arXiv subjects

G. Leckenby

Publications and source records attributed to G. Leckenby.

14 recordsLinked to original sources

arXiv2025

First Proton-Induced Cross Sections on a Stored Rare Ion Beam: Measurement of 118Te(p,γ) for Explosive Nucleosynthesis

We present the first nuclear cross-section measurements of (p,γ) and (p,n) reactions on 118Te at energies relevant for the γ-process nucleosynthesis. Absolute cross-section values for center-of-mass energies of 6, 7 and 10 MeV are provided, together with a theoretical extrapolation to the Gamow window. This experiment marks the first time that direct proton-induced reactions have been measured on a radioactive ion beam at the Experimental Storage Ring (ESR) at GSI, Darmstadt. This paves the way for a large variety of measurements, delivering new constraints for explosive nucleosynthesis and for physics beyond nuclear stability.

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arXiv2025

Intruder structures in $^{32}$Si and $^{29}$Al

We have studied $^{32}$Si and $^{29}$Al using $^{12}$C($^{22}$Ne,2p) and $^{12}$C($^{22}$Ne,$α$p) fusion-evaporation reactions. In both cases, we observed significant population of high-spin structures distinct from the ground-state yrast bands. In $^{32}$Si, most of the high-energy states feed into a $J^π = 5^-$ nanosecond isomer. In $^{29}$Al, we identified a rotor-like negative-parity band with a $J^π = 7/2^-$ band-head. Doppler shift lifetime measurements were performed for all observed states. These results were compared to shell model calculations and interpreted in terms of proton and neutron cross-shell excitation.

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arXiv2025

Bayesian and Monte Carlo approaches to estimating uncertainty for the measurement of the bound-state $β$ decay of $^{205}\mathrm{Tl}^{81+}$

The measurement of the bound-state $β$ decay of $^{205}\mathrm{Tl}^{81+}$ at the Experimental Storage Ring at GSI, Darmstadt, has recently been reported with substantial impact on the use of $^{205}\mathrm{Pb}$ as an early Solar System chronometer and the low-energy measurement of the solar neutrino spectrum via the LOREX project. Due to the technical challenges in producing a high-purity $^{205}\mathrm{Tl}^{81+}$ secondary beam, a robust statistical method needed to be developed to estimate the variation in the contaminant $^{205}\mathrm{Pb}^{81+}$ produced in the fragmentation reaction, which was subsequently transmitted and stored in the ESR. Here we show that Bayesian and Monte Carlo methods produced comparable estimates for the contaminant variation, each with unique advantages and challenges given the complex statistical problems for this experiment. We recommend the adoption of such methods in future experiments that exhibit unknown statistical fluctuations.

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arXiv2025

Half-life determination of heavy ions in a storage ring considering feeding and depleting background processes

Heavy-ion storage rings have relatively large momentum acceptance which allows for multiple ion species to circulate at the same time. This needs to be considered in radioactive decay measurements of highly charged ions, where atomic charge exchange reactions can significantly alter the intensities of parent and daughter ions. In this study, we investigate this effect using the decay curves of ion numbers in the recent $^{205}$Tl$^{81+}$ bound-state beta decay experiment conducted using the Experimental Storage Ring at GSI Darmstadt. To understand the intricate dynamics of ion numbers, we present a set of differential equations that account for various atomic and nuclear reaction processes-bound-state beta decay, atomic electron recombination and capture, and electron ionization. By incorporating appropriate boundary conditions, we develop a set of differential equations that accurately simulate the decay curves of various simultaneously stored ions in the storage ring: $^{205}$Tl$^{81+}$, $^{205}$Pb$^{81+}$, $^{205}$Pb$^{82+}$, $^{200}$Hg$^{79+}$, and $^{200}$Hg$^{80+}$. Through a quantitative comparison between simulations and experimental data, we provide insights into the detailed reaction mechanisms governing stored heavy ions within the storage ring. Our approach effectively models charge-changing processes, reduces the complexity of the experimental setup, and provides a simpler method for measuring the decay half-lives of highly charged ions in storage rings.

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arXiv2025

Investigation of the Excited States of $^{114}\mathrm{Sn}$ Using the GRIFFIN Spectrometer at TRIUMF

The semi-magic $^{110-122}\mathrm{Sn}$ isotopes display signs of shape coexistence in their excited $0^+$ states, which, in contrast to the spherical $0^+$ ground states, are deformed. This paper investigates the nuclear structure of $^{114}\mathrm{Sn}$ using the competing $β^+$ decay and electron capture of a radioactive beam of $^{114}\mathrm{Sb}$ produced at the TRIUMF-ISAC facility using the GRIFFIN spectrometer. This study will allow for an in-depth understanding of the excited $0^+$ states in $^{114}\mathrm{Sn}$, by focusing on their decay patterns. In the present experiment, transitions at 856.2-keV and 1405.0-keV, which were observed in an earlier $β^+$ decay study but not placed in the $^{114}\mathrm{Sn}$ level scheme, have been assigned to the level scheme in connection to the $0^+_3$ level at 2156.0-keV. Properly assigning these transitions refines the level scheme and enhances our understanding of the nuclear structure in $^{114}\mathrm{Sn}$.

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arXiv2025

Bound-State Beta Decay of $\mathbf{\mathrm{^{205}{Tl}^{81+}}}$ Ions and the LOREX Project

Stable $^{205}$Tl ions have the lowest known energy threshold for capturing electron neutrinos ($ν_e$) of ${ E}_{ν_e}\ge50.6$\,keV. The Lorandite Experiment (LOREX), proposed in the 1980s, aims at obtaining the longtime averaged solar neutrino flux by utilizing natural deposits of Tl-bearing lorandite ores. To determine the $ν_e$ capture cross section, it is required to know the strength of the weak transition connecting the ground state of $^{205}$Tl and the 2.3 keV first excited state in $^{205}$Pb. The only way to experimentally address this transition is to measure the bound-state beta decay ($β_{b}$) of fully ionized $\mathrm{^{205}Tl^{81+}}$ ions. After three decades of meticulous preparation, the half-life of the $β_{b}$ decay of $\mathrm{^{205}Tl^{81+}}$ has been measured to be $291_{-27}^{+33}$ days using the Experimental Storage Ring (ESR) at GSI, Darmstadt. The longer measured half-life compared to theoretical estimates reduces the expected signal-to-noise ratio in the LOREX, thus challenging its feasibility.

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arXiv2024

High-temperature $^{205}$Tl decay clarifies $^{205}$Pb dating in early Solar System

Radioactive nuclei with lifetimes on the order of millions of years can reveal the formation history of the Sun and active nucleosynthesis occurring at the time and place of its birth. Among such nuclei whose decay signatures are found in the oldest meteorites, $^{205}$Pb is a powerful example, as it is produced exclusively by slow neutron captures (the s process), with most being synthesized in asymptotic giant branch (AGB) stars. However, making accurate abundance predictions for $^{205}$Pb has so far been impossible because the weak decay rates of $^{205}$Pb and $^{205}$Tl are very uncertain at stellar temperatures. To constrain these decay rates, we measured for the first time the bound-state $β^-$ decay of fully ionized $^{205}$Tl$^{81+}$, an exotic decay mode that only occurs in highly charged ions. The measured half-life is 4.7 times longer than the previous theoretical estimate and our 10% experimental uncertainty has eliminated the main nuclear-physics limitation. With new, experimentally backed decay rates, we used AGB stellar models to calculate $^{205}$Pb yields. Propagating those yields with basic galactic chemical evolution (GCE) and comparing with the $^{205}$Pb/$^{204}$Pb ratio from meteorites, we determined the isolation time of solar material inside its parent molecular cloud. We find positive isolation times that are consistent with the other s-process short-lived radioactive nuclei found in the early Solar System. Our results reaffirm the site of the Sun's birth as a long-lived, giant molecular cloud and support the use of the $^{205}$Pb--$^{205}$Tl decay system as a chronometer in the early Solar System.

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arXiv2024

First simultaneous measurement of the gamma-ray and neutron emission probabilities in inverse kinematics at a heavy-ion storage ring

The probabilities for gamma-ray and particle emission as a function of the excitation energy of a decaying nucleus are valuable observables for constraining the ingredients of the models that describe the de-excitation of nuclei near the particle emission threshold. These models are essential in nuclear astrophysics and applications. In this work, we have for the first time simultaneously measured the gamma-ray and neutron emission probabilities of 208Pb. The measurement was performed in inverse kinematics at the Experimental Storage Ring (ESR) of the GSI/FAIR facility, where a 208Pb beam interacted through the 208Pb(p,p') reaction with a hydrogen gas jet target. Instead of detecting the gamma-rays and neutrons emitted by 208Pb, we detected the heavy beam-like residues produced after gamma and neutron emission. These heavy residues were fully separated by a dipole magnet of the ESR and were detected with outstanding efficiencies. The comparison of the measured probabilities with model calculations has allowed us to test and select different descriptions of the gamma-ray strength function and the nuclear level density available in the literature.

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arXiv2024

First measurement of the neutron-emission probability with a surrogate reaction in inverse kinematics at a heavy-ion storage ring

Neutron-induced reaction cross sections of short-lived nuclei are imperative to understand the origin of heavy elements in stellar nucleosynthesis and for societal applications, but their measurement is extremely complicated due to the radioactivity of the targets involved. One way of overcoming this issue is to combine surrogate reactions with the unique possibilities offered by heavy-ion storage rings. In this work, we describe the first surrogate-reaction experiment in inverse kinematics, which we successfully conducted at the Experimental Storage Ring (ESR) of the GSI/FAIR facility, using the 208Pb(p,p') reaction as a surrogate for neutron capture on 207Pb. Thanks to the outstanding detection efficiencies possible at the ESR, we were able to measure for the first time the neutron-emission probability as a function of the excitation energy of 208Pb. We have used this probability to select different descriptions of the gamma-ray strength function and nuclear level density, and provide reliable results for the neutron-induced radiative capture cross section of 207Pb at energies for which no experimental data exist.

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arXiv2024

Cross-shell excited configurations in the structure of 34Si

The cross-shell excited states of $^{34}$Si have been investigated via $β$-decays of the $4^-$ ground state and the $1^+$ isomeric state of $^{34}$Al. Since the valence protons and valence neutrons occupy different major shells in the ground state as well as the intruder $1^+$ isomeric state of $^{34}$Al, intruder levels of $^{34}$Si are populated via allowed $β$ decays. Spin assignments to such intruder levels of $^{34}$Si were established through $γ$-$γ$ angular correlation analysis for the negative parity states with dominant configurations $(νd_{3/2})^{-1} \otimes (νf_{7/2})^{1}$ as well as the positive parity states with dominant configurations $(νsd)^{-2} \otimes (νf_{7/2}p_{3/2})^2$. The configurations of such intruder states play crucial roles in our understanding of the $N=20$ shell gap evolution. A configuration interaction model derived from the FSU Hamiltonian was utilized in order to interpret the intruder states in $^{34}$Si. Shell model interaction derived from a more fundamental theory with the Valence Space In Medium Similarity Renormalization Group (VS-IMSRG) method was also employed to interpret the structure of $^{34}$Si.

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arXiv2023

Measurement of the Isolated Nuclear Two-Photon Decay in $^{72}\mathrm{Ge}$

The nuclear two-photon or double-gamma ($2γ$) decay is a second-order electromagnetic process whereby a nucleus in an excited state emits two gamma rays simultaneously. To be able to directly measure the $2γ$ decay rate in the low-energy regime below the electron-positron pair-creation threshold, we combined the isochronous mode of a storage ring with Schottky resonant cavities. The newly developed technique can be applied to isomers with excitation energies down to $\sim100$\,keV and half-lives as short as $\sim10$\,ms. The half-life for the $2γ$ decay of the first-excited $0^+$ state in bare $^{72}\mathrm{Ge}$ ions was determined to be $23.9\left(6\right)$\,ms, which strongly deviates from expectations.

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arXiv2023

Identifying the spin trapped character of the $^{32}$Si isomeric state

The properties of a nanosecond isomer in $^{32}$Si, disputed in previous studies, depend on the evolution of proton and neutron shell gaps near the `island of inversion'. We have placed the isomer at 5505.2(2) keV with $J^π = 5^-$, decaying primarily via an $E3$ transition to the $2^+_1$ state. The $E3$ strength of 0.0841(10) W.u. is unusually small and suggests that this isomer is dominated by the $(νd_{3/2})^{-1} \otimes (νf_{7/2})^{1}$ configuration, which is sensitive to the $N=20$ shell gap. A newly observed $4^+_1$ state is placed at 5881.4(13) keV; its energy is enhanced by the $Z=14$ subshell closure. This indicates that the isomer is located in a `yrast trap', a feature rarely seen at low mass numbers.

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arXiv2023

Storage, Accumulation and Deceleration of Secondary Beams for Nuclear Astrophysics

Low-energy investigations on rare ion beams are often limited by the available intensity and purity of the ion species in focus. Here, we present the first application of a technique that combines in-flight production at relativistic energies with subsequent secondary beam storage, accumulation and finally deceleration to the energy of interest. Using the FRS and ESR facilities at GSI, this scheme was pioneered to provide a secondary beam of $^{118}$Te$^{52+}$ for the measurement of nuclear proton-capture at energies of 6 and 7 MeV/u. The technique provided stored beam intensities of about $10^6$ ions at high purity and brilliance, representing a major step towards low-energy nuclear physics studies using rare ion beams.

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arXiv2022

Horizons: Nuclear Astrophysics in the 2020s and Beyond

Nuclear Astrophysics is a field at the intersection of nuclear physics and astrophysics, which seeks to understand the nuclear engines of astronomical objects and the origin of the chemical elements. This white paper summarizes progress and status of the field, the new open questions that have emerged, and the tremendous scientific opportunities that have opened up with major advances in capabilities across an ever growing number of disciplines and subfields that need to be integrated. We take a holistic view of the field discussing the unique challenges and opportunities in nuclear astrophysics in regards to science, diversity, education, and the interdisciplinarity and breadth of the field. Clearly nuclear astrophysics is a dynamic field with a bright future that is entering a new era of discovery opportunities.

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