arXiv subjects

Guido Pupillo

Publications and source records attributed to Guido Pupillo.

At least 55 records · Page 3Linked to original sources

arXiv2020

Mobility edge of the two dimensional Bose-Hubbard model

We analyze the disorder driven localization of the two dimensional Bose-Hubbard model by evaluating the full low energy quasiparticle spectrum via a recently developed fluctuation operator expansion method. For any strength of the local interaction we find a mobility edge that displays an approximately exponential decay with increasing disorder strength. We determine the finite-size scaling collapse and exponents at this critical line finding that the localization of excitations is characterized by weak multi-fractality and a thermal-like critical gap ratio. A direct comparison to a recent experiment yields an excellent match of the predicted finite-size transition point and scaling of single particle correlations.

cond-mat.quant-gas↗

arXiv2020

Collective Dissipative Molecule Formation in a Cavity

We propose a mechanism to realize high-yield molecular formation from ultracold atoms. Atom pairs are continuously excited by a laser, and a collective decay into the molecular ground state is induced by a coupling to a lossy cavity mode. Using a combination of analytical and numerical techniques, we demonstrate that the molecular yield can be improved by simply increasing the number of atoms, and can overcome efficiencies of state-of-the-art association schemes. We discuss realistic experimental setups for diatomic polar and nonpolar molecules, opening up collective light matter interactions as a tool for quantum state engineering, enhanced molecule formation, collective dynamics, and cavity mediated chemistry.

cond-mat.quant-gas↗

arXiv2020

Dark state semilocalization of quantum emitters in a cavity

We study a disordered ensemble of quantum emitters collectively coupled to a lossless cavity mode. The latter is found to modify the localization properties of the "dark" eigenstates, which exhibit a character of being localized on multiple, noncontiguous sites. We denote such states as semi-localized and characterize them by means of standard localization measures. We show that those states can very efficiently contribute to coherent energy transport. Our paper underlines the important role of dark states in systems with strong light-matter coupling.

quant-ph↗

arXiv2020

Cluster self-assembly condition for arbitrary interaction potentials

We present a sufficient criterion for the emergence of cluster phases in an ensemble of interacting classical particles with repulsive two-body interactions. Through a zero-temperature analysis in the low density region we determine the relevant characteristics of the interaction potential that make the energy of a two-particle cluster-crystal become smaller than that of a simple triangular lattice in two dimensions. The method leads to a mathematical condition for the emergence of cluster crystals in terms of the sum of Fourier components of a regularized interaction potential, which can be in principle applied to any arbitrary shape of interactions. We apply the formalism to several examples of bounded and unbounded potentials with and without cluster-forming ability. In all cases, the emergence of self-assembled cluster crystals is well captured by the presented analytic criterion and verified with known results from molecular dynamics simulations at vanishingly temperatures. Our work generalises known results for bounded potentials to repulsive potentials of arbitrary shape.

cond-mat.soft↗

arXiv2020

One-dimensional extended Hubbard model with soft-core potential

We investigate the $T=0$ phase diagram of a variant of the one-dimensional extended Hubbard model where particles interact via a finite-range soft-shoulder potential. Using Density Matrix Renormalization Group (DMRG) simulations, we evidence the appearance of Cluster Luttinger Liquid (CLL) phases, similarly to what first predicted in a hard-core bosonic chain [M. Mattioli, M. Dalmonte, W. Lechner, and G. Pupillo, Phys. Rev. Lett. 111, 165302]. As the interaction strength parameters change, we find different types of clusters, that encode the order of the ground state in a semi-classical approximation and give rise to different types of CLLs. Interestingly, we find that the conventional Tomonaga Luttinger Liquid (TLL) is separated by a critical line with a central charge $c=5/2$, along which the two (spin and charge) bosonic degrees of freedom (corresponding to $c=1$ each) combine in a supersymmetric way with an emergent fermionic excitation ($c=1/2$). We also demonstrate that there are no significant spin correlations.

cond-mat.str-el↗

arXiv2020

Nonequilibrium scenarios in cluster-forming quantum lattice models

We investigate the out-of-equilibrium physics of monodisperse bosonic ensembles on a square lattice. The effective Hamiltonian description of these systems is given in terms of an extended Hubbard model with cluster-forming interactions relevant to experimental realizations with cold Rydberg-dressed atoms. The ground state of the model, recently investigated in Phys. Rev. Lett. 123, 045301 (2019), features, aside from a superfluid and a stripe crystalline phase occurring at small and large interaction strength $V$, respectively, a rare first-order transition between an isotropic and an anisotropic stripe supersolid at intermediate $V$. By means of quantum Monte Carlo calculations we show that the equilibrium crystal may be turned into a glass by simulated temperature quenches and that out-of-equilibrium isotropic (super)solid states may emerge also when their equilibrium counterparts are anisotropic. These out-of-equilibrium states are of experimental interest, their excess energy with respect to the ground state being within the energy window typically accessed in cold atom experiments. We find, after quenching, no evidence of coexistence between superfluid and glassy behavior. Such an absence of superglassiness is qualitatively explained.

cond-mat.quant-gas↗

arXiv2020

Universal algebraic growth of entanglement entropy in many-body localized systems with power-law interactions

Power-law interactions play a key role in a large variety of physical systems. In the presence of disorder, these systems may undergo many-body localization for a sufficiently large disorder. Within the many-body localized phase the system presents in time an algebraic growth of entanglement entropy, $S_{vN}(t)\propto t^γ$. Whereas the critical disorder for many-body localization depends on the system parameters, we find by extensive numerical calculations that the exponent $γ$ acquires a universal value $γ_c\simeq 0.33$ at the many-body localization transition, for different lattice models and decay powers. Moreover, our results suggest an intriguing relation between $γ_c$ and the critical minimal decay power of interactions necessary for the observation of many-body localization.

cond-mat.dis-nn↗

arXiv2020

Quantum Cluster Quasicrystals

Quasicrystals remain among the most intriguing materials in physics and chemistry. Their structure results in many unusual properties including anomalously low friction as well as poor electrical and thermal conductivity but it also supports superconductivity, which shows that quantum effects in quasicrystals can be quite unique. Here we theoretically study superfluidity in a model quantum cluster quasicrystal. Using path-integral Monte Carlo simulations, we explore a 2D ensemble of bosons with the Lifshitz-Petrich-Gaussian pair potential, finding that moderate quantum fluctuations do not destroy the dodecagonal quasicrystalline order. This quasicrystal is characterized by a small yet finite superfluidity, demonstrating that particle clustering combined with the local cogwheel structure can underpin superfluidity even in the almost classical regime. This type of distributed superfluidity may also be expected in certain open crystalline lattices. Large quantum fluctuations are shown to induce transitions to cluster solids, supersolids and superfluids, which we characterize fully quantum-mechanically.

cond-mat.quant-gas↗

arXiv2020

Ensemble-induced strong light-matter coupling of a single quantum emitter

We discuss a technique to strongly couple a single target quantum emitter to a cavity mode, which is enabled by virtual excitations of a nearby mesoscopic ensemble of emitters. A collective coupling of the latter to both the cavity and the target emitter induces strong photon non-linearities in addition to polariton formation, in contrast to common schemes for ensemble strong coupling. We demonstrate that strong coupling at the level of a single emitter can be engineered via coherent and dissipative dipolar interactions with the ensemble, and provide realistic parameters for a possible implementation with SiV$^{-}$ defects in diamond. Our scheme can find applications, amongst others, in quantum information processing or in the field of cavity-assisted quantum chemistry.

quant-ph↗

arXiv2019

Adiabatic elimination for ensembles of emitters in cavities with dissipative couplings

We consider an ensemble of cavity-coupled two-level emitters interacting via full (coherent and dissipative) dipole-dipole interactions. Using an adiabatic elimination procedure we derive effective equations of motion for a subsystem consisting of the cavity and a single emitter. Those equations can be used for schemes to enhance the cavity-coupling of single emitters as shown in [S. Schütz, J. Schachenmayer, D. Hagenmüller, G. K. Brennen, T. Volz, V. Sandoghdar, T. W. Ebbesen, C. Genes, and G. Pupillo, e-print arXiv:1904.08888]. We analyze limitations of effective subsystem parameters, and study how joint dissipative decay processes in the subsystem affect cavity-coupling properties of the single emitter and cavity transmission spectra.

quant-ph↗

arXiv2019

Exploring Superconductivity under Strong Coupling with the Vacuum Electromagnetic Field

Light-matter interactions have generated considerable interest as a means to manipulate material properties. Light-induced superconductivity has been demonstrated using pulsed lasers. An attractive alternative possibility is to exploit strong light-matter interactions arising by coupling phonons to the vacuum electromagnetic field of a cavity mode as has been suggested and theoretically studied. Here we explore this possibility for two very different superconductors, namely YBCO (YBa$_2$Cu$_3$O$_{6+x}$) and Rb$_3$C$_{60}$, coupled to surface plasmon polaritons, using a novel cooperative effect based on the presence of a strongly coupled vibrational environment allowing efficient dressing of the otherwise weakly coupled phonon bands of these compounds. By placing the superconductor-surface plasmon system in a SQUID magnetometer, we find that the superconducting transition temperatures ($T_{c}$) for both compounds are modified in the absence of any external laser field. For YBCO, $T_{c}$ decreases from 92 K to 86 K while for Rb$_3$C$_{60}$, it increases from 30 K to 45 K at normal pressures. In the latter case, a simple theoretical framework is provided to understand these results based on an enhancement of the electron-phonon coupling. This proof-of-principle study opens a new tool box to not only modify superconducting materials but also to understand the mechanistic details of different superconductors.

cond-mat.supr-con↗

arXiv2019

Ultrafast creation of overlapping Rydberg electrons in an atomic BEC and Mott-insulator lattice

An array of ultracold atoms in an optical lattice (Mott insulator) excited to a state where single electron wave-functions spatially overlap would represent a new and ideal platform to simulate exotic electronic many-body phenomena in the condensed phase. However, this highly excited non-equilibrium system is expected to be so short-lived that it has eluded observation so far. Here, we demonstrate the first step toward its realization by exciting high-lying electronic (Rydberg) states of the atomic Mott insulator with a coherent ultrashort laser pulse. Beyond a threshold principal quantum number where Rydberg orbitals of neighboring lattice sites overlap with each other, the atoms efficiently undergo spontaneous Penning ionization resulting in a drastic change of ion-counting statistics, sharp increase of avalanche ionization and the formation of an ultracold plasma. These observations signal the actual creation of exotic electronic states with overlapping wave functions, which is further confirmed by a significant difference in ionization dynamics between a Bose-Einstein condensate and a Mott insulator.

physics.atom-ph↗

arXiv2019

Effects of energy extensivity on the quantum phases of long-range interacting systems

We investigate the ground state properties of one-dimensional hard-core bosons interacting via a variable long-range potential using the density matrix renormalization group. We demonstrate that restoring energy extensivity in the system, which is done by rescaling the interaction potential with a suitable size-dependent factor known as Kac's prescription, has a profound influence on the low-energy properties in the thermodynamic limit. While an insulating phase is found in the absence of Kac's rescaling, the latter leads to a new metallic phase that does not fall into the conventional Luttinger liquid paradigm. Our results in one dimension illustrate the subtlety of determining the thermodynamic properties of generic long-range quantum systems.

cond-mat.str-el↗

arXiv2019

Supersolid stripe crystal from finite-range interactions on a lattice

Strong, long-range interactions present a unique challenge for the theoretical investigation of quantum many-body lattice models, due to the generation of large numbers of competing states at low energy. Here, we investigate a class of extended bosonic Hubbard models with off-site terms interpolating between short and infinite range, thus allowing for an exact numerical solution for all interaction strengths. We predict a novel type of stripe crystal at strong coupling. Most interestingly, for intermediate interaction strengths we demonstrate that the stripes can turn superfluid, thus leading to a self-assembled array of quasi-one-dimensional superfluids. These bosonic superstripes turn into an isotropic supersolid with decreasing the interaction strength. The mechanism for stripe formation is based on cluster self-assembling in the corresponding classical ground state, reminiscent of classical soft-matter models of polymers, different from recently proposed mechanisms for cold gases of alkali or dipolar magnetic atoms.

cond-mat.quant-gas↗

arXiv2019

Phase-change switching in 2D via soft interactions

We present a new type of phase-change behavior relevant for information storage applications, that can be observed in 2D systems with cluster-forming ability. The temperature-based control of the ordering in 2D particle systems depends on the existence of a crystal-to-glass transition. We perform molecular dynamics simulations of models with soft interactions, demonstrating that the crystalline and amorphous structures can be easily tuned by heat pulses. The physical mechanism responsible for this behavior is a self-assembled polydispersity, that depends on the cluster-forming ability of the interactions. Therefore, the range of real materials that can perform such a transition is very wide in nature, reading from colloidal suspensions to vortex matter. The state of the art in soft matter experimental setups, controlling interactions, polydispersity and dimensionality, makes it a very fertile ground for practical applications.

cond-mat.stat-mech↗

arXiv2019

Enhancement of the electron-phonon scattering induced by intrinsic surface plasmon-phonon polaritons

We investigate light-matter coupling in metallic crystals where plasmons coexist with phonons exhibiting large oscillator strength. We demonstrate theoretically that this coexistence can lead to strong light-matter interactions without external resonators. When the frequencies of plasmons and phonons are comparable, hybridization of these collective matter modes occurs in the crystal. We show that the coupling of these modes to photonic degrees of freedom gives rise to intrinsic surface plasmon-phonon polaritons, which offer the unique possibility to control the phonon properties by tuning the electron density and the crystal thickness. In particular, dressed phonons with reduced frequency and large wave vectors arise in the case of quasi-2D crystals, which leads to large enhancements of the electron-phonon scattering in the vibrational ultrastrong coupling regime. This suggests that photons can play a key role in determining the quantum properties of certain materials. A non-perturbative self-consistent Hamiltonian method is presented that is valid for arbitrarily large coupling strengths.

cond-mat.mes-hall↗

arXiv2018

Algebraic Localization from Power-Law Interactions in Disordered Quantum Wires

We analyze the effects of disorder on the correlation functions of one-dimensional quantum models of fermions and spins with long-range interactions that decay with distance $\ell$ as a power-law $1/\ell^α$. Using a combination of analytical and numerical results, we demonstrate that power-law interactions imply a long-distance algebraic decay of correlations within disordered-localized phases, for all exponents $α$. The exponent of algebraic decay depends only on $α$, and not, e.g., on the strength of disorder. We find a similar algebraic localization for wave-functions. These results are in contrast to expectations from short-range models and are of direct relevance for a variety of quantum mechanical systems in atomic, molecular and solid-state physics.

cond-mat.dis-nn↗

arXiv2018

Cavity-assisted mesoscopic transport of fermions: Coherent and dissipative dynamics

We study the interplay between charge transport and light-matter interactions in a confined geometry, by considering an open, mesoscopic chain of two-orbital systems resonantly coupled to a single bosonic mode close to its vacuum state. We introduce and benchmark different methods based on self-consistent solutions of non-equilibrium Green's functions and numerical simulations of the quantum master equation, and derive both analytical and numerical results. It is shown that in the dissipative regime where the cavity photon decay rate is the largest parameter, the light-matter coupling is responsible for a steady-state current enhancement scaling with the cooperativity parameter. We further identify different regimes of interest depending on the ratio between the cavity decay rate and the electronic bandwidth. Considering the situation where the lower band has a vanishing bandwidth, we show that for a high-finesse cavity, the properties of the resonant Bloch state in the upper band are transfered to the lower one, giving rise to a delocalized state along the chain. Conversely, in the dissipative regime with low cavity quality factors, we find that the current enhancement is due to a collective decay of populations from the upper to the lower band.

quant-ph↗