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Gérard Lapertot

Publications and source records attributed to Gérard Lapertot.

17 recordsLinked to original sources

Unusual upper critical field in UTe2 revealed by magnetotransport measurements up to 42 T

The heavy-fermion superconductor UTe2 is unique in that, at ambient pressure, it exhibits three distinct superconducting phases, two of which are induced by magnetic field. When the field is applied along the crystallographic b axis in the orthorhombic structure, the field-induced phase SC2 develops above approximately 20 T and persists up to the metamagnetic transition at Hm about 34 T. When the magnetic field is tilted towards the c axis, another superconducting phase, SC3, emerges at very high fields above about 40 T over a certain angular range. The origin of this exotic phase remains under debate. One of the key open questions regarding the origin of SC3 is whether it is confined to the spin-polarized state above Hm, or whether it already develops at lower fields. Here, we report magnetoresistance measurements performed on a high-quality single crystal of UTe2 in static magnetic fields up to 42 T applied in the (bc) plane at temperatures down to 0.35 K. At this temperature, we find that the SC3 phase first appears at an angle of 20 deg from the b axis. At larger angles, the onset of the SC3 phase, defined by a maximum in resistivity, occurs below Hm. However, zero resistivity is reached only above Hm throughout the entire angular range investigated. These results are summarized in the resulting field-angle phase diagram. Furthermore, we find that at 21 deg the SC3 phase is rapidly suppressed with increasing temperature, whereas at 24 deg it becomes considerably more robust and persists up to about 1 K. Finally, we observe Shubnikov de Haas (SdH) oscillations in the vicinity of the c axis. The observed oscillation frequencies are in good agreement with our previous results. The field dependence of the strongest SdH frequency and of the effective mass is discussed.

cond-mat.str-el↗

Field-induced compensation of magnetic exchange as the possible origin of reentrant superconductivity in UTe$_2$

The potential spin-triplet heavy-fermion superconductor UTe$_2$ exhibits signatures of multiple distinct superconducting phases. For field aligned along the $b$ axis, a metamagnetic transition occurs at $μ_0 H_\mathrm{m}\approx35\,$T. It is associated with magnetic fluctuations that may be beneficial for the field-reinforced superconductivity surviving up to $H_\mathrm{m}$. Once the field is tilted away from the $b$ towards the $c$ axis, a reentrant superconducting phase emerges just above $H_\mathrm{m}$. In order to better understand this remarkably field-resistant superconducting phase, we conducted magnetic-torque and magnetotransport measurements in pulsed magnetic fields. We determine the record-breaking upper critical field of $μ_0 H_\mathrm{c2}\approx 73\,$T and its evolution with angle. Furthermore, the normal-state Hall effect experiences a drastic suppression indicative of a reduced band polarization above $H_\mathrm{m}$ in the angular range around $30^\circ$ caused by a partial compensation between the applied field and an exchange field. This promotes the Jaccarino-Peter effect as a likely mechanism for the reentrant superconductivity above $H_\mathrm{m}$.

cond-mat.supr-con↗

Field-induced tuning of the pairing state in a superconductor

The recently discovered superconductor UTe$_2$, with a T$_c$ between 1.5~K and 2~K, is attracting much attention due to strong suspicion of spin-triplet and topological superconductivity. Its properties under magnetic field are also remarkable, with field-reinforced and field-induced superconducting phases. Here, we report the first complete thermodynamic determination of the phase diagram for fields applied along the three crystallographic directions. Measurements were performed up to 36~T along the hard magnetisation $b$~axis in order to follow the superconducting transition up to the metamagnetic transition at $H_{m} = 34.75$~T. They reveal the existence of a phase transition line within the superconducting phase, and drastic differences occurring between these two phases. Detailed analysis supports a different spin state between the two phases, implying a low-field spin-triplet to high-field spin-singlet transition, a unique case among superconductors, giving insight on the mechanisms leading to spin-triplet superconductivity.

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Thermodynamic signatures of short-range magnetic correlations in UTe$_2$

The normal-state out of which unconventional superconductivity in UTe$_2$ emerges is studied in detail using a variety of thermodynamic and transport probes. Clear evidence for a broad Schottky-like anomaly with roughly R ln 2 entropy around $T^{*} \approx 12$K is observed in all measured quantities. Comparison with high magnetic field transport data allows the construction of an $H\text{-}T$ phase diagram resembling that of the ferromagnetic superconductor URhGe. The low field electronic Grüneisen parameter of $T^{*}$ and that of the metamagnetic transition at $H_m \approx 35$T are comparable pointing to a common origin of both phenomena. Enhanced Wilson and Korringa ratios suggests that the existence of short range ferromagnetic fluctuations cannot be ruled out.

cond-mat.supr-con↗

Evidence of Fermi-Surface Reconstruction at the Metamagnetic Transition of the Strongly Correlated Superconductor UTe2

Thermoelectric power ($S$) and Hall effect ($R_\mathrm{H}$) measurements on the paramagnetic superconductor UTe$_2$ with magnetic field applied along the hard magnetization $b$-axis are reported. The first order nature of the metamagnetic transition at $H_\mathrm{m}=H^b_\mathrm{c2}=35$~T leads to drastic consequences on $S$ and $R_\mathrm{H}$. In contrast to the field dependence of the specific heat in the normal state through $H_\mathrm{m}$, $S(H)$ is not symmetric with respect to $H_\mathrm{m}$. This implies a strong interplay between ferromagnetic (FM) fluctuations and a Fermi-surface reconstruction at $H_\mathrm{m}$. $R_\mathrm{H}$ is very well described by incoherent skew scattering above the coherence temperature $T_\mathrm{m}$ corresponding roughly to the temperature of the maximum in the susceptibility $T_{χ_\mathrm{max}}$ and coherent skew scattering at lower temperatures. The discontinuous field dependence of both, $S(H)$ and the ordinary Hall coefficient $R_0$, at $H_\mathrm{m}$ and at low temperature, provides evidence of a change in the band structure at the Fermi level.

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Anisotropy of the Upper Critical Field in the Heavy-Fermion Superconductor UTe2 under Pressure

We studied the anisotropy of the superconducting upper critical field $H_{\rm c2}$ in the heavy-fermion superconductor UTe$_2$ under hydrostatic pressure by magnetoresistivity measurements. In agreement with previous experiments we confirm that superconductivity disappears near a critical pressure $p_{\rm c} \approx 1.5$~GPa, and a magnetically ordered state appears. The unusual $H_{\rm c2}(T)$ at low temperatures for $H \parallel a$ suggests that the multiple superconducting phases which appear under pressure have quite different $H_{\rm c2}$. For a field applied along the hard magnetization $b$ axis $H_{\rm c2} (0)$ is glued to the metamagnetic transition $H_{\rm m}$ which is suppressed near $p_{\rm c}$. The suppression of $H_{\rm m}$ with pressure follows the decrease of temperature $T_χ^{\rm max}$, at the maximum in the susceptibility along $b$. The strong reinforcement of $H_{\rm c2}$ at ambient pressure for $H \parallel b$ above 16~T is rapidly suppressed under pressure due to the increase of $T_{\rm sc}$ and the decrease of $H_{\rm m}$. The change in the hierarchy of the anisotropy of $H_{\rm c2}(0)$ on approaching $p_{\rm c}$ points out that the $c$ axis becomes the hard magnetization axis.

cond-mat.str-el↗

Fermi-Surface Instabilities in the Heavy-Fermion Superconductor UTe2

We present different transport measurements up to fields of 29~T in the recently discovered heavy-fermion superconductor UTe$_{2}$ with magnetic field $H$ applied along the easy magnetization a-axis of the body-centered orthorhombic structure. The thermoelectric power varies linearly with temperature above the superconducting transition, $T_{SC}= 1.5$ K, indicating that superconductivity develops in a Fermi liquid regime. As a function of field the thermolelectric power shows successive anomalies which are attributed to field-induced Fermi surface instabilities. These Fermi-surface instabilities appear at critical values of the magnetic polarization. Remarkably, the lowest magnetic field instability for $H\parallel a$ occurs for the same critical value of the magnetization (0.4 $μ_B$) than the first order metamagnetic transition at 35~T for field applied along the $b$-axis. The estimated number of charge carriers at low temperature reveals a metallic ground state distinct from LDA calculations indicating that strong electronic correlations are a major issue in this compound.

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Field-reentrant superconductivity close to a metamagnetic transition in the heavy-fermion superconductor UTe$_2$

We present a study of the upper critical field of the newly discovered heavy fermion superconductor UTe$_2$ by magnetoresistivity measurements in pulsed magnetic fields up to 60~T and static magnetic fields up to 35~T. We show that superconductivity survives up to the metamagnetic transition at $H_{\rm m} \approx 35$~T at low temperature. Above $H_{\rm m}$ superconductivity is suppressed. At higher temperature superconductivity is enhanced under magnetic field leading to reentrance of superconductivity or an almost temperature independent increase of $H_{\rm c2}$. By studying the angular dependence of the upper critical field close to the $b$ axis (hard magnetization axis) we show that the maximum of the reentrant superconductivity temperature is depinned from the metamagnetic field. A key ingredient for the field-reinforcement of superconductivity on approaching $H_{\rm m}$ appears to be an immediate interplay with magnetic fluctuations and a possible Fermi-surface reconstruction.

cond-mat.str-el↗

Magnetic-Field-Induced Phenomena in the Paramagnetic Superconductor UTe$_{2}$

We present magnetoresistivity measurements on the heavy-fermion superconductor UTe$_{2}$ in pulsed magnetic fields $μ_0H$ up to 68~T and temperatures $T$ from 1.4 to 80~K. Magnetic fields applied along the three crystallographic directions $\mathbf{a}$ (easy magnetic axis), $\mathbf{b}$, and $\mathbf{c}$ (hard magnetic axes), are found to induce different phenomena - depending on the field direction - beyond the low-field suppression of the superconducting state. For $\mathbf{H}\parallel\mathbf{a}$, a broad anomaly in the resistivity is observed at $μ_0H^*\simeq10$~T and $T = 1.4$~K. For $\mathbf{H}\parallel\mathbf{c}$, no magnetic transition nor crossover are observed. For $\mathbf{H}\parallel\mathbf{b}$, a sharp first-order-like step in the resistivity indicates a metamagnetic transition at the field $μ_0H_m \simeq 35$~T. When the temperature is raised signature of first-order metamagnetism is observed up to a critical endpoint at $T_{CEP}\simeq7$~K. At higher temperatures a crossover persists up to 28~K, i.e., below the temperature $T_χ^{max} = 35$~K where the magnetic susceptibility is maximal. A sharp maximum in the Fermi-liquid quadratic coefficient $A$ of the low-temperature resistivity is found at $H_m$. It indicates an enhanced effective mass associated with critical magnetic fluctuations, possibly coupled with a Fermi surface instability. Similarly to the URhGe case, we show that UTe$_{2}$ is a candidate for field-induced reentrant superconductivity in the proximity of $H_m$.

cond-mat.str-el↗

Fermi-Surface Selective Determination of the $\mathbf{g}$-Factor Anisotropy in URu$_2$Si$_2$

The $g$-factor anisotropy of the heavy quasiparticles in the hidden order state of URu$_2$Si$_2$ has been determined from the superconducting upper critical field and microscopically from Shubnikov-de Haas (SdH) oscillations. We present a detailed analysis of the $g$-factor for the $α$, $β$ and $γ$ Fermi-surface pockets. Our results suggest a strong $g$-factor anisotropy between the $c$ axis and the basal plane for all observed Fermi surface pockets. The observed anisotropy of the $g$-factor from the quantum oscillations is in good agreement with the anisotropy of the superconducting upper critical field at low temperatures, which is strongly limited by the paramagnetic pair breaking along the easy magnetization axis $c$. However, the anisotropy of the initial slope of the upper critical field near $T_c$ cannot be explained by the anisotropy of the effective masses and Fermi velocities derived from quantum oscillations.

cond-mat.str-el↗

The Dominant Role of Critical Valence Fluctuations on High $T_{\rm c}$ Superconductivity in Heavy Fermions

Despite almost 40 years of research, the origin of heavy-fermion superconductivity is still strongly debated. Especially, the pressure-induced enhancement of superconductivity in CeCu$_2$Si$_2$ away from the magnetic breakdown is not sufficiently taken into consideration. As recently reported in CeCu$_2$Si$_2$ and several related compounds, optimal superconductivity occurs at the pressure of a valence crossover, which arises from a virtual critical end point at negative temperature $T_{\rm cr}$. In this context, we did a meticulous analysis of a vast set of top-quality high-pressure electrical resistivity data of several Ce-based heavy fermion compounds. The key novelty is the salient correlation between the superconducting transition temperature $T_{\rm c}$ and the valence instability parameter $T_{\rm cr}$, which is in line with theory of enhanced valence fluctuations. Moreover, it is found that, in the pressure region of superconductivity, electrical resistivity is governed by the valence crossover, which most often manifests in scaling behavior. We develop the new idea that the optimum superconducting $T_{\rm c}$ of a given sample is mainly controlled by the compound's $T_{\rm cr}$ and limited by non-magnetic disorder. In this regard, the present study provides compelling evidence for the crucial role of critical valence fluctuations in the formation of Cooper pairs in Ce-based heavy fermion superconductors besides the contribution of spin fluctuations near magnetic quantum critical points, and corroborates a plausible superconducting mechanism in strongly correlated electron systems in general.

cond-mat.str-el↗

Heavy-Fermion Superconductivity in CeAg$_2$Si$_2$ --Interplay of Spin and Valence Fluctuations--

We present the pressure-temperature phase diagram of the antiferromagnet CeAg$_2$Si$_2$ established via resistivity and calorimetry measurements under quasi-hydrostatic conditions up to 22.5~GPa. With increasing pressure, the Néel temperature [$T_{\mathrm{N}}(p=0)=8.6$~K] slowly increases up to $T_{\mathrm{N}}=13.4$~K at 9.4~GPa and then vanishes abruptly at the magnetic critical pressure $p_{\mathrm{c}}\sim13$~GPa. For the first time, heavy fermion superconductivity is observed in CeAg$_2$Si$_2$ . Superconductivity emerges at $\sim 11$~GPa and persists over roughly 10~GPa. Partial- and bulk-transition temperatures are highest at $p=16$~GPa, with a maximal $T_{\mathrm{c}^{\rm bulk}}=1.25$~K. In the pressure region of superconductivity, Kondo and crystal-field splitting energies become comparable and resistivity exhibits clear signatures of a Ce-ion valence crossover. The crossover line is located at a rapid collapse in resistivity as function of pressure and extrapolates to a valence transition critical endpoint at critical pressure and temperature of $p_{\rm cr}\sim 17$~GPa and $T_{\rm cr}\sim-13~K$, respectively. Both critical spin and valence fluctuations may build up superconductivity in CeAg$_2$Si$_2$.

cond-mat.str-el↗

High-pressure study of the ground- and superconducting-state properties of CeAu$_2$Si$_2$

The pressure-temperature-phase diagram of the new heavy-fermion superconductor CeAu$_2$Si$_2$ is markedly different from those studied previously. Indeed, superconductivity emerges, not on the verge, but deep inside the magnetic phase. In this context, we have carried out ac-calorimetry, resistivity and thermoelectric power measurements on a CeAu$_2$Si$_2$-single crystal under high-pressure. The principal novelties of this experiment are the observation of a new transition line, presumably a magnetic structure rearrangement at $T_{\mathrm{M}}^{\mathrm{mod}}$ inside the antiferromagnetic phase, and the occurrence of quantum critical behavior in resistivity linked to superconductivity. Strong non-Fermi-liquid behavior is observed around the maximum of superconductivity and enhanced scattering rates are observed close to both the emergence and the maximum of superconductivity. Intriguingly, $T_{\mathrm{M}}^{\mathrm{mod}}$ almost coincides with the onset of the superconducting transition over a broad pressure range, where mysteriously Tc increases with the strengthening of magnetism. A comparison of the features in CeAu$_2$Si$_2$ and its parent compounds CeCu$_2$Si$_2$ and CeCu$_2$Ge$_2$ plotted as function of the unit-cell volume leads us to promote that critical fluctuations of a valence crossover play a crucial role in the superconducting paring mechanism. Our study reveals new intriguing features of magnetism and illustrates a complex interplay between magnetism, quantum criticality and superconductivity.

cond-mat.str-el↗

Raman Active High Energy Excitations in URu$_2$Si$_2$

We have performed Raman scattering measurements on URu$_2$Si$_2$ single crystals on a large energy range up to $\sim$ 1300 cm$^{-1}$ and in all the Raman active symmetries as a function of temperature down to 15 K. A large excitation, active only in the E$_{g}$ symmetry, is reported. It has been assigned to a crystal electric field excitation on the Uranium site. We discuss how this constrains the crystal electric field scheme of the Uranium ions. Furthermore, three excitations in the A$_{1g}$ symmetry are observed. They have been associated to double Raman phonon processes consistently with ab initio calculations of the phonons dispersion.

cond-mat.str-el↗

Evidence for Coexistence of Bulk Superconductivity and Itinerant Antiferromagnetism in the Heavy Fermion System CeCo(In$_{1-x}$Cd$_x$)$_5$

In the generic phase diagram of heavy fermion systems, tuning an external parameter such as hydrostatic or chemical pressure modifies the superconducting transition temperature. The superconducting phase forms a dome in the temperature-tuning parameter phase diagram, which is associated with a maximum of the superconducting pairing interaction. Proximity to antiferromagnetism suggests a relation between the disappearance of antiferromagnetic order and superconductivity. We combine muon spin rotation, neutron scattering, and x-ray absorption spectroscopy techniques to gain access to the magnetic and electronic structure of CeCo(In$_{1-x}$Cd$_x$)$_5$ at different time scales. Different magnetic structures are obtained that indicate a magnetic order of itinerant character, coexisting with bulk superconductivity. The suppression of the antiferromagnetic order appears to be driven by a modification of the bandwidth/carrier concentration, implying that the electronic structure and consequently the interplay of superconductivity and magnetism is strongly affected by hydrostatic and chemical pressure.

cond-mat.supr-con↗

Upper critical field of CeCoIn5

We present a detailed analysis of the upper critical field for CeCoIn5 under high pressure. We show that, consistently with other measurements, this system shows a decoupling between maximum of the superconducting transition temperature Tc and maximum pairing strength. This puts forward CeCoIn5 as an important paradigm for this class of unconventional, strongly correlated superconductors.

cond-mat.str-el↗

Evidence for Anisotropic Vortex Dynamics and Pauli Limitation in the Upper Critical Field of FeSe1-xTex

We have determined HC2(T) for FeSe1-xTex (x=0.52) single crystals using resistivity measurements at high static and pulsed magnetic field, as well as specific heat measurements up to 9T. We find that the significant anisotropy of the initial slope of HC2(T) determined from resistivity measurements, is not present when HC2 is determined from the specific heat results. This suggests that the thermodynamic upper critical field is almost isotropic, and that anisotropic vortex dynamics play a role. Further evidence of anisotropic vortex dynamics is found in the behaviour in pulsed field. We also find that Pauli limiting must be included in order to fit the temperature dependence of HC2, indicating probably higher effective mass in FeSe1-xTex than in other Fe superconductors.

cond-mat.supr-con↗