arXiv subjects

Girish S. Agarwal

Publications and source records attributed to Girish S. Agarwal.

At least 55 records · Page 3Linked to original sources

arXiv2020

Observation of photonic spin-momentum locking due to coupling of achiral metamaterials and quantum dots

Here, we report observations of photonic spin-momentum locking in the form of directional and chiral emission from achiral quantum dots (QDs) evanescently coupled to achiral hyperbolic metamaterials (HMM). Efficient coupling between QDs and the metamaterial leads to emergence of these photonic topological modes which can be detected in the far field. We provide theoretical explanation for the emergence of spin-momentum locking through rigorous modeling based on photon Green's function where pseudo spin of light arises from coupling of QDs to evanescent modes of HMM.

physics.optics↗

arXiv2020

Metasurfaces for Quantum Photonics

Rapid progress in the development of metasurfaces allowed to replace bulky optical assemblies with thin nanostructured films, often called metasurfaces, opening a broad range of novel and superior applications to the generation, manipulation, and detection of light in classical optics. Recently, these developments started making a headway in quantum photonics, where novel opportunities arose for the control of nonclassical nature of light, including photon statistics, quantum state superposition, quantum entanglement, and single-photon detection. In this Perspective, we review recent progress in the field of quantum-photonics applications of metasurfaces, focusing on innovative and promising approaches to create, manipulate, and detect nonclassical light.

physics.optics↗

arXiv2020

Squeezed Light Induced Two-photon Absorption Fluorescence of Fluorescein Biomarkers

Two-photon absorption (TPA) fluorescence of biomarkers has been decisive in advancing the fields of biosensing and deep-tissue in vivo imaging of live specimens. However, due to the extremely small TPA cross section and the quadratic dependence on the input photon flux, extremely high peak-intensity pulsed lasers are imperative, which can result in significant photo- and thermal-damage. Previous works on entangled TPA (ETPA) with spontaneous parametric down-conversion (SPDC) light sources found a linear dependence on the input photon-pair flux, but are limited by low optical powers, along with a very broad spectrum. We report that by using a high-flux squeezed light source for TPA, a fluorescence enhancement of 47 is achieved in fluorescein biomarkers as compared to classical TPA. Moreover, a polynomial behavior of the TPA rate is observed in the DCM laser dye.

physics.optics↗

arXiv2020

Nonlinear Spin Currents

The cavity mediated spin current between two ferrite samples has been reported by Bai et. al. [Phys. Rev. Lett. 118, 217201 (2017)]. This experiment was done in the linear regime of the interaction in the presence of external drive. In the current paper we develop a theory for the spin current in the nonlinear domain where the external drive is strong so that one needs to include the Kerr nonlinearity of the ferrite materials. In this manner the nonlinear polaritons are created and one can reach both bistable and multistable behavior of the spin current. The system is driven into a far from equilibrium steady state which is determined by the details of driving field and various interactions. We present a variety of steady state results for the spin current. A spectroscopic detection of the nonlinear spin current is developed, revealing the key properties of the nonlinear polaritons. The transmission of a weak probe is used to obtain quantitative information on the multistable behavior of the spin current. The results and methods that we present are quite generic and can be used in many other contexts where cavities are used to transfer information from one system to another, e.g., two different molecular systems.

quant-ph↗

arXiv2020

Temporal Quantum Noise Reduction Acquired by an Electron-Multiplying Charge-Coupled-Device Camera

Electron-multiplying charge-coupled-device cameras (EMCCDs) have been used to observe quantum noise reductions in beams of light in the transverse spatial degree of freedom. For the quantum noise reduction in the temporal domain, "bucket detectors," usually composed of photodiodes with operational amplifiers, are used to register the intensity fluctuations in beams of light within the bandwidth of the detectors. Spatial information, however, is inevitably washed off by the detector. In this paper, we report on measurements of the temporal quantum noise reduction in bright twin beams using an EMCCD camera. The four-wave mixing process in an atomic rubidium vapor cell is used to generate the bright twin beams of light. We observe more than 25% of temporal quantum noise reduction with respect to the shot-noise limit in images captured by the EMCCD camera. Compared with bucket detectors, EMCCD makes it possible to take advantage of the spatial and temporal quantum properties of light simultaneously, which would greatly benefit many applications using quantum protocols.

physics.optics↗

arXiv2020

Simultaneous excitation of two noninteracting atoms with time-frequency correlated photon pairs in a superconducting circuit

Here we report the first observation of simultaneous excitation of two noninteracting atoms by a pair of time-frequency correlated photons in a superconducting circuit. The strong coupling regime of this process enables the synthesis of a three-body interaction Hamiltonian, which allows the generation of the tripartite Greenberger-Horne-Zeilinger state in a single step with a fidelity as high as 0.95. We further demonstrate the quantum Zeno effect of inhibiting the simultaneous two-atom excitation by continuously measuring whether the first photon is emitted. This work provides a new route in synthesizing many-body interaction Hamiltonian and coherent control of entanglement.

physics.optics↗

arXiv2020

Partial Coherence in modern optics: Emil Wolf's legacy in the 21st century

We highlight the impact of Emil Wolf's work on coherence and polarization on an ever increasing amount of applications in the 21 st century. We present a brief review of how partial coherence at the level of increasing order of coherence functions is leading to evolution in the better methods for microscopy, imaging, optical coherence tomography; speckle imaging; propagation through random media. This evolution in our capabilities is expected to have wide ramifications in Science and Engineering.

physics.optics↗

arXiv2020

Transparency in a periodic chain of quantum emitters strongly coupled to a waveguide

We demonstrate the emergence of transparent behavior in a chain of periodically spaced non-identical quantums emitters coupled to a waveguide, in the special case when the inter-atomic separation is a half-integral multiple of the resonant wavelength, i.e. $kL$ is an integral multiple of $π$, with $k$ being the spatial frequency and $L$ the spatial periodicity. When equal but opposite frequency detunings are assigned in pairs to a system of even number of atoms, perfect transmission ensues. When the chain size is odd, a similar assignment leads to the disappearance of collective effects as the odd atom determines the spectral behavior. We also manifest the robustness of these features against dissipative effects and show, how the spectral behavior hinges significantly on the relative detunings between the atoms as compared to the decay rate. A key distinction from the phenomenon of Electromagnetically Induced Transparency (EIT) is that in the waveguide case, the presence of an intrinsic waveguide mediated phase coupling between the atoms strongly affects the transport properties. Furthermore, while reciprocity in single-photon transport does not generally hold due to the phase coupling, we observe an interesting exception for $kL = nπ$ at which the waveguide demonstrates reciprocal behavior with regard to both the transmission and reflection coefficients.

physics.optics↗

arXiv2019

Quantum drives produce strong entanglement between YIG samples without using intrinsic nonlinearities

We show how to generate an entangled pair of yttrium iron garnet (YIG) samples in a cavity-magnon system without using any nonlinearities which are typically very weak. This is against the conventional wisdom which necessarily requires strong Kerr like nonlinearity. Our key idea, which leads to entanglement, is to drive the cavity by a weak squeezed vacuum field generated by a flux-driven Josephson parametric amplifier (JPA). The two YIG samples interact via the cavity. For modest values of the squeezing of the pump, we obtain significant entanglement. This is the principal feature of our scheme. We discuss entanglement between macroscopic spheres using several different quantitative criteria. We show the optimal parameter regimes for obtaining entanglement which is robust against temperature. We also discuss squeezing of the collective magnon variables.

quant-ph↗

arXiv2019

Squeezed light induced symmetry breaking superradiant phase transition

We theoretically investigate the quantum phase transition in the collective systems of qubits in a high-quality cavity, which is driven by a squeezed light. We show that the squeezed light induced symmetry breaking can result in quantum phase transition without the ultrastrong coupling requirement. Using the standard mean field theory, we derive the condition of the quantum phase transition. Surprisingly, we show that there exists a tricritical point where the first- and second-order phase transitions meet. With specific atom-cavity coupling strengths, both the first- and second-order phase transition can be controlled by the squeezed light, leading to an optical switching from the normal phase to the superradiant phase by just increasing the squeezed light intensity. The signature of these phase transitions can be observed by detecting the phase space Wigner function distribution with different profiles controlled by the squeezed light intensity. Such superradiant phase transition can be implemented in various quantum systems, including atoms, quantum dots and ions in optical cavities as well as the circuit quantum electrodynamics system.

quant-ph↗

arXiv2019

Quantum entanglement between two magnon modes via Kerr nonlinearity

We propose a scheme to entangle two magnon modes via Kerr nonlinear effect when driving the systems far-from-equilibrium. We consider two macroscopic yttrium iron garnets (YIGs) interacting with a single-mode microcavity through the magnetic dipole coupling. The Kittel mode describing the collective excitations of large number of spins are excited through driving cavity with a strong microwave field. We demonstrate how the Kerr nonlineraity creates the entangled quantum states between the two macroscopic ferromagnetic samples, when the microcavity is strongly driven by a blue-detuned microwave field. Such quantum entanglement survives at the steady state. Our work offers new insights and guidance to designate the experiments for observing the entanglement in massive ferromagnetic materials. It can also find broad applications in macroscopic quantum effects and magnetic spintronics.

quant-ph↗

arXiv2019

Multiple Fano interferences due to waveguide-mediated phase-coupling between atoms

We examine quantum interference effects due to absorption and emission from multiple atoms coupled to a waveguide and highlight the modifications they entail in regards to single-photon transport properties. A prominent upshot of these interference phenomena is the resonant suppression of the reflection amplitude, which leads to the observation of multiple Fano minima in the reflection spectrum. Such minima determine the points at which transparency is induced in the system. By taking recourse to the real-space Hamiltonian framework, we calculate analytically the reflectivity and transmissivity for a one-dimensional waveguide that evanescently couples to a chain of equally spaced quantum emitters. The inter-emitter spacing relative to the wavelength of the propagating photon, leading to a waveguide-mediated "phase-coupling" between the atoms, is found to fundamentally affect the existence of Fano minima. For a chain of $N$ atoms, the number of minima can be at most $N-1$. However, suitable choices of the phase can suppress the discernibility of the full range of roots in the reflection spectrum. A principal observation for the case of multiple emitters is the emergence of super-Gaussian characteristics close to zero-detuning and consequently, a plateau-shaped broadband spectrum in the region of high reflectivity. For a large chain size, the plateau gets transformed into a flat-topped quasi-rectangular profile in the frequency domain.

physics.optics↗

arXiv2019

Enhanced molecular chiral signals via molecular coherence

One of the most widely used chiroptical spectroscopic methods for studying chiral molecules is Raman optical activity; however, the chiral Raman optical activity signal is extremely weak. Here, we theoretically examine enhanced chiral signals in a system with strongly prepared molecular coherence. We show that the enhanced chiral signal due to strong molecular coherence is up to four orders of magnitude higher than that of the spontaneous Raman optical activity. We discuss several advantages of studying the heterodyned signal obtained by combining the anti-Stokes signal with a local oscillator. The heterodyning allows direct measurement of the ratio of the chiral and achiral parameters. Taking advantage of the molecular coherence and heterodyne detection, the coherent anti-Stokes Raman scattering technique opens up a new potential application for investigation of biomolecular chirality.

quant-ph↗

arXiv2019

Coherent Anti-Stokes Raman scattering in optically active medium

Early theoretical works on coherent anti-Stokes Raman scattering in optically active medium consider only heterodyne signal and subsequently, fourth- and fifth-rank tensor averages have been used. In this work, we presented a full signal expression of coherent anti-Stokes Raman scattering in optically active medium with the help of eighth- and ninth-rank tensor averaging for simplest experimental configuration namely, measurements of post-selected circularly polarized components of scattered anti-Stokes field in the presence of three incident laser beams all linearly polarized along the same axis.

quant-ph↗

arXiv2019

On three-dimensional rotational averages of odd-rank tensors

The recent growing interest in nonlinear optical spectroscopy in optically active medium demands the three-dimensional rotational average of high-rank tensors. In the present paper, we present a new method for finding the rotational average of odd-rank tensors in an overcomplete basis of isotropic tensors. The method is successfully applied to the rotational averages of tensors of rank 5,7,9,11.

math-ph↗

arXiv2019

Controllable spin-Hall and related effects of light in an atomic medium via coupling fields

We show the existence of spin-Hall effect of light (SHEL) in an atomic medium which is made anisotropic via electromagnetically induced transparency. The medium is made birefringent by applying an additional linearly polarized coupling light beam. The refractive index and the orientation of the optics axis are controlled by the coupling beam. We show that after transmitting the atomic medium, a linearly polarized probe light beam splits into its two spin components by opposite transverse shifts. With proper choice of parameters and atomic density of about $2.5\times10^{17}\,\mathrm{m}^{-3}$, the shifts are about the order of wavelength and can be larger than the wavelength by increasing the atomic density. We propose a novel measurement scheme based on a balanced homodyne detection (BHD). By properly choosing the polarization, phase, and transverse mode of the local oscillator of the BHD, one can independently measure (i) the SHEL shifts of the two spin components; (ii) the spatial and angular shifts; (iii) the transverse and longitudinal shifts. The measurement can reach the quantum limit of precision by detecting signals at the modulation frequency of the electro-optic modulator used to modulate the input probe beam. The precision is estimated to be at the nanometer level limited by the quantum noise.

physics.optics↗

arXiv2018

Quantum fluctuations in Fröhlich condensate of molecular vibrations driven far from equilibrium

Fröhlich discovered the remarkable condensation of polar vibrations into the lowest frequency mode when the system is pumped externally. For a full understanding of the Fröhlich condensate one needs to go beyond the mean field level to describe critical behavior as well as quantum fluctuations. The energy redistribution among vibrational modes with nonlinearity included is shown to be essential for realizing the condensate and the phonon-number distribution, revealing the transition from quasi-thermal to super-Poissonian statistics with the pump. We further study the spectroscopic properties of the Fröhlich condensate, which are especially revealed by the narrow linewidth. This gives the long-lived coherence and the collective motion of the condensate. Finally we show that the proteins such as Bovine Serum Albumin (BSA) and lysozyme are most likely the candidates for observing such collective modes in THz regime by means of Raman or infrared (IR) spectroscopy.

quant-ph↗

arXiv2018

Analysis of superresolution via 3D structured illumination intensity correlation microscopy

Intensity correlation microscopy (ICM), which is prominently known through antibunching microscopy or super-resolution optical fluctuation imaging (SOFI), provides superresolution through a correlation analysis of antibunching of independent quantum emitters or temporal fluctuations of blinking fluorophores. For correlation order $m$ the PSF in the signal is effectively taken to the $m$th power, and is thus directly shrunk by the factor $\sqrt{m}$. Combined with deconvolution a close to linear resolution improvement of factor $m$ can be obtained. Yet, analysis of high correlation orders is challenging, what limits the achievable resolutions. Here we propose to use three dimensional structured illumination along with $m$th-order correlation analysis to obtain an enhanced scaling of up to $m+m=2m$. Including the stokes shift or plasmonic sub-wavelength illumination enhancements beyond $2m$ can be achieved. Hence, resolutions far below the diffraction limit in full 3D imaging can potentially be achieved already with low correlation orders. Since ICM operates in the linear regime our approach may be particularly promising for enhancing the resolution in biological imaging at low illumination levels.

physics.optics↗