arXiv subjects

Gianrico Lamura

Publications and source records attributed to Gianrico Lamura.

6 recordsLinked to original sources

arXiv2026

Anomalous field evolution of the mixed-state linewidth in the second superconducting dome of LaFeAsO$_{1-x}M_x$ ($M={\rm F,H}$)

We report a transverse-field muon-spin rotation/relaxation ($μ$SR) study of the internal-field distribution in the mixed state of LaFeAsO$_{0.89}$F$_{0.11}$ and LaFeAsO$_{0.75}$H$_{0.25}$, representative of the first (SC1) and second (SC2) superconducting domes of the LaFeAsO$_{1-x}M_x$ ($M={\rm F,H}$) family, respectively. Below the superconducting transition temperature $T_{\rm c}$, the linewidth of the internal-field distribution increases in both samples, indicating the formation of a vortex lattice. Above $T_{\rm c}$, the linewidth remains field dependent and increases approximately linearly with field, consistent with broadening of the powder spectrum caused by an anisotropic Knight shift. After subtraction of this normal-state contribution, the superconducting linewidth $σ_{\rm sc}$ exhibits qualitatively different field dependences in the two samples. At 4K, the SC1 ($x_{\rm F}=0.11$) sample shows the expected monotonic decrease with increasing field, whereas the SC2 ($x_{\rm H}=0.25$) sample develops a pronounced local maximum near 3T. A contour representation of $σ_{\rm sc}(T,H)$ further reveals a ridge of local maxima whose field position, $H_{σ,\max}(T)$, shifts to lower fields upon warming and disappears near $T_{\rm c}$. The anomalous field evolution observed in the SC2 sample is consistent with an additional field-induced contribution associated with enhanced Pauli-paramagnetic effects, highlighting the distinct electronic character of the two superconducting domes.

cond-mat.supr-con↗

arXiv2025

Magnetic clusters in the paramagnetic phase of a high-temperature ferromagnetic metal-organic framework

Owing to their exceptional chemical and electronic tunability, metal-organic frameworks can be designed to develop magnetic ground states making a range of applications feasible, from magnetic gas separation to the implementation of lightweight, rare-earth free permanent magnets. However, the typically weak exchange interactions mediated by the diamagnetic organic ligands result in ordering temperatures confined to the cryogenic limit. The itinerant magnetic ground state realized in the chromium-based framework Cr(tri)$_{2}$(CF$_{3}$SO$_{3}$)$_{0.33}$ (Htri, $1H$-$1$,$2$,$3$-triazole) is a remarkable exception to this trend, showing a robust ferromagnetic behavior almost at ambient conditions. Here, we use dc SQUID magnetometry, nuclear magnetic resonance, and ferromagnetic resonance to study the magnetic state realized in this material. We highlight several thermally-activated relaxation mechanisms for the nuclear magnetization due to the tendency of electrons towards localization at low temperatures as well as the rotational dynamics of the charge-balancing triflate ions confined within the pores. Most interestingly, we report the development within the paramagnetic regime of mesoscopic magnetic correlated clusters whose slow dynamics in the MHz range are tracked by the nuclear moments, in agreement with the highly unconventional nature of the magnetic transition detected by dc SQUID magnetometry. We discuss the similarity between the clustered phase in the paramagnetic phase and the magnetoelectronic phase segregation leading to colossal magnetoresistance in manganites and cobaltites. These results demonstrate that high-temperature magnetic metal-organic frameworks can serve as a versatile platform for exploring correlated electron phenomena in low-density, chemically tunable materials.

cond-mat.str-el↗

arXiv2025

Magnetic Trampoline Resonators from (La,Sr)MnO3 Single-Crystal Thin Films

Micro-electro-mechanical resonators employing a magnetic element have been proposed for magnetic field sensing applications, but the integration of magnetic materials with standard semiconductor compounds is challenging and requires complex fabrication protocols. We present a different approach relying on (La0.7,Sr0.3)MnO3 (LSMO), an oxide compound that works both as structural element for the resonator and functional magnetic layer. Suspended trampolines are realized in a single step process from LSMO thin films and show quality factor up to 60k and fQ products reaching 10$^{10}$ Hz. Their magnetic properties are probed by a SQUID magnetometer and magnetic force microscopy, showing saturation magnetization of 240 kA/m at room temperature and in-plane magnetic domains with coercivity of 2.5 mT. Being entirely made from a magnetic material, these resonators exhibit a larger magnetic interaction volume compared to other solutions, making them ideal candidates as building blocks for high-sensitivity magnetic field sensors.

physics.app-ph↗

arXiv2023

Superconductivity induced by gate-driven hydrogen intercalation in the charge-density-wave compound 1T-TiSe2

Hydrogen (H) plays a key role in the near-to-room temperature superconductivity of hydrides at megabar pressures. This suggests that H doping could have similar effects on the electronic and phononic spectra of materials at ambient pressure as well. Here, we demonstrate the non-volatile control of the electronic ground state of titanium diselenide (1T-TiSe$_2$) via ionic liquid gating-driven H intercalation. This protonation induces a superconducting phase, observed together with a charge-density wave through most of the phase diagram, with nearly doping-independent transition temperatures. The H-induced superconducting phase is possibly gapless-like and multi-band in nature, in contrast with those induced in TiSe$_2$ via copper, lithium, and electrostatic doping. This unique behavior is supported by ab initio calculations showing that high concentrations of H dopants induce a full reconstruction of the bandstructure, although with little coupling between electrons and high-frequency H phonons. Our findings provide a promising approach for engineering the ground state of transition metal dichalcogenides and other layered materials via gate-controlled protonation.

cond-mat.supr-con↗

arXiv2021

Inverse magnetic hysteresis of the Josephson supercurrent: study of the magnetic properties of thin niobium/permalloy (Fe_{20}Ni_{80}) interfaces

We propose a picture for the magnetic properties of superconductor/ferromagnet (S/F) heterostructures based on Nb and permalloy (Py: Fe_{20}Ni_{80}). By measuring the magnetic moment as a function of the temperature in S/F/S trilayers for different thicknesses of the middle F layer, we give evidence of the presence of a magnetic stray field of the F layer. For values of F-layer thickness below a threshold, we establish a correlation between the magnetic measurements of the S/F/S trilayers and the anomalous magnetic dependence of the critical current in S/insulator/thin superconducting film/F/S (SIsFS) Josephson junctions (JJs). These complementary investigations provide a self-consistent method to fully characterize S/F heterostructures and possibly demonstrate effects arising from the mutual interactions between ferromagnetism and superconductivity. A shift in the Fraunhofer critical current oscillations has been observed in the opposite direction to the one commonly observed in JJs with F barriers, as it has been recently predicted by inverse and electromagnetic proximity theories. This inverse memory effect is relevant for the design of these heterostructures as memory cells and spintronic devices.

cond-mat.supr-con↗

arXiv2011

Magnetic properties of spin diluted iron pnictides from muSR and NMR in LaFe1-xRuxAsO

The effect of isoelectronic substitutions on the microscopic properties of LaFe1-xRuxAsO, for 0< x< 0.8, has been investigated by means of muSR and 139La NMR. It was found that Ru substitution causes a progressive reduction of the Nèel temperature (T_N) and of the magnetic order parameter without leading to the onset of superconductivity. The temperature dependence of 139La nuclear spin-lattice relaxation rate 1/T_1 can be suitably described within a two-band model. One band giving rise to the spin density wave ground-state, while the other one is characterized by weakly correlated electrons. Fe for Ru substitution yields to a progressive decrease of the density of states at the Fermi level close to the one derived from band structure calculations. The reduction of T_N with doping follows the predictions of the J_1-J_2 model on a square lattice, which appears to be an effective framework to describe the magnetic properties of the spin density wave ground-state.

cond-mat.str-el↗