arXiv subjects

Giuseppe Pirruccio

Publications and source records attributed to Giuseppe Pirruccio.

14 recordsLinked to original sources

arXiv2026

Intercavity phonons and dynamics in coupled polariton cavities

Intercavity polaritons, hybrid quasiparticles with spatially separated photonic and excitonic components, provide a platform to engineer structured light-matter states. We show that resonant driving of the middle polariton branch leads to a qualitatively distinct dynamical regime in which coherent Rabi oscillations are suppressed, and the system evolves monotonically toward its steady state. Including interactions, we demonstrate that this regime supports Bogoliubov excitations with a phonon-like dispersion at low momenta. These collective modes inherit interactions from the excitonic fraction, while preserving the intrinsically intercavity nature of the quasiparticles.

cond-mat.quant-gas↗

arXiv2025

Moiré excitons and exciton-polaritons: A review

Distinguished by their long lifetimes, strong dipolar interactions, and periodic confinement, moiré excitons provide a fertile territory for realizing interaction-driven excitonic phases beyond conventional semiconductor systems. Formed in twisted or lattice-mismatched van der Waals heterostructures, these excitons are shaped by a periodic potential landscape that enables the engineering of flat bands, strong interactions, and long-lived localised states. This has opened pathways to explore strongly correlated phases, including excitonic insulators, superfluids, and supersolids, potentially stable even at room temperature. When embedded in optical cavities, moiré excitons hybridize with photons to form moiré exciton-polaritons, a new class of quasiparticles exhibiting enhanced optical nonlinearities and novel topological features. In this review, we survey the theoretical foundations and experimental progress in the field of moiré excitons and polaritons. We begin by introducing the formation mechanisms of moiré patterns in two-dimensional semiconductors, and describe their impact on exciton confinement, optical selection rules, and spin-valley physics. We then discuss recent advances in the realization of many-body excitonic phases and exciton-based probes of electronic correlations. Finally, we explore the novel aspects of moiré polaritons, highlighting their unique nonlinear and topological properties. By bridging quantum optics, nanophotonics, and correlated electron systems, moiré excitons offer a powerful solid-state platform for quantum simulation, optoelectronic applications, and many-body photonics.

cond-mat.mes-hall↗

arXiv2025

Macroscopic coherence and vorticity in room-temperature polariton condensate confined in a self-assembled perovskite microcavity

Exciton-polariton Bose-Einstein condensation at room temperature offers a promising pathway toward quantum photonic technologies that can operate under ambient conditions. A key challenge in this field is to engineer a controlled platform where strong confinement, nonlinear interactions, and structural disorder coexist, unlocking access to rich collective behavior and unconventional condensate dynamics. We demonstrate polariton condensation in CsPbBr$_3$ microplatelets that self-assemble into whispering gallery mode microresonators featuring tight lateral photon confinement finely balanced with intrinsic disorder. The system exhibits hallmark signatures of out-of-equilibrium condensation, including a non-linear increase in emission intensity, spectral narrowing, and interaction-induced blueshift. Intrinsic disorder subtly reshapes the cavity energy landscape, inducing condensate fragmentation and enabling direct optical access to the condensate wavefunction. Interferometric measurements reveal extended phase coherence, whereas characteristic fork-shaped fringe dislocations confirm the presence of quantized vortices pinned by the disordered potential. These topological excitations underscore the rich physics driven by the interplay of gain, loss, confinement, and disorder. Our work establishes a scalable platform for investigating driven-dissipative quantum fluids of light at room temperature, where the intrinsic disorder balances optical confinement and provides a window into condensate wavefunction, coherence, and vortex phenomena. This study system opens new opportunities for exploring many-body physics and potentially advancing topological photonics in integrable microcavity architectures.

cond-mat.mes-hall↗

arXiv2025

Scalable Dip-Coated Bragg Mirrors for Strong Light-Matter Coupling with 2D Perovskites

We report a scalable and cost-effective method for fabricating high-performance Bragg mirrors using a bottom-up approach that combines evaporation-induced self-assembly (EISA) and dip-coating. The photonic crystals are composed of alternating mesoporous SiO$_2$ and dense TiO$_2$ layers, providing a high refractive index contrast ($\sim$0.8). This enables strong reflectance (up to 96%) with as few as five bilayers and precise control of the photonic stop band across the visible spectrum by simply adjusting the deposition parameters. Integration of a thin film of the two-dimensional perovskite (PEA)$_2$PbI$_4$ leads to strong light--matter coupling at room temperature. Angle-resolved reflectance and photoluminescence measurements reveal the formation of upper and lower polariton branches, with a Rabi splitting of 90 meV. The observed polaritonic dispersion is well described by a two-level system and Green's function formalism. This work demonstrates an efficient strategy for constructing tunable optical cavities using simple solution-based methods. The combination of high optical quality, spectral tunability, and strong coupling performance positions this platform as a promising candidate for low-threshold polariton lasers, nonlinear optics, and integrated optoelectronic devices.

cond-mat.mes-hall↗

arXiv2025

Protecting Intercavity Polaritons in Strongly Coupled Cavities

We theoretically designed and experimentally demonstrated a mechanism to protect a spatially segregated mixed light-matter state, known as intercavity exciton-polariton in strongly coupled optical cavities. This excitation, shared across the coupled cavity array, exhibits remarkable robustness over a wide momentum range, without compromising photon-exciton mixing or the spatial separation of its photonic and excitonic components, which also enables a tunable heavy mass. Additionally, we unveil a direct connection between the transparency window, characteristic of slow-light experiments, and the protection of the intercavity polariton nature. Both phenomena originate from the strategic design of an energy-level landscape featuring a $Λ$-scheme, opening new avenues for exploring and utilizing these unique optical excitations in advanced photonic applications.

cond-mat.mes-hall↗

arXiv2024

Intercavity polariton slows down dynamics in strongly coupled cavities

Band engineering stands as an efficient route to induce strongly correlated quantum many-body phenomena. Besides inspiring analogies among diverse physical fields, tuning on demand the group velocity is highly attractive in photonics because it allows unconventional flows of light. $Λ$-schemes offer a route to control the propagation of light in a lattice-free configurations, enabling exotic phases such as slow-light and allowing for highly optical non-linear systems. Here, we realize room-temperature intercavity Frenkel polaritons excited across two strongly coupled cavities. We demonstrate the formation of a tuneable heavy-polariton, akin to slow light, appearing in the absence of a periodic in-plane potential. Our photonic architecture based on a simple three-level scheme enables the unique spatial segregation of photons and excitons in different cavities and maintains a balanced degree of mixing between them. This unveils a dynamical competition between many-body scattering processes and the underlying polariton nature which leads to an increased fluorescence lifetime. The intercavity polariton features are further revealed under appropriate resonant pumping, where we observe suppression of the polariton fluorescence intensity.

cond-mat.mes-hall↗

arXiv2022

Topological Frenkel Exciton-Polaritons in One-Dimensional Lattices of Strongly Coupled Cavities

Frenkel polaritons, hybrid light-matter quasiparticles, offer promises for the designing of new opto-electronic devices. However, their technological implementations are hindered by sensitivity to imperfections. Topology has raised as a way to circumvent defects and fabrication limitations. Here, we propose a lattice of cavities to realize the one-dimensional Su-Schrieffer-Heeger model (SSH) for topological Frenkel polaritons. By engineering the configuration of the cavities we demonstrate that the SSH topological and trivial phases can be accessed, which we unravel by complementary classical and quantum theories. We demonstrate the polariton edge state robustness under defects and the broadening of the photon and exciton lines. Our findings propose a realistic yet simple experimental setup to realize topological room temperature polaritons.

cond-mat.mes-hall↗

arXiv2022

The Fate of the Upper Polariton: Breakdown of the Quasiparticle Picture in the Continuum

Organic polaritons resulting from the strong hybridisation between photons and matter excitations have arisen as a suitable platform to device light-matter technological interfaces at room temperature. Despite their inherent complexity, organic polaritons are commonly regarded as coherent light-matter excitations that can be described in terms of Landau's quasiparticle approach. Here, we experimentally unveil the role of incoherent matter excitations on the polaritons by exploring the relevant energy-momentum parameter space. We demonstrate the emergence of a well-defined lower polariton branch and an intriguing fading of the upper polariton at its entrance to a continuum of matter excitations. This marks the breakdown of the simplistic quasiparticle picture for this branch and the formation of a more complex quantum state. Our experimental results are sustained by a general theoretical framework that allows understanding the light-matter hybridisation beyond the quasiparticle approach. Our work expands the understanding of organic polaritons in all their complexity and increases their technological significance.

cond-mat.mes-hall↗

arXiv2021

Fabricacion de un magnetron sputtering para deposito de peliculas nanometricas magneticas

This paper presents the development of scientific instrumentation for the fabrication of ferromagnetic thin films, by sputtering technique, for the use of 2-inch-diameter targets. Thin films were deposited using Permalloy alloy (Ni80Fe20) as ferromagnetic material at room temperature on Si (001) substrates. The film thicknesses were measured with profilometry and a deposition rate for this alloy of 16.2 nm/min was calculated. Scanning electron microscopy showed a continuous film formation and a chemical composition similar to the target

physics.ins-det↗

arXiv2018

Spectral thermal gaps due to plasmon-phonon mode interaction in bilayer systems

We present a theoretical study of the modification of the near-field radiative heat transfer due to phonon-plasmon coupling in bilayer systems made of a doped semiconductor and a polar dielectric. By tuning the surface-plasmon mode of the former material in resonance with the phonon modes of the latter one, the near-field spectral radiative heat transfer can be suppressed in a frequency band gap. We distinguish between the interlayer mode coupling within each bilayer and the intragap one between the two bilayers. We elucidate the role of each of them in the formation of the band gap and we determine the distance range at which one mechanism dominates over the other. Furthermore, we show that the surface plasmon polariton of the top-most layer allows optimizing the total heat transfer as a function of the separation of the two bilayers.

cond-mat.mes-hall↗

arXiv2017

Fano interference for tailoring near-field radiative heat transfer

We show the existence of Fano resonances in the context of near-field radiative heat transfer, which enable the strong suppression and enhancement of the spectral heat flux at specific wavelengths. This is demonstrated by making use of the plasmon-phonon coupling in a symmetric nano cavity composed by a polaritonic material coated with a metallic layer, in which each side of the cavity is kept at different temperatures. The strong hybridization of the plasmonic and phononic modes sustained by the multilayer structure is determined by the matching of their polarization. This leads to the opening of a thermal band gap, where heat transfer in the coupled system is inhibited for all wave vectors and for wavelengths at which the individual constituents are thermally transmissive.

cond-mat.mes-hall↗

arXiv2016

Coherent control of the optical absorption in a plasmonic lattice coupled to a luminescent layer

We experimentally demonstrate the coherent control, i.e., phase-dependent enhancement and suppression, of the optical absorption in an array of metallic nanoantennas covered by a thin lu- minescent layer. The coherent control is achieved by using two collinear, counter-propagating and phase-controlled incident waves with wavelength matching the absorption spectrum of dye molecules coupled to the array. Symmetry arguments shed light on the relation between the relative phase of the incident waves and the excitation efficiency of the optical resonances of the system. This coherent control is associated with a phase-dependent distribution of the electromagnetic near-fields in the structure which enables a significant reduction of the unwanted dissipation in the metallic structures.

physics.optics↗

arXiv2013

Coherent absorption and enhanced photoluminescence in thin layers of nanorods

We demonstrate a large light absorptance (80%) in a nanometric layer of quantum dots in rods (QRs) with a thickness of 23 nm. This behavior is explained in terms of the coherent absorption by interference of the light incident at a certain angle onto the very thin QR layer. We exploit this coherent light absorption to enhance the photoluminescent emission from the QRs. Up to a seven- and fivefold enhancement of the photoluminescence is observed for p- and s-polarized incident light, respectively.

physics.optics↗

arXiv2012

Excitation of confined modes on particle arrays

We describe both theoretically and experimentally the existence and excitation of confined modes in planar arrays of gold nanodisks. Ordered 2D lattices of monodispersive nanoparticles are manufactured, embedded in a silica matrix, and exposed to evanescent prism-coupling illumination, leading to dark features in the reflectivity, which signal the presence of confined modes guided along the arrays. We find remarkable agreement between theory and experiment in the frequency-momentum dispersion of the resonances. Direct excitation of these modes reveals long propagation distances and deep extinction features. This characterization of guided modes shows the great potential of metallic particle arrays for optical signal processing and distant sensing applications.

cond-mat.mes-hall↗