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G. Li

Publications and source records attributed to G. Li.

At least 217 records · Page 12Linked to original sources

Electronic properties of single-crystalline Fe$_{1.05}$Te and Fe$_{1.03}$Se$_{0.30}$Te$_{0.70}$

We report on a comprehensive study of the transport, specific heat, magnetic susceptibility and optical spectroscopy on single crystal of Fe$_{1.05}$Te. We confirm that Fe$_{1.05}$Te undergoes a first-order phase transition near 65 K. However, its physical properties are considerably different from other parent compounds of FeAs-based systems, presumably attributed to the presence of excess Fe ions. The charge transport is rather incoherent above the transition, and no clear signature of the gap is observed below the transition temperature. Strong impurity scattering effect exists also in Se-doped superconducting sample Fe$_{1.03}$Se$_{0.30}$Te$_{0.70}$, leading to a relatively low T$_c$ but a rather high upper critical field.

cond-mat.supr-con↗

Magnetic Order of the Iron Spins in NdOFeAs

Polarized and unpolarized neutron diffraction measurements have been carried out to investigate the iron magnetic order in undoped NdOFeAs. Antiferromagnetic order is observed below 141(6) K, which is in close proximity to the structural distortion observed in this material. The magnetic structure consists of chains of parallel spins that are arranged antiparallel between chains, which is the same in-plane spin arrangement as observed in all the other iron oxypnictide materials. Nearest-neighbor spins along the c-axis are antiparallel like LaOFeAs. The ordered moment is 0.25(7) muB, which is the smallest moment found so far in these systems.

cond-mat.supr-con↗

Probing superconducting energy gap from infrared spectroscopy on a Ba$_{0.6}$K$_{0.4}$Fe$_2$As$_2$ single crystal with T$_c$=37 K

We performed optical spectroscopy measurement on a superconducting Ba$_{0.6}$K$_{0.4}$Fe$_2$As$_2$ single crystal with T$_c$=37 K. Formation of the superconducting energy gaps in the far-infared reflectance spectra below T$_c$ is clearly observed. The gap amplitudes match well with the two distinct superconducting gaps observed in angle-resolved photoemission spectroscopy experiments on different Fermi surfaces. We determined absolute value of the penetration depth at 10 K as $λ\simeq2000 Å$. A spectral weight analysis shows that the Ferrell-Glover-Timkham sum rule is satisfied at low energy scale, less than 6$Δ$.

cond-mat.supr-con↗

Superconducting properties of Fe-based layered superconductor LaO$_{0.9}$F$_{0.1-δ}$FeAs

We have employed a new route to synthesize single phase F-doped LaOFeAs compound and confirmed the superconductivity above 20 K in this Fe-based system. We show that the new superconductor has a rather high upper critical field of about 54 T. A clear signature of superconducting gap opening below T$_c$ was observed in the far-infrared reflectance spectra, with 2$Δ/\textit{k}T_c\approx$3.5-4.2. Furthermore, we show that the new superconductor has electron-type conducting carrier with a rather low carrier density.

cond-mat.supr-con↗

Structural and magnetic phase diagram of CeFeAsO1-xFx and its relationship to high-temperature superconductivity

We use neutron scattering to study the structural and magnetic phase transitions in the iron pnictides CeFeAsO1-xFx as the system is tuned from a semimetal to a high-transition-temperature (high-Tc) superconductor through Fluorine (F) doping x. In the undoped state, CeFeAsO develops a structural lattice distortion followed by a stripe like commensurate antiferromagnetic order with decreasing temperature. With increasing Fluorine doping, the structural phase transition decreases gradually while the antiferromagnetic order is suppressed before the appearance of superconductivity, resulting an electronic phase diagram remarkably similar to that of the high-Tc copper oxides. Comparison of the structural evolution of CeFeAsO1-xFx with other Fe-based superconductors reveals that the effective electronic band width decreases systematically for materials with higher Tc. The results suggest that electron correlation effects are important for the mechanism of high-Tc superconductivity in these Fe pnictides.

cond-mat.supr-con↗

Superconductivity in hole-doped (Sr$_{1-x}$K$_x$)Fe$_2$As$_2$

A series of layered (Sr$_{1-x}$K$_x$)Fe$_2$As$_2$ compounds with nominal x=0 to 0.40 are synthesized by solid state reaction method. Similar to other parent compounds of iron-based pnictide superconductors, the pure SrFe$_2$As$_2$ shows a strong resistivity anomaly near 210 K, which was ascribed to the spin-density-wave instability. The anomaly temperature is much higher than those observed in LaOFeAs and BaFe$_2$As$_2$, the two prototype parent compounds with ZrCuSiAs- and ThCr$_2$Si$_2$-type structures. K-doping strongly suppresses this anomaly and induces superconductivity. Like in the case of K-doped BaFe$_2$As$_2$, sharp superconducting transitions at T$_c\sim$38 K was observed. We performed the Hall coefficient measurement, and confirmed that the dominant carriers are hole-type. The carrier density is enhanced by a factor of 3 in comparison to F-doped LaOFeAs superconductor.

cond-mat.supr-con↗

Superconductivity at 41 K and its competition with spin-density-wave instability in layered CeO$_{1-x}$F$_x$FeAs

A series of layered CeO$_{1-x}$F$_x$FeAs compounds with x=0 to 0.20 are synthesized by solid state reaction method. Similar to the LaOFeAs, the pure CeOFeAs shows a strong resistivity anomaly near 145 K, which was ascribed to the spin-density-wave instability. F-doping suppresses this instability and leads to the superconducting ground state. Most surprisingly, the superconducting transition temperature could reach as high as 41 K. The very high superconducting transition temperature strongly challenges the classic BCS theory based on the electron-phonon interaction. The very closeness of the superconducting phase to the spin-density-wave instability suggests that the magnetic fluctuations play a key role in the superconducting paring mechanism. The study also reveals that the Ce 4f electrons form local moments and ordered antiferromagnetically below 4 K, which could coexist with superconductivity.

cond-mat.supr-con↗

Strong-coupling superconductivity in layered nickel-based LaO$_{1-x}$F$_x$NiAs

A series of layered nickel-based LaO$_{1-x}$F$_x$NiAs compounds with x=0 to 0.15 are synthesized by solid state reactions. The pure LaONiAs exhibits bulk superconductivity with Tc $\sim$ 2.75 K. Partial substitution of oxygen by fluorine increases the transition temperature to $\sim 3.8$ K. The LaO$_{0.9}$F$_{0.1}$NiAs sample shows a sharp superconducting transition and a sharp specific heat jump at the critical temperature. The magnitude of the specific heat jump is much larger than that expected from the weak-coupling BCS theory, indicating that this superconductor is in the strong coupling regime. Furthermore, the temperature dependence of the specific heat deviates strongly from the theoretical result for the single-band s- or d-wave superconductor, but shows some character of a multi-gap system.

cond-mat.supr-con↗

Element substitution effect in transition metal oxypnictide Re(O$_{1-x}$F$_x$)TAs (Re=rare earth, T=transition metal)

Different element substitution effects in transition metal oxypnictide Re(O$_{1-x}$F$_x$)TAs with Re=La, Ce, Nd, Eu, Gd, Tm, T=Fe, Ni, Ru, were studied. Similar to the La- or Ce-based systems, we found that the pure NdOFeAs shows a strong resistivity anomaly near 145 K, which was ascribed to the spin-density-wave instability. Electron doping by F increases T$_c$ to about 50 K. While in the case of Gd, the T$_c$ is reduced below 10 K. The tetragonal ZrCuSiAs-type structure could not be formed for Eu or Tm substitution in our preparing process. For Ni-based case, although both pure and F-doped LaONiAs are superconducting, no superconductivity was found when La was replaced by Ce in both cases, instead a ferromagnetic ordering transition was likely to form at low temperature in F-doped sample. We also synthesized LaO$_{1-x}$F$_x$RuAs and CeO$_{1-x}$F$_x$RuAs compounds. Metallic behavior was observed down to 4 K.

cond-mat.supr-con↗

Competing Orders and Spin-Density-Wave Instability in La(O$_{1-x}$F$_x$)FeAs

The interplay between different ordered phases, such as superconducting, charge or spin ordered phases, is of central interest in condensed matter physics. The very recent discovery of superconductivity with a remarkable T$_c$= 26 K in Fe-based oxypnictide La(O$_{1-x}$F$_x$)FeAs is a surprise to the scientific community\cite{Kamihara08}. The pure LaOFeAs itself is not superconducting but shows an anomaly near 150 K in both resistivity and dc magnetic susceptibility. Here we provide combined experimental and theoretical evidences showing that the anomaly is caused by the spin-density-wave (SDW) instability, and electron-doping by F suppresses the SDW instability and recovers the superconductivity. Therefore, the La(O$_{1-x}$F$_x$)FeAs offers an exciting new system showing competing orders in layered compounds.

cond-mat.supr-con↗

Study of Hadron Scattering Using an Asymmetric Box

We propose to study hadron-hadron scattering using lattice QCD in an asymmetric box which allows one to access more non-degenerate low-momentum modes for a given volume. The conventional Lüscher's formula applicable in a symmetric box is modified accordingly. To illustrate the feasibility of this approach, pion-pion elastic scattering phase shifts in the I=2, J=0 channel are calculated within quenched approximation using improved gauge and Wilson fermion actions on anisotropic lattices in an asymmetric box. After the chiral and continuum extrapolation, we find that our quenched results for the scattering phase shifts in this channel are consistent with the experimental data when the three-momentum of the pion is below 300MeV. Agreement is also found when compared with previous theoretical results from lattice and other means. Moreover, with the usage of asymmetric volume, we are able to compute the scattering phases in the low-momentum range (pion three momentum less than about 350MeV in the center of mass frame) for over a dozen values of the pion three-momenta, much more than using the conventional symmetric box with comparable volume.

hep-lat↗

Anomalous metallic state of Cu$_{0.07}$TiSe$_2$: an optical spectroscopy study

We report an optical spectroscopy study on the newly discovered superconductor Cu$_{0.07}$TiSe$_2$. Consistent with the development from a semimetal or semiconductor with a very small indirect energy gap upon doping TiSe$_2$, it is found that the compound has a low carrier density. Most remarkably, the study reveals a substantial shift of the "screened" plasma edge in reflectance towards high energy with decreasing temperature. This phenomenon, rarely seen in metals, indicates either a sizeable increase of the conducting carrier concentration or/and a decrease of the effective mass of carriers with reducing temperature. We attribute the shift primarily to the later effect.

cond-mat.supr-con↗

Semimetal to semimetal charge density wave transition in 1T-TiSe$_2$

We report an infrared study on 1$T$-TiSe$_2$, the parent compound of the newly discovered superconductor Cu$_x$TiSe$_2$. Previous studies of this compound have not conclusively resolved whether it is a semimetal or a semiconductor: information that is important in determining the origin of its unconventional CDW transition. Here we present optical spectroscopy results that clearly reveal that the compound is metallic in both the high-temperature normal phase and the low-temperature CDW phase. The carrier scattering rate is dramatically different in the normal and CDW phases and the carrier density is found to change with temperature. We conclude that the observed properties can be explained within the scenario of an Overhauser-type CDW mechanism.

cond-mat.str-el↗

Optical study of the charge-density-wave mechanism in 2$H$-TaS$_2$ and Na$_x$TaS$_2$

We report an optical study of transition metal dichalcogenide 2$H$-TaS$_2$ and Na intercalated superconductor Na$_x$TaS$_2$ over a broad frequency range at various temperatures. A clear gap feature was observed for 2$H$-TaS$_2$ when it undergoes a CDW transition. The existence of a Drude component in $σ$$_1$($ω$) below T$_{CDW}$ indicates that the Fermi surface of 2$H$-TaS$_2$ is only partially gapped in CDW state. The spectral evolution of two different Na$_x$TaS$_2$ crystals further confirms that the partial gap structure observed in 2$H$-TaS$_2$ has a CDW origin. The CDW mechanism for 2$H$-TaS$_2$, the competition between CDW and superconductivity in Na$_x$TaS$_2$ system are discussed.

cond-mat.supr-con↗

Optical study of MgTi$_2$O$_4$: Evidence for an orbital-Peierls state

Dimension reduction due to the orbital ordering has recently been proposed to explain the exotic charge, magnetic and structural transitions in some three-dimensional (3D) transitional metal oxides. We present optical measurement on a spinel compound MgTi$_2$O$_4$ which undergoes a sharp metal-insulator transition at 240 K, and show that the spectral change across the transition can be well understood from the proposed picture of 1D Peierls transition driven by the ordering of $d_{yz}$ and $d_{zx}$ orbitals. We further elaborate that the orbital-driven instability picture applies also very well to the optical data of another spinel CuIr$_2$S$_4$ reported earlier.

cond-mat.str-el↗

Determining the upper limit of Gamma_{ee} for the Y(4260)

By fitting the R values between 3.7 and 5.0 GeV measured by the BES collaboration, the upper limit of the electron width of the newly discovered resonance Y(4260) is determined to be 580 eV at 90% C.L. Together with the BABAR measurement on the product of Gamma_{ee} and BR(Y(4260) --> pi+pi- J/psi), this implies a large decay width of Y(4260) --> pi+pi- J/psi final states.

hep-ex↗

Doping evolution of chemical potential, spin-correlation gap, and charge dynamics in Nd$_{2-x}$Ce$_x$CuO$_4$

We report optical reflectivity study on Nd$_{2-x}$Ce$_x$CuO$_4$ over a broad doping range 0$\leq x\leq$0.20. The study reveals a systematic shift of chemical potential with doping. A pronounced peak structure specific to the electron-doped cuprate is observed in optical scattering rate based on the extended Drude model analysis. The energy scale of the peak could be very different from that of the peak in conductivity spectrum. We clarify that the "hot spots" gap probed in photoemission experiments correlates directly with the sharp suppression feature in scattering rate rather than conductivity spectra. The gap is associated with the short-range antiferromagnetic correlation, and disappears in a manner of fading away with increasing doping and temperature. In the heavily overdoped region, a dominant $ω^2$-dependence of the scattering rate is identified up to very high energy.

cond-mat.supr-con↗