arXiv subjects

Gianpietro Cagnoli

Publications and source records attributed to Gianpietro Cagnoli.

18 recordsLinked to original sources

arXiv2026

Elastic and structural anisotropy in silica thin films for gravitational-wave detectors

The thermal noise of mirror coatings for gravitational-wave detectors critically depends on the elastic properties of the constituent materials. Data analyses and theoretical models typically assume each material is homogeneous and isotropic, but isotropy has never been explicitly verified. Using Brillouin light scattering (BLS), we demonstrate for the first time that ion-beam-sputtered SiO2 -- a material still viable for future mirror coatings -- exhibits cylindrical elastic symmetry, with in-plane isotropy but a notable 6% compressive anisotropy along the film normal. This anisotropy remains unchanged after the post-deposition heat treatment currently used in ground-based detectors (500 $^\circ$C, 10 h) but is nearly eliminated at 900 $^\circ$C. Infrared reflectivity experiments support these findings by directly revealing heterogeneities in the distribution of bridging and non-bridging oxygen structures along the growth axis. While BLS measures the real part of the elastic constants at GHz frequencies, the data reveal negligible contributions from mechanical relaxations in the kHz-GHz range, making BLS a valid substitute for low-frequency properties obtained from standard anisotropy-insensitive techniques. Our results highlight that restoring isotropy through heat treatment -- by softening the material, enabling more than 7% out-of-plane expansion, and smoothing out structural heterogeneities -- may play a key role in reducing thermal noise. This proof-of-concept study extends beyond silica, providing critical insights for the design of future coatings.

physics.optics↗

arXiv2025

Mechanical Characterisation of Silicon for the ETpathfinder Test Masses

The next generation of gravitational-wave detectors, such as the Einstein Telescope, is designed to reduce noise in a wide band of frequencies compared to the current generation, through the use of new technologies. ETpathfinder, designed as an R&D facility for these technologies, is a prototype for which the mirrors were chosen to be made of crystalline silicon, produced by the Leibniz-Institut für Kristallzüchtung. This material choice was made to pave the way for a low thermal noise level at cryogenic temperatures in the Einstein Telescope. This paper shows the mechanical loss of silicon designated to become the test masses for ETpathfinder in the range between room temperature and 53K. In addition, the effect of the anisotropic nature of silicon on the measurement procedure is addressed. Predictions are made of the contribution of the mirror substrate material to the overall ETpathfinder noise budget.

physics.ins-det↗

arXiv2023

TiO2 doping effect on reflective coating mechanical loss for gravitational wave detection at low temperature

We measured the mechanical loss of a dielectric multilayer reflective coating (ion-beam-sputtered SiO2 and Ta2O5) with and without TiO2 on sapphire disks between 6 and 77 K. The measured loss angle exhibited a temperature dependence, and the local maximum was found at approximately 20 K. This maximum was 7.0*10^(-4) (with TiO2) and 7.7*10^(-4) (without TiO2), although the previous measurement for the coating on sapphire disks showed almost no temperature dependence (Phys. Rev. D 74 022002 (2006)). We evaluated the coating thermal noise in KAGRA and discussed future investigation strategies.

gr-qc↗

arXiv2022

A Systematic Error in the Internal Friction Measurement of Coatings for Gravitational Waves Detectors

Low internal friction coatings are key components of advanced technologies such as optical atomic clocks and high-finesse optical cavity and often lie at the forefront of the most advanced experiments in Physics. Notably, increasing the sensitivity of gravitational-wave detectors depends in a very large part on developing new coatings, which entails developing more suitable methods and models to investigate their loss angle. In fact, the most sensitive region of the detection band in such detectors is limited by the coating thermal noise, which is related to the loss angle of the coating. Until now, models which describe only ideal physical properties have been adopted, wondering about the use of one or more loss angles to describe the mechanical properties of coatings. Here we show the presence of a systematic error ascribed to inhomogeneity of the sample at its edges in measuring the coating loss angle. We present a model for disk-shaped resonators, largely used in loss angle measurements, and we compare the theory with measurements showing how this systematic error impacts on the accuracy with which the loss model parameters are known.

astro-ph.IM↗

arXiv2022

Effects of mixing and annealing on the optical and mechanical properties of TiO$_{2}$:Ta$_{2}$O$_{5}$ amorphous coatings

Amorphous mixed titania-tantala coatings are key components of Bragg reflectors in the gravitational wave detectors (GWDs). Attaining the lowest possible values of optical absorption and mechanical losses in the coatings is of paramount importance for GWDs, and this requires a complex optimization of the coating deposition and post-deposition annealing. We present here a systematic investigation of the optical properties and internal friction of amorphous mixed titania-tantala coatings grown by ion beam sputtering. We consider coatings with six different cation mixing ratios and we study them both in the as-deposited and annealed state. By exploiting spectroscopic ellipsometry data and modelling, along with ancillary techniques, we retrieved the dielectric function of the coatings in a wide spectral range. When varying the mixing ratio and performing the annealing we find monotonic trends for most of the aforementioned properties. Remakably, the post-annealing Urbach energy displays a definite minimum for a mixing ratio around 20%, very close to the composition of the coatings showing the lowest optical absorption for GWDs applications. We suggest that the observed minimum in the Urbach energy depends not only on the mixing ratio, but also on the annealing parameters. On the other hand, the minimum coating loss angle was found to be weakly dependent on the considered measurement frequency and to lie within a rather broad range of Ti content, suggesting that the search for an absolute minimum following post-deposition annealing should be rather sought in the study of the best annealing parameters for each specific cation ratio considered. This work constitutes a reference for the optical properties of the amorphous mixed titania-tantala coatings, and highlights the relevance of the Urbach energy in the optimization process of materials for high-performing Bragg reflectors.

physics.app-ph↗

arXiv2020

Point defects in IBS coating for very low loss mirrors

High reflective coatings are used in many physics experiments. Despite the high quality of the opticalcoating, the performances of the mirrors is altered by the scattered light induced by micrometers sizedefects in the coating layers. The topic of this paper is the study of the point-like scatterers present in thespecific coating of the mirrors used in state of the art, high sensitivity optical experiments. We studied thebehavior of the materials according to different thicknesses, and how the defects change after annealing.To our knowledge, this is a first insight into the formation of such defects for different materials andthickness and how this is reduced when samples are annealed.

physics.ins-det↗

arXiv2020

Observation of a Correlation Between Internal friction and Urbach Energy in Amorphous Oxides Thin Films

We have investigated by spectroscopic ellipsometry (SE, 190-1700 nm) the optical properties of uniform, amorphous thin films of Ta2O5 and Nb2O5 as deposited and after annealing, and after so-called "doping" with Ti atoms which leads to mixed oxides. Ta2O5 and Ti:Ta2O5 are currently used as high-index components in Bragg reflectors for Gravitational Wave Detectors. Parallel to the optical investigation, we measured the mechanical energy dissipation of the same coatings, through the so-called "loss angle" phi = Q^-1, which quantifies the energy loss in materials. By applying the well-known Cody-Lorentz model in the analysis of SE data we have been able to derive accurate information on the fundamental absorption edge through important parameters related to the electronic density of states, such as the optical gap (E_g) and the energy width of the exponential Urbach tail (the Urbach energy E_U). We have found that E_U is neatly reduced by suitable annealing as is also perceptible from direct inspection of SE data. Ti-doping also points to a minor decrease of E_U. The reduction of E_U parallels a lowering of the mechanical losses quantified by the loss angle phi. The correlation highlights that both the electronic states responsible of Urbach tail and the internal friction are sensitive to a self-correlation of defects on a medium-range scale, which is promoted by annealing and in our case, to a lesser extent, by doping. These observations may contribute to a better understanding of the relationship between structural and mechanical properties in amorphous oxides.

physics.optics↗

arXiv2020

Progress in the measurement and reduction of thermal noise in optical coatings for gravitational-wave detectors

Coating thermal noise is a fundamental limit for precision experiments based on optical and quantum transducers. In this review, after a brief overview of the techniques for coating thermal noise measurements, we present the latest world-wide research activity on low-noise coatings, with a focus on the results obtained at the Laboratoire des Matériaux Avancés. We report new updated values for the Ta$_2$O$_5$, Ta$_2$O$_5$-TiO$_2$ and SiO$_2$ coatings of the Advanced LIGO, Advanced Virgo and KAGRA detectors, and new results from sputtered Nb$_2$O$_5$, TiO$_2$-Nb$_2$O$_5$, Ta$_2$O$_5$-ZrO$_2$, MgF$_2$, AlF$_3$ and silicon nitride coatings. Amorphous silicon, crystalline coatings, high-temperature deposition, multi-material coatings and composite layers are also briefly discussed, together with the latest developments of structural analyses and models.

physics.ins-det↗

arXiv2019

Amorphous optical coatings of present gravitational-wave interferometers

We report on the results of an extensive campaign of optical and mechanical characterization of the ion-beam sputtered oxide layers (Ta$_2$O$_5$, TiO$_2$, Ta$_2$O$_5$-TiO$_2$, SiO$_2$) within the high-reflection coatings of the Advanced LIGO, Advanced Virgo and KAGRA gravitational-wave detectors: refractive index, thickness, optical absorption, composition, density, internal friction and elastic constants have been measured; the impact of deposition rate and post-deposition annealing on coating internal friction has been assessed. For Ta$_2$O$_5$ and SiO$_2$ layers, coating internal friction increases with the deposition rate, whereas the annealing treatment either erases or largely reduces the gap between samples with different deposition history. For Ta$_2$O$_5$-TiO$_2$ layers, the reduction of internal friction due to TiO$_2$ doping becomes effective only if coupled with annealing. All measured samples showed a weak dependence of internal friction on frequency ($ϕ_c(f) = af^{b}$, with $-0.208 < b < 0.140$ depending on the coating material considered). SiO$_2$ films showed a mode-dependent loss branching, likely due to spurious losses at the coated edge of the samples. The reference loss values of the Advanced LIGO and Advanced Virgo input (ITM) and end (ETM) mirror HR coatings have been updated by using our estimated value of Young's modulus of Ta$_2$O$_5$-TiO$_2$ layers (120 GPa) and are about 10\% higher than previous estimations.

physics.ins-det↗

arXiv2018

LSST: from Science Drivers to Reference Design and Anticipated Data Products

(Abridged) We describe here the most ambitious survey currently planned in the optical, the Large Synoptic Survey Telescope (LSST). A vast array of science will be enabled by a single wide-deep-fast sky survey, and LSST will have unique survey capability in the faint time domain. The LSST design is driven by four main science themes: probing dark energy and dark matter, taking an inventory of the Solar System, exploring the transient optical sky, and mapping the Milky Way. LSST will be a wide-field ground-based system sited at Cerro Pachón in northern Chile. The telescope will have an 8.4 m (6.5 m effective) primary mirror, a 9.6 deg$^2$ field of view, and a 3.2 Gigapixel camera. The standard observing sequence will consist of pairs of 15-second exposures in a given field, with two such visits in each pointing in a given night. With these repeats, the LSST system is capable of imaging about 10,000 square degrees of sky in a single filter in three nights. The typical 5$σ$ point-source depth in a single visit in $r$ will be $\sim 24.5$ (AB). The project is in the construction phase and will begin regular survey operations by 2022. The survey area will be contained within 30,000 deg$^2$ with $δ<+34.5^\circ$, and will be imaged multiple times in six bands, $ugrizy$, covering the wavelength range 320--1050 nm. About 90\% of the observing time will be devoted to a deep-wide-fast survey mode which will uniformly observe a 18,000 deg$^2$ region about 800 times (summed over all six bands) during the anticipated 10 years of operations, and yield a coadded map to $r\sim27.5$. The remaining 10\% of the observing time will be allocated to projects such as a Very Deep and Fast time domain survey. The goal is to make LSST data products, including a relational database of about 32 trillion observations of 40 billion objects, available to the public and scientists around the world.

astro-ph↗

arXiv2017

High-Reflection Coatings for Gravitational-Wave Detectors: State of The Art and Future Developments

We report on the optical, mechanical and structural characterization of the sputtered coating materials of Advanced LIGO, Advanced Virgo and KAGRA gravitational-waves detectors. We present the latest results of our research program aiming at decreasing coating thermal noise through doping, optimization of deposition parameters and post-deposition annealing. Finally, we propose sputtered Si3N4 as a candidate material for the mirrors of future detectors.

physics.ins-det↗

arXiv2017

Correlated evolution of structure and mechanical loss of a sputtered silica film

Energy dissipation in amorphous coatings severely affects high-precision optical and quantum transducers. In order to isolate the source of coating loss, we performed an extensive study of Raman scattering and mechanical loss of a thermally-treated sputtered silica coating. Our results show that loss is correlated with the population of three-membered rings of Si-O$_4$ tetrahedral units, and support the evidence that thermal treatment reduces the density of metastable states separated by a characteristic energy of about 0.5 eV, in favour of an increase of the states separated by smaller activation energies. Finally, we conclude that three-fold rings are involved in the relaxation mechanisms only if they belong to more complex chain-like structures of 10 to 100 tetrahedra.

cond-mat.mtrl-sci↗

arXiv2016

A new method of probing mechanical losses of coatings at cryogenic temperatures

A new method of probing mechanical losses and comparing the corresponding deposition processes of metallic and dielectric coatings in 1-100 MHz frequency range and cryogenic temperatures is presented. The method is based on the use of extremely high-quality quartz acoustic cavities whose internal losses are orders of magnitude lower than any available coatings nowadays. The approach is demonstrated for Chromium, Chromium/Gold and a multilayer tantala/silica coatings. The ${\rm Ta}_2{\rm O}_5/{\rm Si}{\rm O}_2$ coating has been found to exhibit a loss angle lower than $1.6\times10^{-5}$ near 30 {\rm MHz} at 4 {\rm K}. The results are compared to the previous measurements.

physics.ins-det↗

arXiv2016

Mechanical loss in state-of-the-art amorphous optical coatings

We present the results of mechanical characterizations of many different high-quality optical coatings made of ion-beam-sputtered titania-doped tantala and silica, developed originally for interferometric gravitational-wave detectors. Our data show that in multi-layer stacks (like high-reflection Bragg mirrors, for example) the measured coating dissipation is systematically higher than the expectation and is correlated with the stress condition in the sample. This has a particular relevance for the noise budget of current advanced gravitational-wave interferometers, and, more generally, for any experiment involving thermal-noise limited optical cavities.

physics.ins-det↗

arXiv2014

Measurements of mechanical thermal noise and energy dissipation in optical dielectric coatings

In recent years an increasing number of devices and experiments are shown to be limited by mechanical thermal noise. In particular sub-Hertz laser frequency stabilization and gravitational wave detectors, that are able to measure fluctuations of 1E-18 m/rtHz or less, are being limited by thermal noise in the dielectric coatings deposited on mirrors. In this paper we present a new measurement of thermal noise in low absorption dielectric coatings deposited on micro-cantilevers and we compare it with the results obtained from the mechanical loss measurements. The coating thermal noise is measured on the widest range of frequencies with the highest signal to noise ratio ever achieved. In addition we present a novel technique to deduce the coating mechanical losses from the measurement of the mechanical quality factor which does not rely on the knowledge of the coating and substrate Young moduli. The dielectric coatings are deposited by ion beam sputtering. The results presented here give a frequency independent loss angle of (4.70 $\pm$ 0.2)x1E-4 with a Young's modulus of 118 GPa for annealed tantala from 10 Hz to 20 kHz. For as-deposited silica, a weak frequency dependence (~ f^{-0.025}) is observed in this frequency range, with a Young's modulus of 70 GPa and an internal damping of (6.0 $\pm$ 0.3)x1E-4 at 16 kHz, but this value decreases by one order of magnitude after annealing and the frequency dependence disappears.

physics.ins-det↗

arXiv2006

Titania-doped tantala/silica coatings for gravitational-wave detection

Reducing thermal noise from optical coatings is crucial to reaching the required sensitivity in next generation interferometric gravitational-waves detectors. Here we show that adding TiO$_2$ to Ta$_2$O$_5$ in Ta$_2$O$_5$/SiO$_2$ coatings reduces the internal friction and in addition present data confirming it reduces thermal noise. We also show that TiO$_2$-doped Ta$_2$O$_5$/SiO$_2$ coatings are close to satisfying the optical absorption requirements of second generation gravitational-wave detectors.

gr-qc↗

arXiv2003

Mechanical Loss in Tantala/Silica Dielectric Mirror Coatings

Current interferometric gravitational wave detectors use test masses with mirror coatings formed from multiple layers of dielectric materials, most commonly alternating layers of SiO2 (silica) and Ta2O5 (tantala). However, mechanical loss in the Ta2O5/SiO2 coatings may limit the design sensitivity for advanced detectors. We have investigated sources of mechanical loss in the Ta2O5/SiO2 coatings, including loss associated with the coating-substrate interface, with the coating-layer interfaces, and with the bulk material. Our results indicate that the loss is associated with the bulk coating materials and that the loss of Ta2O5 is substantially larger than that of SiO2.

gr-qc↗

arXiv2001

Thermal noise in interferometric gravitational wave detectors due to dielectric optical coatings

We report on thermal noise from the internal friction of dielectric coatings made from alternating layers of Ta2O5 and SiO2 deposited on fused silica substrates. We present calculations of the thermal noise in gravitational wave interferometers due to optical coatings, when the material properties of the coating are different from those of the substrate and the mechanical loss angle in the coating is anisotropic. The loss angle in the coatings for strains parallel to the substrate surface was determined from ringdown experiments. We measured the mechanical quality factor of three fused silica samples with coatings deposited on them. The loss angle of the coating material for strains parallel to the coated surface was found to be (4.2 +- 0.3)*10^(-4) for coatings deposited on commercially polished slides and (1.0 +- 0.3)*10^{-4} for a coating deposited on a superpolished disk. Using these numbers, we estimate the effect of coatings on thermal noise in the initial LIGO and advanced LIGO interferometers. We also find that the corresponding prediction for thermal noise in the 40 m LIGO prototype at Caltech is consistent with the noise data. These results are complemented by results for a different type of coating, presented in a companion paper.

gr-qc↗