arXiv subjects

Gerhard Rempe

Publications and source records attributed to Gerhard Rempe.

At least 55 records · Page 3Linked to original sources

arXiv2016

Optoelectrical cooling of polar molecules to sub-millikelvin temperatures

We demonstrate direct cooling of gaseous formaldehyde (H2CO) to the microkelvin regime. Our approach, optoelectrical Sisyphus cooling, provides a simple dissipative cooling method applicable to electrically trapped dipolar molecules. By reducing the temperature by three orders of magnitude and increasing the phase-space density by a factor of ~$10^4$ we generate an ensemble of $3\cdot10^5$ molecules with a temperature of about 420μK, populating a single rotational state with more than 80% purity.

physics.atom-ph↗

arXiv2016

Interference and dynamics of light from a distance-controlled atom pair in an optical cavity

Interference is central to quantum physics and occurs when indistinguishable paths exist, like in a double-slit experiment. Replacing the two slits with two single atoms introduces optical non-linearities for which nontrivial interference phenomena are predicted. Their observation, however, has been hampered by difficulties in preparing the required atomic distribution, controlling the optical phases and detecting the faint light. Here we overcome all of these experimental challenges by combining an optical lattice for atom localisation, an imaging system with single-site resolution, and an optical resonator for light steering. We observe resonator-induced saturation of resonance fluorescence for constructive interference of the scattered light and nonzero emission with huge photon bunching for destructive interference. The latter is explained by atomic saturation and photon pair generation. Our experimental setting is scalable and allows one to realize the Tavis-Cummings model for any number of atoms and photons, explore fundamental aspects of light-matter interaction, and implement new quantum information processing protocols.

quant-ph↗

arXiv2015

Rotational cooling of trapped polyatomic molecules

Controlling the internal degrees of freedom is a key challenge for applications of cold and ultracold molecules. Here, we demonstrate rotational-state cooling of trapped methyl fluoride molecules (CH3F) by optically pumping the population of 16 M-sublevels in the rotational states J=3,4,5, and 6 into a single level. By combining rotational-state cooling with motional cooling, we increase the relative number of molecules in the state J=4, K=3, M=4 from a few percent to over 70%, thereby generating a translationally cold (~30mK) and nearly pure state ensemble of about 10^6 molecules. Our scheme is extendable to larger sets of initial states, other final states and a variety of molecule species, thus paving the way for internal-state control of ever larger molecules.

physics.atom-ph↗

arXiv2015

Breakdown of atomic hyperfine coupling in a deep optical-dipole trap

We experimentally study the breakdown of hyperfine coupling for an atom in a deep optical-dipole trap. One-color laser spectroscopy is performed at the resonance lines of a single $^{87}$Rb atom for a trap wavelength of 1064 nm. Evidence of hyperfine breakdown comes from three observations, namely a nonlinear dependence of the transition frequencies on the trap intensity, a splitting of lines which are degenerate for small intensities, and the ability to drive transitions which would be forbidden by selection rules in the absence of hyperfine breakdown. From the data, we infer the hyperfine interval of the $5P_{1/2}$ state and the scalar and tensor polarizabilities for the $5P_{3/2}$ state.

physics.atom-ph↗

arXiv2015

Cavity-based quantum networks with single atoms and optical photons

Distributed quantum networks will allow users to perform tasks and to interact in ways which are not possible with present-day technology. Their implementation is a key challenge for quantum science and requires the development of stationary quantum nodes that can send and receive as well as store and process quantum information locally. The nodes are connected by quantum channels for flying information carriers, i.e. photons. These channels serve both to directly exchange quantum information between nodes as well as to distribute entanglement over the whole network. In order to scale such networks to many particles and long distances, an efficient interface between the nodes and the channels is required. This article describes the cavity-based approach to this goal, with an emphasis on experimental systems in which single atoms are trapped in and coupled to optical resonators. Besides being conceptually appealing, this approach is promising for quantum networks on larger scales, as it gives access to long qubit coherence times and high light-matter coupling efficiencies. Thus, it allows one to generate entangled photons on the push of a button, to reversibly map the quantum state of a photon onto an atom, to transfer and teleport quantum states between remote atoms, to entangle distant atoms, to detect optical photons nondestructively, to perform entangling quantum gates between an atom and one or several photons, and even provides a route towards efficient heralded quantum memories for future repeaters. The presented general protocols and the identification of key parameters are applicable to other experimental systems.

quant-ph↗

arXiv2015

Heralded Storage of a Photonic Quantum Bit in a Single Atom

Combining techniques of cavity quantum electrodynamics, quantum measurement, and quantum feedback, we have realized the heralded transfer of a polarization qubit from a photon onto a single atom with 39% efficiency and 86% fidelity. The reverse process, namely, qubit transfer from the atom onto a given photon, is demonstrated with 88% fidelity and an estimated efficiency of up to 69%. In contrast to previous work based on two-photon interference, our scheme is robust against photon arrival-time jitter and achieves much higher efficiencies. Thus, it constitutes a key step toward the implementation of a long-distance quantum network.

quant-ph↗

arXiv2015

Frequency splitting of polarization eigenmodes in microscopic Fabry-Perot cavities

We study the frequency splitting of the polarization eigenmodes of the fundamental transverse mode in CO2 laser-machined, high-finesse optical Fabry-Perot cavities and investigate the influence of the geometry of the cavity mirrors. Their highly reflective surfaces are typically not rotationally symmetric but have slightly different radii of curvature along two principal axes. We observe that the eccentricity of such elliptical mirrors lifts the degeneracy of the polarization eigenmodes. The impact of the eccentricity increases for smaller radii of curvature. A model derived from corrections to the paraxial resonator theory is in excellent agreement with the measurements, showing that geometric effects are the main source of the frequency splitting of polarization modes for the type of microscopic cavity studied here. By rotating one of the mirrors around the cavity axis, the splitting can be tuned. In the case of an identical differential phase shift per mirror, it can even be eliminated, despite a nonvanishing eccentricity of each mirror. We expect our results to have important implications for many experiments in cavity quantum electrodynamics, where Fabry-Perot cavities with small mode volumes are required.

physics.optics↗

arXiv2014

Rotational state detection of electrically trapped polyatomic molecules

Detecting the internal state of polar molecules is a substantial challenge when standard techniques such as resonance-enhanced multi photon ionization (REMPI) or laser-induced fluorescense (LIF) do not work. As this is the case for most polyatomic molecule species, we here investigate an alternative based on state selective removal of molecules from an electrically trapped ensemble. Specifically, we deplete molecules by driving rotational and/or vibrational transitions to untrapped states. Fully resolving the rotational state with this method can be a considerable challenge as the frequency differences between various transitions is easily substantially less than the Stark broadening in an electric trap. However, making use of a unique trap design providing homogeneous fields in a large fraction of the trap volume, we successfully discriminate all rotational quantum numbers, including the rotational M-substate.

physics.atom-ph↗

arXiv2014

Single-Photon Transistor Using a Förster Resonance

An all-optical transistor is a device in which a gate light pulse switches the transmission of a target light pulse with a gain above unity. The gain quantifies the change of the transmitted target photon number per incoming gate photon. We study the quantum limit of one incoming gate photon and observe a gain of 20. The gate pulse is stored as a Rydberg excitation in an ultracold gas. The transmission of the subsequent target pulse is suppressed by Rydberg blockade which is enhanced by a Förster resonance. The detected target photons reveal in a single shot with a fidelity above 0.86 whether a Rydberg excitation was created during the gate pulse. The gain offers the possibility to distribute the transistor output to the inputs of many transistors, thus making complex computational tasks possible.

quant-ph↗

arXiv2014

A Quantum Gate between a Flying Optical Photon and a Single Trapped Atom

The steady increase in control over individual quantum systems has backed the dream of a quantum technology that provides functionalities beyond any classical device. Two particularly promising applications have been explored during the past decade: First, photon-based quantum communication, which guarantees unbreakable encryption but still has to be scaled to high rates over large distances. Second, quantum computation, which will fundamentally enhance computability if it can be scaled to a large number of quantum bits. It was realized early on that a hybrid system of light and matter qubits could solve the scalability problem of both fields - that of communication via quantum repeaters, that of computation via an optical interconnect between smaller quantum processors. To this end, the development of a robust two-qubit gate that allows to link distant computational nodes is "a pressing challenge". Here we demonstrate such a quantum gate between the spin state of a single trapped atom and the polarization state of an optical photon contained in a faint laser pulse. The presented gate mechanism is deterministic, robust and expected to be applicable to almost any matter qubit. It is based on reflecting the photonic qubit from a cavity that provides strong light-matter coupling. To demonstrate its versatility, we use the quantum gate to create atom-photon, atom-photon-photon, and photon-photon entangled states from separable input states. We expect our experiment to break ground for various applications, including the generation of atomic and photonic cluster states, Schrödinger-cat states, deterministic photonic Bell-state measurements, and quantum communication using a redundant quantum parity code.

quant-ph↗

arXiv2014

Single-Photon Switch based on Rydberg Blockade

All-optical switching is a technique in which a gate light pulse changes the transmission of a target light pulse without the detour via electronic signal processing. We take this to the quantum regime, where the incoming gate light pulse contains only one photon on average. The gate pulse is stored as a Rydberg excitation in an ultracold atomic gas using electromagnetically induced transparency. Rydberg blockade suppresses the transmission of the subsequent target pulse. Finally, the stored gate photon can be retrieved. A retrieved photon heralds successful storage. The corresponding postselected subensemble shows an extinction of 0.05. The single-photon switch offers many interesting perspectives ranging from quantum communication to quantum information processing.

quant-ph↗

arXiv2013

Nondestructive Detection of an Optical Photon

All optical detectors to date annihilate photons upon detection, thus excluding repeated measurements. Here, we demonstrate a robust photon detection scheme which does not rely on absorption. Instead, an incoming photon is reflected off an optical resonator containing a single atom prepared in a superposition of two states. The reflection toggles the superposition phase which is then measured to trace the photon. Characterizing the device with faint laser pulses, a single-photon detection efficiency of 74% and a survival probability of 66% is achieved. The efficiency can be further increased by observing the photon repeatedly. The large single-photon nonlinearity of the experiment should enable the development of photonic quantum gates and the preparation of novel quantum states of light.

quant-ph↗

arXiv2013

Generation of single photons from an atom-cavity system

A single rubidium atom trapped within a high-finesse optical cavity is an efficient source of single photons. We theoretically and experimentally study single-photon generation using a vacuum stimulated Raman adiabatic passage. We experimentally achieve photon generation efficiencies of up to 34% and 56% on the D1 and D2 line, respectively. Output coupling with 89% results in record-high efficiencies for single photons in one spatiotemporally well-defined propagating mode. We demonstrate that the observed generation efficiencies are constant in a wide range of applied pump laser powers and virtual level detunings. This allows for independent control over the frequency and wave packet envelope of the photons without loss in efficiency. In combination with the long trapping time of the atom in the cavity, our system constitutes a significant advancement toward an on-demand, highly efficient single-photon source for quantum information processing tasks.

quant-ph↗

arXiv2013

Ground-State Cooling of a Single Atom at the Center of an Optical Cavity

A single neutral atom is trapped in a three-dimensional optical lattice at the center of a high-finesse optical resonator. Using fluorescence imaging and a shiftable standing-wave trap, the atom is deterministically loaded into the maximum of the intracavity field where the atom-cavity coupling is strong. After 5ms of Raman sideband cooling, the three-dimensional motional ground state is populated with a probability of (89+/-2)%. Our system is the first to simultaneously achieve quantum control over all degrees of freedom of a single atom: its position and momentum, its internal state, and its coupling to light.

physics.atom-ph↗

arXiv2013

Efficient Teleportation between Remote Single-Atom Quantum Memories

We demonstrate teleportation of quantum bits between two single atoms in distant laboratories. Using a time-resolved photonic Bell-state measurement, we achieve a teleportation fidelity of (88.0+/-1.5)%, largely determined by our entanglement fidelity. The low photon collection efficiency in free space is overcome by trapping each atom in an optical cavity. The resulting success probability of 0.1% is almost 5 orders of magnitude larger than in previous experiments with remote material qubits. It is mainly limited by photon propagation and detection losses and can be enhanced with a cavity-based deterministic Bell-state measurement.

quant-ph↗

arXiv2012

Coherent Logic Gate for Light Pulses based on Storage in a Bose-Einstein Condensate

A classical logic gate connecting input and output light pulses is demonstrated. The gate operation is based on three steps: First, two incoming light pulses are stored in a Bose-Einstein condensate, second, atomic four-wave mixing generates a new matter wave, and third, the light pulses are retrieved. In the presence of the new matter wave, the retrieval generates a new optical wave. The latter will only be generated if both input light pulses are applied, thus realizing an AND gate. Finally, we show that the gate operation is phase coherent, an essential prerequisite for a quantum logic gate.

quant-ph↗

arXiv2012

Observation of squeezed light from one atom excited with two photons

Single quantum emitters like atoms are well-known as non-classical light sources which can produce photons one by one at given times, with reduced intensity noise. However, the light field emitted by a single atom can exhibit much richer dynamics. A prominent example is the predicted ability for a single atom to produce quadrature-squeezed light, with sub-shot-noise amplitude or phase fluctuations. It has long been foreseen, though, that such squeezing would be "at least an order of magnitude more difficult" to observe than the emission of single photons. Squeezed beams have been generated using macroscopic and mesoscopic media down to a few tens of atoms, but despite experimental efforts, single-atom squeezing has so far escaped observation. Here we generate squeezed light with a single atom in a high-finesse optical resonator. The strong coupling of the atom to the cavity field induces a genuine quantum mechanical nonlinearity, several orders of magnitude larger than for usual macroscopic media. This produces observable quadrature squeezing with an excitation beam containing on average only two photons per system lifetime. In sharp contrast to the emission of single photons, the squeezed light stems from the quantum coherence of photon pairs emitted from the system. The ability of a single atom to induce strong coherent interactions between propagating photons opens up new perspectives for photonic quantum logic with single emitters

quant-ph↗

arXiv2012

An Elementary Quantum Network of Single Atoms in Optical Cavities

Quantum networks are distributed quantum many-body systems with tailored topology and controlled information exchange. They are the backbone of distributed quantum computing architectures and quantum communication. Here we present a prototype of such a quantum network based on single atoms embedded in optical cavities. We show that atom-cavity systems form universal nodes capable of sending, receiving, storing and releasing photonic quantum information. Quantum connectivity between nodes is achieved in the conceptually most fundamental way: by the coherent exchange of a single photon. We demonstrate the faithful transfer of an atomic quantum state and the creation of entanglement between two identical nodes in independent laboratories. The created nonlocal state is manipulated by local qubit rotation. This efficient cavity-based approach to quantum networking is particularly promising as it offers a clear perspective for scalability, thus paving the way towards large-scale quantum networks and their applications.

quant-ph↗