arXiv subjects

Gonzalo Usaj

Publications and source records attributed to Gonzalo Usaj.

At least 37 records · Page 2Linked to original sources

arXiv2018

Floquet Spectrum and Two-Terminal Conductance of a Transition Metal Dichalcogenide Ribbon under a Circularly Polarized Laser Field

We study the transport properties of a monolayer transition metal dichalcogenide (TMDC) ribbon subject to a time periodic circularly polarized laser field. First, we calculate the quasienergy spectrum within the framework of the Floquet theory and analyze the nontrivial topology of the Floquet bulk gaps. The later is revealed by the presence of chiral edge states inside the bulk gaps in finite samples, in agreement with the calculation of the appropriate winding numbers as a function of both the energy and the amplitude of the laser field. The effect of the time dependent perturbation on the equilibrium edge states is also analyzed. Finally, we calculate the two-terminal conductance and discuss how the above mentioned effects manifest on it. In particular, besides the expected suppression of the bulk conductance and the emergence of edge transport at the Floquet gaps, we find that there is an asymmetry between left and right transmission coefficients (in the zigzag case), leading to pumping effects. In addition, we found that the laser field can lead to a complete switch off of the linear conductance when the later is dominated by the equilibrium edge states.

cond-mat.mes-hall↗

arXiv2018

Population inversion and dynamical phase transitions in a driven superconductor

We consider a superconductor in which the density of states at the Fermi level or the pairing interaction is driven periodically with a frequency larger than the superconducting gap in the collisionless regime. We show by numerical and analytical computations that a subset of quasiparticle excitations enter into resonance and perform synchronous Rabi oscillations leading to cyclic population inversion with a frequency that depends on the amplitude of the drive. As a consequence a new "Rabi-Higgs" mode emerges. Turning off the drive at different times and modulating the strength allows access to all known dynamical phases of the order parameter: persistent oscillations, oscillations with damping and overdamped dynamics. We discuss physical realizations of the drive and methods to detect the dynamics.

cond-mat.supr-con↗

arXiv2018

Time-resolved Hall conductivity of pulse-driven topological quantum systems

We address the question of how the time-resolved bulk Hall response of a two dimensional honeycomb lattice develops when driving the system with a pulsed perturbation. A simple toy model that switches a valley Hall signal by breaking inversion symmetry is studied in detail for slow quasi-adiabatic ramps and sudden quenches, obtaining an oscillating dynamical response that depends strongly on doping and time-averaged values that are determined both by the out of equilibrium occupations and the Berry curvature of the final states. On the other hand, the effect of irradiating the sample with a circularly-polarized infrared pump pulse that breaks time reversal symmetry and thus ramps the system into a non-trivial topological regime is probed. Even though there is a non quantized average signal due to the break down of the Floquet adiabatical picture, some features of the photon-dressed topological bands are revealed to be present even in a few femtosecond timescale. Small frequency oscillations during the transient response evidence the emergence of dynamical Floquet gaps which are consistent with the instantaneous amplitude of the pump envelope. On the other hand, a characteristic heterodyining effect is manifested in the model. The presence of a remnant Hall response for ultra-short pulses that contain only a few cycles of the radiation field is briefly discussed.

cond-mat.mes-hall↗

arXiv2018

Berry curvature tomography and realization of topological Haldane model in driven three-terminal Josephson junctions

We propose a protocol to locally detect the Berry curvature of a three terminal Josephson junction with a quantum dot based on a synchronic detection when an AC modulation is applied in the device. This local gauge invariant quantity is expressed in terms of the instantaneous Green function of the Bogoliubov-de Gennes Hamiltonian. We analyze the contribution to the Berry curvature from both the quasi-particle excitations and the Andreev bound state levels by introducing an effective low-energy model. In addition, we propose to induce topological properties in the junction by breaking time-reversal symmetry with a microwave field in the non-resonant regime. In the last case, the Floquet-Andreev levels are the ones that determine the topological structure of the junction, which is formally equivalent to a 2D-honeycomb Haldane lattice. A relation between the Floquet Berry curvature and the transconductance of the driven system is derived.

cond-mat.mes-hall↗

arXiv2016

Photo-electrons unveil topological transitions in graphene-like systems

The topological structure of the wavefunctions of particles in periodic potentials is characterized by the Berry curvature $Ω_{kn}$ whose integral on the Brillouin zone is a topological invariant known as the Chern number. The bulk-boundary correspondence states that these numbers define the number of edge or surface topologically protected states. It is then of primary interest to find experimental techniques able to measure the Berry curvature. However, up to now, there are no spectroscopic experiments that proved to be capable to obtain information on $Ω_{kn}$ to distinguish different topological structures of the $\it{bulk}$ wavefunctions of semiconducting materials. Based on experimental results of the dipolar matrix elements for graphene, here we show that ARPES experiments with the appropriate x-ray energies and polarization can unambiguously detect changes of the Chern numbers in dynamically driven graphene and graphene-like materials opening new routes towards the experimental study of topological properties of condensed matter systems.

cond-mat.mes-hall↗

arXiv2016

Floquet bound states around defects and adatoms in graphene

Recent studies have focused on laser-induced gaps in graphene which have been shown to have a topological origin, thereby hosting robust states at the sample edges. While the focus has remained mainly on these topological chiral edge states, the Floquet bound states around defects lack a detailed study. In this paper we present such a study covering large defects of different shape and also vacancy-like defects and adatoms at the dynamical gap at $\hbarΩ/2$ ($\hbarΩ$ being the photon energy). Our results, based on analytical calculations as well as numerics for full tight-binding models, show that the bound states are chiral and appear in a number which grows with the defect size. Furthermore, while the bound states exist regardless the type of the defect's edge termination (zigzag, armchair, mixed), the spectrum is strongly dependent on it. In the case of top adatoms, the bound states quasi-energies depend on the adatoms energy. The appearance of such bound states might open the door to the presence of topological effects on the bulk transport properties of dirty graphene.

cond-mat.mes-hall↗

arXiv2016

Bilayer graphene under pressure: Electron-hole Symmetry Breaking, Valley Hall Effect, and Landau Levels

The electronic structure of bilayer graphene under pressure develops very interesting features with an enhancement of the trigonal warping and a splitting of the parabolic touching bands at the K point of the reciprocal space into four Dirac cones, one at K and three along the T symmetry lines. As pressure is increased, these cones separate in reciprocal space and in energy, breaking the electron-hole symmetry. Due to their energy separation, their opposite Berry curvature can be observed in valley Hall effect experiments and in the structure of the Landau levels. Based on the electronic structure obtained by Density Functional Theory, we develop a low energy Hamiltonian that describes the effects of pressure on measurable quantities such as the Hall conductivity and the Landau levels of the system.

cond-mat.mtrl-sci↗

arXiv2015

Floquet interface states in illuminated three-dimensional topological insulators

Recent experiments showed that the surface of a three dimensional topological insulator develops gaps in the Floquet-Bloch band spectrum when illuminated with a circularly polarized laser. These Floquet-Bloch bands are characterized by non-trivial Chern numbers which only depend on the helicity of the polarization of the radiation field. Here we propose a setup consisting of a pair of counter-rotating lasers, and show that one-dimensional chiral states emerge at the interface between the two lasers. These interface states turn out to be spin-polarized and may trigger interesting applications in the field of optoelectronics and spintronics.

cond-mat.mes-hall↗

arXiv2015

Hierarchy of Floquet gaps and edge states for driven honeycomb lattices

Electromagnetic driving in a honeycomb lattice can induce gaps and topological edge states with a structure of increasing complexity as the frequency of the driving lowers. While the high frequency case is the most simple to analyze we focus on the multiple photon processes allowed in the low frequency regime to unveil the hierarchy of Floquet edge-states. In the case of low intensities an analytical approach allows us to derive effective Hamiltonians and address the topological character of each gap in a constructive manner. At high intensities we obtain the net number of edge states, given by the winding number, with a numerical calculation of the Chern numbers of each Floquet band. Using these methods, we find a hierarchy that resembles that of a Russian nesting doll. This hierarchy classifies the gaps and the associated edge states in different orders according to the electron-photon coupling strength. For large driving intensities, we rely on the numerical calculation of the winding number, illustrated in a map of topological phase transitions. The hierarchy unveiled with the low energy effective Hamiltonians, alongside with the map of topological phase transitions discloses the complexity of the Floquet band structure in the low frequency regime. The proposed method for obtaining the effective Hamiltonian can be easily adapted to other Dirac Hamiltonians of two dimensional materials and even the surface of a 3D topological insulator.

cond-mat.mes-hall↗

arXiv2015

Impurities and electronic localization in graphene bilayers

We analyze the electronic properties of bilayer graphene with Bernal stacking and a low concentration of adatoms. Assuming that the host bilayer lies on top of a substrate, we consider the case where impurities are adsorbed only on the upper layer. We describe non-magnetic impurities as a single orbital hybridized with carbon's pz states. The effect of impurity doping on the local density of states with and without a gated electric field perpendicular to the layers is analyzed. We look for Anderson localization in the different regimes and estimate the localization length. In the biased system, the field induced gap is partially filled by strongly localized impurity states. Interestingly, the structure, distribution and localization length of these states depend on the field polarization.

cond-mat.mes-hall↗

arXiv2015

Gate induced enhancement of spin-orbit coupling in dilute fluorinated graphene

We analyze the origin of spin-orbit coupling (SOC) in fluorinated graphene using Density Functional Theory (DFT) and a tight-binding model for the relevant orbitals. As it turns out, the dominant source of SOC is the atomic spin-orbit of fluorine adatoms and not the impurity induced SOC based on the distortion of the graphene plane as in hydrogenated graphene. More interestingly, our DFT calculations show that SOC is strongly affected by both the type and concentrations of the graphene's carriers, being enhanced by electron doping and reduced by hole doping. This effect is due to the charge transfer to the fluorine adatom and the consequent change in the fluorine-carbon bonding. Our simple tight-binding model, that includes the SOC of the $2p$ orbitals of F and effective parameters based on maximally localized Wannier functions, is able to account for the effect. The strong enhancement of the SOC induced by graphene doping opens the possibility to tune the spin relaxation in this material.

cond-mat.mes-hall↗

arXiv2014

Irradiated graphene as a tunable Floquet topological insulator

In the presence of a circularly polarized mid-infrared radiation graphene develops dynamical band gaps in its quasi-energy band structure and becomes a Floquet insulator. Here we analyze how topologically protected edge states arise inside these gaps in the presence of an edge. Our results show that the gap appearing at $\hbarΩ/2$, where $\hbar Ω$ is the photon energy, is bridged by two chiral edge states whose propagation direction is set by the direction of the polarization of the radiation field. Therefore, both the propagation direction and the energy window where the states appear can be controlled externally. We present both analytical and numerical calculations that fully characterize these states. This is complemented by simple topological arguments that account for them and by numerical calculations for the case of semi-infinite sample, thereby eliminating finite size effects.

cond-mat.mes-hall↗

arXiv2014

Diffusion of fluorine adatoms on doped graphene

We calculate the diffusion barrier of fluorine adatoms on doped graphene in the diluted limit using Density Functional Theory. We found that the barrier $Δ$ strongly depends on the magnitude and character of the graphene's doping ($δn$): it increases for hole doping ($δn<0$) and decreases for electron doping ($δn>0$). Near the neutrality point the functional dependence can be approximately by $Δ=Δ_0-α\, δn$ where $α\simeq6\times10^{-12}$ meVcm$^2$. This effect leads to significant changes of the diffusion constant with doping even at room temperature and could also affect the low temperature diffusion dynamics due to the presence of substrate induced charge puddles. In addition, this might open up the possibility to engineer the F dynamics on graphene by using local gates.

cond-mat.mes-hall↗

arXiv2014

Ballistic spin resonance in multisubband quantum wires

Ballistic spin resonance was experimentally observed in a quasi-one-dimensional wire by Frolov et al. [Nature (London) 458, 868 (2009)]. The spin resonance was generated by a combination of an external static magnetic field and the oscillating effective spin-orbit magnetic field due to periodic bouncings of the electrons off the boundaries of a narrow channel. An increase of the D'yakonov-Perel spin relaxation rate was observed when the frequency of the spin-orbit field matched that of the Larmor precession frequency around the external magnetic field. Here we develop a model to account for the D'yakonov-Perel mechanism in multisubband quantum wires with both the Rashba and Dresselhaus spin-orbit interactions. Considering elastic spin-conserving impurity scatterings in the time-evolution operator (Heisenberg representation), we extract the spin relaxation time by evaluating the time-dependent average of the spin operators. The magnetic field dependence of the nonlocal voltage, which is related to the spin relaxation time behavior, shows a wide plateau, in agreement with the experimental observation. This plateau arises due to injection in higher subbands and small-angle scattering. In this quantum mechanical approach, the spin resonance occurs near the spin-orbit induced energy anticrossings of the quantum wire subbands with opposite spins. We also predict anomalous dips in the spin relaxation time as a function of the magnetic field in systems with strong spin-orbit couplings.

cond-mat.mes-hall↗

arXiv2014

Floquet chiral edge states in graphene

We report on the emergence of laser-induced chiral edge states in graphene ribbons. Insights on the nature of these Floquet states is provided by an analytical solution which is complemented with numerical simulations of the transport properties. Guided by these results we show that graphene can be used for realizing non-equilibrium topological states with striking tunability: While the laser intensity can be used to control their velocity and decay length, changing the laser polarization switches their propagation direction.

cond-mat.mes-hall↗

arXiv2014

Partial preservation of chiral symmetry and colossal magnetoresistance in adatom doped graphene

We analyze the electronic properties of adatom doped graphene in the low impurity concentration regime. We focus on the Anderson localized regime and calculate the localization length ($ξ$) as a function of the electron doping and an external magnetic field. The impurity states hybridize with carbon's $p_z$ states and form a partially filled band close to the Dirac point. Near the impurity band center, the chiral symmetry of the system's effective Hamiltonian is partially preserved which leads to a large enhancement of $ξ$. The sensitivity of transport properties, namely Mott's variable range hopping scale $T_0$, to an external magnetic field perpendicular to the graphene sheet leads to a colossal magnetoresistance effect, as observed in recent experiments.

cond-mat.mes-hall↗

arXiv2012

Spin-orbit induced chirality of Andreev states in Josephson junctions

We study Josephson junctions (JJs) in which the region between the two superconductors is a multichannel system with Rashba spin-orbit coupling (SOC) where a barrier or a quantum point contact (QPC) is present. These systems might present unconventional Josephson effects such as Josephson currents for zero phase difference or critical currents that \textit{depend on} the current direction. Here, we discuss how the spin polarizing properties of the system in the normal state affect the spin characteristic of the Andreev bound states inside the junction. This results in a strong correlation between the spin of the Andreev states and the direction in which they transport Cooper pairs. While the current-phase relation for the JJ at zero magnetic field is qualitatively unchanged by SOC, in the presence of a weak magnetic field a strongly anisotropic behavior and the mentioned anomalous Josephson effects follow. We show that the situation is not restricted to barriers based on constrictions such as QPCs and should generically arise if in the normal system the direction of the carrier's spin is linked to its direction of motion.

cond-mat.mes-hall↗

arXiv2012

Tunable Charge and Spin Seebeck Effects in Magnetic Molecular Junctions

We study the charge and spin Seebeck effects in a spin-1 molecular junction as a function of temperature (T), applied magnetic field (H), and magnetic anisotropy (D) using Wilson's numerical renormalization group. A hard-axis magnetic anisotropy produces a large enhancement of the charge Seebeck coefficient Sc (\sim k_B/|e|) whose value only depends on the residual interaction between quasiparticles in the low temperature Fermi-liquid regime. In the underscreened spin-1 Kondo regime, the high sensitivity of the system to magnetic fields makes it possible to observe a sizable value for the spin Seebeck coefficient even for magnetic fields much smaller than the Kondo temperature. Similar effects can be obtain in C60 junctions where the control parameter is the gap between a singlet and a triplet molecular state.

cond-mat.str-el↗