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Gonzalo Usaj

Publications and source records attributed to Gonzalo Usaj.

At least 55 records · Page 3Linked to original sources

Transport through side-coupled double quantum dots: from weak to strong interdot coupling

We report low-temperature transport measurements through a double quantum dot device in a configuration where one of the quantum dots is coupled directly to the source and drain electrodes, and a second (side-coupled) quantum dot interacts electrostatically and via tunneling to the first one. As the interdot coupling increases, a crossover from weak to strong interdot tunneling is observed in the charge stability diagrams that present a complex pattern with mergings and apparent crossings of Coulomb blockade peaks. While the weak coupling regime can be understood by considering a single level on each dot, in the intermediate and strong coupling regimes, the multi-level nature of the quantum dots needs to be taken into account. Surprisingly, both in the strong and weak coupling regimes, the double quantum dot states are mainly localized on each dot for most values of the parameters. Only in an intermediate coupling regime the device presents a single dot-like molecular behavior as the molecular wavefunctions weight is evenly distributed between the quantum dots. At temperatures larger than the interdot coupling energy scale, a loss of coherence of the molecular states is observed.

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Magnetic Structure of Hydrogen Induced Defects on Graphene

Using density functional theory (DFT), Hartree-Fock, exact diagonalization, and numerical renormalization group methods we study the electronic structure of diluted hydrogen atoms chemisorbed on graphene. A comparison between DFT and Hartree-Fock calculations allows us to identify the main characteristics of the magnetic structure of the defect. We use this information to formulate an Anderson-Hubbard model that captures the main physical ingredients of the system, while still allowing a rigorous treatment of the electronic correlations. We find that the large hydrogen-carbon hybridization puts the structure of the defect half-way between the one corresponding to an adatom weakly coupled to pristine graphene and a carbon vacancy. The impurity's magnetic moment leaks into the graphene layer where the electronic correlations on the C atoms play an important role in stabilizing the magnetic solution. Finally, we discuss the implications for the Kondo effect.

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Electrical Control of the Chemical Bonding of Fluorine on Graphene

We study the electronic structure of diluted F atoms chemisorbed on graphene using density functional theory calculations. We show that the nature of the chemical bonding of a F atom adsorbed on top of a C atom in graphene strongly depends on carrier doping. In neutral samples the F impurities induce a sp^3-like bonding of the C atom below, generating a local distortion of the hexagonal lattice. As the graphene is electron-doped, the C atom retracts back to the graphene plane and for high doping (10^14 cm^-2) its electronic structure corresponds to a nearly pure sp^2 configuration. We interpret this sp^3-sp^2 doping-induced crossover in terms of a simple tight binding model and discuss the physical consequences of this change.

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Out of equilibrium transport through an Anderson impurity: Probing scaling laws within the equation of motion approach

We study non-equilibrium electron transport through a quantum impurity coupled to metallic leads using the equation of motion technique at finite temperature T. Assuming that the interactions are taking place solely in the impurity and focusing in the infinite Hubbard limit, we compute the out of equilibrium density of states and the differential conductance G_2(T,V) to test several scaling laws. We find that G_2(T,V)/G_2(T,0) is a universal function of both eV/T_K and T/T_K, being T_K the Kondo temperature. The effect of an in plane magnetic field on the splitting of the zero bias anomaly in the differential conductance is also analyzed. For a Zeeman splitting Δ, the computed differential conductance peak splitting depends only on Δ/T_K, and for large fields approaches the value of 2Δ. Besides the traditional two leads setup, we also consider other configurations that mimics recent experiments, namely, an impurity embedded in a mesoscopic wire and the presence of a third weakly coupled lead. In these cases, a double peak structure of the Kondo resonance is clearly obtained in the differential conductance while the amplitude of the highest peak is shown to decrease as \ln(eV/T_K). Several features of these results are in qualitative agreement with recent experimental observations reported on quantum dots.

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Edge states interferometry and spin rotations in zigzag graphene nanoribbons

An interesting property of zigzag graphene nanoribbons is the presence of edge states which are extended along its borders but localized in the transverse direction. We show that because of this property, electron transport through an externally induced potential well displays two-paths-interference oscillations when subject either to a magnetic or a transverse electric field. This effect does not require the existence of an actual `hole' in the nanoribbon's geometry. Moreover, since edge states are spin polarized, having opposite polarization on opposite sides, such interference effect can be used to rotate the spin of the incident carriers in a controlled way.

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Localized Spins on Graphene

The problem of a magnetic impurity, atomic or molecular, absorbed on top of a carbon atom in otherwise clean graphene is studied using the numerical renormalization group. The spectral, thermodynamic, and scattering properties of the impurity are described in detail. In the presence of a small magnetic field, the low energy electronic features of graphene make possible to inject spin polarized currents through the impurity using a scanning tunneling microscope (STM). Furthermore, the impurity scattering becomes strongly spin dependent and for a finite impurity concentration it leads to spin polarized bulk currents and a large magnetoresistance. In gated graphene the impurity spin is Kondo screened at low temperatures. However, at temperatures larger than the Kondo temperature, the anomalous magnetotransport properties are recovered.

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Magnetic breakdown of cyclotron orbits in systems with Rashba and Dresselhaus spin-orbit coupling

We study the effect of the interplay between the Rashba and the Dresselhaus spin-orbit couplings on the transverse electron focusing in two-dimensional electron gases. Depending on their relative magnitude, the presence of both couplings can result in the splitting of the first focusing peak into two or three. This splitting has information about the relative value of spin-orbit couplings and therefore about the shape of the Fermi surface. More interesting, the presence of the third peak is directly related to the tunneling probability ("magnetic breakdown") between orbits corresponding to the different sheets of the Fermi surface. In addition, destructive interference effects between paths that involve tunneling and those that do not can be observed in the second focusing condition. Such electron paths (orbits) could be experimentally detected using current techniques for imaging the electron flow opening the possibility to directly observe and characterize the magnetic breakdown effect in this system.

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Anomalous Josephson Current in Junctions with Spin-Polarizing Quantum Point Contacts

We consider a ballistic Josephson junction with a quantum point contact in a two-dimensional electron gas with Rashba spin-orbit coupling. The point contact acts as a spin filter when embedded in a circuit with normal electrodes. We show that with an in-plane external magnetic field an anomalous supercurrent appears even for zero phase difference between the superconducting electrodes. In addition, the external field induces large critical current asymmetries between the two flow directions, leading to supercurrent rectifying effects.

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Level Spacings in Random Matrix Theory and Coulomb Blockade Peaks in Quantum Dots

We obtain analytic formulae for the spacing between conductance peaks in the Coulomb blockade regime, based on the universal Hamiltonian model of quantum dots. New random matrix theory results are developed in order to treat correlations between two and three consecutive spacings in the energy level spectrum. These are generalizations of the Wigner surmise for the probability distribution of single level spacing. The analytic formulae are shown to be in good agreement with numerical evaluation.

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Electronic Transport through Magnetic Molecules with Soft Vibrating Modes

The low-temperature transport properties of a molecule are studied in the field-effect transitor geometry. The molecule has an internal mechanical mode that modulates its electronic levels and renormalizes both the interactions and the coupling to the electrodes. For a soft mechanical mode the spin fluctuations in the molecule are dominated by the bare couplings while the valence changes are determined by the dressed energies. In this case, the transport properties present an anomalous behavior and the Kondo temperature has a weak gate voltage dependence. These observations are in agreement with recent experimental data.

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Imaging transverse electron focusing in semiconducting heterostructures with spin-orbit coupling

Transverse electron focusing in two-dimensional electron gases (2DEGs) with strong spin-orbit coupling is revisited. The transverse focusing is related to the transmission between two contacts at the edge of a 2DEG when a perpendicular magnetic field is applied. Scanning probe microscopy imaging techniques can be used to study the electron flow in these systems. Using numerical techniques we simulate the images that could be obtained in such experiments. We show that hybrid edge states can be imaged and that the outgoing flux can be polarized if the microscope tip probe is placed in specific positions.

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Slave boson theory for transport through magnetic molecules with vibronic states

We study the electron transport through a magnetic molecular transistor in the Kondo limit using the slave boson technique. We include the electron-phonon coupling and analyze the cases where the spin of the molecule is either S=1/2 or S=1. We use the Schrieffer-Wolff transformation to write down a low energy Hamiltonian for the system. In the presence of electron-phonon coupling, and for $S\smeq1$, the resulting Kondo Hamiltonian has two active channels. At low temperature, these two channels interfere destructively, leading to a zero conductance.

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Detection of spin polarized currents in quantum point contacts via transverse electron focusing

It has been predicted recently that an electron beam can be polarized when it flows adiabatically through a quantum point contact in a system with spin-orbit interaction. Here, we show that a simple transverse electron focusing setup can be used to detect such polarized current. It uses the amplitude's asymmetry of the spin-split transverse electron focusing peak to extract information about the electron's spin polarization. On the other hand, and depending on the quantum point contact geometry, including this one-body effect can be important when using the focusing setup to study many-body effects in quantum point contacts.

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Spin Hall effect in clean two dimensional electron gases with Rashba spin-orbit coupling

We study the spin polarization induced by a current flow in clean two dimensional electron gases with Rashba spin-orbit coupling. This geometric effect originates from special properties of the electron's scattering at the edges of the sample. In wide samples, the spin polarization has it largest value at low energies (close to the bottom of the band) and goes to zero at higher energies. In this case, the spin polarization is dominated by the presence of evanescent modes which have an explicit spin component outside the plane. In quantum wires, on the other hand, the spin polarization is dominated by interference effects induced by multiple scattering at the edges. Here, the spin polarization is quite sensitive to the value of the Fermi energy, especially close to the point where a new channel opens up. We analyzed different geometries and found that the spin polarization can be strongly enhanced.

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Anisotropy in Ferromagnetic Nanoparticles: Level-to-Level Fluctuations of a Collective Effect

We calculate the mesoscopic fluctuations of the magnetic anisotropy of ferromagnetic nanoparticles. A microscopic spin-orbit Hamiltonian considered as a perturbation of the much stronger exchange interaction first yields an explicit expression for the anisotropy tensor. Then, assuming a simple random matrix model for the spin-orbit coupling allows us to describe the fluctuation of such a tensor. In the case of uniaxial anisotropy, we calculate the distribution of the anisotropy constant for a given number of electrons, and its variation upon increasing this number by one. The magnitude of the latter is sufficient to account for the experimental data.

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Spin Accumulation and Equilibrium Currents at the Edge of 2DEGs with Spin-Orbit Coupling

We show that in a two dimensional electron gas (2DEG) the interplay between the Rashba spin-orbit coupling and a potential barrier (eg., the sample edge) generates interesting spin effects. In the presence of an external charge current, a spin accumulation is built up near the barrier while in equilibrium there is an inhomogeneous spin current which is localized at the barrier and flows parallel to it. When an in-plane magnetic field perpendicular to the barrier is applied, the system also develops an inhomogeneous charge current density. These effects originate purely from the structure of the eigenstates near the boundary.

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Design and control of spin gates in two quantum dots arrays

We study the spin-spin interaction between quantum dots coupled through a two dimensional electron gas with spin-orbit interaction. We show that the interplay between transverse electron focusing and spin-orbit coupling allows to dynamically change the symmetry of the effective spin-spin Hamiltonian. That is, the interaction can be changed from Ising-like to Heisenberg-like and vice versa. The sign and magnitude of the coupling constant can also be tuned.

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Tuning the Non-local Spin-Spin Interaction between Quantum Dots with a Magnetic Field

We describe a device where the non-local spin-spin interaction between two quantum dots can be turned on and off and even changed sign with a very small magnetic field. The setup consists of two quantum dots at the edge of two two-dimensional electron gases (2DEGs). The quantum dots' spins are coupled through a RKKY-like interaction mediated by the electrons in the 2DEGs. A small magnetic field perpendicular to the plane of the 2DEG is used as a tuning parameter. When the cyclotron radius is commensurate with the interdot distance, the spin-spin interaction is amplified by a few orders of magnitude. The sign of the interaction is controlled by finely tuning the magnetic field. Our setup allows for several dots to be coupled in a linear arrangement and it is not restricted to nearest-neighbors interaction.

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