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Giacomo Scalari

Publications and source records attributed to Giacomo Scalari.

At least 19 recordsLinked to original sources

Dynamically reconfigurable THz quantum walk comb laser through subharmonic excitation

On-chip frequency combs are increasingly relevant to both laser science and applications. Broad bandwidths and flat-top spectral envelopes are especially desirable for precision spectroscopy and dense wavelength-division multiplexed communications. Toward these goals, active microwave modulation has emerged as a powerful strategy for generating, stabilizing, and reconfiguring frequency combs at the source. However, practical challenges associated with high-frequency modulation imposes an upper bound on the accessible cavity free spectral ranges. Here, we demonstrate a subharmonic locking scheme in a quantum walk comb laser, a recently introduced platform for broadband and highly controllable comb states. Using a THz ring quantum cascade laser, we realize quantum walk comb formation under strong microwave injection at successive subharmonics of the cavity round-trip frequency, tuning the comb spacing from 15.8 to 1.58 GHz. The resulting states arise from fast-gain dynamics and nonlinear microwave mixing in the laser cavity. Through two-tone injection, we exploit this mixing to dynamically control the comb bandwidth and spectral shape. These results establish subharmonic excitation as a route to broadband, reconfigurable semiconductor comb generation in high-FSR cavities.

physics.optics

Amplitude- and frequency-modulated combs from an actively locked metasurface external-cavity laser

Optical frequency combs are key components of several photonics applications including spectroscopy, communications, and ultrafast photonics. A central challenge in frequency-comb photonics is to develop sources whose operating state can be precisely controlled and adapted to different application needs. We introduce frequency comb functionality to a THz metasurface vertical-external-cavity-surface-emitting laser (VECSEL), combining its characteristic high output power and excellent beam quality with a reconfigurable comb output. The source exhibits reversible switching between actively mode-locked 3.5 ps-long pulses and stable frequency-modulated quantum walk comb states. The flexible control of the intermodal phase relation is achieved through careful dispersion engineering via a Gires-Tournois interferometer (GTI) output-coupler combined with resonant RF bias modulation of the metasurface. These results pave the way for on-demand comb control in the THz range and provide a versatile strategy that could be extended to other semiconductor frequency-comb platforms and wavelength ranges.

physics.optics

Profiling THz Beams With Off-Label Use of Infrared Microbolometric Cameras

Visualizing the spatial profile of light beams is essential for evaluating irradiance, characterizing beam quality, and achieving precise alignment. In the optical spectral range, this is readily performed using silicon-based CCD and CMOS cameras. In the terahertz (THz) range, however, it typically requires specialized detectors with prohibitive costs. Here, we show that an infrared (IR) camera can be used outside of its labeled specifications to achieve similar performance as a dedicated microbolometric THz camera, at under 1% of the THz camera's cost. We compared the cameras by characterizing THz beam profiles from two sources: a pulsed broadband THz beam produced through optical rectification in organic crystals, and a narrowband quasi-continuous-wave (quasi-CW) THz beam emitted by a quantum cascade laser. For the broadband THz radiation, the beam width measured by the two cameras differed by only ~ 6%, well within the pixel resolution limit, and in the narrowband quasi-CW case by just ~ 1.3%. Additionally, the IR camera exhibits a lower minimum detectable power (down to 1.5 THz) than the THz camera, while also maintaining a linear and polarization-independent responsivity. These results expand the applicability of conventional IR cameras to the THz range, suggesting that they will become routine tools for high-fidelity THz beam diagnostics and imaging in scientific and industrial applications.

physics.optics

Absence of a Superradiant Phase Transition in Dirac Landau Polaritons

One of the most striking predictions in cavity quantum electrodynamics is the condensation of photons into a macroscopically populated ground state, the so-called superradiant phase transition (SRPT). SRPTs are theorized to occur in light-matter coupled systems above a critical coupling strength, yet have not been experimentally realized in equilibrium. On the contrary, the very existence of SRPTs has been largely disputed by No-Go theorems. In cavity-coupled electronic systems with Dirac dispersion, the diamagnetic $\vec{A}^2$-term crucial to No-go theorems is not present at leading order, making graphene Landau level transitions ultrastrongly coupled to terahertz cavities good candidates for SRPTs. In this work, we present the first terahertz spectroscopic measurements of an hBN-encapsulated monolayer graphene flake coupled to a highly sub-wavelength resonator mode. By tuning the graphene carrier density, we drive the resulting Landau polaritons into the ultrastrong coupling regime, with the normalized coupling reaching $\approx 40 \%$, approaching criticality. In this regime, the continuous SRPT would lead to a unique spectroscopic polariton softening, which we consistently rule out. The full polariton dispersion is instead quantitatively reproduced by a Hopfield Hamiltonian using a quasistatic near-field model that accounts for the sub-wavelength character of the cavity.

cond-mat.mes-hall

Ultrabroadband Gain-Switched and Superluminescent Terahertz Semiconductor Lasers

Terahertz quantum cascade lasers (THz QCLs) are chip-scale semiconductor lasers operating in the frequency range between 1-6 THz, useful as compact sources for spectroscopy, communications, and non-destructive imaging and testing. Here, we apply low-frequency microwave modulation on a planarized THz QCL to generate ultrabroadband emission in the THz range. For very low modulation frequencies below 1 GHz, a gain-switched octave-spanning spectrum with a smooth spectral envelope is generated between 1.9 - 4.1 THz. Increasing the modulation frequency broadens the lasing modes until a low-coherence, continuous emission spectrum is achieved in the superluminescent regime, covering the spectral region between around 3 - 4 THz, without any discrete lasing modes or spectral gaps. We complement the experimental results with extensive analytical models and numerical simulations that capture the intracavity laser dynamics and fully explain the different operation regimes. These devices could prove useful for absorption spectroscopy without any spectral gaps, and as ultrabroadband sources of THz radiation.

physics.optics

Spectral shaping of fast-gain frequency combs through phases in synthetic dimensions

Optical frequency comb devices have unlocked new capabilities in telecommunications, sensing, and metrology. Yet, precise in situ control of the comb spectral envelope remains extremely challenging. By introducing mode coupling with non-trivial phases, we demonstrate a spectral shaping technique that enables continuous tuning of a dominant spectral lobe across the full bandwidth of a semiconductor laser frequency comb. We achieve this jointly leveraging the engineered geometry of the synthetic lattice formed by the cavity modes of the laser and the coherent dynamics enabled by its fast-gain recovery. We use dual-tone modulation of the cavity at its repetition rate and twice this frequency with a controlled relative phase to couple the comb modes into a triangular lattice. The relative phase between the two tones defines a lattice phase that breaks time-reversal symmetry and steers the lattice dynamics through the fast gain. With this approach, we experimentally control the spectral envelope of the comb such that a targeted region contains more than twice the intensity expected from a uniform distribution, demonstrating tunable spectral selectivity. This capability, achieved directly at the light generation stage in a fast-gain device, opens routes for efficient programmable waveform engineering with potential applications in ranging, data transmission, and sensing.

physics.optics

Cavity modification of magnetoplasmon mode through coupling with intersubband polaritons

We investigate the coupling of a multi-mode metal-insulator-metal cavity to a two-dimensional electron gas (2DEG) in a quantum well in the presence of a strong magnetic field. The TM cavity mode is strongly hybridized with an intersubband transition of the 2DEG, forming a polaritonic mode in the ultrastrong coupling regime, while the TE mode remains an almost purely cavity mode. The magnetoplasmon excitation emerging from the presence of the magnetic field couples with both TM and TE modes, exhibiting different coupling strengths and levels of spatial field inhomogeneity. While the strong homogeneity of the bare TE mode gives rise to the standard anticrossing of strong coupling, the inhomogeneous polaritonic TM mode is shown to activate an observable Coulombic effect in the spectral response, often referred to as non-locality. This experiment demonstrates a cavity-induced modification of the 2DEG response and offers a new route to probing the effect of Coulomb interactions in ultrastrongly coupled systems via reshaping of their cavity mode profiles.

cond-mat.mes-hall

Quantum cascade laser roadmap

Quantum cascade lasers (QCLs) are unipolar semiconductor lasers first demonstrated in 1994. Since then, they have played a central role in advancing mid-infrared and terahertz photonics, becoming among the most reliable light sources in these regions of the electromagnetic spectrum. Their importance is further reinforced by their ability to generate self-starting optical frequency combs, whose investigation is motivated both by fundamental physics and by a wide range of applications, including molecular spectroscopy and free-space optical communications. This Roadmap provides a unified overview of current advances and emerging directions in QCL research. The chapters are organized into three main sections: device design and technology; frequency combs and pulse formation; and applications of QCLs. Each chapter reviews the relevant background, summarizes the current state of the art, and identifies key challenges and future directions within its specific research area.

physics.optics

Short period InGaAs/AlInAs THz quantum cascade laser in thin double metal cavities operating up to 188K

We present a two-well terahertz (THz) quantum cascade laser designed for high temperature operation based on the InGaAs/AlInAs material system. The lighter effective mass and higher energy barriers increase the gain at high temperatures (T > 150K). When processed in copper-based double metal waveguides the devices show laser action up to a maximum operating temperature of 188K with a maximum current density of 1.4kA/cm$^2$. The low Joule heating due to reduced active region thickness and low electrical bias allows operation at 10% duty cycle up to a temperature of 170K.

physics.optics

Short mode-locked pulses from planarized Y-coupled THz lasers

Short THz pulses are highly attractive both for fundamental research and practical applications in this underdeveloped region of the electromagnetic spectrum. Typically, THz pulses are generated using nonlinear optical methods, starting from a high-power visible or near-IR mode-locked source, but usually suffer from low conversion efficiencies. Here, we present a direct on-chip THz source of coherent short pulse trains based on active mode-locking of an inverse-designed planarized Y-coupled THz quantum cascade laser. By employing quasi-resonant microwave modulation of the asymmetric laser cavity, mode-locked pulses as short as 2.3 ps are generated, with emission bandwidths spanning 500 and 700 GHz at a central frequency of 2.9 THz.

physics.optics

Multi-mode Deep Strong Coupling in a Multi Quantum Well Fabry-Perot Cavity

We present multi-mode deep-strong coupling in a multi-quantum well (N=166) heterostructure. The heterostructure itself acts as a Fabry-Perot cavity, for which the even cavity modes strongly couple to the cyclotron resonance to form Landau polaritons. The experimentally observed vacuum Rabi splitting is larger than the mode spacing and well into the deep-strong coupling regime ($η>1$) resulting in a rich multi-mode polaritonic spectrum which is accurately reproduced by an all-to-all multi-photonic, multi-electronic Hopfield coupling model. Remarkably, light-matter decoupling is observed across the whole measurable spectrum, including in the low frequency limit ($λ>>L_{cav}$) where the normalized coupling strength reaches $η=8.1$. The system demonstrates a robust platform for exploring extreme coupling regimes and its chiral nature holds potential for chiral cavity and chiral mirror applications.

physics.optics

Gate-tunable single terahertz meta-atom ultrastrong light-matter coupling

We study the electrical tunability of ultrastrong light-matter interactions between a single terahertz circuit-based complementary split ring resonator (cSRR) and a two-dimensional electron gas. For this purpose, transmission spectroscopy measurements are performed under the influence of a strong magnetic field at different set points for the electric gate bias. The resulting Landau polariton dispersion depends on the applied electric bias, as the gating technique confines the electrons in-plane down to extremely sub-wavelength dimensions as small as d = 410 nm. This confinement allows for the excitation of standing plasma waves at zero magnetic field and an effective tunability of the electron number coupled to the THz resonator. This allows the normalized coupling strength to be tuned in-situ from $η$ = 0.46 down to $η$ = 0.18. This is the first demonstration of terahertz far-field spectroscopy of an electrically tunable interaction between a single terahertz resonator and electrons in a GaAs quantum well heterostructure.

cond-mat.mes-hall

Terahertz chiral sub-wavelength cavities breaking time-reversal symmetry via ultra-strong light-matter interaction

We demonstrate terahertz chiral sub-wavelength cavities that break time-reversal symmetry by coupling the degenerate linearly polarized modes of two orthogonal sets of nano-antenna arrays using the inter-Landau level transition of a two-dimensional electron gas in a perpendicular magnetic field, realizing normalized light-matter coupling rates up to $Ω_R/ω_{\mathrm{cav}} = 0.78$ with a dispersion that is modified by the parasitic capacitive coupling between the orthogonal antennas. The deep sub-wavelength confinement of the nano-antennas means that the ultra-strong coupling regime can be reached even with a small number of carriers compared to Fabry-Perot cavities, making it viable to be used with a variety of 2D materials. The non-degenerate circularly polarized ground state was only obtained after carefully optimizing the optical design to minimize the parasitic coupling to linearly polarized light.

cond-mat.mes-hall

Hybrid interfaces at the single quantum level in fluorescent molecules

We theoretically investigate a single fluorescent molecule as a hybrid quantum optical device, in which multiple external laser sources exert control of the vibronic states. In the high-saturation regime, a coherent interaction is established between the vibrational and electronic degrees of freedom, and molecules can simulate several cavity QED models, whereby a specific vibrational mode plays the role of the cavity mode. Focusing on the specific example where the system is turned into an analogue simulator of the quantum Rabi model, the steady state exhibits vibrational bi-modality resulting in a statistical mixture of highly non-classical vibronic cat states. Applying our paradigm to molecules with prominent spatial asymmetry and combining an optical excitation with a THz(IR) driving, the system can be turned into a single photon transducer. Two possible implementations are discussed based on the coupling to a subwavelength THz patch antenna or a resonant metamaterial. In a nutshell, this work assesses the role of molecules as an optomechanical quantum toolbox for creating hybrid entangled states of electrons, photons, and vibrations, hence enabling frequency conversion over very different energy scales.

quant-ph

Cavity QED Control of Quantum Hall Stripes

Controlling quantum phases of materials with vacuum field fluctuations in engineered cavities is a novel route towards the optical control of emergent phenomena. We demonstrate, using magnetotransport measurements of a high-mobility two-dimensional electron gas, striking cavity-induced anisotropies in the electronic transport, including the suppression of the longitudinal resistance well below the resistivity at zero magnetic field. Our cavity-induced effects occur at ultra-low temperatures (< 200 mK) when the magnetic field lies between quantized Hall plateaus. We interpret our results as arising from the stabilization of thermally-disordered quantum Hall stripes. Our work presents a clear demonstration of the cavity QED control of a correlated electronic phase.

cond-mat.mes-hall

On-chip, inverse-designed active wavelength division multiplexer at THz frequencies

The development of photonic integrated components for terahertz has become an active and growing research field. Despite its numerous applications, several challenges are still present in hardware design. We demonstrate an on-chip active wavelength division multiplexer (WDM) operating at THz frequencies. The WDM architecture is based on an inverse design topology optimization, which is applied in this case to the active quantum cascade heterostructure material embedded within a polymer in a planarized double metal cavity. Such an approach enables the fabrication of a strongly subwavelength device, with a normalized volume of only $V/λ^3 \simeq 0.5$. The WDM input is integrated with a THz quantum cascade laser frequency comb, providing three broadband output ports, ranging from 2.2 THz to 3.2 THz, with $\approx$ 330 GHz bandwidth and a maximum crosstalk of -6 dB. The three ports are outcoupled via integrated broadband patch array antennas with surface emission. Such a device can be also function as a stand-alone element, unlocking complex on-chip signal processing in the THz range

physics.optics

Continuously tunable coherent pulse generation in semiconductor lasers

In a laser, the control of its spectral emission depends on the physical dimensions of the optical resonator, limiting it to a set of discrete cavity modes at specific frequencies. Here, we overcome this fundamental limit by demonstrating a monolithic semiconductor laser with a continuously tunable repetition rate from 4 up to 16 GHz, by employing a microwave driving signal that induces a spatiotemporal gain modulation along the entire laser cavity, generating intracavity mode-locked pulses with a continuously tunable group velocity. At the output, frequency combs with continuously tunable mode spacings are generated in the frequency domain, and coherent pulse trains with continuously tunable repetition rates are generated in the time domain. Our results pave the way for fully tunable chip-scale lasers and frequency combs, advantageous for use in a diverse variety of fields, from fundamental studies to applications such as high-resolution and dual-comb spectroscopy.

physics.optics

A Quantum Walk Comb Source at Telecommunication Wavelengths

We demonstrate a quantum walk comb in synthetic frequency space formed by externally modulating a semiconductor optical amplifier operating in the telecommunication wavelength range in a unidirectional ring cavity. The ultrafast gain saturation dynamics of the gain medium and its operation at high current injections is responsible for the stabilization of the comb in a broad frequency modulated state. Our device produces a nearly flat broadband comb with a tunable repetition frequency reaching a bandwidth of 1.8THz at the fundamental repetition rate of 1GHz while remaining fully locked to the RF drive. Comb operation at harmonics of the repetition rate up to 14.1GHz is also demonstrated. This approach paves the way for next-generation optical frequency comb devices with potential applications in precision ranging and high-speed communications.

physics.optics