arXiv subjects

G. D. Gu

Publications and source records attributed to G. D. Gu.

At least 109 records · Page 6Linked to original sources

arXiv2018

Observation of topological superconductivity on the surface of an iron-based superconductor

Topological superconductors, whose edge hosts Majorana bound states or Majorana fermions that obey non-Abelian statistics, can be used for low-decoherence quantum computations. Most of the proposed topological superconductors are realized with spin-helical states through proximity effect to BCS superconductors. However, such approaches are difficult for further studies and applications because of the low transition temperatures and complicated hetero-structures. Here by using high-resolution spin-resolved and angle-resolved photoelectron spectroscopy, we discover that the iron-based superconductor FeTe1-xSex (x = 0.45, Tc = 14.5 K) hosts Dirac-cone type spin-helical surface states at Fermi level, which open an s-wave SC gap below Tc. Our study proves that the surface states of FeTe0.55Se0.45 are 2D topologically superconducting, and thus provides a simple and possibly high-Tc platform for realizing Majorana fermions.

cond-mat.supr-con↗

arXiv2018

Remarkable Stability of Charge Density Wave Order in La$_{1.875}$Ba$_{0.125}$CuO$_4$

The occurrence of charge-density-wave (CDW) order in underdoped cuprates is now well established, although the precise nature of the CDW and its relationship with superconductivity is not. Theoretical proposals include contrasting ideas such as that pairing may be driven by CDW fluctuations or that static CDWs may intertwine with a spatially-modulated superconducting wave function. We test the dynamics of CDW order in La$_{1.825}$Ba$_{0.125}$CuO$_4$ by using x-ray photon correlation spectroscopy (XPCS) at the CDW wave vector, detected resonantly at the Cu $L_3$-edge. We find that the CDW domains are strikingly static, with no evidence of significant fluctuations up to 2\,\nicefrac{3}{4} hours. We discuss the implications of these results for some of the competing theories.

cond-mat.supr-con↗

arXiv2018

Topological Dirac semimetal phase in the iron-based superconductor Fe(Te,Se)

Topological Dirac semimetals (TDSs) exhibit bulk Dirac cones protected by time reversal and crystal symmetry, as well as surface states originating from non-trivial topology. While there is a manifold possible onset of superconducting order in such systems, few observations of intrinsic superconductivity have so far been reported for TDSs. We observe evidence for a TDS phase in FeTe$_{1-x}$Se$_x$ ($x$ = 0.45), one of the high transition temperature ($T_c$) iron-based superconductors. In angle-resolved photoelectron spectroscopy (ARPES) and transport experiments, we find spin-polarized states overlapping with the bulk states on the (001) surface, and linear magnetoresistance (MR) starting from 6 T. Combined, this strongly suggests the existence of a TDS phase, which is confirmed by theoretical calculations. In total, the topological electronic states in Fe(Te,Se) provide a promising high $T_c$ platform to realize multiple topological superconducting phases.

cond-mat.supr-con↗

arXiv2017

Incommensurate phonon anomaly and the nature of charge density waves in cuprates

While charge density wave (CDW) instabilities are ubiquitous to superconducting cuprates, the different ordering wavevectors in various cuprate families have hampered a unified description of the CDW formation mechanism. Here we investigate the temperature dependence of the low energy phonons in the canonical CDW ordered cuprate La$_{1.875}$Ba$_{0.125}$CuO$_{4}$. We discover that the phonon softening wavevector associated with CDW correlations becomes temperature dependent in the high-temperature precursor phase and changes from a wavevector of 0.238 reciprocal space units (r.l.u.) below the ordering transition temperature up to 0.3~r.l.u. at 300~K. This high-temperature behavior shows that "214"-type cuprates can host CDW correlations at a similar wavevector to previously reported CDW correlations in non-"214"-type cuprates such as YBa$_{2}$Cu$_{3}$O$_{6+δ}$. This indicates that cuprate CDWs may arise from the same underlying instability despite their apparently different low temperature ordering wavevectors.

cond-mat.supr-con↗

arXiv2017

Superconducting and normal-state anisotropy of the doped topological insulator Sr$_{0.1}$Bi$_2$Se$_3$

Sr$_x$Bi$_2$Se$_3$ and the related compounds Cu$_x$Bi$_2$Se$_3$ and Nb$_x$Bi$_2$Se$_3$ have attracted considerable interest, as these materials may be realizations of unconventional topological superconductors. Superconductivity with T$_c$ ~ 3 K in Sr$_x$Bi$_2$Se$_3$ arises upon intercalation of Sr into the layered topological insulator Bi$_2$Se$_3$. Here we elucidate the anisotropy of the normal and superconducting state of Sr$_{0.1}$Bi$_2$Se$_3$ with angular dependent magnetotransport and thermodynamic measurements. High resolution x-ray diffraction studies underline the high crystalline quality of the samples. We demonstrate that the normal state electronic and magnetic properties of Sr$_{0.1}$Bi$_2$Se$_3$ are isotropic in the basal plane while we observe a large two-fold in-plane anisotropy of the upper critical field in the superconducting state. Our results support the recently proposed odd-parity nematic state characterized by a nodal gap of $E_u$ symmetry in Sr$_x$Bi$_2$Se$_3$.

cond-mat.supr-con↗

arXiv2017

Light-induced new collective modes in La$_{1.905}$Ba$_{0.095}$CuO$_4$ superconductor

We report near and mid-infrared pump c-axis terahertz probe measurement on a superconducting single crystal La$_{1.905}$Ba$_{0.095}$CuO$_4$ with T$_c$=32 K. The measurement reveals that the pump-induced change occurs predominantly at the Josephson plasma edge position below T$_c$. Upon excited by the strong near-infrared pulses, the superconducting state is severely disturbed and incoherent quasiparticle excitations develop in frequency regime above the static plasma edge. However, within very short time delay ($\sim$1.5 ps) we observe the reappearance of a very sharp Josephson plasma edge at frequency lower than the static Josephson plasma edge and the emergence of a new light-induced Josephson mode at higher energy. The results imply that the light can induce new Josephson couplings with different coupling strengths. Similar but weaker effect is observed for the mid-infrared pump. No pump induced effect is detected above T$_c$.

cond-mat.supr-con↗

arXiv2017

Superconductivity, pairing symmetry, and disorder in the doped topological insulator Sn$_{1-x}$In$_x$Te for x $\geq$ 0.10

The temperature dependence of the London penetration depth $Δλ(T)$ in the superconducting doped topological crystalline insulator Sn$_{1-x}$In$_x$Te was measured down to 450 mK for two different doping levels, x $\approx$ 0.45 (optimally doped) and x $\approx$ 0.10 (underdoped), bookending the range of cubic phase in the compound. The results indicate no deviation from fully gapped BCS-like behavior, eliminating several candidate unconventional gap structures. Critical field values below 1 K and other superconducting parameters are also presented. The introduction of disorder by repeated particle irradiation with 5 MeV protons does not enhance $T_c$, indicating that ferroelectric interactions do not compete with superconductivity.

cond-mat.supr-con↗

arXiv2017

High-temperature charge density wave correlations in La$_{1.875}$Ba$_{0.125}$CuO$_{4}$ without spin-charge locking

Although all superconducting cuprates display charge-ordering tendencies, their low-temperature properties are distinct, impeding efforts to understand the phenomena within a single conceptual framework. While some systems exhibit stripes of charge and spin, with a locked periodicity, others host charge density waves (CDWs) without any obviously related spin order. Here we use resonant inelastic x-ray scattering (RIXS) to follow the evolution of charge correlations in the canonical stripe ordered cuprate La$_{1.875}$Ba$_{0.125}$CuO$_{4}$ (LBCO~$1/8$) across its ordering transition. We find that high-temperature charge correlations are unlocked from the wavevector of the spin correlations, signaling analogies to CDW phases in various other cuprates. This indicates that stripe order at low temperatures is stabilized by the coupling of otherwise independent charge and spin density waves, with important implications for the relation between charge and spin correlations in the cuprates.

cond-mat.supr-con↗

arXiv2017

Growth and structural characterization of large superconducting crystals of La$_{2-x}$Ca$_{1+x}$Cu$_2$O$_{6}$

Large crystals of La$_{2-x}$Ca$_{1+x}$Cu$_2$O$_{6}$ (La-Ca-2126) with $x=0.10$ and 0.15 have been grown and converted to bulk superconductors by high-pressure oxygen annealing. The superconducting transition temperature, $T_c$, is as high as 55~K; this can be raised to 60~K by post-annealing in air. Here we present structural and magnetic characterizations of these crystals using neutron scattering and muon spin rotation techniques. While the as-grown, non-superconducting crystals are single phase, we find that the superconducting crystals contain 3 phases forming coherent domains stacked along the $c$ axis: the dominant La-Ca-2126 phase, very thin (1.5 unit-cell) intergrowths of La$_2$CuO$_4$, and an antiferromagnetic La$_8$Cu$_8$O$_{20}$ phase. We propose that the formation and segregation of the latter phases increases the Ca concentration of the La-Ca-2126, thus providing the hole-doping that supports superconductivity.

cond-mat.supr-con↗

arXiv2017

Static Charge Density Wave Order in the Superconducting State of La2-xBaxCuO4

Charge density wave (CDW) correlations feature prominently in the phase diagram of the cuprates, motivating competing theories of whether fluctuating CDW correlations aid superconductivity or whether static CDW order coexists with superconductivity in inhomogeneous or spatially modulated states. Here we report Cu $L$-edge resonant x-ray photon correlation spectroscopy (XPCS) measurements of CDW correlations in superconducting La$_{2-x}$Ba$_x$CuO$_4$ $x=0.11$. Static CDW order is shown to exist in the superconducting state at low temperatures and to persist up to at least 85\% of the CDW transition temperature. We discuss the implications of our observations for how \emph{nominally} competing order parameters can coexist in the cuprates.

cond-mat.supr-con↗

arXiv2017

First-Order Reversal Curves of the Magnetostructural Phase Transition in FeTe

We apply the first-order reversal curve (FORC) method, borrowed from studies of ferromagnetic materials, to the magneto-structural phase transition of FeTe. FORC measurements reveal two features in the hysteretic phase transition, even in samples where traditional temperature measurements display only a single transition. For Fe1.13Te, the influence of magnetic field suggests that the main feature is primarily structural while a smaller, slightly higher-temperature transition is magnetic in origin. By contrast Fe1.03Te has a single transition which shows a uniform response to magnetic field, indicating a stronger coupling of the magnetic and structural phase transitions. We also introduce uniaxial stress, which spreads the distribution width without changing the underlying energy barrier of the transformation. The work shows how FORC can help disentangle the roles of the magnetic and structural phase transitions in FeTe.

cond-mat.str-el↗

arXiv2017

Andreev Reflection without Fermi surface alignment in High T$_{c}$-Topological heterostructures

We address the controversy over the proximity effect between topological materials and high T$_{c}$ superconductors. Junctions are produced between Bi$_{2}$Sr$_{2}$CaCu$_{2}$O$_{8+δ}$ and materials with different Fermi surfaces (Bi$_{2}$Te$_{3}$ \& graphite). Both cases reveal tunneling spectra consistent with Andreev reflection. This is confirmed by magnetic field that shifts features via the Doppler effect. This is modeled with a single parameter that accounts for tunneling into a screening supercurrent. Thus the tunneling involves Cooper pairs crossing the heterostructure, showing the Fermi surface mis-match does not hinder the ability to form transparent interfaces, which is accounted for by the extended Brillouin zone and different lattice symmetries.

cond-mat.supr-con↗

arXiv2017

Vertical temperature-boundary of the pseudogap under the superconducting dome of the Bi2Sr2CaCu2O8+d phase-diagram

Combining electronic Raman scattering experiments with cellular dynamical mean field theory, we present evidence of the pseudogap in the superconducting state of various hole-doped cuprates. In Bi2Sr2CaCu2O8+d we track the superconducting pseudogap hallmark, a peak-dip feature, as a function of temperature T and doping p, well beyond the optimal one. We show that, at all temperatures under the superconducting dome, the pseudogap disappears at the doping pc, between 0.222 and 0.226, where also the normal-state pseudogap collapses at a Lifshitz transition. This demonstrates that the superconducting pseudogap boundary forms a vertical line in the T-p phase diagram.

cond-mat.supr-con↗

arXiv2017

Doping Dependence of Collective Spin and Orbital Excitations in Spin 1 Quantum Antiferromagnet La$_{2-x}$Sr$_x$NiO$_4$ Observed by X-rays

We report the first empirical demonstration that resonant inelastic x-ray scattering (RIXS) is sensitive to \emph{collective} magnetic excitations in $S=1$ systems by probing the Ni $L_3$-edge of La$_{2-x}$Sr$_x$NiO$_4$ ($x = 0, 0.33, 0.45$). The magnetic excitation peak is asymmetric, indicating the presence of single and multi spin-flip excitations. As the hole doping level is increased, the zone boundary magnon energy is suppressed at a much larger rate than that in hole doped cuprates. Based on the analysis of the orbital and charge excitations observed by RIXS, we argue that this difference is related to the orbital character of the doped holes in these two families. This work establishes RIXS as a probe of fundamental magnetic interactions in nickelates opening the way towards studies of heterostructures and ultra-fast pump-probe experiments.

cond-mat.str-el↗

arXiv2017

Spectroscopic evidence for bulk-band inversion and three-dimensional massive Dirac fermions in ZrTe5

Three-dimensional topological insulators (3D TIs) represent novel states of quantum matters in which surface states are protected by time-reversal symmetry and an inversion occurs between bulk conduction- and valence-bands. However, the bulk-band inversion which is intimately tied to the topologically nontrivial nature of 3D TIs has rarely been investigated by experiments. Besides, 3D massive Dirac fermions with nearly near band dispersions were seldom observed in TIs. Recently, a van der Waals crystal, ZrTe5, was theoretically predicted to be a TI. Here, we report an infrared transmission study of a high-mobility (~33,000 cm$^2$/(Vs)) multilayer ZrTe5 flake at magnetic fields ($B$) up to 35 T. Our observation of a linear relationship between the zero-magnetic-field optical absorption and the photon energy, a bandgap of ~10 meV and a $\sqrt{B}$ dependence of the Landau level (LL) transition energies at low magnetic fields demonstrates 3D massive Dirac fermions with nearly linear band dispersions in this system. More importantly, the reemergence of the intra-LL transitions at magnetic fields higher than 17 T reveals the energy cross between the two zeroth LLs, which reflects the inversion between the bulk conduction- and valence-bands. Our results not only provide spectroscopic evidence for the TI state in ZrTe5 but also open up a new avenue for fundamental studies of Dirac fermions in van der Waals materials.

cond-mat.mes-hall↗

arXiv2016

Modeling Tunneling for the Unconventional Superconducting Proximity Effect

Recently there has been reinvigorated interest in the superconducting proximity effect, driven by predictions of the emergence of Majorana fermions. To help guide this search, we have developed a phenomenological model for the tunneling spectra in anisotropic superconductor-normal metal proximity devices. We combine successful approaches used in s-wave proximity and standard d-wave tunneling to reproduce tunneling spectra in d-wave proximity devices, and clarify the origin of various features. Different variations of the pair potential are considered, resulting from the proximity-induced superconductivity. Furthermore, the effective pair potential felt by the quasiparticles is momentum-dependent in contrast to s-wave superconductors. The probabilities of reflection and transmission are calculated by solving the Bogoliubov equations. Our results are consistent with experimental observations of the unconventional proximity effect and provide important experimental parameters such as the size and length scale of the proximity induced gap, as well as the conditions needed to observe the reduced and full superconducting gaps.

cond-mat.supr-con↗

arXiv2016

Electronic structure of the ingredient planes of cuprate superconductor Bi2Sr2CuO6+δ: a comparison study with Bi2Sr2CaCu2O8+δ

By means of low-temperature scanning tunneling microscopy, we report on the electronic structures of BiO and SrO planes of Bi2Sr2CuO6+δ (Bi-2201) superconductor prepared by argon-ion bombardment and annealing. Depending on post annealing conditions, the BiO planes exhibit either pseudogap (PG) with sharp coherence peaks and an anomalously large gap of 49 meV or van Hove singularity (VHS) near the Fermi level, while the SrO is always characteristic of a PG-like feature. This contrasts with Bi2Sr2CaCu2O8+δ (Bi-2212) superconductor where VHS occurs solely on the SrO plane. We disclose the interstitial oxygen dopants (δ in the formulas) as a primary cause for the occurrence of VHS, which are located dominantly around the BiO and SrO planes, respectively, in Bi-2201 and Bi-2212. This is supported by the contrasting structural buckling amplitude of BiO and SrO planes in the two superconductors. Our findings provide solid evidence for the irrelevance of PG to the superconductivity in the two superconductors, as well as insights into why Bi-2212 can achieve a higher superconducting transition temperature than Bi-2201, and by implication, the mechanism of cuprate superconductivity.

cond-mat.supr-con↗

arXiv2016

Restoring Interlayer Josephson Coupling in La_{1.885}Ba_{0.115}CuO_4 by Charge Transfer Melting of Stripe Order

We show that disruption of charge-density-wave (stripe) order by charge transfer excitation, enhances the superconducting phase rigidity in La_{1.885}Ba_{0.115}CuO_4 (LBCO). Time-Resolved Resonant Soft X-Ray Diffraction demonstrates that charge order melting is prompt following near-infrared photoexcitation whereas the crystal structure remains intact for moderate fluences. THz time-domain spectroscopy reveals that, for the first 2 ps following photoexcitation, a new Josephson Plasma Resonance edge, at higher frequency with respect to the equilibrium edge, is induced indicating enhanced superconducting interlayer coupling. The fluence dependence of the charge-order melting and the enhanced superconducting interlayer coupling are correlated with a saturation limit of about 0.5 mJ/cm2. Using a combination of x-ray and optical spectroscopies we establish a hierarchy of timescales between enhanced superconductivity, melting of charge order and rearrangement of the crystal structure.

cond-mat.supr-con↗