arXiv subjects

Frank Vewinger

Publications and source records attributed to Frank Vewinger.

At least 19 recordsLinked to original sources

arXiv2026

Fluctuations of a Photon Bose-Einstein Condensate Coupled to a Reservoir: Describing Coherence Properties in a Free-Energy Model

Photons are mutually nearly noninteracting particles, so thermalized photon ensembles are commonly obtained not from direct particle-particle-interactions but rather from contact with matter, which can constitute a reservoir for the photon gas. We develop a theory model for photons in a material-filled (e.g. liquid dye) optical microcavity, with the aim to study the fluctuation properties using a free-energy description for noninteracting photons coupled to a reservoir of material electronic excitations. To begin with, we use a single mode description for the condensate. For a small relative size of the material reservoir, corresponding to the canonical regime, condensate number fluctuations are small, and the derived free energy landscape takes the usual Mexican-hat shaped form such that spontaneous symmetry breaking occurs. In contrast, for a large relative size of the reservoir, corresponding to the grand canonical regime, fluctuations become as large as the average particle number. We show that the resulting free energy landscape acquires a bowl-shaped form, with a single minimum at the origin. Thus, a macroscopic occupation of the ground state (i.e., Bose-Einstein condensation) in the absence of spontaneous symmetry breaking is expected. We also provide a model for the treatment of a photon gas trapped in a box-shaped potential with spatially distributed coupling to a reservoir. The model predicts, for example, a statistically fluctuating pattern of islands with long-range coherence, resembling transient microcondensates.

cond-mat.quant-gas↗

arXiv2026

Universal critical behavior in ideal Bose-Einstein condensation

Ideal Bose-Einstein condensation (BEC) remains a paradigmatic example of a continuous phase transition and a cornerstone for understanding quantum degenerate bosonic matter. We demonstrate that critical behavior of the ideal Bose gas near the BEC phase transition falls into three distinct classes, determined exclusively by the low-energy scaling of the density of states. Depending on its scaling exponent, which is controlled by dimensionality and confinement, the transition displays either the usual algebraic divergences of thermodynamic susceptibilities, divergent behavior with marginal logarithmic corrections, or a more subtle form of criticality, where only the correlation length diverges. Our work provides a unified framework for criticality in noninteracting bosonic systems. This classification applies broadly to atomic, photonic, polaritonic, and magnonic condensates, where dimensionality, confinement, and spectral engineering can strongly reshape the density of states.

cond-mat.quant-gas↗

arXiv2025

Observation of critical scaling in the Bose gas universality class

Critical exponents characterize the divergent scaling of thermodynamic quantities near phase transitions and allow for the classification of physical systems into universality classes. While quantum gases thermalizing by interparticle interactions fall into the XY model universality class, the ideal Bose gas has been predicted to form a distinct universality class whose signatures have not yet been revealed experimentally. Here, we report the observation of critical scaling in a two-dimensional quantum gas of essentially noninteracting photons, which thermalize by radiative contact to a reservoir of molecules inside a microcavity. By measuring the spatial correlations near the condensation transition, we determine the critical exponent for the correlation length to be $\nu = 0.52(3)$. Our results constitute a first experimental test of the long-standing scaling predictions for the Bose gas universality class.

cond-mat.quant-gas↗

arXiv2025

3D micro-printing: An enabling technique for arbitrary potential landscapes for photonic quantum-gases

Photonic quantum gases explore the physics of open driven-dissipative quantum systems under ambient conditions and thus open access to thermodynamics and transport phenomena in quantum gases in the weakly interacting regime. Here we introduce the technology of 3D micro-printing to create potential landscapes for photonic quantum gases in dye-filled micro cavities, which surpass the current state of the art in terms of potential size and definition, potential depth, coupling strength, and number of coupled potentials by at least an order of magnitude. We realize as demonstration of the capabilities box potentials with rectangular side walls, anisotropic harmonic potentials, double-well potentials with dimensions on the scale of the wavelength of light as well as potential lattices with topological non-trivial properties. This approach paves the way for experimentally studying the physics of open quantum systems on lattices and might find applications in solving complex ground-state problems like the XY-model.

quant-ph↗

arXiv2025

An optical frequency shifter based on continuous-wave pump fields

Practical implementations of quantum information networks require frequency conversion of individual photons. Approaches based on a molecular gas as the nonlinear medium cover a wide range of the optical spectrum and promise high efficiency at negligible background. We present polarization-preserving frequency conversion in a hydrogen-loaded hollow core fiber using continuous-wave pump fields. We demonstrate conversion efficiency at the level of a few per mille, discuss various limitations and loss mechanisms, and present a route to increase conversion efficiency to near unity.

quant-ph↗

arXiv2025

Polarization properties of photon Bose-Einstein condensates

The first experimental realization of a photon Bose-Einstein condensate was demonstrated more than a decade ago. However, the polarization of the condensate has not been fully understood and measured in this weakly driven-dissipative system. In this letter, we experimentally investigate the polarization of thermal and condensed light depending on the power and polarization of the pump beam. With full control over the polarization of the pump, it is possible to create arbitrary states on the surface of the Poincar\'e sphere. We show that, in agreement with previous theoretical work, there is a remarkable increase in the polarization strength of the condensate above the threshold for a fully linearly polarized pump. Above a certain threshold also the degenerate orthogonal polarized state of the cavity is occupied, limiting the degree of polarization to approximately 90%.

quant-ph↗

arXiv2025

One- and two-photon spectroscopy with a test of the Kennard-Stepanov relation in high-pressure two-species xenon-noble gas mixtures

Between the absorption and the emission spectral lineshapes of dense atomic and molecular media, such as dye solutions and alkali-noble buffer gas mixtures at high pressure, in many cases there exists a universal scaling, the Kennard-Stepanov relation, which is a manifestation of detailed balance. This relation plays a crucial role in recent Bose-Einstein condensation experiments of visible-spectral-photons in e.g.~dye-solution-filled optical microcavities. It has recently been proposed to use high-pressure xenon-noble gas mixtures as a thermalization medium for vacuum-ultraviolet regime photons, so as to extend the achievable wavelength range of such Bose-Einstein-condensed optical sources from the visible to the vacuum-ultraviolet regime. In this work, we report two-photon excitation spectroscopy measurements of ground state ($5p^6$) xenon atoms subject to up to 80bar of helium or krypton buffer gas pressure, respectively, in the 220-260nm wavelength range. The study of such two-photon spectra is of interest e.g.~for the exploration of possible pumping schemes of a future vacuum-ultraviolet photon Bose-Einstein condensate. We have also recorded absorption and emission spectra of the $5p^6 \leftrightarrow 5p^56s$ single-photon transition near 147nm wavelength of xenon atoms subject to 80bar of krypton buffer gas pressure. We find that the ratio of absorption and emission shows a Kennard-Stepanov scaling, which suggests that such gas mixtures are promising candidates as a thermalization medium for a Bose-Einstein condensate of vacuum-ultraviolet photons.

physics.optics↗

arXiv2025

Time-periodic driving of a bath-coupled open quantum gas of light

We study the frequency-resolved density response of a photon Bose-Einstein condensate coupled to a bath of dye molecules by time-periodic driving. By monitoring the photon number dynamics for different drive frequencies, we obtain the spectral response of the condensate in a phase-sensitive way. We find that as the photon number increases, the response of the coupled condensate-bath system transitions from overdamped to resonant behavior, indicating a transition from closed to open system dynamics. Our spectroscopy method paves the way for studies of collective excitations in complex driven-dissipative systems.

cond-mat.quant-gas↗

arXiv2025

Frequency conversion in a hydrogen-filled hollow-core fiber: power scaling, background, and bandwidth

Large-area quantum networks based on optical fibers allow photons at near-infrared wavelengths to travel with minimal loss. Quantum frequency conversion is a method to alter the wavelength of a single photon while maintaining its quantum state. Most commonly, nonlinear crystals are employed for this conversion process, where near-unity conversion efficiency at high fidelity has been demonstrated. Still, the crystal-based conversion process is plagued by strong background noise, very limited spectral bandwidth, and inhomogeneous temperature profiles at strong pump fields. In previous work, we have demonstrated frequency conversion in hydrogen-filled hollow-core fibers and claimed that this conversion process does not compromise performance at strong pump fields, is essentially free of background noise, and intrinsically broadband. Here, we demonstrate that these three claims are justified.

quant-ph↗

arXiv2024

Thermodynamics and State Preparation in a Two-State System of Light

The coupling of two-level quantum systems to the thermal environment is a fundamental problem, with applications ranging from qubit state preparation to spin models. However, for the elementary problem of the thermodynamics of an ensemble of bosons populating a two-level system despite its conceptual simplicity experimental realizations are scarce. Using an optical dye microcavity platform, we thermalize photons in a two-mode system with tunable chemical potential, demonstrating N bosons populating a two-level system coupled to a heat bath. Under pulsed excitation, Josephson oscillations between the two quantum states demonstrate the possibility for coherent manipulation. In contrast, under stationary conditions the thermalization of the two-mode system is observed. As the energetic splitting between eigenstates is two orders of magnitude smaller than thermal energy, at low occupations an almost equal distribution of the modes occupation is observed, as expected from Boltzmann statistics. For larger occupation, we observe efficient population of the ground state and saturation of the upper level at high filling, expected from quantum statistics. Our experiment holds promise for state preparation in quantum technologies as well as for quantum thermodynamics studies.

cond-mat.quant-gas↗

arXiv2024

Frequency conversion in a hydrogen-filled hollow-core fiber using continuous-wave fields

In large-area quantum networks based on optical fibers, photons are the fundamental carriers of information as so-called flying qubits. They may also serve as the interconnect between different components of a hybrid architecture, which might comprise atomic and solid state platforms operating at visible or near-infrared wavelengths, as well as optical links in the telecom band. Quantum frequency conversion is the pathway to change the color of a single photon while preserving its quantum state. Currently, nonlinear crystals are utilized for this process. However, their performance is limited by their acceptance bandwidth, tunability, polarization sensitivity, as well as undesired background emission. A promising alternative is based on stimulated Raman scattering in gases. Here, we demonstrate polarization-preserving frequency conversion in a hydrogen-filled anti-resonant hollow-core fiber. This approach holds promises for seamless integration into optical fiber networks and interfaces to single emitters. Disparate from related experiments that employ a pulsed pump field, we here take advantage of two coherent continuous-wave pump fields.

quant-ph↗

arXiv2024

Observation of Nonlinear Response and Onsager Regression in a Photon Bose-Einstein Condensate

The quantum regression theorem states that the correlations of a system at two different times are governed by the same equations of motion as the temporal response of the average values. Such a relation provides a powerful framework for the investigation of physical systems by establishing a formal connection between intrinsic microscopic behaviour and a macroscopic 'effect' due to an external 'cause'. Measuring the response to a controlled perturbation in this way allows to determine, for example, structure factors in condensed matter systems as well as other correlation functions of material systems. Here we experimentally demonstrate that the two-time particle number correlations in a photon Bose-Einstein condensate inside a dye-filled microcavity exhibit the same dynamics as the response of the condensate to a sudden perturbation of the dye molecule bath. This confirms the regression theorem for a quantum gas and, moreover, establishes a test of this relation in an unconventional form where the perturbation acts on the bath and only the condensate response is monitored. For strong perturbations, we observe nonlinear relaxation dynamics which our microscopic theory relates to the equilibrium fluctuations, thereby extending the regression theorem beyond the regime of linear response. The demonstrated nonlinearity of the condensate-bath system paves the way for studies of novel elementary excitations in lattices of driven-dissipative photon condensates.

cond-mat.quant-gas↗

arXiv2024

Frequency conversion to the telecom O-band using pressurized hydrogen

Large-scale quantum networks rely on optical fiber networks and photons as so-called flying qubits for information transport. While dispersion and absorption of optical fibers are minimum at the infrared telecom wavelengths, most atomic and solid state platforms operate at visible or near-infrared wavelengths. Quantum frequency conversion is required to bridge these two wavelength regimes, and nonlinear crystals are currently employed for this process. Here, we report on a novel approach of frequency conversion to the telecom band. This interaction is based on coherent Stokes Raman scattering (CSRS), a four-wave mixing process resonantly enhanced in a dense molecular hydrogen gas. We show the conversion of photons from \SI{863}{\nano\meter} to the telecom O-Band and demonstrate that the input polarization state is preserved. This process is intrinsically broad-band and can be adapted to any other wavelength.

quant-ph↗

arXiv2023

Bose-Einstein Condensation of Photons in a Four-Site Quantum Ring

Thermalization of radiation by contact to matter is a well-known concept, but the application of thermodynamic methods to complex quantum states of light remains a challenge. Here we observe Bose-Einstein condensation of photons into the hybridized ground state of a four-site ring potential with coherent tunnel couplings. In our experiment, the periodically-closed ring lattice superimposed by a weak harmonic trap for photons is realized inside a spatially structured dye-filled microcavity. Photons thermalize to room temperature, and above a critical photon number macroscopically occupy the symmetric linear combination of the site eigenstates with zero phase winding, which constitutes the ground state of the system. The mutual phase coherence of photons at different lattice sites is verified by optical interferometry.

cond-mat.quant-gas↗

arXiv2023

Dimensional Crossover in a Quantum Gas of Light

The dimensionality of a system profoundly influences its physical behaviour, leading to the emergence of different states of matter in many-body quantum systems. In lower dimensions, fluctuations increase and lead to the suppression of long-range order. For example, in bosonic gases, Bose-Einstein condensation (BEC) in one dimension requires stronger confinement than in two dimensions. We experimentally study the properties of a harmonically trapped photon gas undergoing Bose-Einstein condensation along the dimensional crossover from one to two dimensions. The photons are trapped in a dye microcavity where polymer nanostructures provide the trapping potential for the photon gas. By varying the aspect ratio of the harmonic trap, we tune from an isotropic two-dimensional confinement to an anisotropic, highly elongated one-dimensional trapping potential. Along this transition we determine the caloric properties of the photon gas and find a softening of the second-order Bose-Einstein condensation phase transition observed in two dimensions to a crossover behaviour in one dimension.

cond-mat.quant-gas↗

arXiv2023

Two-photon excitation and absorption spectroscopy of gaseous and supercritical xenon

Spectroscopy of gases under high-pressure conditions is of interest in various fields such as plasma physics and astrophysics. Recently, it has also been proposed to utilize a high-pressure noble gas environment as a thermalization medium to extend the wavelength range of photon Bose-Einstein condensates to the vacuum-ultraviolet regime, from the presently accessible visible and near-infrared spectral regimes. In this work, we report on experimental results of two-photon spectroscopy of gaseous and supercritical xenon for pressures as high as $95 \; \text{bar}$, probing the transitions from the $5p^6$ electronic ground-state to the $5p^56p$ and $5p^56p^\prime$ excited-state configurations. Aiming at the exploration of possible pumping schemes for future vacuum-ultraviolet photon condensates, we have recorded degenerate two-photon excitation spectra of such dense xenon samples. In further measurements, we have investigated whether irradiation of an auxiliary light field can enhance the reabsorption of the emission on the second excimer continuum of xenon, which is subject to a large Stokes shift. To this end, absorption measurements have been conducted, driving the $5p^6 \rightarrow 5p^56p$ two-photon transitions nondegenerately.

quant-ph↗

arXiv2023

Fluctuation-dissipation relation for a Bose-Einstein condensate of photons

For equilibrium systems, the magnitude of thermal fluctuations is closely linked to the dissipative response to external perturbations. This fluctuation-dissipation relation has been described for material particles in a wide range of fields. Here we experimentally probe the relation between the number fluctuations and the response function for a Bose-Einstein condensate of photons coupled to a dye reservoir, demonstrating the fluctuation-dissipation relation for a quantum gas of light. The observed agreement of the scale factor with the environment temperature both directly confirms the thermal nature of the optical condensate and demonstrates the validity of the fluctuation-dissipation theorem for a Bose-Einstein condensate.

cond-mat.quant-gas↗

arXiv2022

Frequency Conversion in High-Pressure Hydrogen

State-preserving frequency conversion in the optical domain is a necessary component in many configurations of quantum information processing and communication. Thus far, nonlinear crystals are used for this purpose. Here, we report on a new approach based on coherent anti-Stokes Raman scattering (CARS) in a dense molecular hydrogen gas. This four-wave mixing process sidesteps the limitations imposed by crystal properties, it is intrinsically broadband and does not generate an undesired background. We demonstrate this method by converting photons from 434 nm to 370 nm and show that their polarization is preserved.

quant-ph↗