arXiv subjects

Gerhard Rempe

Publications and source records attributed to Gerhard Rempe.

At least 37 records · Page 2Linked to original sources

arXiv2021

A Quantum-Logic Gate between Distant Quantum-Network Modules

The big challenge in quantum computing is to realize scalable multi-qubit systems with cross-talk free addressability and efficient coupling of arbitrarily selected qubits. Quantum networks promise a solution by integrating smaller qubit modules to a larger computing cluster. Such a distributed architecture, however, requires the capability to execute quantum-logic gates between distant qubits. Here we experimentally realize such a gate over a distance of 60m. We employ an ancillary photon that we successively reflect from two remote qubit modules, followed by a heralding photon detection which triggers a final qubit rotation. We use the gate for remote entanglement creation of all four Bell states. Our non-local quantum-logic gate could be extended both to multiple qubits and many modules for a tailor-made multi-qubit computing register.

quant-ph↗

arXiv2021

Continuous quantum light from a dark atom

Cycling processes are important in many areas of physics ranging from lasers to topological insulators, often offering surprising insights into dynamical and structural aspects of the respective system. Here we report on a quantum-nonlinear wave-mixing experiment where resonant lasers and an optical cavity define a closed cycle between several ground and excited states of a single atom. We show that, for strong atom-cavity coupling and steady-state driving, the entanglement between the atomic states and intracavity photon number suppresses the excited-state population via quantum interference, effectively reducing the cycle to the atomic ground states. The system dynamics then result from transitions within a harmonic ladder of entangled dark states, one for each cavity photon number, and a quantum Zeno blockade that generates antibunching in the photons emitted from the cavity. The reduced cycle suppresses unwanted optical pumping into atomic states outside the cycle, thereby enhancing the number of emitted photons.

quant-ph↗

arXiv2020

A Quantum Network Node with Crossed Optical Fibre Cavities

Quantum networks provide unique possibilities for resolving open questions on entanglement and promise innovative applications ranging from secure communication to scalable computation. While two quantum nodes coupled by a single channel are adequate for basic quantum communication tasks between two parties, fully functional large-scale quantum networks require a web-like architecture with multiply connected nodes. Efficient interfaces between network nodes and channels can be implemented with optical cavities. Using two optical fibre cavities coupled to one atom, we here realise a quantum network node that connects to two quantum channels. It functions as a passive, heralded and high-fidelity quantum memory that requires neither amplitude- and phase-critical control fields nor error-prone feedback loops. Our node is robust, fits naturally into larger fibre-based networks, can be scaled to more cavities, and thus provides clear perspectives for a quantum internet including qubit controlled quantum switches, routers, and repeaters.

quant-ph↗

arXiv2020

Buffer-gas cooling of molecules in the low-density regime: Comparison between simulation and experiment

Cryogenic buffer gas cells have been a workhorse for the cooling of molecules in the last decades. The straightforward sympathetic cooling principle makes them applicable to a huge variety of different species. Notwithstanding this success, detailed simulations of buffer gas cells are rare, and have never been compared to experimental data in the regime of low to intermediate buffer gas densities. Here, we present a numerical approach based on a trajectory analysis, with molecules performing a random walk in the cell due to collisions with a homogeneous buffer gas. This method can reproduce experimental flux and velocity distributions of molecules emerging from the buffer gas cell for varying buffer gas densities. This includes the strong decrease in molecule output from the cell for increasing buffer gas density and the so-called boosting effect, when molecules are accelerated by buffer-gas atoms after leaving the cell. The simulations provide various insights which could substantially improve buffer-gas cell design.

physics.chem-ph↗

arXiv2020

Dark-time decay of the retrieval efficiency of light stored as a Rydberg excitation in a noninteracting ultracold gas

We study the dark-time decay of the retrieval efficiency for light stored in a Rydberg state in an ultracold gas of $^{87}$Rb atoms based on electromagnetically induced transparency (EIT). Using low atomic density to avoid dephasing caused by atom-atom interactions, we measure a $1/e$ time of 30 $μ$s for the $80S$ state in free expansion. One of the dominant limitations is the combination of photon recoil and thermal atomic motion at 0.2 $μ$K. If the 1064-nm dipole trap is left on, then the $1/e$ time is reduced to 13 $μ$s, in agreement with a model taking differential light shifts and gravitational sag into account. To characterize how coherent the retrieved light is, we overlap it with reference light and measure the visibility $V$ of the resulting interference pattern, obtaining $V> 90\%$ for short dark time. Our experimental work is accompanied by a detailed model for the dark-time decay of the retrieval efficiency of light stored in atomic ensembles. The model is generally applicable for photon storage in Dicke states, such as in EIT with $Λ$-type or ladder-type level schemes and in Duan-Lukin-Cirac-Zoller single-photon sources. The model includes a treatment of the dephasing caused by thermal atomic motion combined with net photon recoil, as well as the influence of trapping potentials. It takes into account that the signal light field is typically not a plane wave. The model maps the retrieval efficiency to single-atom properties and shows that the retrieval efficiency is related to the decay of fringe visibility in Ramsey spectroscopy and to the spatial first-order coherence function of the gas.

quant-ph↗

arXiv2019

A Photon-Photon Quantum Gate Based on Rydberg Interactions

The interaction between Rydberg states of neutral atoms is strong and long-range, making it appealing to put it to use in the context of quantum technologies. Recently, first applications of this idea have been reported in the fields of quantum computation and quantum simulation. Furthermore, electromagnetically induced transparency allows to map these Rydberg interactions to light. Here we exploit this mapping and the resulting interaction between photons to realize a photon-photon quantum gate, demonstrating the potential of Rydberg systems as a platform also for quantum communication and quantum networking. We measure a controlled-NOT truth table with a fidelity of 70(8)% and an entangling-gate fidelity of 63.7(4.5)%, both post-selected upon detection of a control and a target photon. The level of control reached here is an encouraging step towards exploring novel many-body states of photons or for future applications in quantum communication and quantum networking.

quant-ph↗

arXiv2019

Deterministic creation of entangled atom-light Schrödinger-cat states

Quantum physics allows for entanglement between microscopic and macroscopic objects, described by discrete and continuous variables, respectively. As in Schrödinger's famous cat gedanken experiment, a box enclosing the objects can keep the entanglement alive. For applications in quantum information processing, however, it is essential to access the objects and manipulate them with suitable quantum tools. Here we reach this goal and deterministically generate entangled light-matter states by reflecting a coherent light pulse with up to four photons on average from an optical cavity containing one atom. The quantum light propagates freely and reaches a remote receiver for quantum state tomography. We produce a plethora of quantum states and observe negative-valued Wigner functions, a characteristic sign of non-classicality. As a first application, we demonstrate a quantum-logic gate between an atom and a light pulse, with the photonic qubit encoded in the phase of the light field.

quant-ph↗

arXiv2019

Single-Photon Distillation via a Photonic Parity Measurement Using Cavity QED

Single photons with tailored temporal profiles are a vital resource for future quantum networks. Here we distill them out of custom-shaped laser pulses that reflect from a single atom strongly coupled to an optical resonator. A subsequent measurement on the atom is employed to herald a successful distillation. Out of vacuum-dominated light pulses, we create single photons with fidelity $66(1)\%$, two-and-more-photon suppression $95.5(6)\%$, and a Wigner function with negative value $-0.125(6)$. Our scheme applied to state-of-the-art fiber resonators could boost the single-photon fidelity to up to $96\%$.

quant-ph↗

arXiv2018

High-resolution spectroscopy on cold electrically trapped formaldehyde

We present precision spectroscopy on electrically trapped formaldehyde (H$_2$CO), demonstrating key attributes which will enable molecular spectroscopy with unprecedented precision. Our method makes use of a microstructured electric trap with homogeneous fields in the trap center and rotational transitions with minimal Stark broadening at a 'magic' offset electric field. Using molecules cooled to the low millikelvin temperature regime via optoelectrical Sisyphus cooling, we reduce Stark broadening on the $J=5\leftarrow4$ ($K=3$) transition at 364 GHz to well below 1 kHz, observe Doppler-limited linewidths down to 3.8 kHz, and determine the line position with sub-kHz uncertainty. Our results and clear prospects for even narrower spectra pave the way towards in-trap precision spectroscopy on diverse molecule species.

physics.atom-ph↗

arXiv2018

Increased Dimensionality of Raman Cooling in a Slightly Nonorthogonal Optical Lattice

We experimentally study the effect of a slight nonorthogonality in a two-dimensional optical lattice onto resolved-sideband Raman cooling. We find that when the trap frequencies of the two lattice directions are equal, the trap frequencies of the combined potential exhibit an avoided crossing and the corresponding eigenmodes are rotated by 45 degrees relative to the lattice beams. Hence, tuning the trap frequencies makes it possible to rotate the eigenmodes such that both eigenmodes have a large projection onto any desired direction in the lattice plane, in particular, onto the direction along which Raman cooling works. Using this, we achieve two-dimensional Raman ground-state cooling in a geometry where this would be impossible, if the eigenmodes were not rotated. Our experiment is performed with a single atom inside an optical resonator but this is inessential and the scheme is expected to work equally well in other situations.

quant-ph↗

arXiv2018

Photon-Mediated Quantum Gate between Two Trapped Neutral Atoms in an Optical Cavity

Quantum logic gates are fundamental building blocks of quantum computers. Their integration into quantum networks requires strong qubit coupling to network channels, as can be realized with neutral atoms and optical photons in cavity quantum electrodynamics. Here we demonstrate that the long-range interaction mediated by a flying photon performs a gate between two stationary atoms inside an optical cavity from which the photon is reflected. This single step executes the gate in $2\,\mathrm{μs}$. We show an entangling operation between the two atoms by generating a Bell state with 76(2)% fidelity. The gate also operates as a CNOT. We demonstrate 74.1(1.6)% overlap between the observed and the ideal gate output, limited by the state preparation fidelity of 80.2(0.8)%. As the atoms are efficiently connected to a photonic channel, our gate paves the way towards quantum networking with multiqubit nodes and the distribution of entanglement in repeater-based long-distance quantum networks.

quant-ph↗

arXiv2017

A cryofuge for cold-collision experiments with slow polar molecules

Ultracold molecules represent a fascinating research frontier in physics and chemistry, but it has proven challenging to prepare dense samples at low velocities. Here we present a solution to this goal by a non-conventional approach dubbed cryofuge. It employs centrifugal force to bring cryogenically cooled molecules to kinetic energies below $1\,$K$\times k_B$ in the laboratory frame, with corresponding fluxes exceeding $10^{10}$/s at velocities below $20\,$m/s. By attaining densities higher than $10^9$/cm$^3$ and interaction times longer than $25\,$ms in samples of fluoromethane as well as deuterated ammonia, we observe cold dipolar collisions between molecules and determine their collision cross sections.

physics.atom-ph↗

arXiv2017

Cavity Carving of Atomic Bell States

We demonstrate entanglement generation of two neutral atoms trapped inside an optical cavity. Entanglement is created from initially separable two-atom states through carving with weak photon pulses reflected from the cavity. A polarization rotation of the photons heralds the entanglement. We show the successful implementation of two different protocols and the generation of all four Bell states with a maximum fidelity of (90+-2)%. The protocol works for any distance between cavity-coupled atoms, and no individual addressing is required. Our result constitutes an important step towards applications in quantum networks, e.g. for entanglement swapping in a quantum repeater.

quant-ph↗

arXiv2017

Two-Photon Blockade in an Atom-Driven Cavity QED System

Photon blockade is a dynamical quantum-nonlinear effect that occurs in driven systems with an anharmonic excitation ladder. For a single atom strongly coupled to an optical cavity, we show that driving the atom gives a decisively larger optical nonlinearity than driving the cavity. This enhances single-photon blockade and allows for the implementation of two-photon blockade where the absorption of two photons suppresses the absorption of further photons. As a signature, we report on three-photon antibunching with simultaneous two-photon bunching observed in the light emitted from the cavity. Our experiment constitutes a significant step towards multi-photon quantum-nonlinear optics.

quant-ph↗

arXiv2017

A photon-photon quantum gate based on a single atom in an optical resonator

Two photons in free space pass each other undisturbed. This is ideal for the faithful transmission of information, but prohibits an interaction between the photons as required for a plethora of applications in optical quantum information processing. The long-standing challenge here is to realise a deterministic photon-photon gate. This requires an interaction so strong that the two photons can shift each others phase by pi. For polarisation qubits, this amounts to the conditional flipping of one photon's polarisation to an orthogonal state. So far, only probabilistic gates based on linear optics and photon detectors could be realised, as "no known or foreseen material has an optical nonlinearity strong enough to implement this conditional phase shift..." [Science 318, 1567]. Meanwhile, tremendous progress in the development of quantum-nonlinear systems has opened up new possibilities for single-photon experiments. Platforms range from Rydberg blockade in atomic ensembles to single-atom cavity quantum electrodynamics. Applications like single-photon switches and transistors, two-photon gateways, nondestructive photon detectors, photon routers and nonlinear phase shifters have been demonstrated, but none of them with the ultimate information carriers, optical qubits. Here we employ the strong light-matter coupling provided by a single atom in a high-finesse optical resonator to realise the Duan-Kimble protocol of a universal controlled phase flip (CPF, pi phase shift) photon-photon quantum gate. We achieve an average gate fidelity of F=(76.2+/-3.6)% and specifically demonstrate the capability of conditional polarisation flipping as well as entanglement generation between independent input photons. Our gate could readily perform most of the hitherto existing two-photon operations. It also discloses avenues towards new quantum information processing applications where photons are essential.

quant-ph↗

arXiv2017

Fast, precise, and widely tunable frequency control of an optical parametric oscillator referenced to a frequency comb

Optical frequency combs (OFC) provide a convenient reference for the frequency stabilization of continuous-wave lasers. We demonstrate a frequency control method relying on tracking over a wide range and stabilizing the beat note between the laser and the OFC. The approach combines fast frequency ramps on a millisecond timescale in the entire mode-hop free tuning range of the laser and precise stabilization to single frequencies. We apply it to a commercially available optical parametric oscillator (OPO) and demonstrate tuning over more than 60 GHz with a ramping speed up to 3 GHz/ms. Frequency ramps spanning 15 GHz are performed in less than 10 ms, with the OPO instantly relocked to the OFC after the ramp at any desired frequency. The developed control hardware and software is able to stabilize the OPO to sub-MHz precision and to perform sequences of fast frequency ramps automatically.

physics.ins-det↗

arXiv2016

Optical $π$ Phase Shift Created with a Single-Photon Pulse

A deterministic photon-photon quantum-logic gate is a long-standing goal. Building such a gate becomes possible if a light pulse containing only one photon imprints a phase shift of $π$ onto another light field. Here we experimentally demonstrate the generation of such a $π$ phase shift with a single-photon pulse. A first light pulse containing less than one photon on average is stored in an atomic gas. Rydberg blockade combined with electromagnetically induced transparency creates a phase shift for a second light pulse which propagates through the medium. Postselected on the detection of a retrieved photon from the first pulse, we measure a $π$ phase shift of the second pulse. This demonstrates a crucial step toward a photon-photon gate and offers a variety of applications in the field of quantum information processing.

quant-ph↗

arXiv2016

An integrated quantum repeater at telecom wavelength with single atoms in optical fiber cavities

Quantum repeaters promise to enable quantum networks over global distances by circumventing the exponential decrease in success probability inherent in direct photon transmission. We propose a realistic, functionally integrated quantum repeater implementation based on single atoms in optical cavities. Entanglement is directly generated between the single-atom quantum memory and a photon at telecom wavelength. The latter is collected with high efficiency and adjustable temporal and spectral properties into a spatially well-defined cavity mode. It is heralded by a near-infrared photon emitted from a second, orthogonal cavity. Entanglement between two remote quantum memories can be generated via an optical Bell-state measurement, while we propose entanglement swapping based on a highly efficient, cavity-assisted atom-atom gate. Our quantum repeater scheme eliminates any requirement for wavelength conversion such that only a single system is needed at each node. We investigate a particular implementation with rubidium and realistic parameters for Fabry-Perot cavities based on CO$_2$ laser-machined optical fibers. We show that the scheme enables the implementation of a rather simple quantum repeater that outperforms direct entanglement generation over large distances and does not require any improvements in technology beyond the state of the art.

quant-ph↗