arXiv subjects

Gary A. Steele

Publications and source records attributed to Gary A. Steele.

At least 55 records · Page 3Linked to original sources

arXiv2017

Giant modulation of the electronic band gap of carbon nanotubes by dielectric screening

Carbon nanotubes (CNTs) are a promising material for high-performance electronics beyond silicon. But unlike silicon, the nature of the transport band gap in CNTs is not fully understood. The transport gap in CNTs is predicted to be strongly driven by electron-electron (e-e) interactions and correlations, even at room temperature. Here, we use dielectric liquids to screen e-e interactions in individual suspended ultra-clean CNTs. Using multiple techniques, the transport gap is measured as dielectric screening is increased. Changing the dielectric environment from air to isopropanol, we observe a 25% reduction in the transport gap of semiconducting CNTs, and a 32% reduction in the band gap of narrow-gap CNTs. Additional measurements are reported in dielectric oils. Our results elucidate the nature of the transport gap in CNTs, and show that dielectric environment offers a mechanism for significant control over the transport band gap.

cond-mat.mes-hall↗

arXiv2017

A split-cavity design for the incorporation of a DC bias in a 3D microwave cavity

We report on a technique for applying a DC bias in a 3D microwave cavity. We achieve this by isolating the two halves of the cavity with a dielectric and directly using them as DC electrodes. As a proof of concept, we embed a variable capacitance diode in the cavity and tune the resonant frequency with a DC voltage, demonstrating the incorporation of a DC bias into the 3D cavity with no measurable change in its quality factor at room temperature. We also characterize the architecture at millikelvin temperatures and show that the split cavity design maintains a quality factor $Q_\text{i} \sim 8.8 \times 10^5$, making it promising for future quantum applications.

cond-mat.mes-hall↗

arXiv2017

Multi-mode ultra-strong coupling in circuit quantum electrodynamics

With the introduction of superconducting circuits into the field of quantum optics, many novel experimental demonstrations of the quantum physics of an artificial atom coupled to a single-mode light field have been realized. Engineering such quantum systems offers the opportunity to explore extreme regimes of light-matter interaction that are inaccessible with natural systems. For instance the coupling strength $g$ can be increased until it is comparable with the atomic or mode frequency $ω_{a,m}$ and the atom can be coupled to multiple modes which has always challenged our understanding of light-matter interaction. Here, we experimentally realize the first Transmon qubit in the ultra-strong coupling regime, reaching coupling ratios of $g/ω_{m}=0.19$ and we measure multi-mode interactions through a hybridization of the qubit up to the fifth mode of the resonator. This is enabled by a qubit with 88% of its capacitance formed by a vacuum-gap capacitance with the center conductor of a coplanar waveguide resonator. In addition to potential applications in quantum information technologies due to its small size and localization of electric fields in vacuum, this new architecture offers the potential to further explore the novel regime of multi-mode ultra-strong coupling.

quant-ph↗

arXiv2017

Approaching ultra-strong coupling in Transmon circuit-QED using a high-impedance resonator

In this experiment, we couple a superconducting Transmon qubit to a high-impedance $645\ Ω$ microwave resonator. Doing so leads to a large qubit-resonator coupling rate $g$, measured through a large vacuum Rabi splitting of $2g\simeq 910$ MHz. The coupling is a significant fraction of the qubit and resonator oscillation frequencies $ω$, placing our system close to the ultra-strong coupling regime ($\bar{g}=g/ω=0.071$ on resonance). Combining this setup with a vacuum-gap Transmon architecture shows the potential of reaching deep into the ultra-strong coupling $\bar{g} \sim 0.45$ with Transmon qubits.

quant-ph↗

arXiv2016

Strong and tunable couplings in flux-mediated optomechanics

We investigate superconducting interference device (SQUID) with two asymmetric Josephson junctions coupled to a mechanical resonator embedded in the loop of the SQUID. We quantize this system in the case when the frequency of the mechanical resonator is much lower than the cavity frequency of the SQUID and in the case when they are comparable. In the first case, the radiation pressure and cross-Kerr type interactions arise and are modified by asymmetry. Cross-Kerr type coupling is the leading term at the extremum points where radiation pressure is zero. In the second case, the main interaction is single-photon beam splitter, which exists only at finite asymmetry. Another interaction in this regime is of cross-Kerr type, which exists at all asymmetries, but generally much weaker than the beam splitter interaction. Increasing magnetic field can substantially enhance optomechanical couplings strength with the potential for the radiation pressure coupling to reach the single-photon strong coupling regime, even the ultrastrong coupling regime, in which the single-photon coupling rate exceeds the mechanical frequency.

cond-mat.mes-hall↗

arXiv2016

Thickness dependent interlayer transport in vertical MoS2 Josephson junctions

We report on observations of thickness dependent Josephson coupling and multiple Andreev reflections (MAR) in vertically stacked molybdenum disulfide (MoS2) - molybdenum rhenium (MoRe) Josephson junctions. MoRe, a chemically inert superconductor, allows for oxide free fabrication of high transparency vertical MoS2 devices. Single and bilayer MoS2 junctions display relatively large critical currents (up to 2.5 uA) and the appearance of sub-gap structure given by MAR. In three and four layer thick devices we observe orders of magnitude lower critical currents (sub-nA) and reduced quasiparticle gaps due to proximitized MoS2 layers in contact with MoRe. We anticipate that this device architecture could be easily extended to other 2D materials.

cond-mat.mes-hall↗

arXiv2016

Enhanced superconductivity in atomically thin TaS2

The ability to exfoliate layered materials down to the single layer limit has opened the opportunity to understand how a gradual reduction in dimensionality affects the properties of bulk materials. Here we use this top-down approach to address the problem of superconductivity in the two-dimensional limit. The transport properties of electronic devices based on 2H tantalum disulfide flakes of different thicknesses are presented. We observe that superconductivity persists down to the thinnest layer investigated (3.5 nm), and interestingly, we find a pronounced enhancement in the critical temperature from 0.5 K to 2.2 K as the layers are thinned down. In addition, we propose a tight-binding model, which allows us to attribute this phenomenon to an enhancement of the effective electron-phonon coupling constant. This work provides evidence that reducing dimensionality can strengthen superconductivity as opposed to the weakening effect that has been reported in other 2D materials so far.

cond-mat.supr-con↗

arXiv2016

Folded MoS2 layers with reduced interlayer coupling

We study molybdenum disulfide (MoS2) structures generated by folding single- and bilayer MoS2 flakes. We find that this modified layer stacking leads to a decrease in the interlayer coupling and an enhancement of the photoluminescence emission yield. We additionally find that folded single-layer MoS2 structures show a contribution to photoluminescence spectra of both neutral and charged excitons, which is a characteristic feature of single-layer MoS2 that has not been observed in multilayer MoS2. The results presented here open the door to fabrication of multilayered MoS2 samples with high optical absorption while maintaining the advantageous enhanced photoluminescence emission of single-layer MoS2 by controllably twisting the MoS2 layers.

cond-mat.mes-hall↗

arXiv2015

Gate-tunable diode and photovoltaic effect in an organic-2D layered material p-n junction

The semiconducting p-n junction is a simple device structure with great relevance for electronic and optoelectronic applications. The successful integration of low-dimensional materials in electronic circuits has opened the way forward for producing gate-tunable p-n junctions. In that context, here we present an organic (Cu-phthalocyanine)-2D layered material (MoS2) hybrid p-n junction with both gate-tunable diode characteristics and photovoltaic effect. Our proof-of-principle devices show multifunctional properties with diode rectifying factors of up to 10^4, while under light exposure they exhibit photoresponse with a measured external quantum efficiency of ~ 11 %. As for their photovoltaic properties, we found open circuit voltages of up to 0.6 V and optical-to-electrical power conversion efficiency of 0.7 %. The extended catalogue of known organic semiconductors and two-dimensional materials offer the prospect for tailoring the properties and the performance of the resulting devices, making organic-2D p-n junctions promising candidates for future technological applications.

cond-mat.mtrl-sci↗

arXiv2015

Broadband architecture for galvanically accessible superconducting microwave resonators

In many hybrid quantum systems, a superconducting circuit is required that combines DC-control with a coplanar waveguide (CPW) microwave resonator. The strategy thus far for applying a DC voltage or current bias to microwave resonators has been to apply the bias through a symmetry point in such a way that it appears as an open circuit for certain frequencies. Here, we introduce a microwave coupler for superconducting CPW cavities in the form of a large shunt capacitance to ground. Such a coupler acts as a broadband mirror for microwaves while providing galvanic connection to the center conductor of the resonator. We demonstrate this approach with a two-port $λ/4$-transmission resonator with linewidths in the MHz regime ($Q\sim10^3$) that shows no spurious resonances and apply a voltage bias up to $80$ V without affecting the quality factor of the resonator. This resonator coupling architecture, which is simple to engineer, fabricate and analyse, could have many potential applications in experiments involving superconducting hybrid circuits.

cond-mat.mes-hall↗

arXiv2015

Large cooperativity and microkelvin cooling with a three-dimensional optomechanical cavity

In cavity optomechanics, light is used to control mechanical motion. A central goal of the field is achieving single-photon strong coupling, which would enable the creation of quantum superposition states of motion. Reaching this limit requires significant improvements in optomechanical coupling and cavity coherence. Here we introduce an optomechanical architecture consisting of a silicon nitride membrane coupled to a three-dimensional superconducting microwave cavity. Exploiting their large quality factors, we achieve an optomechanical cooperativity of 146,000 and perform sideband cooling of the kilohertz-frequency membrane motion to 34$\pm$5 $μ$K, the lowest mechanical mode temperature reported to date. The achieved cooling is limited only by classical noise of the signal generator, and should extend deep into the ground state with superconducting filters. Our results suggest that this realization of optomechanics has the potential to reach the regimes of ultra-large cooperativity and single-photon strong coupling, opening up a new generation of experiments.

cond-mat.mes-hall↗

arXiv2015

Negative nonlinear damping of a graphene mechanical resonator

We experimentally investigate the nonlinear response of a multilayer graphene resonator using a superconducting microwave cavity to detect its motion. The radiation pressure force is used to drive the mechanical resonator in an optomechanically induced transparency configuration. By varying the amplitudes of drive and probe tones, the mechanical resonator can be brought into a nonlinear limit. Using the calibration of the optomechanical coupling, we quantify the mechanical Duffing nonlinearity. By increasing the drive force, we observe a decrease in the mechanical dissipation rate at large amplitudes, suggesting a negative nonlinear damping mechanism in the graphene resonator. Increasing the optomechanical backaction, we observe a nonlinear regime not described by a Duffing response that includes new instabilities of the mechanical response.

cond-mat.mes-hall↗

arXiv2015

Optomechanical response of a non-linear mechanical resonator

We investigate theoretically in detail the non-linear effects in the response of an optical/microwave cavity coupled to a Duffing mechanical resonator. The cavity is driven by a laser at a red or blue mechanical subband, and a probe laser measures the reflection close to the cavity resonance. Under these conditions, we find that the cavity exhibits optomechanically induced reflection (OMIR) or absorption (OMIA) and investigate the optomechanical response in the limit of non-linear driving of the mechanics. Similar to linear mechanical drive, an overcoupled cavity the red-sideband drive may lead to both OMIA and OMIR depending on the strength of the drive, whereas the blue-sideband drive only leads to OMIR. The dynamics of the phase of the mechanical resonator leads to the difference between the shapes of the response of the cavity and the amplitude response of the driven Duffing oscillator, for example, at weak red-sideband drive the OMIA dip has no inflection point. We also verify that mechanical non-linearities beyond Duffing model have little effect on the size of the OMIA dip though they affect the width of the dip.

cond-mat.mes-hall↗

arXiv2015

Photocurrent generation with two-dimensional van der Waals semiconductors

Two-dimensional (2D) materials have attracted a great deal of interest in recent years. This family of materials allows for the realization of versatile electronic devices and holds promise for next-generation (opto)electronics. Their electronic properties strongly depend on the number of layers, making them interesting from a fundamental standpoint. For electronic applications, semiconducting 2D materials benefit from sizable mobilities and large on/off ratios, due to the large modulation achievable via the gate field-effect. Moreover, being mechanically strong and flexible, these materials can withstand large strain (>10\%) before rupture, making them interesting for strain engineering and flexible devices. Even in their single layer form, semiconducting 2D materials have demonstrated efficient light absorption, enabling large responsivity in photodetectors. Therefore, semiconducting layered 2D materials are strong candidates for optoelectronic applications, especially for photodetection. Here, we review the state-of-the-art in photodetectors based on semiconducting 2D materials, focusing on the transition metal dichalcogenides, novel van der Waals materials, black phosphorus, and heterostructures.

cond-mat.mes-hall↗

arXiv2015

High-Q Tantalum Oxide Nanomechanical Resonators by Laser-Oxidation of TaSe2

Controlling the strain in two-dimensional materials is an interesting avenue to tailor the mechanical properties of nanoelectromechanical systems. Here we demonstrate a technique to fabricate ultrathin tantalum oxide nanomechanical resonators with large stress by laser-oxidation of nano-drumhead resonators made out of tantalum diselenide (TaSe2), a layered 2D material belonging to the metal dichalcogenides. Prior to the study of their mechanical properties with a laser interferometer, we checked the oxidation and crystallinity of the freely-suspended tantalum oxide in a high-resolution electron microscope. We show that the stress of tantalum oxide resonators increase by 140 MPa (with respect to pristine TaSe2 resonators) which causes an enhancement of quality factor (14 times larger) and resonance frequency (9 times larger) of these resonators.

cond-mat.mes-hall↗

arXiv2015

Observation of decoherence in a carbon nanotube mechanical resonator

In physical systems, decoherence can arise from both dissipative and dephasing processes. In mechanical resonators, the driven frequency response measures a combination of both, while time domain techniques such as ringdown measurements can separate the two. Here, we report the first observation of the mechanical ringdown of a carbon nanotube mechanical resonator. Comparing the mechanical quality factor obtained from frequency- and time-domain measurements, we find a spectral quality factor four times smaller than that measured in ringdown, demonstrating dephasing-induced decoherence of the nanomechanical motion. This decoherence is seen to arise at high driving amplitudes, pointing to a non-linear dephasing mechanism. Our results highlight the importance of time-domain techniques for understanding dissipation in nano-mechanical resonators, and the relevance of decoherence mechanisms in nanotube mechanics.

cond-mat.mes-hall↗

arXiv2015

Environmental instability of few-layer black phosphorus

We study the environmental instability of mechanically exfoliated few-layer black phosphorus (BP). From continuous measurements of flake topography over several days, we observe an increase of over 200% in volume due to the condensation of moisture from air. We find that long term exposure to ambient conditions results in a layer-by-layer etching process of BP flakes. Interestingly, flakes can be etched down to single layer (phosphorene) thicknesses. BP's strong affinity for water greatly modifies the performance of fabricated field-effect transistors (FETs) measured in ambient conditions. Upon exposure to air, we differentiate between two timescales for doping of BP FET transfer characterisitcs: a short timescale (minutes) in which a shift in the threshold voltage occurs due to physisorbed oxygen and nitrogen, and a long timescale (hours) in which p-type doping occurs from water absorption. Continuous measurements of BP FETs in air reveal eventual degradation and break-down of the channel material after several days due to the layer-by-layer etching process.

cond-mat.mtrl-sci↗

arXiv2015

Mechanical manipulation and exfoliation of boron nitride flakes by micro-plowing with an AFM tip

We demonstrate a simple method to manipulate and exfoliate thick hexagonal boron nitride (h-BN) flakes using an atomic force microscope (AFM) cantilever and tip mounted to a micromanipulator stage. Thick flakes of tens to hundreds of nanometers can be thinned down to large area, few-layer and monolayer flakes. We characterize the resulting thinned-down flakes using AFM and Raman spectroscopy. This technique is extendable to other two dimensional, van der Waals materials.

cond-mat.mtrl-sci↗