arXiv subjects

Frank Vewinger

Publications and source records attributed to Frank Vewinger.

At least 37 records · Page 2Linked to original sources

arXiv2022

Frequency Conversion in High-Pressure Hydrogen

State-preserving frequency conversion in the optical domain is a necessary component in many configurations of quantum information processing and communication. Thus far, nonlinear crystals are used for this purpose. Here, we report on a new approach based on coherent anti-Stokes Raman scattering (CARS) in a dense molecular hydrogen gas. This four-wave mixing process sidesteps the limitations imposed by crystal properties, it is intrinsically broadband and does not generate an undesired background. We demonstrate this method by converting photons from 434 nm to 370 nm and show that their polarization is preserved.

quant-ph↗

arXiv2022

Spectroscopy of high pressure rubidium-noble gas mixtures

Spectroscopy of alkali-buffer gas mixtures at high pressures from single-digit to several 100 bars in the regime of substantial collisional broadening is relevant in a wide range of fields, ranging from collisional redistribution cooling to laboratory astrophysics. Here we report on spectroscopic measurements of dense rubidium-noble gas mixtures recorded in a pressure cell equipped with soldered sapphire optical viewports, which allows for the controlled realization of extreme conditions of high temperature and high pressure in a table top laboratory experiment. In the gas cell, we have recorded absorption and emission spectra of rubidium subject to 250 bar helium buffer gas pressure at 500 K temperature. The spectra to good accuracy fulfill the thermodynamic Kennard- Stepanov frequency scaling of the ratio of absorption and emission spectral profiles. Further, the long optical path length in the cell allowed to both record spectra of rubidium-argon mixtures at moderate temperatures and high pressures and to observe redistributional laser cooling in this system.

physics.atom-ph↗

arXiv2022

Nonlocality-induced surface localization in Bose-Einstein condensates of light

The ability to create and manipulate strongly correlated quantum many-body states is of central importance to the study of collective phenomena in several condensed-matter systems. In the last decades, a great amount of work has been focused on ultracold atoms in optical lattices, which provide a flexible platform to simulate peculiar phases of matter both for fermionic and bosonic particles. The recent experimental demonstration of Bose-Einstein condensation (BEC) of light in dye-filled microcavities has opened the intriguing possibility to build photonic simulators of solid-state systems, with potential advantages over their atomic counterpart. A distinctive feature of photon BEC is the thermo-optical nature of the effective photon-photon interaction, which is intrinsically nonlocal and can thus induce interactions of arbitrary range. This offers the opportunity to systematically study the collective behaviour of many-body systems with tunable interaction range. In this paper, we theoretically study the effect of nonlocal interactions in photon BEC. We first present numerical results of BEC in a double-well potential, and then extend our analysis to a short one-dimensional lattice with open boundaries. By resorting to a numerical procedure inspired by the Newton-Raphson method, we simulate the time-independent Gross-Pitaevskii equation and provide evidence of surface localization induced by nonlocality, where the condensate density is localized at the boundaries of the potential. Our work paves the way towards the realization of synthetic matter with photons, where the interplay between long-range interactions and low dimensionality can lead to the emergence of unexplored nontrivial collective phenomena.

physics.optics↗

arXiv2021

Compressibility and the Equation of State of an Optical Quantum Gas in a Box

The compressibility of a medium, quantifying its response to mechanical perturbations, is a fundamental property determined by the equation of state. For gases of material particles, studies of the mechanical response are well established, in fields from classical thermodynamics to cold atomic quantum gases. Here we demonstrate a measurement of the compressibility of a two-dimensional quantum gas of light in a box potential and obtain the equation of state for the optical medium. The experiment is carried out in a nanostructured dye-filled optical microcavity. We observe signatures of Bose-Einstein condensation at high phase-space densities in the finite-size system. Strikingly, upon entering the quantum degenerate regime, the measured density response to an external force sharply increases, hinting at the peculiar prediction of an infinite compressibility of the deeply degenerate Bose gas.

cond-mat.quant-gas↗

arXiv2021

Converting single photons from an InAs/GaAs quantum dot into the ultraviolet: preservation of second-order correlations

Wavelength conversion at the single-photon level is required to forge a quantum network from distinct quantum devices. Such devices include solid-state emitters of single or entangled photons, as well as network nodes based on atoms or ions. Here we demonstrate the conversion of single photons emitted from a III-V semiconductor quantum dot at 853nm via sum frequency conversion to the wavelength of the strong transition of Yb ions at 370nm. We measure the second-order correlation function of both the unconverted and of the converted photon and show that the single-photon character of the quantum dot emission is preserved during the conversion process.

quant-ph↗

arXiv2021

Sapphire optical viewport for high pressure and temperature applications

We describe the design of a soldered sapphire optical viewport, useful for spectroscopic applications of samples at high temperatures and high pressures. The sapphire window is bonded via active soldering to a metal flange with a structure of two c-shaped rings made of different metallic materials in between, as to mitigate thermally induced stress. A spectroscopic cell equipped with two of the optical viewports has been successfully operated with alkali metals in a noble gas environment at temperatures in the range $20\,$°C to $450\,$°C at noble gas pressures from $10^{-6}\,$mbar to $330\,$bar. At the upper pressure range, we observe a leakage rate smaller than our readout accuracy of $30\,$mbar per day.

physics.atom-ph↗

arXiv2021

Observation of a non-Hermitian phase transition in an optical quantum gas

Quantum gases of light, as photons or polariton condensates in optical microcavities, are collective quantum systems enabling a tailoring of dissipation from e.g. cavity loss. This makes them a tool to study dissipative phases, an emerging subject in quantum manybody physics. Here we experimentally demonstrate a non-Hermitian phase transition of a photon Bose-Einstein condensate to a new dissipative phase, characterized by a biexponential decay of the condensate's second-order coherence. The phase transition occurs due to the emergence of an exceptional point in the quantum gas. While Bose-Einstein condensation is usually connected to ordinary lasing by a smooth crossover, the observed phase transition separates the novel, biexponential phase from both lasing and an intermediate, oscillatory condensate regime. Our findings pave the way for studies of a wide class of dissipative quantum phases, for instance in topological or lattice systems.

cond-mat.quant-gas↗

arXiv2021

Vacuum-Ultraviolet Absorption and Emission Spectroscopy of Gaseous, Liquid, and Supercritical Xenon

Bose-Einstein condensation, an effect long known for material particles as cold atomic gases, has in recent years also been observed for photons in microscopic optical cavitites. Here, we report absorption and emission spectroscopic measurements on the lowest electronic transition ($5\text{p}^6 \rightarrow 5\text{p}^5 6\text{s}$) of xenon, motivated by the search for a thermalization medium for photon Bose-Einstein condensation in the vacuum-ultraviolet spectral regime. We have recorded pressure-broadened xenon spectra in the 135 nm to 190 nm wavelength regime at conditions near the critical point. The explored pressure and temperature range includes high pressure gaseous xenon below the critical pressure and supercritical xenon at room temperature, as well as liquid xenon close to the boiling point near the critical pressure.

physics.atom-ph↗

arXiv2020

Realizing arbitrary trapping potentials for light via direct laser writing of mirror surface profiles

The versatility of quantum gas experiments greatly benefits from the ability to apply variable potentials. Here we describe a method which allows the preparation of potential structures for microcavity photons via spatially selective deformation of optical resonator geometries with a heat induced mirror surface microstructuring technique. We investigate the thermalization of a two-dimensional photon gas in a dye-filled microcavity composed of the custom surface-structured mirrors at wavelength-scale separation. Specifically, we describe measurements of the spatial redistribution of thermal photons in a coupled double-ridge structure, where photons form a Bose-Einstein condensate in a spatially split ground state, as a function of different pumping geometries.

cond-mat.quant-gas↗

arXiv2019

Rubidium spectroscopy at high-pressure buffer gas conditions: detailed balance in the optical interaction of an absorber coupled to a reservoir

Optical spectroscopy of atoms and molecules is a field where one usually operates very far from thermal equilibrium conditions. A prominent example is spectroscopy of thin vapors, where the pump irradiation leads to a non equilibrium distribution within the electronic structure that is well shielded from the environment. Here we describe experimental work investigating absorption and emission lines of rubidium vapor subject to a noble buffer gas environment with pressure 100 to 200 bar, a regime interpolating between usual gas phase and liquid solid state conditions. Frequent elastic collisions in the dense buffer gas sample cause a large coupling to the environment. We give a detailed account of recent observations of the Kennard Stepanov scaling, a Boltzmann like thermodynamic frequency scaling between absorption and emission profiles, for both atomic and molecular rubidium species in the gaseous environment. Our observations are interpreted as due to the thermalization of alkali noble gas submanifolds in both ground and electronically excited states respectively. Both pressure broadening and shift of the high pressure buffer gas D lines system are determined. We also discuss some prospects, including possible advances in collisional laser cooling and optical thermometry.

physics.atm-clus↗

arXiv2019

Thermally Condensing Photons into a Coherently Split State of Light

Techniques to control the quantum state of light play a crucial role in a wide range of fields, from quantum information science to precision measurements. While for electrons in solid state materials complex quantum states can be created by mere cooling, in the field of optics manipulation and control currently builds on non-thermodynamic methods. Using an optical dye microcavity, we have split photon wavepackets by thermalization within a potential with two minima subject to tunnel coupling. Even at room temperature, photons condense into a quantum-coherent bifurcated ground state. Fringe signals upon recombination show the relative coherence between the two wells, demonstrating a working interferometer with the non-unitary thermodynamic beamsplitter. This energetically driven optical state preparation opens up an avenue for exploring novel correlated and entangled optical manybody states.

cond-mat.quant-gas↗

arXiv2019

Fluctuation dynamics of an open photon Bose-Einstein condensate

Bosonic gases coupled to a particle reservoir have proven to support a regime of operation where Bose-Einstein condensation coexists with unusually large particle-number fluctuations. Experimentally, this situation has been realized with two-dimensional photon gases in a dye-filled optical microcavity. Here, we investigate theoretically and experimentally the open-system dynamics of a grand canonical Bose-Einstein condensate of photons. We identify a regime with temporal oscillations of the second-order coherence function $g^{(2)}(τ)$, even though the energy spectrum closely matches the predictions for an equilibrium Bose-Einstein distribution and the system is operated deeply in the regime of weak light-matter coupling. The observed temporal oscillations are attributed to the nonlinear, weakly driven-dissipative nature of the system which leads to time-reversal symmetry breaking.

quant-ph↗

arXiv2019

Collective Modes of a Photon Bose-Einstein Condensate with Thermo-Optic Interaction

Although for photon Bose-Einstein condensates the main mechanism of the observed photon-photon interaction has already been identified to be of thermo-optic nature, its influence on the condensate dynamics is still unknown. Here a mean-field description of this effect is derived, which consists of an open-dissipative Schrödinger equation for the condensate wave function coupled to a diffusion equation for the temperature of the dye solution. With this system at hand, the lowest-lying collective modes of a harmonically trapped photon Bose-Einstein condensate are calculated analytically via a linear stability analysis. As a result, the collective frequencies and, thus, the strength of the effective photon-photon interaction turn out to strongly depend on the thermal diffusion in the cavity mirrors. In particular, a breakdown of the Kohn theorem is predicted, i.e.~the frequency of the centre-of-mass oscillation is reduced due to the thermo-optic photon-photon interaction.

cond-mat.quant-gas↗

arXiv2017

Variable Potentials for Thermalized Light and Coupled Condensates

For over a decade, cold atoms in lattice potentials have been an attractive platform to simulate phenomena known from solid state theory, as the Mott-insulator transition. In contrast, the field of photonics usually deals with non-equilibrium physics. Recent advances towards photonic simulators of solid state equilibrium effects include polariton double-site and lattice experiments, as well as the demonstration of a photon condensate in a dye-filled microcavity. Here we demonstrate a technique to create variable micropotentials for light using thermo-optic imprinting within an ultrahigh-reflectivity mirror microcavity filled with a dye-polymer solution that is compatible with photon gas thermalization. By repeated absorption-emission cycles photons thermalize to the temperature of the dye solution, and in a single microsite we observe a photon Bose-Einstein microcondensate. Effective interactions between the otherwise nearly non-interacting photons are observed due to thermo-optic effects, and in a double-well system tunnel coupling between sites is demonstrated, as well as the hybridization of eigenstates. Prospects of the new experimental platform include photonic structures in which photons thermalize into entangled manybody states.

cond-mat.quant-gas↗

arXiv2017

First-order spatial coherence measurements in a thermalized two-dimensional photonic quantum gas

Phase transitions between different states of matter can profoundly modify the order in physical systems, with the emergence of ferromagnetic or topological order constituting important examples. Correlations allow to quantify the degree of order and classify different phases. Here we report measurements of first-order spatial correlations in a harmonically trapped two-dimensional photon gas below, at, and above the critical particle number for Bose-Einstein condensation, using interferometric measurements of the emission of a dye-filled optical microcavity. For the uncondensed gas, the transverse coherence decays on a length scale determined by the thermal de Broglie wavelength of the photons, which shows the expected scaling with temperature. At the onset of Bose-Einstein condensation true long-range order emerges, and we observe quantum statistical effects as the thermal wave packets overlap. The excellent agreement with equilibrium Bose gas theory prompts microcavity photons as promising candidates for studies of critical scaling and universality in optical quantum gases.

cond-mat.quant-gas↗

arXiv2016

Absorption spectroscopy of xenon and ethylene-noble gas mixtures at high pressure: Towards Bose-Einstein condensation of vacuum ultraviolet photons

Bose-Einstein condensation is a phenomenon well known for material particles as cold atomic gases, and this concept has in recent years been extended to photons confined in microscopic optical cavities. Essential for the operation of such a photon condensate is a thermalization mechanism that conserves the average particle number, as in the visible spectral regime can be realized by subsequent absorption re-emission processes in dye molecules. Here we report on the status of an experimental effort aiming at the extension of the concept of Bose-Einstein condensation of photons towards the vacuum ultraviolet spectral regime, with gases at high pressure conditions serving as a thermalization medium for the photon gas. We have recorded absorption spectra of xenon gas at up to 30 bar gas pressure of the $5p^6 - 5p^56s$ transition with a wavelength close to 147 nm. Moreover, spectra of ethylene noble gas mixtures between 155 and 180 nm wavelength are reported.

physics.atom-ph↗

arXiv2016

Bose-Einstein Condensation of Photons versus Lasing and Hanbury Brown-Twiss Measurements with a Condensate of Light

The advent of controlled experimental accessibility of Bose-Einstein condensates, as realized with e.g. cold atomic gases, exciton-polaritons, and more recently photons in a dye-filled optical microcavity, has paved the way for new studies and tests of a plethora of fundamental concepts in quantum physics. We here describe recent experiments studying a transition between laser-like dynamics and Bose-Einstein condensation of photons in the dye microcavity system. Further, measurements of the second-order coherence of the photon condensate are presented. In the condensed state we observe photon number fluctuations of order of the total particle number, as understood from effective particle exchange with the photo-excitable dye molecules. The observed intensity fluctuation properties give evidence for Bose-Einstein condensation occurring in the grand-canonical statistical ensemble regime.

cond-mat.quant-gas↗

arXiv2016

Calorimetry of a Bose-Einstein condensed photon gas

Phase transitions, as the condensation of a gas to a liquid, are often revealed by a discontinuous behavior of thermodynamic quantities. For liquid Helium, for example, a divergence of the specific heat signals the transition from the normal fluid to the superfluid state. Apart from liquid helium, determining the specific heat of a Bose gas has proven to be a challenging task, for example for ultracold atomic Bose gases. Here we examine the thermodynamic behavior of a trapped two-dimensional photon gas, a system that allows us to spectroscopically determine the specific heat and the entropy of a nearly ideal Bose gas from the classical high temperature to the Bose-condensed quantum regime. The critical behavior at the phase transition is clearly revealed by a cusp singularity of the specific heat. Regarded as a test of quantum statistical mechanics, our results demonstrate a quantitative agreement with its predictions at the microscopic level.

cond-mat.quant-gas↗