arXiv subjects

G. D. Gu

Publications and source records attributed to G. D. Gu.

At least 91 records · Page 5Linked to original sources

arXiv2019

Disorder raises the critical temperature of a cuprate superconductor

With the discovery of charge density waves (CDW) in most members of the cuprate high temperature superconductors, the interplay between superconductivity and CDW has become a key point in the debate on the origin of high temperature superconductivity. Some experiments in cuprates point toward a CDW state competing with superconductivity, but others raise the possibility of a CDW-superconductivity intertwined order, or more elusive pair-density wave (PDW). Here we have used proton irradiation to induce disorder in crystals of La$_{1.875}$Ba$_{0.125}$CuO$_4$ and observed a striking 50% increase of $T_\mathrm{c}$ accompanied by a suppression of the CDW. This is in clear contradiction with the behaviour expected of a d-wave superconductor for which both magnetic and non-magnetic defects should suppress $T_\mathrm{c}$. Our results thus make an unambiguous case for the strong detrimental effect of the CDW on bulk superconductivity in La$_{1.875}$Ba$_{0.125}$CuO$_4$. Using tunnel diode oscillator (TDO) measurements, we find evidence for dynamic layer decoupling in PDW phase. Our results establish irradiation-induced disorder as a particularly relevant tuning parameter for the many families of superconductors with coexisting density waves, which we demonstrate on superconductors such as the dichalcogenides and Lu$_5$Ir$_4$Si$_{10}$.

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arXiv2019

Gapless spin excitations in superconducting La$_{2-x}$Ca$_{1+x}$Cu$_{2}$O$_{6}$ with $T_c$ up to 55 K

We report inelastic neutron scattering on single crystals of the bilayer cuprate family La$_{2-x}$Ca$_{1+x}$Cu$_{2}$O$_{6+δ}$, including two crystals made superconducting (transitions at 45 and 55 K) by high-pressure annealing in an oxygen-containing atmosphere. The magnetic excitations in the non-superconducting crystal have a similar temperature-dependence as those in weakly hole-doped cuprates. In the superconducting crystals, there is a near-uniform suppression of the magnetic spectral weight with increasing temperature; in particular, there are no signs of a spin gap or "resonance" peak. This is different from the temperature dependence seen in many optimally-doped cuprates but similar to the behavior seen in certain underdoped cuprates. We discuss the possible connection with pair-density-wave superconductivity.

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arXiv2019

Disappearance of Superconductivity Due to Vanishing Coupling in the Overdoped Bi$_2$Sr$_2$CaCu$_2$O$_{8+δ}$

In high-temperature cuprate superconductors, superconductivity is accompanied by a "plethora of orders", and phenomena that may compete, or cooperate with superconductivity, but which certainly complicate our understanding of origins of superconductivity in these materials. While prominent in the underdoped regime, these orders are known to significantly weaken or completely vanish with overdoping. Here, we approach the superconducting phase from the more conventional highly overdoped side. We present angle-resolved photoemission spectroscopy (ARPES) studies of Bi$_2$Sr$_2$CaCu$_2$O$_{8+δ}$ (Bi2212) single crystals cleaved and annealed in ozone to increase the doping all the way to the metallic, non-superconducting phase. We show that the mass renormalization in the antinodal region of the Fermi surface, associated with the structure in the quasiparticle self-energy, that possibly reflects the pairing interaction, monotonically weakens with increasing doping and completely disappears precisely where superconductivity disappears. This is the direct evidence that in the overdoped regime, superconductivity is determined by the coupling strength. A strong doping dependence and an abrupt disappearance above the transition temperature ($T_{\mathrm c}$) eliminate the conventional phononic mechanism of the observed mass renormalization and identify the onset of spin-fluctuations as its likely origin.

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arXiv2019

On the interplay of paramagnetism and topology in the Fe-based High Tc Superconductors

The high Tc superconductor FeTe0.55Se0.45 has recently been shown to support a surface state with topological character. Here we use low-energy laser-based ARPES with variable light polarization, including both linear and circular polarization, to re-examine the same material and the related FeTe0.7Se0.3, with larger Te concentration. In both cases we observe the presence of a surface state displaying linear dispersion in a cone-like configuration. The use of circular polarization confirms the presence of helical spin structure. These experimental studies are compared with theoretical studies that account for the local magnetic effects related to the paramagnetism observed in this system in the normal state. In contrast to previous studies we find that including the magnetic contributions is necessary to bring the chemical potential of the calculated electronic band structure naturally into alignment with the experimental observations.

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arXiv2019

A strongly inhomogeneous superfluid in an iron-based superconductor

Among the mysteries surrounding unconventional, strongly correlated superconductors is the possibility of spatial variations in their superfluid density. We use atomic-resolution Josephson scanning tunneling microscopy to reveal a strongly inhomogeneous superfluid in the iron-based superconductor FeTe0.55Se0.45. By simultaneously measuring the topographic and electronic properties, we find that this inhomogeneity in the superfluid density is not caused by structural disorder or strong inter-pocket scattering, and does not correlate with variations in Cooper pair-breaking gap. Instead, we see a clear spatial correlation between superfluid density and quasiparticle strength, putting the iron-based superconductors on equal footing with the cuprates and demonstrating that locally, the quasiparticles are sharpest when the superconductivity is strongest. When repeated at different temperatures, our technique could further help elucidate what local and global mechanisms limit the critical temperature in unconventional superconductors.

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arXiv2018

Magnetic-Field Tuning of Light-Induced Superconductivity in Striped La$_{2-x}$Ba$_x$CuO$_4$

Optical excitation of stripe-ordered La$_{2-x}$Ba$_x$CuO$_4$ has been shown to transiently enhance superconducting tunneling between the CuO$_2$ planes. This effect was revealed by a blue-shift, or by the appearance of a Josephson Plasma Resonance in the terahertz-frequency optical properties. Here, we show that this photo-induced state can be strengthened by the application of high external magnetic fields oriented along the c-axis. For a 7-Tesla field, we observe up to a ten-fold enhancement in the transient interlayer phase correlation length, accompanied by a two-fold increase in the relaxation time of the photo-induced state. These observations are highly surprising, since static magnetic fields suppress interlayer Josephson tunneling and stabilize stripe order at equilibrium. We interpret our data as an indication that optically-enhanced interlayer coupling in La$_{2-x}$Ba$_x$CuO$_4$ does not originate from a simple optical melting of stripes, as previously hypothesized. Rather, we speculate that the photo-induced state may emerge from activated tunneling between optically-excited stripes in adjacent planes.

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arXiv2018

Low-energy antiferromagnetic spin fluctuations limit the coherent superconducting gap in cuprates

Motivated by recent attention to a potential antiferromagnetic quantum critical point at $x_c\sim 0.19$, we have used inelastic neutron scattering to investigate the low-energy spin excitations in crystals of La$_{2-x}$Sr$_x$CuO$_4$ bracketing $x_c$. We observe a peak in the normal-state spin-fluctuation weight at $\sim20$~meV for both $x=0.21$ and 0.17, inconsistent with quantum critical behavior. The presence of the peak raises the question of whether low-energy spin fluctuations limit the onset of superconducting order. Empirically evaluating the spin gap $Δ_{\rm spin}$ in the superconducting state, we find that $Δ_{\rm spin}$ is equal to the coherent superconducting gap $Δ_c$ determined by electronic spectroscopies. To test whether this is a general result for other cuprate families, we have checked through the literature and find that $Δ_c\leΔ_{\rm spin}$ for cuprates with uniform $d$-wave superconductivity. We discuss the implications of this result.

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arXiv2018

Phase Diagram of Bi$_2$Sr$_2$CaCu$_2$O$_{8+δ}$ Revisited

In cuprate superconductors, the doping of carriers into the parent Mott insulator induces superconductivity and various other phases whose characteristic temperatures are typically plotted versus the doping level $p$. In most materials, $p$ cannot be determined from the chemical composition, but it is derived from the superconducting transition temperature, $T_\mathrm{c}$, using the assumption that $T_\mathrm{c}$ dependence on doping is universal. Here, we present angle-resolved photoemission studies of Bi$_2$Sr$_2$CaCu$_2$O$_{8+δ}$, cleaved and annealed in vacuum or in ozone to reduce or increase the doping from the initial value corresponding to $T_\mathrm{c}=91$ K. We show that $p$ can be determined from the underlying Fermi surfaces and that $in-situ$ annealing allows mapping of a wide doping regime, covering the superconducting dome and the non-superconducting phase on the overdoped side. Our results show a surprisingly smooth dependence of the inferred Fermi surface with doping. In the highly overdoped regime, the superconducting gap approaches the value of $2Δ_0=(4\pm1)k_\mathrm{B}T_\mathrm{c}$

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arXiv2018

Signatures of pair-density wave order in phase-sensitive measurements of La$_{2-x}$Ba$_x$CuO$_4$-Nb Josephson junctions and SQUIDs

The interplay of charge order, spin order, and superconductivity in La$_{2-x}$Ba$_x$CuO$_4$ creates a complex physical system that hosts several interesting phases, such as two-dimensional superconductivity within the CuO$_2$ planes and the ordered pair-density wave state in which charge ordering is intertwined with superconductivity. Using Josephson interferometry techniques, we measure the current-phase relation of junctions and SQUIDs incorporating this material and observe a significant sin($2ϕ$)-component indicative of closely-spaced alternations of the sign of the Josephson coupling predicted by the pair-density wave model. We find that the ratio of the sin(2$ϕ$)-component to the conventional sin($ϕ$)-component to be largest near x=1/8 doping, where the pair-density wave state is believed to be the strongest, and that it increases with increasing temperature as the Josephson coupling in the junction weakens.

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arXiv2018

Sign reversing Hall effect in atomically thin high temperature superconductors

We fabricate van der Waals heterostructure devices using few unit cell thick Bi$_2$Sr$_2$CaCu$_2$O$_{8+δ}$ for magnetotransport measurements. The superconducting transition temperature and carrier density in atomically thin samples can be maintained to close to that of the bulk samples. As in the bulk sample, the sign of the Hall conductivity is found to be opposite to the normal state near the transition temperature but with a drastic enlargement of the region of Hall sign reversal in the temperature-magnetic field phase diagram as the thickness of samples decreases. Quantitative analysis of the Hall sign reversal based on the excess charge density in the vortex core and superconducting fluctuations suggests a renormalized superconducting gap in atomically thin samples at the 2-dimensional limit.

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arXiv2018

Multiple topological states in iron-based superconductors

Topological insulators and semimetals as well as unconventional iron-based superconductors have attracted major recent attention in condensed matter physics. Previously, however, little overlap has been identified between these two vibrant fields, even though the principal combination of topological bands and superconductivity promises exotic unprecedented avenues of superconducting states and Majorana bound states (MBSs), the central building block for topological quantum computation. Along with progressing laser-based spin-resolved and angle-resolved photoemission spectroscopy (ARPES) towards high energy and momentum resolution, we have resolved topological insulator (TI) and topological Dirac semimetal (TDS) bands near the Fermi level ($E_{\text{F}}$) in the iron-based superconductors Li(Fe,Co)As and Fe(Te,Se), respectively. The TI and TDS bands can be individually tuned to locate close to $E_{\text{F}}$ by carrier doping, allowing to potentially access a plethora of different superconducting topological states in the same material. Our results reveal the generic coexistence of superconductivity and multiple topological states in iron-based superconductors, rendering these materials a promising platform for high-$T_{\text{c}}$ topological superconductivity.

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arXiv2018

Directly visualizing the sign change of d-wave superconducting gap in Bi2Sr2CaCu2O8+δ by phase-referenced quasiparticle interference

The superconducting state is achieved by the condensation of Cooper pairs and is protected by the superconducting gap. The pairing interaction between the two electrons of a Cooper pair determines the superconducting gap function. Thus, it is very pivotal to detect the gap structure for understanding the mechanism of superconductivity. In cuprate superconductors, it has been well established that the superconducting gap may have a d-wave function Δ = Δ_0cos2θ. This gap function has an alternative sign change by every pi/2 in the momentum space when the in-plane azimuthal angle theta is scanned. It is very hard to visualize this sign change. Early experiments for recommending or proving this d-wave gap function were accomplished by the specially designed phase sensitive measurements based on the Josephson effect. Here we report the measurements of scanning tunneling spectroscopy in one of the model cuprate system Bi2Sr2CaCu2O8+δ and conduct the analysis of phase-referenced quasiparticle interference (QPI). Due to the unique quasiparticle excitations in the superconducting state of cuprate, we have seen the seven basic scattering vectors that connect each pair of the terminals of the banana-shaped contour of constant quasiparticle energy (CCE). The phase-referenced QPI clearly visualizes the sign change of the d-wave gap. Our results illustrate a very effective way for determining the sign change of unconventional superconductors.

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arXiv2018

Persistent Charge Density Wave Memory in a Cuprate Superconductor

Although charge density wave (CDW) correlations appear to be a ubiquitous feature of the superconducting cuprates, their disparate properties suggest a crucial role for coupling or pinning of the CDW to lattice deformations and disorder. While diffraction intensities can demonstrate the occurrence of CDW domain formation, the lack of scattering phase information has limited our understanding of this process. Here, we report coherent resonant x-ray speckle correlation analysis, which directly determines the reproducibility of CDW domain patterns in La1.875Ba0.125CuO4 (LBCO 1/8) with thermal cycling. While CDW order is only observed below 54 K, where a structural phase transition results in equivalent Cu-O bonds, we discover remarkably reproducible CDW domain memory upon repeated cycling to temperatures well above that transition. That memory is only lost on cycling across the transition at 240(3) K that restores the four-fold symmetry of the copper-oxide planes. We infer that the structural-domain twinning pattern that develops below 240 K determines the CDW pinning landscape below 54 K. These results open a new view into the complex coupling between charge and lattice degrees of freedom in superconducting cuprates.

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arXiv2018

Continuous doping of a cuprate surface: new insights from in-situ ARPES

The cuprate superconductors distinguish themselves from the conventional superconductors in that a small variation in the carrier doping can significantly change the superconducting transition temperature (T_c), giving rise to a superconducting dome where a pseudogap (ref. 1,2) emerges in the underdoped region and a Fermi liquid appears in the overdoped region. Thus a systematic study of the properties over a wide doping range is critical for understanding the superconducting mechanism. Here, we report a new technique to continuously dope the surface of Bi2Sr2CaCu2O8+x through an ozone/vacuum annealing method. Using in-situ ARPES, we obtain precise quantities of energy gaps and the coherent spectral weight over a wide range of doping. We discover that the d-wave component of the quasiparticle gap is linearly proportional to the Nernst temperature that is the onset of superconducting vortices (ref. 3), strongly suggesting that the emergence of superconducting pairing is concomitant with the onset of free vortices, with direct implications for the onset of superconducting phase coherence at T_c and the nature of the pseudogap phenomena.

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arXiv2018

Anomalous density fluctuations in a strange metal

A central mystery in high temperature superconductivity is the origin of the so-called "strange metal," i.e., the anomalous conductor from which superconductivity emerges at low temperature. Measuring the dynamic charge response of the copper-oxides, $χ''(q,ω)$, would directly reveal the collective properties of the strange metal, but it has never been possible to measure this quantity with meV resolution. Here, we present the first measurement of $χ''(q,ω)$ for a cuprate, optimally doped Bi$_2$Sr$_2$CaCu$_2$O$_{8+x}$ ($T_c=91$ K), using momentum-resolved inelastic electron scattering. In the medium energy range 0.1-2 eV relevant to the strange metal, the spectra are dominated by a featureless, temperature- and momentum-independent continuum persisting to the eV energy scale. This continuum displays a simple power law form, exhibiting $q^2$ behavior at low energy and $q^2/ω^2$ behavior at high energy. Measurements of an overdoped crystal ($T_c=50$ K) showed the emergence of a gap-like feature at low temperature, indicating deviation from power law form outside the strange metal regime. Our study suggests the strange metal exhibits a new type of charge dynamics in which excitations are local to such a degree that space and time axes are decoupled.

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arXiv2018

Decoupled Pairing Amplitude and Electronic Coherence in Iron-Based Superconductors

Here we use angle-resolved photoemission spectroscopy to study superconductivity that emerges in two extreme cases, from a Fermi liquid phase (LiFeAs) and an incoherent bad-metal phase (FeTe0.55Se0.45). We find that although the electronic coherence can strongly reshape the single-particle spectral function in the superconducting state, it is decoupled from the maximum superconducting pairing amplitude, which shows a universal scaling that is valid for all FeSCs. Our observation excludes pairing scenarios in the BCS and the BEC limit for FeSCs and calls for a universal strong coupling pairing mechanism for the FeSCs.

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arXiv2018

Unambiguous connection between the Fermi surface topology and the pseudogap in Bi$_{2}$Sr$_2$CaCu$_2$O$_{8+d}$

We study the behavior of the pseudogap in overdoped Bi$_{2}$Sr$_2$CaCu$_2$O$_{8+d}$ by electronic Raman scattering (ERS) and angle-resolved photoemission spectroscopy (ARPES) on the same single crystals. Using both techniques we find that, unlike the superconducting gap, the pseudogap related to the anti-bonding band vanishes above the critical doping p$_c$ = 0.22. Concomitantly, we show from ARPES measurements that the Fermi surface of the anti-bonding band is hole-like below pc and becomes electron-like above p$_c$. This reveals that the appearance of the pseudogap depends on the Fermi surface topology in Bi$_{2}$Sr$_2$CaCu$_2$O$_{8+d}$ , and more generally, puts strong constraint on theories of the pseudogap phase.

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arXiv2018

Collapse of superconductivity in cuprates via ultrafast quenching of phase coherence

The possibility of driving phase transitions in low-density condensates through the loss of phase coherence alone has far-reaching implications for the study of quantum phases of matter. This has inspired the development of tools to control and explore the collective properties of condensate phases via phase fluctuations. Electrically-gated oxide interfaces, ultracold Fermi atoms, and cuprate superconductors, which are characterized by an intrinsically small phase-stiffness, are paradigmatic examples where these tools are having a dramatic impact. Here we use light pulses shorter than the internal thermalization time to drive and probe the phase fragility of the Bi$_2$Sr$_2$CaCu$_2$O$_{8+δ}$ cuprate superconductor, completely melting the superconducting condensate without affecting the pairing strength. The resulting ultrafast dynamics of phase fluctuations and charge excitations are captured and disentangled by time-resolved photoemission spectroscopy. This work demonstrates the dominant role of phase coherence in the superconductor-to-normal state phase transition and offers a benchmark for non-equilibrium spectroscopic investigations of the cuprate phase diagram.

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