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G. D. Gu

Publications and source records attributed to G. D. Gu.

At least 73 records · Page 4Linked to original sources
arXiv2020

Absence of $μ$SR evidence for magnetic order in the pseudogap phase of Bi$_{2+x}$Sr$_{2-x}$CaCu$_2$O$_{8+δ}$

We present an extended zero-field muon spin relaxation (ZF-$μ$SR) study of overdoped Bi$_{2+x}$Sr$_{2-x}$CaCu$_2$O$_{8+δ}$ (Bi2212) single crystals, intended to elucidate the origin of weak quasistatic magnetism previously detected by $μ$SR in the superconducting and normal states of optimally-doped and overdoped samples. New results on heavily-overdoped single crystals show a similar monotonically decreasing ZF-$μ$SR relaxation rate with increasing temperature that persists above the pseudogap (PG) temperature $T^*$ and does not evolve with hole doping ($p$). Additional measurements using an ultra-low background apparatus confirm that this behavior is an intrinsic property of Bi2212, which cannot be due to magnetic order associated with the PG phase. Instead we show that the temperature-dependent relaxation rate is most likely caused by structural changes that modify the contribution of the nuclear dipole fields to the ZF-$μ$SR signal. Our results for Bi2212 emphasize the importance of not assuming the nuclear-dipole field contribution is independent of temperature in ZF-$μ$SR studies of high-temperature (high-$T_c$) cuprate superconductors, and do not support a recent $μ$SR study of YBa$_2$Cu$_3$O$_{6+x}$ that claims to detect magnetic order in the PG phase.

cond-mat.supr-con↗
arXiv2020

Nature of the charge-density wave excitations in cuprates

The discovery of charge-density wave (CDW)-related effects in the resonant inelastic x-ray scattering (RIXS) spectra of cuprates holds the tantalizing promise of clarifying the interactions that stabilize the electronic order. Here, we report a comprehensive RIXS study of La2-xSrxCuO4 (LSCO) finding that CDW effects persist up to a remarkably high doping level of x = 0.21 before disappearing at x = 0.25. The inelastic excitation spectra remain essentially unchanged with doping despite crossing a topological transition in the Fermi surface. This indicates that the spectra contain little or no direct coupling to electronic excitations near the Fermi surface, rather they are dominated by the resonant cross-section for phonons and CDW-induced phonon-softening. We interpret our results in terms of a CDW that is generated by strong correlations and a phonon response that is driven by the CDW-induced modification of the lattice.

cond-mat.supr-con↗
arXiv2020

Reconstruction of the Bi$_2$Sr$_2$CaCu$_2$O$_{8+δ}$ Fermi Surface

The effects of structural supermodulation with the period $λ\approx26$ Å\ along the $b$-axis of Bi$_2$Sr$_2$CaCu$_2$O$_{8+δ}$ have been observed in photoemission studies from the early days as the presence of diffraction replicas of the intrinsic electronic structure. Although predicted to affect the electronic structure of the Cu-O plane, the influence of supermodulation potential on Cu-O electrons has never been observed in photoemission. In the present study, we clearly see, for the first time, the effects on the Bi$_2$Sr$_2$CaCu$_2$O$_{8+δ}$ electronic structure - we observe a hybridization of the intrinsic bands with the supermodulation replica bands in the form of avoided crossings and a corresponding reconstruction of the Fermi surface. We estimate the hybridization gap, $2Δ_h\sim25$ meV in the slightly underdoped samples. The hybridization weakens with doping and the anti-crossing can no longer be resolved in strongly overdoped samples. In contrast, the shadow replica, shifted by $(π, π)$, is found not to hybridize with the original bands within our detection limits.

cond-mat.supr-con↗
arXiv2019

Probing intraband excitations in ZrTe$_5$: a high-pressure infrared and transport study

Zirconium pentatetelluride, ZrTe5, shows remarkable sensitivity to hydrostatic pressure. In this work we address the high-pressure transport and optical properties of this compound, on samples grown by flux and charge vapor transport. The high-pressure resistivity is measured up to 2 GPa, and the infrared transmission up to 9 GPa. The dc conductivity anisotropy is determined using a microstructured sample. Together, the transport and optical measurements allow us to discern band parameters with and without the hydrostatic pressure, in particular the Fermi level, and the effective mass in the less conducting, out-of-plane direction. The results are interpreted within a simple two-band model characterized by a Dirac-like, linear in-plane band dispersion, and a parabolic out-of-plane dispersion.

cond-mat.mtrl-sci↗
arXiv2019

Nature and impact of stripe freezing in La$_{1.67}$Sr$_{0.33}$NiO$_4$

La$_{1.67}$Sr$_{0.33}$NiO$_4$ develops charge and spin stripe orders at temperatures of roughly 200 K, with modulation wave vectors that are temperature independent. Various probes of spin and charge response have provided independent evidence for some sort of change below $\sim50$ K. In combination with a new set of neutron scattering measurements, we propose a unified interpretation of all of these observations in terms of a freezing of Ni-centered charges stripes, together with a glassy ordering of the spin stripes that shows up in neutron scattering as a slight rotation of the average spin direction.

cond-mat.str-el↗
arXiv2019

Evidence for photoinduced sliding of the charge-order condensate in La$_{1.875}$Ba$_{0.125}$CuO$_4$

We use femtosecond resonant soft x-ray scattering to measure the ultrafast optical melting of charge-order correlations in La$_{1.875}$Ba$_{0.125}$CuO$_4$. By analyzing both the energy-resolved and energy-integrated order parameter dynamics, we find evidence of a short-lived nonequilibrium state, whose features are compatible with a sliding charge density wave coherently set in motion by the pump. This transient state exhibits shifts in both the quasielastic line energy and its wave vector, as expected from a classical Doppler effect. The wave vector change is indeed found to directly follow the pump propagation direction. These results demonstrate the existence of sliding charge order behavior in an unconventional charge density wave system and underscore the power of ultrafast optical excitation as a tool to coherently manipulate electronic condensates.

cond-mat.str-el↗
arXiv2019

Crossover of Charge Fluctuations across the Strange Metal Phase Diagram

A normal metal exhibits a valence plasmon, which is a sound wave in its conduction electron density. The mysterious strange metal is characterized by non-Boltzmann transport and violates most fundamental Fermi liquid scaling laws. A fundamental question is: Do strange metals have plasmons? Using momentum-resolved inelastic electron scattering (M-EELS) we recently showed that, rather than a plasmon, optimally-doped Bi$_{2.1}$Sr$_{1.9}$Ca$_{1.0}$Cu$_{2.0}$O$_{8+x}$ (Bi-2212) exhibits a featureless, temperature-independent continuum with a power-law form over most energy and momentum scales [M. Mitrano, PNAS 115, 5392-5396 (2018)]. Here, we show that this continuum is present throughout the fan-shaped, strange metal region of the phase diagram. Outside this region, dramatic changes in spectral weight are observed: In underdoped samples, spectral weight up to 0.5 eV is enhanced at low temperature, biasing the system towards a charge order instability. The situation is reversed in the overdoped case, where spectral weight is strongly suppressed at low temperature, increasing quasiparticle coherence in this regime. Optimal doping corresponds to the boundary between these two opposite behaviors at which the response is temperature-independent. Our study suggests that plasmons do not exist as well-defined excitations in Bi-2212, and that a featureless continuum is a defining property of the strange metal, which is connected to a peculiar crossover where the spectral weight change undergoes a sign reversal.

cond-mat.str-el↗
arXiv2019

Signature of Dispersing 1D Majorana Channels in an Iron-based Superconductor

The possible realization of Majorana fermions as quasiparticle excitations in condensed matter physics has created much excitement. Most recent studies have focused on Majorana bound states which can serve as topological qubits. More generally, akin to elementary particles, Majorana fermions can propagate and display linear dispersion. These excitations have not yet been directly observed, and can also be used for quantum information processing. One route to realizing this is in a line junction between two phase-shifted superconductors coupled to topological surface states. Recent theory indicates that in iron-based superconductors, a particular type of crystalline defect, i.e., a domain wall (DW) between two regions with a half-unit cell shift between them, should create a $π$-phase shift in the superconducting order parameter. Combined with recent data showing topological surface states in FeSe$_x$Te$_{1-x}$ we find that this is the ideal system to realize helical 1D-dispersing Majorana modes. Here we report scanning tunneling spectroscopic (STS) measurements of crystalline DWs in FeSe$_{0.45}$Te$_{0.55}$. By analyzing large-area superconducting gap maps, we identify the gap in the topological surface state, demonstrating that our sample is an effective Fu-Kane proximitized topological system. We further locate DWs across which the atoms shift by half a unit cell. STS data on these DWs reveal a flat density of states inside the superconducting gap, a hallmark of linearly dispersing modes in 1D. This unique signature is absent in DWs in the related superconductor, FeSe which is not in the topological phase. Our combined data are consistent with the observation of dispersing Majorana states at a $π$-phase shift DW in a proximitized topological material.

cond-mat.supr-con↗
arXiv2019

Two-dimensional conical dispersion in ZrTe5 evidenced by optical spectroscopy

Zirconium pentatelluride was recently reported to be a 3D Dirac semimetal, with a single conical band, located at the center of the Brillouin zone. The cone's lack of protection by the lattice symmetry immediately sparked vast discussions about the size and topological/trivial nature of a possible gap opening. Here we report on a combined optical and transport study of ZrTe5, which reveals an alternative view of electronic bands in this material. We conclude that the dispersion is approximately linear only in the a-c plane, while remaining relatively flat and parabolic in the third direction (along the b axis). Therefore, the electronic states in ZrTe5 cannot be described using the model of 3D Dirac massless electrons, even when staying at energies well above the band gap 6 meV found in our experiments at low temperatures.

cond-mat.mes-hall↗
arXiv2019

Low-energy phonons in Bi$_2$Sr$_2$CaCu$_2$O$_{8+δ}$ and their possible interaction with electrons measured by inelastic neutron scattering

Electron-phonon interaction in copper oxide superconductors is still enigmatic. Strong coupling for certain optic phonons is now well established experimentally, but theoretical understanding is challenging. Scattering of electrons near the Fermi surface by the longitudinal acoustic (LA) phonons is expected from basic theory because these phonons modulate electron density. We used inelastic neutron scattering on a large single crystal sample of optimally-doped Bi$_2$Sr$_2$CaCu$_2$O$_{8+δ}$ to show that low-energy LA phonons could couple to electronic density fluctuations only at small phonon wavevectors, which naturally limits any interaction to forward scattering. Such scattering should not be pairbreaking in the case of the d-wave gap. We also found that previously the reported low energy phonon spectral weight half-way to the zone boundary is consistent with conventional lattice dynamics and does not reflect an incipient charge density wave.

cond-mat.supr-con↗
arXiv2019

Scaling Behaviour of Low-Temperature Orthorhombic Domains in Prototypical High-Temperature Superconductor La$_{1.875}$Ba$_{0.125}$CuO$_{4}$

Translational/rotational symmetry breaking and recovery in condensed matter systems are closely related to exotic physical properties such as superconductivity (SC), magnetism, spin density waves (SDW) and charge density waves (CDW). The interplay between different order parameters is intricate and often subject to intense debate, as in the case of CDW order and superconductivity. In La1:875Ba0:125CuO4 (LBCO), the locations of CDW domains are found to be pinned on the nanometer size scale. Coherent X-ray diffraction techniques open routes to directly visualize the domain structures associated with these symmetry changes. We have pushed Bragg Coherent Diffractive Imaging (BCDI) into the cryogenic regime where most phase transitions in quantum materials reside. Utilizing BCDI, we image the structural evolution of LBCO microcrystal samples during the high-temperature-tetragonal (HTT) to low-temperature-orthorhombic (LTO) phase transition. Our results show the formation of LTO domains close to the transition temperature and how the domain size varies with temperature. The LTO domain size is shown to decrease with temperature and to be inversely proportional to the magnitude of the orthorhombic distortion. The number of domains follows the secondary order parameter (or orthorhombic strain) measurement with a critical exponent that is consistent with the 3D universality class.

cond-mat.mes-hall↗
arXiv2019

Formation of Incommensurate Charge Density Waves in Cuprates

Although charge density waves (CDWs) are omnipresent in cuprate high-temperature superconductors, they occur at significantly different wavevectors, confounding efforts to understand their formation mechanism. Here, we use resonant inelastic x-ray scattering to investigate the doping- and temperature-dependent CDW evolution in La2-xBaxCuO4 (x=0.115-0.155). We discovered that the CDW develops in two stages with decreasing temperature. A precursor CDW with quasi-commensurate wavevector emerges first at high-temperature. This doping-independent precursor CDW correlation originates from the CDW phase mode coupled with a phonon and "seeds" the low-temperature CDW with strongly doping dependent wavevector. Our observation reveals the precursor CDW and its phase mode as the building blocks of the highly intertwined electronic ground state in the cuprates.

cond-mat.supr-con↗
arXiv2019

Large surface conductance and two-dimensional superconductivity in microstructured crystalline topological insulators

Controllable geometric manipulation via micromachining techniques provides a promising tool for enhancing useful topological electrical responses relevant to future applications such as quantum information science. Here we present microdevices fabricated with focused ion beam from indium-doped topological insulator Pb1-xSnxTe. With device thickness on the order of 1 μm and an extremely large bulk resistivity, we achieve an unprecedented enhancement of the surface contribution to about 30% of the total conductance near room temperature. The surface contribution increases as the temperature is reduced, becoming dominant below approximately 180 K, compared to 30 K in mm-thickness crystals. In addition to the enhanced surface contribution to normal-state transport, we observe the emergence of a two-dimensional superconductivity below 6 K. Measurements of magnetoresistivity at high magnetic fields reveal a weak antilocalization behavior in the normal-state magnetoconductance at low temperature and a variation in the power-law dependence of resistivity on temperature with field. These results demonstrate that interesting electrical response relevant to practical applications can be achieved by suitable engineering of single crystals.

cond-mat.mtrl-sci↗
arXiv2019

Evidence for Helical Hinge Zero Modes in an Fe-Based Superconductor

Combining topology and superconductivity provides a powerful tool for investigating fundamental physics as well as a route to fault-tolerant quantum computing. There is mounting evidence that the Fe-Based Superconductor FeTe$_{0.55}$Se$_{0.45}$ (FTS) may also be topologically non-trivial. Should the superconducting order be s$^{\pm}$, then FTS could be a higher order topological superconductor with Helical Hinge Zero Modes (HHZM).To test the presence of these modes we developed a new method for making normal metal/superconductor junctions via 2D atomic crystal heterostructures. As expected,junctions in contact with the hinge reveal a sharp zero-bias anomaly whose suppression with temperature and magnetic field only along the c-axis are completely consistent with the presence of HHZM. This feature is completely absent when tunneling purely into the c-axis, and its characteristics are also inconsistent with other origins of zero bias anomalies. Furthermore, additional measurements with soft-point contacts in bulk samples with various Fe interstitial contents demonstrate the intrinsic nature of the observed mode. Thus we provide evidence that FTS is indeed a higher order topological superconductor as well as a new method for probing 2D atomic crystals.

cond-mat.supr-con↗
arXiv2019

Tuning from failed superconductor to failed insulator with magnetic field

Do charge modulations compete with electron pairing in high-temperature copper-oxide superconductors? We investigated this question by suppressing superconductivity in a stripe-ordered cuprate compound at low temperature with high magnetic fields. With increasing field, loss of three-dimensional superconducting order is followed by reentrant two-dimensional superconductivity and then an ultra-quantum metal phase. Circumstantial evidence suggests that the latter state is bosonic and associated with the charge stripes. These results provide experimental support to the theoretical perspective that local segregation of doped holes and antiferromagnetic spin correlations underlies the electron-pairing mechanism in cuprates.

cond-mat.supr-con↗
arXiv2019

Four-legged starfish-shaped Cooper pairs with ultrashort antinodal length scales in cuprate superconductors

Cooper pairs of mutually attracting electrons form the building blocks of superconductivity. Thirty years after the discovery of high-temperature superconductivity in cuprates, many details of the pairs remain unknown, including their size and shape. Here we apply brand new ARPES-based methods that allow us to reconstruct the shape and size of the pairs in Bi$_2$Sr$_2$CaCu$_2$O$_{8+δ}$. The pairs are seen to form a characteristic starfish shape that is very long (>50Å) in the near-nodal direction but extremely short (~4.5Å) in the antinodal (Cu-O) direction. We find that this ultrashort antinodal length scale, which is of order a lattice constant, is approximately constant over a wide range of doping levels even as many other parameters including the pairing strength change. This suggests that this new length scale, along with the pair shape, is one of the most fundamental characteristics of the pairs. Further, the shape and ultrashort length scale should make the pairs create or intertwine with variations in charge and pair density, center on various types of lattice positions, and potentially explain aspects of the nematic order in these materials.

cond-mat.supr-con↗
arXiv2019

Nanocalorimetric Evidence for Nematic Superconductivity in the Doped Topological Insulator Sr$_{0.1}$Bi$_{2}$Se$_{3}$

Spontaneous rotational-symmetry breaking in the superconducting state of doped $\mathrm{Bi}_2\mathrm{Se}_3$ has attracted significant attention as an indicator for topological superconductivity. In this paper, high-resolution calorimetry of the single-crystal $\mathrm{Sr}_{0.1}\mathrm{Bi}_2\mathrm{Se}_3$ provides unequivocal evidence of a two-fold rotational symmetry in the superconducting gap by a \emph{bulk thermodynamic} probe, a fingerprint of nematic superconductivity. The extremely small specific heat anomaly resolved with our high-sensitivity technique is consistent with the material's low carrier concentration proving bulk superconductivity. The large basal-plane anisotropy of $H_{c2}$ is attributed to a nematic phase of a two-component topological gap structure $\vecη = (η_{1}, η_{2})$ and caused by a symmetry-breaking energy term $δ(|η_{1}|^{2} - |η_{2}|^{2}) T_{c}$. A quantitative analysis of our data excludes more conventional sources of this two-fold anisotropy and provides the first estimate for the symmetry-breaking strength $δ\approx 0.1$, a value that points to an onset transition of the second order parameter component below 2K.

cond-mat.supr-con↗