arXiv subjects

Gavin W. Morley

Publications and source records attributed to Gavin W. Morley.

At least 19 recordsLinked to original sources

arXiv2026

Microkelvin resolution thermometry at the nanometre scale

Accurate temperature readings of transient events at the nanometer scale are challenging due to the low sensitivity of available sensors. Nanodiamonds containing nitrogen-vacancy (NV) centers have been used for nanoscale thermometry in complex environments, including inside living cells. However, their performance has been limited by short coherence times and low photon counts. In this work, we use isotopically-purified dual-NV nanodiamonds and a bespoke quantum sensing chip to showcase an order of magnitude improvement in temperature measurement sensitivity compared with previous reports. We demonstrate robust temperature measurements with an error of 682 $μ$K, experimental sensitivities below 50 mK/$\surd \text{Hz}$ and a shot-noise limited sensitivity of 9.6 mK/$\surd \text{Hz}$. To confirm the utility of these high-performance nanothermometers, we quantify the temperature change induced by the thermometry measurement itself, specifically the optical excitation laser used to probe the NV spin state. In addition, we observe directly at the nanometre scale the transient heating caused by the exothermic mixing of dimethyl sulfoxide in water. Sub-millikelvin resolution and millikelvin sensitivity thermometry unlock the possibility of monitoring minute thermal fluctuations in living systems and assessing catalyst performance at the nanometre scale.

quant-ph↗

arXiv2026

High-Resolution Electron Paramagnetic Resonance

Electron paramagnetic resonance (EPR) is a valuable tool for physics, chemistry, biology and medicine, providing complementary spectroscopic information to NMR. It has long been known that EPR at high magnetic fields offers greater spectral resolution, but limitations in the THz instrumentation have prevented the full realization of these opportunities. Here we describe an EPR spectrometer at the high magnetic field of 14 T using 396 GHz excitation, which adapts techniques from liquid-state NMR to obtain sharp EPR resonances with a width of 210 ppb (full-width half-maximum). We use this to measure resonance positions, and hence g-factors, with a precision that reaches $\pm$16 ppb. Our use of in-situ liquid-state NMR of our solvent within the same sample improves the accuracy of these measurements: it allows us to reference our EPR measurement back to dilute gas 3He NMR for which quantum calculations are accurate. We measure the g-factor of N@C60 in deuterated toluene as g = 2.002 099 09 (3), where the 3 in brackets means that the uncertainty on the last digit is $\pm$3.

physics.ins-det↗

arXiv2025

A Spin-Based Pathway to Testing the Quantum Nature of Gravity

A key open problem in physics is the correct way to combine gravity (described by general relativity) with everything else (described by quantum mechanics). This problem suggests that general relativity and possibly also quantum mechanics need fundamental corrections. Most physicists expect that gravity should be quantum in character, but gravity is fundamentally different to the other forces because it alone is described by spacetime geometry. Experiments are needed to test whether gravity, and hence space-time, is quantum or classical. We propose an experiment to test the quantum nature of gravity by checking whether gravity can entangle two micron-sized crystals. A pathway to this is to create macroscopic quantum superpositions of each crystal first using embedded spins and Stern-Gerlach forces. These crystals could be nanodiamonds containing nitrogen-vacancy (NV) centres. The spins can subsequently be measured to witness the gravitationally generated entanglement. This is based on extensive theoretical feasibility studies and experimental progress in quantum technology. The eventual experiment will require a medium-sized consortium with excellent suppression of decoherence including vibrations and gravitational noise. In this white paper, we review the progress and plans towards realizing this. While implementing these plans, we will further explore the most macroscopic superpositions that are possible, which will test theories that predict a limit to this.

quant-ph↗

arXiv2025

Nitrogen vacancy center in diamond-based Faraday magnetometer

The nitrogen vacancy (NV) center in diamond is a versatile color center used for magnetometry, quantum computing, and quantum communications. In this article, using a single laser beam as a pump and probe, we measure the spin states of the NV center using the Faraday effect and use such measurements to develop a novel magnetic field sensor. Using the spin-state-dependent effect on the left and right circularly polarized light, we probe and confirm the existence of spin-orbit coupling in the NV center at room temperature. The sensitivity of our magnetometer is $350~$nT/$\sqrt{Hz}$, limited by the background produced by the laser trapped inside the diamond. We argue that by using an optical cavity and a high-purity diamond, sensitivities in the femtotesla level can be achieved.

physics.app-ph↗

arXiv2025

Broadband Fourier transform spectroscopy of quantum emitters photoluminescence with sub-nanosecond temporal resolution

The spectral characterization of quantum emitter luminescence over broad wavelength ranges and fast timescales is important for applications ranging from biophysics to quantum technologies. Here we present the application of time-domain Fourier transform spectroscopy, based on a compact and stable birefringent interferometer coupled to low-dark-count superconducting single-photon detectors, to the study of quantum emitters. We experimentally demonstrate that the system enables spectroscopy of quantum emitters over a broad wavelength interval from the near-infrared to the telecom range, where grating-based spectrometers coupled to InGaAs cameras are typically noisy and inefficient. We further show that the high temporal resolution of single-photon detectors, which can be on the order of tens of picoseconds, enables the monitoring of spin-dependent spectral changes on sub-nanosecond timescales.

quant-ph↗

arXiv2025

Long-Baseline Atom Interferometry

Long-baseline atom interferometry is a promising technique for probing various aspects of fundamental physics, astrophysics and cosmology, including searches for ultralight dark matter (ULDM) and for gravitational waves (GWs) in the frequency range around 1~Hz that is not covered by present and planned detectors using laser interferometry. The MAGIS detector is under construction at Fermilab, as is the MIGA detector in France. The PX46 access shaft to the LHC has been identified as a very suitable site for an atom interferometer of height $\sim 100$m, sites at the Boulby mine in the UK and the Canfranc Laboratory are also under investigation, and possible sites for km-class detectors have been suggested. The Terrestrial Very-Long-Baseline Atom Interferometry (TVLBAI) Proto-Collaboration proposes a coordinated programme of interferometers of increasing baselines.

hep-ex↗

arXiv2024

Real-time adaptive estimation of decoherence timescales for a single qubit

Characterising the time over which quantum coherence survives is critical for any implementation of quantum bits, memories and sensors. The usual method for determining a quantum system's decoherence rate involves a suite of experiments probing the entire expected range of this parameter, and extracting the resulting estimation in post-processing. Here we present an adaptive multi-parameter Bayesian approach, based on a simple analytical update rule, to estimate the key decoherence timescales ($T_1$, $T_2^*$ and $T_2$) and the corresponding decay exponent of a quantum system in real time, using information gained in preceding experiments. This approach reduces the time required to reach a given uncertainty by a factor up to an order of magnitude, depending on the specific experiment, compared to the standard protocol of curve fitting. A further speed-up of a factor $\sim 2$ can be realised by performing our optimisation with respect to sensitivity as opposed to variance.

quant-ph↗

arXiv2023

Additive GaN solid immersion lenses for enhanced photon extraction efficiency from diamond color centers

Effective light extraction from optically active solid-state spin centres inside high-index semiconductor host crystals is an important factor in integrating these pseudo-atomic centres in wider quantum systems. Here we report increased fluorescent light collection efficiency from laser-written nitrogen vacancy centers (NV) in bulk diamond facilitated by micro-transfer printed GaN solid immersion lenses. Both laser-writing of NV centres and transfer printing of micro-lens structures are compatible with high spatial resolution, enabling deterministic fabrication routes towards future scalable systems development. The micro-lenses are integrated in a non-invasive manner, as they are added on top of the unstructured diamond surface and bond by Van-der-Waals forces. For emitters at 5 micrometer depth, we find approximately 2x improvement of fluorescent light collection using an air objective with a numerical aperture of NA = 0.95 in good agreement with simulations. Similarly, the solid immersion lenses strongly enhance light collection when using an objective with NA = 0.5, significantly improving the signal-to-noise ratio of the NV center emission while maintaining the NV's quantum properties after integration.

physics.optics↗

arXiv2022

Snowmass 2021: Quantum Sensors for HEP Science -- Interferometers, Mechanics, Traps, and Clocks

A wide range of quantum sensing technologies are rapidly being integrated into the experimental portfolio of the high energy physics community. Here we focus on sensing with atomic interferometers; mechanical devices read out with optical or microwave fields; precision spectroscopic methods with atomic, nuclear, and molecular systems; and trapped atoms and ions. We give a variety of detection targets relevant to particle physics for which these systems are uniquely poised to contribute. This includes experiments at the precision frontier like measurements of the electron dipole moment and electromagnetic fine structure constant and searches for fifth forces and modifications of Newton's law of gravity at micron-to-millimeter scales. It also includes experiments relevant to the cosmic frontier, especially searches for gravitional waves and a wide variety of dark matter candidates spanning heavy, WIMP-scale, light, and ultra-light mass ranges. We emphasize here the need for more developments both in sensor technology and integration into the broader particle physics community.

quant-ph↗

arXiv2022

Snowmass White Paper: Precision Studies of Spacetime Symmetries and Gravitational Physics

High-energy physics is primarily concerned with uncovering the laws and principles that govern nature at the fundamental level. Research in this field usually relies on probing the boundaries of established physics, an undertaking typically associated with extreme energy and distance scales. It is therefore unsurprising that particle physics has traditionally been dominated by large-scale experimental methods often involving high energies, such as colliders and storage rings, cosmological and astrophysical observations, large-volume detector systems, etc. However, high-sensitivity measurements in smaller experiments, often performed at lower energies, are presently experiencing a surge in importance for particle physics for at least two reasons. First, they exploit synergies to adjacent areas of physics with recent advances in experimental techniques and technology. Together with intensified phenomenological explorations, these advances have led to the realization that challenges associated with weak couplings or the expected suppression factors for new physics can be overcome with such methods while maintaining a large degree of experimental control. Second, many of these measurements broaden the range of particle-physics phenomena and observables relative to the above set of more conventional methodologies. Combining such measurements with the conventional efforts above therefore casts both a wider and tighter net for possible effects originating from physics beyond the Standard Model (BSM). This paper argues that this assessment points at a growing impact of such methods and measurements on high-energy physics, and therefore warrants direct support as particle-physics research. Leveraging the recent rapid progress and bright outlook associated with such studies for high-energy physics, could yield high returns, but requires substantial and sustained efforts by funding agencies.

hep-ex↗

arXiv2022

MAQRO -- BPS 2023 Research Campaign Whitepaper

The objective of the proposed MAQRO mission is to harness space for achieving long free-fall times, extreme vacuum, nano-gravity, and cryogenic temperatures to test the foundations of physics in macroscopic quantum experiments. This will result in the development of novel quantum sensors and a means to probe the foundations of quantum physics at the interface with gravity. Earlier studies showed that the proposal is feasible but that several critical challenges remain, and key technologies need to be developed. These new technologies will open up the potential for achieving additional science objectives. The proposed research campaign aims to advance the state of the art and to perform the first macroscopic quantum experiments in space. Experiments on the ground, in micro-gravity, and in space will drive the proposed research campaign during the current decade to enable the implementation of MAQRO within the subsequent decade.

quant-ph↗

arXiv2021

Towards a test of quantum gravity with a levitated nanodiamond containing a spin

There is significant interest in potential experimental tests of macroscopic quantum effects, both to test potential modifications to quantum theory and to probe the quantum nature of gravity. A proposed platform with which to generate the required macroscopic quantum spatial superposition is a nanodiamond containing a negatively charged nitrogen vacancy (${\text{NV}}^{-}$) centre. In this review, methods to fabricate nanodiamonds containing ${\text{NV}}^{-}$ suitable for these quantum applications are discussed. The proposed probes of the macroscopic limits of quantum theory are presented along with the spin physics of the ${\text{NV}}^{-}$ centre relevant to those tests.

quant-ph↗

arXiv2021

Microscopic processes during ultra-fast laser generation of Frenkel defects in diamond

Engineering single atomic defects into wide bandgap materials has become an attractive field in recent years due to emerging applications such as solid-state quantum bits and sensors. The simplest atomic-scale defect is the lattice vacancy which is often a constituent part of more complex defects such as the nitrogen-vacancy (NV) centre in diamond, therefore an understanding of the formation mechanisms and precision engineering of vacancies is desirable. We present a theoretical and experimental study into the ultra-fast laser generation of vacancy-interstitial pairs (Frenkel defects) in diamond. The process is described by a set of coupled rate equations of the pulsed laser interaction with the material and of the non-equilibrium dynamics of charge carriers during and in the wake of the pulse. We find that a model for Frenkel defect generation via the recombination of a bound biexciton as the electron plasma cools provides good agreement with experimental data, reproducing an effective non-linearity of $\sim$ 40 for Frenkel defect generation with respect to laser pulse energy.

cond-mat.mtrl-sci↗

arXiv2020

Mesoscopic Interference for Metric and Curvature (MIMAC) & Gravitational Wave Detection

A compact detector for space-time metric and curvature is highly desirable. Here we show that quantum spatial superpositions of mesoscopic objects, of the type which would in principle become possible with a combination of state of the art techniques and taking into account the known sources of decoherence, could be exploited to create such a detector. By using Stern-Gerlach (SG) interferometry with masses much larger than atoms, where the interferometric signal is extracted by measuring spins, we show that accelerations as low as $5\times10^{-15}\textrm{ms}^{-2}\textrm{Hz}^{-1/2}$ or better, as well as the frame dragging effects caused by the Earth, could be sensed. Constructing such an apparatus to be non-symmetric would also enable the direct detection of curvature and gravitational waves (GWs). The GW sensitivity scales differently from the stray acceleration sensitivity, a unique feature of MIMAC. We have identified mitigation mechanisms for the known sources of noise, namely Gravity Gradient Noise (GGN), uncertainty principle and electro-magnetic forces. Hence it could potentially lead to a meter sized, orientable and vibrational noise (thermal/seismic) resilient detector of mid (ground based) and low (space based) frequency GWs from massive binaries (the predicted regimes are similar to those targeted by atom interferometers and LISA).

gr-qc↗

arXiv2019

Motional Dynamical Decoupling for Matter-Wave Interferometry

Matter-wave interferometry provides a remarkably sensitive tool for probing minute forces and, potentially, the foundations of quantum physics by making use of interference between spatially separated matter waves. Furthering this development requires ever-increasing stability of the interferometer, typically achieved by improving its physical isolation from the environment. Here we introduce as an alternative strategy the concept of dynamical decoupling applied to spatial degrees of freedom of massive objects. We show that the superposed matter waves can be driven along paths in space that render their superposition resilient to many important sources of noise. As a concrete implementation, we present the case of matter-wave interferometers in a magnetic field gradient based on either levitated or free-falling nanodiamonds hosting a color center. We present an in-depth analysis of potential sources of decoherence in such a setup and of the ability of our protocol to suppress them. These effects include gravitational forces, interactions of the net magnetic and dipole moments of the diamond with magnetic and electric fields, surface dangling bonds, rotational degrees of freedom, Casimir-Polder forces, and diamagnetic forces. Contrary to previous analyses, diamagnetic forces are not negligible in this type of interferometers and, if not acted upon lead to small separation distances that scale with the inverse of the magnetic field gradient. We show that our motional dynamical decoupling strategy renders the system immune to such limitations while continuing to protect its coherence from environmental influences, achieving a linear-in-time growth of the separation distance independent of the magnetic field gradient. Hence, motional dynamical decoupling may become an essential tool in driving the sensitivity of matter-wave interferometry to the next level.

quant-ph↗

arXiv2018

Matter and spin superposition in vacuum experiment (MASSIVE)

A free-falling nanodiamond containing a nitrogen vacancy centre in a spin superposition should experience a superposition of forces in an inhomogeneous magnetic field. We propose a practical design that brings the internal temperature of the diamond to under 10 K. This extends the expected spin coherence time from 2 ms to 500 ms, so the spatial superposition distance could be increased from 0.05 nm to over 1 $μ$m, for a 1 $μ$m diameter diamond and a magnetic inhomogeneity of only 10$^4$ T/m. The low temperature allows single-shot spin readout, reducing the number of nanodiamonds that need to be dropped by a factor of 10,000. We also propose solutions to a generic obstacle that would prevent such macroscopic superpositions.

quant-ph↗

arXiv2018

Laser writing of individual atomic defects in a crystal with near-unity yield

Atomic defects in wide band gap materials show great promise for development of a new generation of quantum information technologies, but have been hampered by the inability to produce and engineer the defects in a controlled way. The nitrogen-vacancy (NV) color center in diamond is one of the foremost candidates, with single defects allowing optical addressing of electron spin and nuclear spin degrees of freedom with potential for applications in advanced sensing and computing. Here we demonstrate a method for the deterministic writing of individual NV centers at selected locations with high positioning accuracy using laser processing with online fluorescence feedback. This method provides a new tool for the fabrication of engineered materials and devices for quantum technologies and offers insight into the diffusion dynamics of point defects in solids.

quant-ph↗

arXiv2017

A Spin Entanglement Witness for Quantum Gravity

Understanding gravity in the framework of quantum mechanics is one of the great challenges in modern physics. Along this line, a prime question is to find whether gravity is a quantum entity subject to the rules of quantum mechanics. It is fair to say that there are no feasible ideas yet to test the quantum coherent behaviour of gravity directly in a laboratory experiment. Here, we introduce an idea for such a test based on the principle that two objects cannot be entangled without a quantum mediator. We show that despite the weakness of gravity, the phase evolution induced by the gravitational interaction of two micron size test masses in adjacent matter-wave interferometers can detectably entangle them even when they are placed far apart enough to keep Casimir-Polder forces at bay. We provide a prescription for witnessing this entanglement, which certifies gravity as a quantum coherent mediator, through simple correlation measurements between two spins: one embedded in each test mass. Fundamentally, the above entanglement is shown to certify the presence of non-zero off-diagonal terms in the coherent state basis of the gravitational field modes.

quant-ph↗