spectroscopy, that combines the advantages of two well-established methods -- correlation spectroscopy and quantum heterodyne detection -- to enable temporally efficient measurements of statistically polarized samples at the nanoscale with spin ensembles. We present a theoretical framework for this approach and demonstrate an experimental proof of concept with a nitrogen vacancy center in diamond. We achieve single hertz uncertainty in the estimated signal frequency, highlighting the potential applications of the technique for nanoscale nuclear magnetic resonance.

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arXiv2025

High-Fidelity Single-Shot Readout and Selective Nuclear Spin Control for a Spin-1/2 Quantum Register in Diamond

Quantum networks offer a way to overcome the size and complexity limitations of single quantum devices by linking multiple nodes into a scalable architecture. Group-IV color centers in diamond, paired with long-lived nuclear spins, have emerged as promising building blocks demonstrating proof-of-concept experiments such as blind quantum computing and quantum-enhanced sensing. However, realizing a large-scale electro-nuclear register remains a major challenge. Here we establish the germanium-vacancy (GeV) center as a viable platform for such network nodes. Using correlation spectroscopy, we identify single nuclear spins within a convoluted spin environment, overcoming limitations imposed by the color center's spin-$1/2$ nature and thereby enabling indirect control of these nuclear spins. We further demonstrate high-fidelity single-shot readout of both the GeV center ($95.8\,\%$) and a neighboring ${}^{13}\text{C}$ nuclear spin ($93.7\,\%$), a key tool for feed-forward error correction. These critical advances position the GeV center as a compelling candidate for next-generation quantum network nodes.

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arXiv2025

Weak convexity of Fisher information matrix and superresolved localization of blinking sources of light

A group of techniques known by the general name of single-molecule localization microscopy reaches a nanometer-scale spatial resolution of point light emitters, well below the diffraction limit of the traditional microscopy. The key feature of these techniques is blinking, alternation of bright and dark states, of each emitter so that no more than one emitter is bright within the width of the point-spread function of the microscope during a time sufficient for its localization. We give a formulation of the optical part of these techniques in terms of quantum metrology, where the limit of precision is determined by the Fisher information on the emitters positions contained in the measurement data. We show that the advantage in resolution provided by making the emitters blink is a consequence of the fundamental property of Fisher information, its convexity. In particular, we prove the weak matrix convexity and the trace convexity of the Fisher information matrix -- two fundamental results in the multiparameter estimation theory. We show also that the advantage in information is inherent to the quantum state of light itself before the measurement and is related to the convexity of the quantum Fisher information matrix.

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arXiv2025

Quantum Sensing Enhancement through a Nuclear Spin Register in Nitrogen-Vacancy Centers in Diamond

Quantum sensing has seen rapid progress from laboratory research to real-world applications. Solid-state spin systems, particularly nitrogen-vacancy (NV) centers in diamond, are attractive for their ability to operate at room temperature with high sensitivity. However, electron spin coherence due to noise from the surrounding spin bath and this environment effect limits the sensitivity of NV centers. Thus, a critical task in NV center-based quantum sensing is sensitivity enhancement through coherence protection. Nuclear spin assisted protocols have demonstrated greater enhancement of electron spin coherence due to the naturally occurring electron and nuclear spin pair. The longer nuclear coherence times allow for long-lived memory bit for quantum information protocols. This review discusses the physics of NV centers, the mechanisms and variations of nuclear spin-assisted protocols, and their applications in nuclear spin spectroscopy, atomic imaging, and magnetic sensing. Challenges in sensitivity enhancement, commercialization prospects, and future research directions are also explored.

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arXiv2025

Optimization and characterization of laser excitation for quantum sensing with single nitrogen-vacancy centres

In this work we present a comprehensive method of characterization and optimization of laser irradiation within a confocal microscope tailored to quantum sensing experiments using nitrogen-vacancy (NV) centres. While confocal microscopy is well-suited for such experiments, precise control and understanding of several optical parameters are essential for reliable single-emitter studies. We investigate the laser beam intensity profile, single-photon emission statistics, fluorescence response under varying polarization and saturation conditions, spectral characteristics, and the temporal profiles of readout and reinitialization pulses. The beam quality is assessed using the beam propagation factor $M^2$, determined via the razorblade technique. Optical fluorescence spectrum is recorded to confirm NV centre emission. To confirm single-emitter operation, we measure second-order autocorrelation function $g^{(2)}(τ)$. Saturation behaviour is analysed by varying laser power and recording the corresponding fluorescence, while polarization dependence is studied using a half-wave ($λ/2$) plate. Temporal laser pulse profile is examined by modulating the power of an acousto-optic modulator. After optimizing all relevant parameters, we demonstrate the microscope's capabilities in driving spin transitions of a single NV centre. This work establishes a straightforward and effective protocol for laser excitation optimization, enhancing the performance and reliability of NV-based quantum sensors.

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arXiv2025

High-Fidelity Electron Spin Gates for Scaling Diamond Quantum Register

Diamond is a promising platform for quantum information processing as it can host highly coherent qubits that could allow for the construction of large quantum registers. A prerequisite for such devices is a coherent interaction between nitrogen vacancy (NV) electron spins. Entanglement between dipolar-coupled NV spin pairs has been demonstrated, but with a limited entanglement fidelity and its error sources have not been characterized. Here, we design and implement a robust, easy to implement entangling gate between NV spins in diamond and quantify the influence of multiple error sources on the gate performance. Experimentally, we demonstrate a record gate fidelity of $F=(96.0 \pm 2.5)$ % under ambient conditions. Our identification of the dominant errors paves the way towards NV-NV gates beyond the error correction threshold.

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arXiv2025

Extending and measuring dephasing times of nuclear spins in NV centers of diamond

Long coherence times rank among the most important performance measures for many different types of quantum technology. In NV centers of diamond, the nuclear spins provide particularly long dephasing times. However, since initialization and readout require assistance from the electron spin, the apparent dephasing times can be reduced by the electron spin lifetime. Here we propose and implement schemes for measuring and extending the dephasing times of nuclear spins, resulting in dephasing times that are longer than the longitudinal relaxation time $T_{1}$ of the electron spin.

quant-ph↗

arXiv2025

Robust Noise Suppression and Quantum Sensing by Continuous Phased Dynamical Decoupling

We propose and demonstrate experimentally continuous phased dynamical decoupling (CPDD), where we apply a continuous field with discrete phase changes for quantum sensing and robust compensation of environmental and amplitude noise. CPDD does not use short pulses, making it particularly suitable for experiments with limited driving power or nuclear magnetic resonance at high magnetic fields. It requires control of the timing of the phase changes, offering much greater precision than the Rabi frequency control needed in standard continuous sensing schemes. We successfully apply our method to nanoscale nuclear magnetic resonance and combine it with quantum heterodyne detection, achieving microhertz uncertainty in the estimated signal frequency for a 120 s measurement. Our Letter expands significantly the applicability of dynamical decoupling and opens the door for a wide range of experiments, e.g., in nitrogen-vacancy centers, trapped ions, or trapped atoms.

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arXiv2025

Vector Magnetometry Using Shallow Implanted NV Centers in Diamond with Waveguide-Assisted Dipole Excitation and Readout

On-chip magnetic field sensing with Nitrogen-Vacancy (NV) centers in diamond requires scalable integration of 3D waveguides into diamond substrates. Here, we develop a sensing array device with an ensemble of shallow implanted NV centers integrated with arrays of laser-written waveguides for excitation and readout of NV signals. Our approach enables an easy-to-operate on-chip magnetometer with a pixel size proportional to the Gaussian mode area of each waveguide. The performed continuous wave optically detected magnetic resonance on each waveguide gives an average dc-sensitivity value of $195 \pm 3 {nT}/\sqrt{Hz}$, which can be improved with lock-in-detection or pulsed-microwave sequences. We apply a magnetic field to separate the four NV crystallographic orientations of the magnetic resonance and then utilize a DC current through a straight wire antenna close to the waveguide to prove the sensor capabilities of our device. We reconstruct the complete vector magnetic field in the NV crystal frame using three different NV crystallographic orientations. By knowing the polarization axis of the waveguide mode, we project the magnetic field vector into the lab frame.

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arXiv2025

Coherent Control of a Long-Lived Nuclear Memory Spin in a Germanium-Vacancy Multi-Qubit Node

The ability to process and store information on surrounding nuclear spins is a major requirement for group-IV color center-based repeater nodes. We demonstrate coherent control of a ${}^{13}$C nuclear spin strongly coupled to a negatively charged germanium-vacancy center in diamond with coherence times beyond 2.5s at mK temperatures, which is the longest reported for group-IV defects. Detailed analysis allows us to model the system's dynamics, extract the coupling parameters, and characterize noise. We estimate an achievable memory time of 18.1s with heating limitations considered, paving the way to successful applications as a quantum repeater node.

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arXiv2024

Efficiency of optimal control for noisy spin qubits in diamond

Decoherence is a major challenge for quantum technologies. A way to mitigate its negative impact is by employing quantum optimal control. The decoherence dynamics varies significantly based on the characteristics of the surrounding environment of qubits, consequently affecting the outcome of the control optimization. In this work, we investigate the dependence of the shape of a spin inversion control pulse on the correlation time of the environment noise. Furthermore, we analyze the effects of constraints and optimization options on the optimization outcome and identify a set of strategies that improve the optimization performance. Finally, we present an experimental realization of the numerically-optimized pulses validating the optimization feasibility. Our work serves as a generic yet essential guide to implementing optimal control in the presence of realistic noise, e.g., in nitrogen-vacancy centers in diamond.

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arXiv2024

Robust Nuclear Spin Polarization via Ground-State Level Anti-Crossing of Boron Vacancy Defects in Hexagonal Boron Nitride

Nuclear spin polarization plays a crucial role in quantum information processing and quantum sensing. In this work, we demonstrate a robust and efficient method for nuclear spin polarization with boron vacancy ($\mathrm{V_B^-}$) defects in hexagonal boron nitride (h-BN) using ground-state level anti-crossing (GSLAC). We show that GSLAC-assisted nuclear polarization can be achieved with significantly lower laser power than excited-state level anti-crossing, making the process experimentally more viable. Furthermore, we have demonstrated direct optical readout of nuclear spins for $\mathrm{V_B^-}$ in h-BN. Our findings suggest that GSLAC is a promising technique for the precise control and manipulation of nuclear spins in $\mathrm{V_B^-}$ defects in h-BN.

quant-ph↗

arXiv2024

Gate-set evaluation metrics for closed-loop optimal control on nitrogen-vacancy center ensembles in diamond

A recurring challenge in quantum science and technology is the precise control of their underlying dynamics that lead to the desired quantum operations, often described by a set of quantum gates. These gates can be subject to application-specific errors, leading to a dependence of their controls on the chosen circuit, the quality measure and the gate-set itself. A natural solution would be to apply quantum optimal control in an application-oriented fashion. In turn, this requires the definition of a meaningful measure of the contextual gate-set performance. Therefore, we explore and compare the applicability of quantum process tomography, linear inversion gate-set tomography, randomized linear gate-set tomography, and randomized benchmarking as measures for closed-loop quantum optimal control experiments, using a macroscopic ensemble of nitrogen-vacancy centers in diamond as a test-bed. Our work demonstrates the relative trade-offs between those measures and how to significantly enhance the gate-set performance, leading to an improvement across all investigated methods.

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arXiv2024

$^{13}$C Hyperpolarization with Nitrogen-Vacancy Centers in Micro- and Nanodiamonds for Sensitive Magnetic Resonance Applications

Nuclear hyperpolarization is a known method to enhance the signal in nuclear magnetic resonance (NMR) by orders of magnitude. The present work addresses the $^{13}$C hyperpolarization in diamond micro- and nanoparticles, using the optically-pumped nitrogen-vacancy center (NV) to polarize $^{13}$C spins at room temperature. Consequences of the small particle size are mitigated by using a combination of surface treatment improving the $^{13}$C relaxation ($T_1$) time, as well as that of NV, and applying a technique for NV illumination based on a microphotonic structure. Monitoring the light-induced redistribution of the NV spin state populations with electron paramagnetic resonance, a strong polarization enhancement for the NV spin state is observed in a narrow spectral region corresponding to about 4\% of these defect centers. By combining adjustments to the `PulsePol' sequence and slow sample rotation, the NV-$^{13}$C polarization transfer rate is improved further. The hyperpolarized $^{13}$C NMR signal is observed in particles of 2 $μ$m and 100 nm median sizes, with enhancements over the thermal signal (at 0.29 T magnetic field), of 1500 and 940, respectively. The present demonstration of room-temperature hyperpolarization anticipates the development of agents based on nanoparticles for sensitive magnetic resonance applications.

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arXiv2024

Rapid transform optimisation strategy for decoherence-protected quantum register in diamond

Decoherence-protected spins associated with nitrogen-vacancy color centers in diamond possess remarkable long coherence time, which make them one of the most promising and robust quantum registers. The current demand is to explore practical rapid control strategies for preparing and manipulating the such register. Our work provides all-microwave control strategies optimized using multiple optimization methods to significantly reduce the processing time by $80\%$ with a set of smooth near-zero-endpoints control fields that are shown to be experimentally realizable. Furthermore, we optimize and analyze the robustness of these strategies under frequency and amplitude imperfections of the control fields, during which process we use only $16$ samples to give a fair estimation of the robustness map with $2500$ pixels. Overall, we provide a ready-to-implement recipe to facilitate high-performance information processing via decoherence-protected quantum register for future quantum technology applications.

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