arXiv subjects

G. Knebel

Publications and source records attributed to G. Knebel.

At least 37 records · Page 2Linked to original sources

arXiv2020

Comparison of two superconducting phases induced by a magnetic field in UTe2

Superconductivity induced by a magnetic field near metamagnetism is a striking manifestation of magnetically-mediated superconducting pairing. After being observed in itinerant ferromagnets, this phenomenon was recently reported in the orthorhombic paramagnet UTe$_2$. Under a magnetic field applied along the hard magnetization axis b, superconductivity is reinforced on approaching metamagnetism at $μ_0H_m$ = 35 T, but it abruptly disappears beyond $H_m$. On the contrary, field-induced superconductivity was reported beyond $μ_0H_m$ = 40-50 T in a magnetic field tilted by $\simeq25-30°$ from b in the (b,c) plane. Here we explore the phase diagram of UTe2 under these two magnetic-field directions. Zero-resistance measurements permit to confirm unambiguously that superconductivity is established beyond Hm in the tilted-field direction. While superconductivity is locked exactly at fields either smaller (for a H || b), or larger (for H tilted by $\simeq27°$ from b to c), than Hm, the variations of the Fermi-liquid coefficient in the electrical resistivity and of the residual resistivity are surprisingly similar for the two field directions. The resemblance of the normal states for the two field directions puts constraints for theoretical models of superconductivity and implies that some subtle ingredients must be in play.

cond-mat.supr-con↗

arXiv2019

Multiple superconducting phases in a nearly ferromagnetic system

Multiple superconducting order parameters are extremely rare. Here we show that a very small pressure can induce this phenomenon in the recently discovered heavy fermion superconductor UTe2. This nearly ferromagnetic system shows several intriguing phenomena, including an extraordinary reinforcement of superconductivity in very strong magnetic fields. We find that pressure can tune the system to a more correlated state and probable magnetic order. The superconducting critical temperature is strongly enhanced, reaching almost 3K, a new record for Ce- and U-based heavy fermion superconductors. Most spectacularly under pressure we find a transition within the superconducting state, putting UTe2 among the very rare systems having multiple superconducting phases. UTe2 under pressure is a treasure trove of several of the most fascinating phenomena in unconventional superconductivity and may well be a keystone in their understanding.

cond-mat.str-el↗

arXiv2016

Thermoelectric power quantum oscillations in the ferromagnet UGe$_2$

We present thermoelectric power and resistivity measurements in the ferromagnet UGe$_2$ as a function of temperature and magnetic field. At low temperature, huge quantum oscillations are observed in the thermoelectric power as a function of the magnetic field applied along the $a$ axis. The frequencies of the extreme orbits are determined and an analysis of the cyclotron masses is performed following different theoretical approaches for quantum oscillations detected in the thermoelectric power. They are compared to those obtained by Shubnikov-de Haas experiments on the same crystal and previous de Haas-van Alphen experiments. The agreement of the different probes confirms thermoelectric power as an excellent probe to extract simultaneously both microscopic and macroscopic information on the Fermi-surface properties. Band-structure calculations of UGe$_2$ in the ferromagnetic state are compared to the experiment.

cond-mat.str-el↗

arXiv2015

Fermi surface instabilities in CeRh2Si2 at high magnetic field and pressure

We present thermoelectric power (TEP) studies under pressure and high magnetic field in the antiferromagnet CeRh2Si2 at low temperature. Under magnetic field, large quantum oscillations are observed in the TEP, S(H), in the antiferromagnetic phase. They suddenly disappear when entering in the polarized paramagnetic (PPM) state at Hc pointing out an important reconstruction of the Fermi surface (FS). Under pressure, S/T increases strongly of at low temperature near the critical pressure Pc, where the AF order is suppressed, implying the interplay of a FS change and low energy excitations driven by spin and valence fluctuations. The difference between the TEP signal in the PPM state above Hc and in the paramagnetic state (PM) above Pc can be explained by different FS. Band structure calculations at P = 0 stress that in the AF phase the 4f contribution at the Fermi level (EF) is weak while it is the main contribution in the PM domain. By analogy to previous work on CeRu2Si2, in the PPM phase of CeRh2Si2 the 4f contribution at EF will drop.

cond-mat.str-el↗

arXiv2015

Thermal conductivity through the quantum critical point in YbRh2Si2 at very low temperature

The thermal conductivity of YbRh2Si2 has been measured down to very low temperatures under field in the basal plane. An additional channel for heat transport appears below 30 mK, both in the antiferromagnetic and paramagnetic states, respectively below and above the critical field suppressing the magnetic order. This excludes antiferromagnetic magnons as the origin of this additional contribution to thermal conductivity. Moreover, this low temperature contribution prevails a definite conclusion on the validity or violation of the Wiedemann-Franz law at the field-induced quantum critical point. At high temperature in the paramagnetic state, the thermal conductivity is sensitive to ferromagnetic fluctuations, previously observed by NMR or neutron scattering and required for the occurrence of the sharp electronic spin resonance fracture.

cond-mat.str-el↗

arXiv2014

Switching of the magnetic order in CeRhIn$_{5-x}$Sn$_{x}$ in the vicinity of its quantum critical point

We report neutron diffraction experiments performed in the tetragonal antiferromagnetic heavy fermion system CeRhIn$_{5-x}$Sn$_{x}$ in its ($x$, $T$) phase diagram up to the vicinity of the critical concentration $x_c$ $\approx$ 0.40, where long range magnetic order is suppressed. The propagation vector of the magnetic structure is found to be $\bf{k_{IC}}$=(1/2, 1/2, $k_l$) with $k_l$ increasing from $k_l$=0.298 to $k_l$=0.410 when $x$ increases from $x$=0 to $x$=0.26. Surprisingly, for $x$=0.30, the order has changed drastically and a commensurate antiferromagnetism with $\bf{k_{C}}$=(1/2, 1/2, 0) is found. This concentration is located in the proximity of the quantum critical point where superconductivity is expected.

cond-mat.str-el↗

arXiv2013

Quantum criticality and Lifshitz transition in the Ising system CeRu2Si2: Comparison with YbRh2Si2

New thermoelectric power (TEP) measurements on prototype heavy-fermion compounds close to magnetic quantum criticality are presented. The highly sensitive technique of TEP is an unique tool to reveal Fermi surface instabilities, referred here as Lifshitz transitions. The first focus is on the Ising CeRu2Si2 series. Doping CeRu2Si2 with Rh produces a decoupling between the first order metamagnetic transition and the pseudo-metamagnetism observed in the pure compound. Comparison is made with the case of YbRh2Si2 which is often considered as the archetype of local quantum criticality by contrast to CeRu2Si2, taken as an example of spin-density wave criticality. Up to now for ferromagnetic materials showing ferromagnetic wings, no simple case appears where the Fermi surface is preserved between the ferromagnetic and paramagnetic phases. An open issue is the consequence of Lifshitz transitions on superconductivity in these multiband systems.

cond-mat.str-el↗

arXiv2013

Fermi surface in the hidden-order state of URu$_2$Si$_2$ under intense pulsed magnetic fields up to 81~T

We present measurements of the resistivity $ρ_{x,x}$ of URu2Si2 high-quality single crystals in pulsed high magnetic fields up to 81~T at a temperature of 1.4~K and up to 60~T at temperatures down to 100~mK. For a field \textbf{H} applied along the magnetic easy-axis \textbf{c}, a strong sample-dependence of the low-temperature resistivity in the hidden-order phase is attributed to a high carrier mobility. The interplay between the magnetic and orbital properties is emphasized by the angle-dependence of the phase diagram, where magnetic transition fields and crossover fields related to the Fermi surface properties follow a 1/$\cosθ$-law, $θ$ being the angle between \textbf{H} and \textbf{c}. For $\mathbf{H}\parallel\mathbf{c}$, a crossover defined at a kink of $ρ_{x,x}$, as initially reported in [Shishido et al., Phys. Rev. Lett. \textbf{102}, 156403 (2009)], is found to be strongly sample-dependent: its characteristic field $μ_0H^*$ varies from $\simeq20$~T in our best sample with a residual resistivity ratio RRR of $225$ to $\simeq25$~T in a sample with a RRR of $90$. A second crossover is defined at the maximum of $ρ_{x,x}$ at the sample-independent characteristic field $μ_0H_{ρ,max}^{LT}\simeq30$~T. Fourier analyzes of SdH oscillations show that $H_{ρ,max}^{LT}$ coincides with a sudden modification of the Fermi surface, while $H^*$ lies in a regime where the Fermi surface is smoothly modified. For $\mathbf{H}\parallel\mathbf{a}$, i) no phase transition is observed at low temperature and the system remains in the hidden-order phase up to 81~T, ii) quantum oscillations surviving up to 7~K are related to a new and almost-spherical orbit - for the first time observed here - at the frequency $F_λ\simeq1400$~T and associated with a low effective mass $m^*_λ=(1\pm0.5)\cdot m_0$, and iii) no Fermi surface modification occurs up to 81~T.

cond-mat.str-el↗

arXiv2013

Magnetic order in Ce0.95Nd0.05CoIn5: the Q-phase at zero magnetic field

We report neutron scattering experiment results revealing the nature of the magnetic order occurring in the heavy fermion superconductor Ce0.95Nd0.05CoIn5, a case for which an antiferromagnetic state is stabilized at a temperature below the superconducting transition one. We evidence an incommensurate order and its propagation vector is found to be identical to that of the magnetic field induced antiferromagnetic order occurring in the stoichiometric superconductor CeCoIn5, the so-called Q-phase. The commonality between these two cases suggests that superconductivity is a requirement for the formation of this kind of magnetic order and the proposed mechanism is the enhancement of nesting condition by d-wave order parameter with nodes in the nesting area.

cond-mat.str-el↗

arXiv2013

Magnetic Polarization and Fermi Surface Instability: Case of YbRh2Si2

We report thermoelectric and resitivity measurements of antiferromagnetic heavy fermion compound YRh2Si2 at low temperatures down and under high magnetic field. At low temperature, the thermoelectric power and the resistivity present several distinct anomalies as a function of field around H_0 ~ 9.5 T when the magnetic polarization reaches a critical value. The anomalies are accompanied with a change of sign from negative at low magnetic field to positive at high field (H>H_0) and are resulting from a Lifshitz-type topological transition of the Fermi surface. A logarithmic divergence of S/T at T \to 0 K just above H_0 (H=11.5 T) is quite comparable to the well known divergence of S/T in the temperature range above the antiferromagnetic order at H=0 T referred to as non Fermi liquid behavior. The transition will be compared to the well characterized Fermi surface change in CeRu2Si2 at its pseudo-metamagnetic transition.

cond-mat.str-el↗

arXiv2013

Metamagnetic Transition in UCoAl Probed by Thermoelectricity Measurements

We report field and temperature dependent measurements of the thermoelectric power (TEP) and the Nernst effect in the itinerant metamagnet UCoAl. The magnetic field is applied along the easy magnetization c-axis in the hexagonal crystal structure. The metamagnetic transition from the paramagnetic phase at zero field to the field induced ferromagnetic (FM) state is of first order at low temperatures and becomes a broad crossover above the critical temperature $T^{\star}_{M} \sim 11$ K. The field-dependence of the TEP reveals that the effective mass of the hole carriers changes significantly at the metamagnetic transition. The TEP experiment reflects the existence of different carrier types in good agreement with band structure calculations and previous Hall effect experiments. According to the temperature dependence of the TEP, no Fermi liquid behavior appears in the paramagnetic state down to 150 mK, but is achieved only in the field induced ferromagnetic state.

cond-mat.str-el↗

arXiv2012

Verification of the Wiedemann-Franz law in YbRh2Si2 at a quantum critical point

The thermal conductivity measurements have been performed on the heavy-fermion compound YbRh2Si2 down to 0.04 K and under magnetic fields through a quantum critical point (QCP) at Bc = 0.66 T || c-axis. In the limit as T -> 0, we find that the Wiedemann-Franz law is satisfied within experimental error at the QCP despite the destruction of the standard signature of Fermi liquid. Our results place strong constraints on models that attempt to describe the nature of unconventional quantum criticality of YbRh2Si2.

cond-mat.str-el↗

arXiv2012

(p,T,H) phase diagram of Heavy Fermion systems : Some systematics and some surprises from ytterbium

Pressure is the cleanest way to tune heavy fermion systems to a quantum phase transition in order to study the rich physics and competing phases, and the comparison between ytterbium and cerium systems is particularly fruitful. We briefly review the mechanisms in play and show some examples of expected and unexpected behaviour. We emphasize the importance of the valence changes under pressure and show how modern synchrotron techniques can accurately determine this, including at low temperature.

cond-mat.str-el↗

arXiv2012

Thermoelectric response near a quantum critical point of beta-YbAlB4 and YbRh2Si2: A comparative study

The thermoelectric coefficients have been measured on the Yb-based heavy fermion compounds beta-YbAlB4 and YbRh2Si2 down to a very low temperature. We observe a striking difference in the behavior of the Seebeck coefficient, S in the vicinity of the Quantum Critical Point (QCP) in the two systems. As the critical field is approached, S/T enhances in beta-YbAlB4 but is drastically reduced in YbRh2Si2. While in the former system, the ratio of thermopower-to-specific heat remains constant, it drastically drops near the QCP in YbRh2Si2. In both systems, on the other hand, the Nernst coefficient shows a diverging behavior near the QCP. The results provide a new window to the way various energy scales of the system behave and eventually vanish near a QCP.

cond-mat.str-el↗

arXiv2011

Phase diagram of CeVSb3 under pressure and its dependence on pressure conditions

We present temperature dependent resistivity and ac-calorimetry measurements of CeVSb3 under pressure up to 8 GPa in a Bridgman anvil cell modified to use a liquid medium and in a diamond anvil cell using argon as a pressure medium, respectively. We observe an initial increase of the ferromagnetic transition temperature Tc with pressures up to 4.5 GPa, followed by decrease of Tc on further increase of pressure and finally its disappearance, in agreement with the Doniach model. We infer a ferromagnetic quantum critical point around 7 GPa under hydrostatic pressure conditions from the extrapolation to 0 K of Tc and the maximum of the A coefficient from low temperature fits of the resistivity ρ(T)=ρ_{0}+AT^{n}. No superconductivity under pressure was observed down to 0.35 K for this compound. In addition, differences in the Tc(P) behavior when a slight uniaxial component is present are noticed and discussed and correlated to choice of pressure medium.

cond-mat.str-el↗

arXiv2010

Tricritical point and wing structure in the itinerant ferromagnet UGe2

Precise resistivity measurements on the ferromagnetic superconductor UGe2 under pressure p and magnetic field H reveal a previously unobserved change of the anomaly at the Curie temperature. Therefore, the tricritical point (TCP) where the paramagnetic-to-ferromagnetic transition changes from a second order to a first order transition is located in the p-T phase diagram. Moreover, the evolution of the TCP can be followed under the magnetic field in the same way. It is the first report of the boundary of the first order plane which appears in the p-T-H phase diagram of weak itinerant ferromagnets. This line of critical points starts from the TCP and will terminate at a quantum critical point. These measurements provide the first estimation of the location of the quantum critical point in the p-H plane and will inspire similar studies of the other weak itinerant ferromagnets.

cond-mat.str-el↗

arXiv2010

Trends in Heavy Fermion Matter

A brief review on major advances in heavy fermion physics is presented including the Ce metal phase diagram, the huge effective mass detected in CeAl3, and the successive discoveries of unconventional superconductivity in CeCu2Si2 and three U based compounds, UBe13, UPt3 and URu2Si2. In order to track the origin of the huge effective mass, the case of intermediate valence compounds is discussed with emphasis of the differences between Yb and Ce materials. The formation of the effective mass is analyzed by two regular- and singular-part contributions. Examples are given for both, antiferromagnetic (CeRu2Si2 series) and ferromagnetic tricriticalities (UGe2). Pressure and magnetic-field studies on the ferromagnetic superconductor URhGe illustrate the role of the singular effective mass enhancement on the superconducting pairing. The discovery of the Ce-115 material gives the opportunity to study deeply the interplay of antiferromagnetism and superconductivity. This is clearly demonstrated by field re-entrance AF inside the SC phase just below the superconducting upper critical field (Hc2) for CeCoIn5 or on both side of Hc2 within a restricted pressure window for CeRhIn5. The present status of the search for the hidden-order parameter of URu2Si2 is given and we emphasize that it may correspond to a lattice unit-cell doubling which leads to a drastic change in the band structure and spin dynamic, with the possibility of competition between multipolar ordering and antiferromagnetism.

cond-mat.str-el↗

arXiv2010

Similarity of Fermi Surface in the Hidden Order State and in the Antiferromagnetic State of URu2Si2

Shubnikov-de Haas measurements of high quality URu2Si2 single crystals reveal two previously unobserved Fermi surface branches in the so-called hidden order phase. Therefore about 55% of the enhanced mass is now detected. Under pressure in the antiferromagnetic state, the Shubnikov-de Haas frequencies for magnetic fields applied along the crystalline c axis show little change compared with the zero pressure data. This implies a similar Fermi surface in both the hidden order and antiferromagnetic states, which strongly suggests that the lattice doubling in the antiferromagnetic phase due to the ordering vector QAF = (0 0 1) already occurs in the hidden order. These measurements provide a good test for existing or future theories of the hidden order parameter.

cond-mat.str-el↗