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Francisco Domínguez-Adame

Publications and source records attributed to Francisco Domínguez-Adame.

At least 19 recordsLinked to original sources

Emergent Quantum Geometric Phases in Holey Graphene

In graphene and other two-dimensional materials, periodic modulations of the electron density can significantly alter the energy spectrum and transport properties. Here, we report magnetotransport measurements in encapsulated monolayer graphene with ultra-high-quality patterned periodic antidot lattices that preserve the intrinsic electronic properties of the material. This lithographically defined platform enables controlled access to commensurability and superlattice phenomena at length scales otherwise difficult to achieve. By systematically tuning the lattice dimensions, we reveal a hierarchy of classical commensurability features arising from cyclotron orbits with comparable radii that follow multiple classical trajectories, resulting in broadened resistance peaks beyond the conventional single-orbit picture. Superimposed on these features, we observe pronounced Brown-Zak oscillations arising from the quantum commensurability between the magnetic flux quantum and the unit cell of the engineered Bravais lattices. We demonstrate that the intrinsic geometric phase of our system is directly measurable and show a precise matching of the magnetic field periodicity to the lithographic periodic patterning, where moiré-like electronic spectra can be geometrically generated in single-layer graphene without the need for twist, lattice mismatch, or multilayer stacking. Our results establish nanopatterned graphene as a clean, tunable, and scalable platform for realizing and exploring moiré physics through on-demand real-space design

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Dissociation of one-dimensional excitons by static electric field

The quantum states of an electron-hole pair in one-dimensional semiconductors under a static electric field are theoretically analyzed using a two-band model with on-site Coulomb interaction. In the absence of static field, the electron and hole are always bound, forming an exciton regardless of the Coulomb interaction strength, in contrast to what occurs in higher-dimensional semiconductors. The static field modifies the wave function of the electron-hole pair, turning bound states into continuum states. However, at low static fields, the linear optical spectra resemble those of the unbiased semiconductor, exhibiting a quadratic redshift of the main exciton absorption line as the field increases. When the static field exceeds a critical threshold, the exciton dissociates and the linear optical spectra exhibit signatures of the Wannier-Stark ladder with squally spaced peaks, making them a valuable tool for experimentally probing exciton dissociation.

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Unconventional Floquet topological phases in the SSH lattice

Topological materials, known for their edge states robust against local perturbations, hold promise for next-generation quantum technologies, but remain scarce in nature and challenging to realize in static systems. The Su-Schrieffer-Heeger chain is a one-dimensional system for topological phases, although its static control is limited. To overcome these limitations, we propose to use high-frequency monochromatic driving and modulated amplitude pulses to dynamically induce and switch the Floquet topological phases. Using a Kramers-Henneberger-like transformation, we encode all Floquet sidebands into a single effective Hamiltonian. We demonstrate that both monochromatic and experimental pulse protocols (Gaussian and fast-beating envelopes) can induce topological edge states, enabling dynamic phase switching. Notably, fast-beating modulations require significantly lower field strengths than monochromatic ones, especially with larger inter-dimer separations. Our findings offer an experimentally feasible route for Floquet engineering, paving the way for ultrafast and energy efficient control of topological phases in quantum platforms, opening up new possibilities in the field of dynamic quantum materials.

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Superballistic conduction in hydrodynamic antidot graphene superlattices

Viscous electron flow exhibits exotic signatures such as superballistic conduction. In order to observe hydrodynamics effects, a 2D device where the current flow is as inhomogeneous as possible is desirable. To this end, we build three antidot graphene superlattices with different hole diameters. We measure their electrical properties at various temperatures and under the effect of a perpendicular magnetic field. We find an enhanced superballistic effect, suggesting the effectiveness of the geometry at bending the electron flow. In addition, superballistic conduction, which is related to a transition from a non-collective to a collective regime of transport, behaves non-monotonically with the magnetic field. We also analyze the device resistance as a function of the size of the antidot superlattice to find characteristic scaling laws describing the different transport regimes. We prove that the antidot superlattice is a convenient geometry for realizing hydrodynamic flow and provide valuable explanations for the technologically relevant effects of superballistic conduction and scaling laws.

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Superballistic paradox in electron fluids: Evidence of tomographic transport

Electron hydrodynamics encompasses the exotic fluid-like behavior of electrons in two-dimensional materials such as graphene. It accounts for superballistic conduction, also known as the Gurzhi effect, where increasing temperature reduces the electrical resistance. In analogy with conventional fluids, the Gurzhi effect is only expected in the hydrodynamic regime, with the decrease in the resistance occurring at intermediate temperatures. Nonetheless, experiments on electron fluids consistently show that superballistic conduction starts at close-to-zero temperatures. To address this paradox, we study hydrodynamic flow, and we find that replacing the classical dynamics with tomographic dynamics, where only head-on collisions are allowed between electrons, solves the dilemma. The latter strengthens superballistic conduction, with potential applications in low-dissipation devices, and explains its differences with the Molenkamp effect and conventional fluids dynamics. Our study reveals that the superballistic paradox is resolved by considering the electrons not as classical particles but as fermions.

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Monolayer transition metal dichalcogenides under finite-pulse polarized radiation

Recent advances in time-resolved angle-resolved photoemission spectroscopy have enabled access to ultrafast electron states and their spin dynamics in solids. Atomically thin transition metal dichalcogenides are paradigmatic two-dimensional materials where electron momentum and spin degrees of freedom are coupled, being suitable candidates for time-resolved spectroscopy studies. In this work, we present a thorough study of the electron dynamics when these materials are subject to an intense finite-pulse driving radiation. We extend the scope of the conventional Floquet engineering and rely of the so-called $t-t^{\prime}$ formalism to deal with driving fields described with two distinct time scales, namely the envelope amplitude timescale and the time period of the external field. The interplay between the finite-pulse timescales and the intrinsic properties of the electrons gives rise to transient valley polarization and dynamical modifications of band structures, revealed by the time-dependent circular dichroism of the sample.

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Tuning magnetism in graphene nanoribbons via strain and adatoms

We investigate the impact of strain and adsorbed H adatoms on the magnetic properties of zigzag graphene nanoribbons (ZGNRs) using a combination of tight-binding and density functional theory methods for both, ferromagnetic (FM) and antiferromagnetic edge configurations (AFM). Our study reveals that longitudinal strain induces a significant enhancement in the edge magnetic moment, that we attribute to strain-driven modifications in the band structure. In addition, we describe H~adatoms within the tight-binding approach by employing both an unrelaxed vacancy model and the Anderson impurity model. By comparing to density functional theory results, we corroborate that the Anderson impurity model is best suited to describe H adsorption. We then focus on the metallic FM edge configuration of the ZGNRs to better exploit the tuning of its properties. We find that the magnetic configuration of H~adatoms is strongly influenced by the edges, with an AFM coupling between edges and the H~adatom. In fact, the magnetic spatial pattern of the H adatom differs to that found in graphene due to this edge coupling. Importantly, we find robust discrete plateaus of integer magnetic moment as strain is varied in the defected ZGNRs, that we relate to changes in the band structure, namely, a half-metallic character or the opening of a gap. This behavior can be of interest for magnetic applications of carbon-based nanostructures

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Radiation-induced dynamical formation of Floquet-Bloch bands in Dirac Hamiltonians

Recent experiments, combing ultrafast strong-field irradiation of surfaces with time- and angle-resolved photoemission spectroscopy, allow for monitoring the time-dependent charge carrier dynamics and the build-up of transient sidebands due to the radiation pulses. While these structures are reminiscent of Floquet-Bloch bands, standard Floquet theory is not applicable since it requires a strictly time-periodic driving field. To study the emergence and formation of such sidebands, i.e. to provide a link between common Floquet physics and dynamical mechanisms underlying short driving pulses, we consider a generalization of Floquet theory, the so-called $t-t^{\prime}$ formalism. This approach naturally extents Floquet theory to driving field amplitudes with a superimposed envelope shape. Motivated by experiments we study 2D Dirac Hamiltonians subject to linearly and circularly polarised light waves with a Gaussian field envelope of a few cycles. For these Floquet-Bloch Hamiltonians we study the evolution of their Floquet-Bloch spectra, accompanied by a systematic analysis of the time-dependent (sideband) transitions. We show that sideband occupation requires circularly polarized light for linear Dirac systems such as graphene, while for Dirac models with trigonal warping, describing surface states of topological insulators such as Bi$_2$ Se$_3$, both linearly and circularly polarised pulses induce sideband excitations.

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Alternative routes to electron hydrodynamics

Viscous flow of interacting electrons in two dimensional materials features a bunch of exotic effects. A model resembling the Navier-Stokes equation for classical fluids accounts for them in the so called hydrodynamic regime. We performed a detailed analysis of the physical conditions to achieve electron hydrodynamic transport and found three new alternative routes: favouring frequent inelastic collisions, the application of a magnetic field or a high-frequency electric field. As a mayor conclusion, we show that the conventional requirement of frequent electron-electron collisions is too restrictive and, as a consequence, materials and phenomena to be described using hydrodynamics are widened. In view of our results, we discuss recent experimental evidence on viscous flow and point out alternative avenues to reduce electric dissipation in optimized devices.

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Impact of vacancies on twisted bilayer graphene quantum point contacts

We carry out an extensive numerical study of low-temperature electronic transport in quantum point contacts based on twisted bilayer graphene. Assuming ballistic electron dynamics, quantized plateaus in the conductance are observed in defect-free samples when the twisting angle is large enough. However, plateaus are smeared out and hardly noticeable on decreasing the angle. Close to the magic angle, the conductance around the charge neutrality point drops significantly and the quantization steps visible at higher angles are no longer appreciable. Furthermore, we consider the effects of a random distribution of vacancies on the quantum point contact. Whereas the electron-hole symmetry is broken in pristine samples, we find that this symmetry is restored upon increasing the concentration of vacancies. We explain this effect by a reduction of the effective interlayer coupling due to the presence of the vacancies.

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Anomalous spin textures in a 2D topological superconductor induced by point impurities

Topological superconductors are foreseen as good candidates for the search of Majorana zero modes, where they appear as edge states and can be used for quantum computation. In this context, it becomes necessary to study the robustness and behavior of electron states in topological superconductors when a magnetic or non-magnetic impurity is present. We focus on scattering resonances in the bands and on spin texture to know what the spin behavior of the electrons in the system will be. We find that the scattering resonances appear outside the superconducting gap, thus providing evidence of topological robustness. We also find non-trivial and anisotropic spin textures related to the Dzyaloshinskii-Moriya interaction. The spin textures show a Ruderman-Kittel-Kasuya-Yosida interaction governed by Friedel oscillations. We believe that our results are useful for further studies which consider many-point-impurity scattering or a more structured impurity potential with a finite range.

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Effect of the external fields in high Chern number quantum anomalous Hall insulators

A quantum anomalous Hall state with high Chern number has so far been realized in multiplayer structures consisting of alternating magnetic and undoped topological insulator layers. However, in previous proposals, the Chern number can be only tuned by varying the doping concentration or the width of the magnetic topological insulator layers. This drawback largely restrict the applications of dissipationless chiral edge currents in electronics since the number of conducting channels remains fixed. In this work, we propose a way of varying the Chern number at will in these multilayered structures by means of an external electric field applied along the stacking direction. In the presence of an electric field in the stacking direction, the inverted bands of the unbiased structure coalesce and hybridize, generating new inverted bands and collapsing the previously inverted ones. In this way, the number of Chern states can be tuned externally in the sample, without the need of modifying the number and width of the layers or the doping level. We showed that this effect can be uncovered by the variation of the transverse conductance as a function of the electric field at constant injection energy at the Fermi level.

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Persistence of symmetry-protected Dirac points at the surface of the topological crystalline insulator SnTe upon impurity doping

We investigate the effect of a non-magnetic donor impurity located at the surface of the SnTe topological crystalline insulator. In particular, the changes on the surface states due to a Sb impurity atom are analyzed by means of ab initio simulations of pristine and impurity-doped SnTe. Both semi-infinite and slab geometries are considered within the first-principles approach. Furthermore, minimal and Green's function continuum models are proposed with the same goal. We find that the Dirac cones are shifted down in energy upon doping; this shift strongly depends on the position of the impurity with respect to the surface. In addition, we observe that the width of the impurity band presents an even-odd behavior by varying the position of the impurity. This behavior is related to the position of the nodes of the wave function with respect to the surface, and hence it is a manifestation of confinement effects. We compare slab and semi-infinite geometries within the ab initio approach, demonstrating that the surface states remain gapless and their spin textures are unaltered in the doped semi-infinite system. In the slab geometry, a gap opens due to hybridization of the states localized at opposite surfaces. Finally, by means of a continuum model, we extrapolate our results to arbitrary positions of the impurity, clearly showing a non-monotonic behavior of the Dirac cone.

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Generation and control of non-local chiral currents in graphene superlattices by orbital Hall effect

Graphene-based superlattices offer a new materials playground to exploit and control a higher number of electronic degrees of freedom, such as charge, spin, or valley for disruptive technologies. Recently, orbital effects, emerging in multivalley band structure lacking inversion symmetry, have been discussed as possible mechanisms for developing orbitronics. Here, we report non-local transport measurements in small gap hBN/graphene/hBN moiré superlattices which reveal very strong magnetic field-induced chiral response which is stable up to room temperature. The measured sign dependence of the non-local signal with respect to the magnetic field orientation clearly indicates the manifestation of emerging orbital magnetic moments. The interpretation of experimental data is well supported by numerical simulations, and the reported phenomenon stands as a formidable way of in-situ manipulation of the transverse flow of orbital information, that could enable the design of orbitronic devices.

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Impact of electron-electron interactions on the thermoelectric efficiency of graphene quantum point contacts

Thermoelectric materials open a way to harness dissipated energy and make electronic devices less energy-demanding. Heat-to-electricity conversion requires materials with a strongly suppressed thermal conductivity but still high electronic conduction. This goal is largely achieved with the help of nanostructured materials, even if the bulk counterpart is not highly efficient. In this work, we investigate how thermoelectric efficiency is enhanced by many-body effects in graphene nanoribbons at low temperature. To this end, starting from the Kane-Mele-Hubbard model within a mean-field approximation, we carry out an extensive numerical study of the impact of electron-electron interactions on the thermoelectric efficiency of graphene nanoribbons with armchair or zigzag edges. We consider two different regimes, namely trivial and topological insulator. We find that electron-electron interactions are crucial for the appearance of interference phenomena that give rise to an enhancement of the thermoelectric efficiency of the nanoribbons. Lastly, we also propose an experimental setup that would help to test the validity of our conclusions.

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Fast response photogating in monolayer MoS2 phototransistors

Two-dimensional transition metal dichalcogenide (TMD) phototransistors have been object of intensive research during the last years due to their potential for photodetection. Photoresponse in these devices is typically caused by a combination of two physical mechanisms: photoconductive effect (PCE) and photogating effect (PGE). In earlier literature for monolayer (1L) MoS2 phototransistors PGE is generally attributed to charge trapping by polar molecules adsorbed to the semiconductor channel, giving rise to a very slow photoresponse. Thus, the photoresponse of 1L-MoS2 phototransistors at high-frequency light modulation is assigned to PCE alone. Here we investigate the photoresponse of a fully h-BN encapsulated monolayer (1L) MoS2 phototransistor. In contrast with previous understanding, we identify a rapidly responding PGE mechanism that becomes the dominant contribution to photoresponse under high-frequency light modulation. Using a Hornbeck-Haynes model for the photocarrier dynamics, we fit the illumination power dependence of this PGE and estimate the energy level of the involved traps. The resulting energies are compatible with shallow traps in MoS2 caused by the presence of sulfur vacancies.

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Tailoring topological states of core-shell nanoparticles

In this work we investigate novel spherical core-shell nanoparticles with band inversion. The core and the embedding medium are normal semiconductors while the shell material is assumed to be a topological insulator. The envelope functions are found to satisfy a Dirac-like equation that can be solved in a closed form. The core-shell nanoparticle supports midgap bound states located at both interfaces due to band inversion. These states are robust since they are topologically protected. The energy spectrum presents mirror symmetry due to the chiral symmetry of the Dirac-like Hamiltonian. As a major result, we show that the thickness of the shell acts as an additional parameter for the fine tuning of the energy levels, which paves the way for electronics and optoelectronics applications.

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Rashba coupling and spin switching through surface states of Dirac semimetals

We study the effect of the Rashba spin-orbit coupling on the Fermi arcs of topological Dirac semimetals. The Rashba coupling is induced by breaking the inversion symmetry at the surface. Remarkably, this coupling could be enhanced by the interaction with the substrate and controlled by an external electric field. We study analytically and numerically the rotation of the spin of the surface states as a function of the electron's momentum and the coupling strength. Furthermore, a detailed analysis of the spin-dependent two-terminal conductance is presented in the clean limit and with the addition of a random distribution of impurities. Depending on the magnitude of the quadratic terms in the Hamiltonian, the spin-flip conductance may become dominant, thus showing the potential of the system for spintronic applications, since the effect is robust even in the presence of disorder.

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