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G. Bollen

Publications and source records attributed to G. Bollen.

At least 19 recordsLinked to original sources

High-Precision Mass Measurements of 52Ni and 51Co Reveal Breakdown of the Isobaric Multiplet Mass Equation in the f p Shell

We performed high-precision mass measurements of the proton-rich nuclei $^{52}$Ni and $^{51}$Co with the LEBIT Penning trap at the Facility for Rare Isotope Beams (FRIB). For $^{52}$Ni, a mass excess of $-22474.8(2.2)$~keV was determined, which is consistent with a recent storage-ring measurement at the Cooler-Storage Ring (CSRe) but has a factor 37 improved precision. For $^{51}$Co, we obtained a mass excess of $-27375.1(5.7)$~keV, agreeing with a recent CSRe result, while reducing the uncertainty by a factor~2. Combining our mass value for $^{52}$Ni with the known two-proton decay energy of $^{54}$Zn, we determined the mass excess of $^{54}$Zn to be $-6463(42)$~keV. These new mass values reveal a substantial breakdown of the isobaric mass multiplet equation for $A=52$ and $A=54$, and provide stringent benchmarks for isospin-symmetry-breaking effects in the proton-rich $fp$-shell, favoring theoretical descriptions that omit the Coulomb-exchange term.

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A high-voltage MR-ToF mass spectrometer and separator for the study of exotic isotopes at FRIB

The Facility for Rare Isotope Beams (FRIB) delivers a wide variety of rare isotopes as fast, stopped, or reaccelerated beams to enable forefront research in nuclear structure, astrophysics, and fundamental interactions. To expand the scientific potential of FRIB's stopped and reaccelerated beam programs, we are designing a Multi-Reflection Time-of-Flight mass spectrometer and separator (MR-ToF MS). It will enable high-precision mass measurements of short-lived isotopes, improve beam diagnostics, and deliver isobarically and isomerically purified beams to downstream experimental stations. It is designed to store ions at a kinetic energy of 30 keV, significantly enhancing ion throughput while maintaining high mass resolving power. We present the scientific motivation, technical design, and simulations demonstrating the expected performance of the system, which has the potential to significantly enhance FRIB's mass measurement, diagnostic, and mass separation capabilities.

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High-precision Penning trap mass measurements of neutron-rich chlorine isotopes at the N=28 shell closure

Although it is known that the $N=28$ spherical shell closure erodes, the strength of the closure with decreasing proton number $Z<20$ is an open question in nuclear structure. In this region of interest, direct high-precision mass measurements of neutron-rich $^{43-45}$Cl isotopes were performed at the Low Energy Beam and Ion Trap (LEBIT) when coupled to the National Superconducting Cyclotron Lab. The resulting mass excesses (MEs) are ME($^{43}$Cl) = -24114.4(1.7) keV, ME($^{44}$Cl) = -20450.8(10.6) keV, and ME($^{45}$Cl) = -18240.1(3.7) keV, and improve the uncertainty of these masses by up to a factor of ~40 compared to the previous values reported in the 2020 Atomic Mass Evaluation. Comparison to $\textit{ab initio}$ calculations using the Valence-Space In-Medium Similarity Renormalization Group (VS-IMSRG) shows good agreement up to and including the closure.

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Exploring Isospin Symmetry Breaking in Exotic Nuclei: High-Precision Mass Measurement of 23Si and Shell-Model Calculations of T = 5/2 Nuclei

We present a high-precision mass measurement of the proton-rich nucleus 23Si, performed with the LEBIT Penning trap at the Facility for Rare Isotope Beams (FRIB) utilizing the time-of-flight ion cyclotron resonance (TOF-ICR) technique. We determined a mass excess of 23362.9(5.8) keV, which agrees with a recent storage-ring measurement from CSRe but has a factor 20 improved precision. 23Si is hence the nucleus with the most precisely known mass of all nuclei with an isospin projection of Tz =-5/2. We performed shell-model calculations with the USDC and USDCm Hamiltonians to study binding energy differences and Thomas-Ehrmann shifts in mirror systems with an isospin up to T = 5/2. Our experimental result and other recently reported masses of neutron-deficient sd-shell nuclei agree well with the theoretical predictions, demonstrating that isospin symmetry breaking in sd-shell nuclei, even at high isospin values, is well described by modern shell-model calculations.

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High-precision mass measurement of $^{103}$Sn restores smoothness of the mass surface

As a step towards the ultimate goal of a high-precision mass measurement of doubly-magic $^{100}$Sn, the mass of $^{103}$Sn was measured at the Low Energy Beam and Ion Trap (LEBIT) located at the Facility for Rare Isotope Beams (FRIB). Utilizing the time-of-flight ion cyclotron resonance (ToF-ICR) technique, a mass uncertainty of 3.7~keV was achieved, an improvement by more than an order of magnitude compared to a recent measurement performed in 2023 at the Cooler Storage Ring (CSRe) in Lanzhou. Although the LEBIT and CSRe mass measurements of $^{103}$Sn are in agreement, they diverge from the experimental mass value reported in the 2016 version of the Atomic Mass Evaluation (AME2016), which was derived from the measured $Q_{\beta^+}$ value and the mass of $^{103}$In. In AME2020, this indirectly measured $^{103}$Sn mass was classified as a `seriously irregular mass' and replaced with an extrapolated value, which aligns with the most recent measured values from CSRe and LEBIT. As such, the smoothness of the mass surface is confidently reestablished for $^{103}$Sn. Furthermore, LEBIT's mass measurement of $^{103}$Sn enabled a significant reduction in the mass uncertainties of five parent isotopes which are now dominated by uncertainties in their respective $Q$-values.

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Precision Mass Measurement of Proton-Dripline Halo Candidate $^{22}$Al

We report the first mass measurement of the proton-halo candidate $^{22}$Al performed with the LEBIT facility's 9.4~T Penning trap mass spectrometer at FRIB. This measurement completes the mass information for the lightest remaining proton-dripline nucleus achievable with Penning traps. $^{22}$Al has been the subject of recent interest regarding a possible halo structure from the observation of an exceptionally large isospin asymmetry [Phys. Rev. Lett. \textbf{125} 192503 (2020)]. The measured mass excess value of $\text{ME}=18\;093.6(7)$~keV, corresponding to an exceptionally small proton separation energy of $S_p = 99.2(1.0)$~keV, is compatible with the suggested halo structure. Our result agrees well with predictions from \textit{sd}-shell USD Hamiltonians. While USD Hamiltonians predict deformation in $^{22}$Al ground-state with minimal $1s_{1/2}$ occupation in the proton shell, a particle-plus-rotor model in the continuum suggests that a proton halo could form at large quadrupole deformation. These results emphasize the need for a charge radius measurement to conclusively determine the halo nature.

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First direct $^{7}$Be electron capture $Q$-value measurement towards high-precision BSM neutrino physics searches

We report the first direct measurement of the nuclear electron capture (EC) decay $Q$-value of $^{7}$Be $\rightarrow$ $^{7}$Li via high-precision Penning trap mass spectrometry (PTMS). This was performed using the LEBIT Penning trap located at the National Superconducting Cyclotron Laboratory/Facility for Rare Isotope Beams (NSCL/FRIB) using the newly commissioned Batch-Mode Ion-Source (BMIS) to deliver the unstable $^{7}$Be$^{+}$ samples. With a measured value of $Q_{EC}$ = 861.963(23) keV this result is also three times more precise than any previous determination of this quantity. This improved precision, and accuracy of the $^7$Be EC decay $Q$-value is critical for ongoing experiments that measure the recoiling nucleus in this system as a signature to search for beyond Standard Model (BSM) neutrino physics using $^7$Be-doped superconducting sensors.

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Mass Measurement of $^{27}$P to Constrain Type-I X-ray Burst Models and Validate the IMME for the A=27, T=$\frac{3}{2}$ Isospin Quartet

Light curves are the primary observable of type-I x-ray bursts. Computational x-ray burst models must match simulations to observed light curves. Most of the error in simulated curves comes from uncertainties in $rp$ process reaction rates, which can be reduced via precision mass measurements of neutron-deficient isotopes in the $rp$ process path. We perform a precise Penning trap mass measurement of $^{27}$P utilizing the ToF-ICR technique. We use this measurement to calculate $rp$ process reaction rates and input these rates into an x-ray burst model to reduce simulated light curve uncertainty. We also use the mass measurement of $^{27}$P to validate the Isobaric Multiplet Mass Equation (IMME) for the A=27 T=$\frac{3}{2}$ isospin quartet which $^{27}$P belongs to. The mass excess of $^{27}$P was measured to be -670.7(6) keV, a fourteen-fold precision increase over the mass reported in the 2020 Atomic Mass Evaluation (AME2020). X-ray burst light curves were produced with the MESA (Modules for Experiments in Stellar Astrophysics) code using the new mass and associated reaction rates. Changes in the mass of $^{27}$P seem to have minimal effect on light curves, even in burster systems tailored to maximize impact. The mass of $^{27}$P does not play a significant role in x-ray burst light curves. It is important to understand that more advanced models do not just provide more precise results, but often qualitatively different ones. This result brings us a step closer to extracting stellar parameters from individual x-ray burst observations. The IMME has been validated for the $A=27, T=3/2$ quartet. The normal quadratic form of the IMME using the latest data yields a reduced $\chi^2$ of 2.9. The cubic term required to generate an exact fit to the latest data matches theoretical attempts to predict this term.

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Identification of a potential ultra-low Q value electron capture decay branch in $^{75}$Se via a precise Penning trap measurement of the mass of $^{75}$As

Background: Low energy $\beta$ and electron capture (EC) decays are important systems in neutrino mass determination experiments. An isotope with an ultra-low Q value $\beta$-decay to an excited state in the daughter with Qes < 1 keV could provide a promising alternative candidate for future experiments. $^{75}$Se EC and $^{75}$Ge $\beta$-decay represent such candidates, but a more precise determination of the mass of the common daughter, $^{75}$As, is required to evaluate whether their potential decay branches are energetically allowed and ultra-low. Purpose: Perform a precise atomic mass measurement of $^{75}$As and combine the result with the precisely known atomic masses of $^{75}$Se and $^{75}$Ge, along with nuclear energy level data for $^{75}$As to evaluate potential ultra-low Q value decay branches in the EC decay of $^{75}$Se and the $\beta$-decay of $^{75}$Ge. Method: The LEBIT Penning trap mass spectrometer at the Facility for Rare Isotope Beams was used to perform a high-precision measurement of the atomic mass of $^{75}$As via cyclotron frequency ratio measurements of $^{75}$As$^{+}$ to a $^{12}$C$_{6}^{+}$ reference ion. Results: The $^{75}$As mass excess was determined to be ME($^{75}$As)= -73 035.98(43) keV, from which the ground-state to ground-state Q values for $^{75}$Se EC and $^{75}$Ge $\beta$-decay were determined to be 866.50(44) keV and 1179.01(44) keV, respectively. These results were compared to energies of excited states in $^{75}$As at 865.4(5) keV and 1172.0(6) keV to determine Q values of 1.1(7) keV and 7.0(7) keV for the potential ultra-low EC and $\beta$-decay branches of $^{75}$Se and $^{75}$Ge, respectively. Conclusion: The $^{75}$Se EC decay to the 865.4 keV excited state in $^{75}$As is potentially ultra-low with Qes $\approx$ 1 keV. However, a more precise determination of the 865.4(5) keV level in $^{75}$As is required.

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Measurements and computational analysis on the natural decay of $^{176}$Lu

Mainly because of its long half-life and despite its scientific relevance, spectroscopic measurements of $^{176}$Lu forbidden $\beta$-decays are very limited and lack formulation of shape factors. A direct precise measurement of its $Q$ value is also presently unreported. In addition, the description of forbidden decays provides interesting challenges for nuclear theory. The comparison of precise experimental results with theoretical calculations for these decays can help to test underlying models and can aid the interpretation of data from other experiments.

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High-precision mass measurement of $^{24}$Si and a refined determination of the $rp$ process at the $A=22$ waiting point

We report a high precision mass measurement of $^{24}{\rm Si}$, performed with the LEBIT facility at the National Superconducting Cyclotron Laboratory. The atomic mass excess, $10\;753.8$(37) keV, is a factor of 5 more precise than previous results. This substantially reduces the uncertainty of the $^{23}{\rm Al}(p,\gamma)^{24}{\rm Si}$ reaction rate, which is a key part of the rapid proton capture ($rp$) process powering Type I X-ray bursts. The updated rate constrains the onset temperature of the $(\alpha,p)$ process at the $^{22}{\rm Mg}$ waiting-point to a precision of 9%.

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Investigating nuclear structure near $N = 32$ and $N = 34$: Precision mass measurements of neutron-rich Ca, Ti and V isotopes

Nuclear mass measurements of isotopes are key to improving our understanding of nuclear structure across the chart of nuclides, in particular for the determination of the appearance or disappearance of nuclear shell closures. We present high-precision mass measurements of neutron-rich Ca, Ti and V isotopes performed at the TITAN and LEBIT facilities. These measurements were made using the TITAN multiple-reflection time-of-flight mass spectrometer (MR-ToF-MS) and the LEBIT 9.4T Penning trap mass spectrometer. In total, 13 masses were measured, eight of which represent increases in precision over previous measurements. These measurements refine trends in the mass surface around $N = 32$ and $N = 34$, and support the disappearance of the $N = 32$ shell closure with increasing proton number. Additionally, our data does not support the presence of a shell closure at $N = 34$.

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Improved Nuclear Physics Near $A=61$ Refines Urca Neutrino Luminosities in Accreted Neutron Star Crusts

We performed a Penning trap mass measurement of $^{61}{\rm Zn}$ at the National Superconducting Cyclotron Laboratory and NuShellX calculations of the $^{61}{\rm Zn}$ and $^{62}{\rm Ga}$ structure using the GXPF1A Hamiltonian to obtain improved estimates of the $^{61}{\rm Zn}(p,\gamma)^{62}{\rm Ga}$ and $^{60}{\rm Cu}(p,\gamma)^{61}{\rm Zn}$ reaction rates. Surveying astrophysical conditions for type-I X-ray bursts with the code MESA, implementing our improved reaction rates, and taking into account updated nuclear masses for $^{61}{\rm V}$ and $^{61}{\rm Cr}$ from the recent literature, we refine the neutrino luminosity from the important mass number $A=61$ urca cooling source in accreted neutron star crusts. This improves our understanding of the thermal barrier between deep heating in the crust and the shallow depths where extra heat is needed to explain X-ray superbursts, as well as the expected signature of crust urca neutrino emission in light curves of cooling transients.

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Lightweight self-conjugate nucleus $^{80}$Zr

Protons and neutrons in the atomic nucleus move in shells analogous to the electronic shell structures of atoms. Nuclear shell structure varies across the nuclear landscape due to changes of the nuclear mean field with the number of neutrons $N$ and protons $Z$. These variations can be probed with mass differences. The $N=Z=40$ self-conjugate nucleus $^{80}$Zr is of particular interest as its proton and neutron shell structures are expected to be very similar, and its ground state is highly deformed. In this work, we provide evidence for the existence of a deformed double shell closure in $^{80}$Zr through high precision Penning trap mass measurements of $^{80-83}$Zr. Our new mass values show that $^{80}$Zr is significantly lighter, and thus more bound than previously determined. This can be attributed to the deformed shell closure at $N=Z=40$ and the large Wigner energy. Our statistical Bayesian model mixing analysis employing several global nuclear mass models demonstrates difficulties with reproducing the observed mass anomaly using current theory.

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Particle-in-Cell Techniques for the Study of Space Charge Effects in the Advanced Cryogenic Gas Stopper

Linear gas stoppers are widely used to convert high-energy, rare-isotope beams and reaction products into low-energy beams with small transverse emittance and energy spread. Stopping of the high-energy ions is achieved through interaction with a buffer gas, typically helium, generating large quantities of He$^+$/e$^-$ pairs. The Advanced Cryogenic Gas Stopper (ACGS) was designed for fast, efficient stopping and extraction of high-intensity, rare-isotope beams. As part of the design process, a comprehensive particle-in-cell code was developed to optimize the transport and extraction of rare isotopes from the ACGS in the presence of space charge, including He$^+$/e$^-$ dynamics, buffer gas interactions including gas flow, RF carpets, and ion extraction through a nozzle or orifice. Details of the simulations are presented together with comparison to experiment when available.

physics.acc-ph

Precision mass measurements of neutron-rich scandium isotopes refine the evolution of $N=32$ and $N=34$ shell closures

We report high-precision mass measurements of $^{50-55}$Sc isotopes performed at the LEBIT facility at NSCL and at the TITAN facility at TRIUMF. Our results provide a substantial reduction of their uncertainties and indicate significant deviations, up to 0.7 MeV, from the previously recommended mass values for $^{53-55}$Sc. The results of this work provide an important update to the description of emerging closed-shell phenomena at neutron numbers $N=32$ and $N=34$ above proton-magic $Z=20$. In particular, they finally enable a complete and precise characterization of the trends in ground state binding energies along the $N=32$ isotone, confirming that the empirical neutron shell gap energies peak at the doubly-magic $^{52}$Ca. Moreover, our data, combined with other recent measurements, does not support the existence of closed neutron shell in $^{55}$Sc at $N=34$. The results were compared to predictions from both \emph{ab initio} and phenomenological nuclear theories, which all had success describing $N=32$ neutron shell gap energies but were highly disparate in the description of the $N=34$ isotone.

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First Penning trap mass measurement of $^{36}$Ca

Isobaric quintets provide the best test of the isobaric multiplet mass equation (IMME) and can uniquely identify higher order corrections suggestive of isospin symmetry breaking effects in the nuclear Hamiltonian. The Generalized IMME (GIMME) is a novel microscopic interaction theory that predicts an extension to the quadratic form of the IMME. Only the $A=20, 32$ $T=2$ quintets have the exotic $T_z = -2$ member ground state mass determined to high-precision by Penning trap mass spectrometry. In this work, we establish $A=36$ as the third high-precision $T=2$ isobaric quintet with the $T_z = -2$ member ground state mass measured by Penning trap mass spectrometry and provide the first test of the predictive power of the GIMME. A radioactive beam of neutron-deficient $^{36}$Ca was produced by projectile fragmentation at the National Superconducting Cyclotron Laboratory. The beam was thermalized and the mass of $^{36}$Ca$^+$ and $^{36}$Ca$^{2+}$ measured by the Time of Flight - Ion Cyclotron Resonance method in the LEBIT 9.4 T Penning trap. We measure the mass excess of $^{36}$Ca to be ME$ = -6483.6(56)$ keV, an improvement in precision by a factor of 6 over the literature value. The new datum is considered together with evaluated nuclear data on the $A=36$, $T=2$ quintet. We find agreement with the quadratic form of the IMME given by isospin symmetry, but only coarse qualitative agreement with predictions of the GIMME. A total of three isobaric quintets have their most exotic members measured by Penning trap mass spectrometry. The GIMME predictions in the $T = 2$ quintet appear to break down for $A = 32$ and greater.

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High precision mass measurements of the isomeric and ground states of $^{44}$V: improving constraints on the IMME parameters of the A=44, $\text{0}^{\text{+}}$ quintet

The Isobaric Multiplet Mass Equation (IMME) has been successful at predicting the masses of isobaric analogue states in the same multiplet, while its coefficients are known to follow trends as functions of mass number. The Atomic Mass Evaluation 2016 [Chin. Phys. C 41, 030003 (2017)] $^{44}$V mass value results in an negative $c$ coefficient for the IMME quadratic term. The $b$ and $c$ coefficients can provide constraints for construction of the isospin-nonconserving (INC) Hamiltonians for the $pf$ shell. The excitation energy of the $0^+, T=2$ level in $^{44}$V is currently unknown and can be used to constrain the $^{44}$Cr mass. The aim of the experiment was to perform high-precision mass measurements to resolve the difference between $^{44}$V isomeric and ground states, to test the IMME, and to provide ingredients for identifying the $0^+$, $T=2$ state in $^{44}$V. High-precision Penning trap mass spectrometry was performed at LEBIT, to measure the cyclotron frequency ratios of [$^{44g,m}$VO]$^+$ versus [$^{32}$SCO]$^+$, a reference mass, to extract both the isomeric and ground state masses of $^{44}$V. The mass excess of the ground and isomeric states in $^{44}$V were measured to be $-23\ 804.9(80)$ keV/$\text{c}^2$ and $-23\ 537.0(55)$ keV/$\text{c}^2$. This yielded a new proton separation energy of $S_p$ = 1\ 773(10) keV. The new mass values of $^{44}$V have been used to deduce the IMME $b$ and $c$ coefficients of the lowest $2^+$ and $6^+$ triplets in $A=44$. The $2^+$ $c$ coefficient is verified with the IMME trend and agrees with the shell-model predictions using charge-dependent Hamiltonians. The mirror energy differences were determined between $^{44}$V and $^{44}$Sc, in line with isospin-symmetry. The new value of the proton separation energy determined will be important for the determination of the $0^+$, $T=2$ state in $^{44}$V and for prediction of the mass of $^{44}$Cr.

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