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Guido Pupillo

Publications and source records attributed to Guido Pupillo.

At least 73 records · Page 4Linked to original sources

Rydberg optical Feshbach resonances in cold gases

We propose a novel scheme to efficiently tune the scattering length of two colliding ground-state atoms by off-resonantly coupling the scattering-state to an excited Rydberg-molecular state using laser light. For the s-wave scattering of two colliding ${^{87}}\mathrm{Rb}$ atoms, we demonstrate that the effective optical length and pole strength of this Rydberg optical Feshbach resonance can be tuned over several orders of magnitude, while incoherent processes and losses are minimised. Given the ubiquity of Rydberg molecular states, this technique should be generally applicable to homo-nuclear atomic pairs as well as to atomic mixtures with s-wave (or even p-wave) scattering.

cond-mat.quant-gas↗

Cavity-enhanced transport of charge

We theoretically investigate charge transport through electronic bands of a mesoscopic one-dimensional system, where inter-band transitions are coupled to a confined cavity mode, initially prepared close to its vacuum. This coupling leads to light-matter hybridization where the dressed fermionic bands interact via absorption and emission of dressed cavity-photons. Using a self-consistent non-equilibrium Green's function method, we compute electronic transmissions and cavity photon spectra and demonstrate how light-matter coupling can lead to an enhancement of charge conductivity in the steady-state. We find that depending on cavity loss rate, electronic bandwidth, and coupling strength, the dynamics involves either an individual or a collective response of Bloch states, and explain how this affects the current enhancement. We show that the charge conductivity enhancement can reach orders of magnitudes under experimentally relevant conditions.

quant-ph↗

Glass transitions in monodisperse cluster-forming ensembles: vortex matter in type-1.5 superconductors

At low enough temperatures and high densities, the equilibrium configuration of an ensemble of ultrasoft particles is a self-assembled, ordered, cluster-crystal. In the present work we explore the out-of-equilibrium dynamics for a two-dimensional realization, which is relevant to superconducting materials with multi-scale intervortex forces. We find that for small temperatures following a quench, the suppression of the thermally-activated particle hopping hinders the ordering. This results in a glass transition for a monodispersed ensemble, for which we derive a microscopic explanation in terms of an "effective polydispersity" induced by multi-scale interactions. This demonstrates that a vortex glass can form in clean systems of thin films of "type-1.5" superconductors. An additional setup to study this physics can be layered superconducting systems, where the shape of the effective vortex-vortex interactions can be engineered.

cond-mat.supr-con↗

Direct observation of ultrafast many-body electron dynamics in an ultracold Rydberg gas

Many-body correlations govern a variety of important quantum phenomena such as the emergence of superconductivity and magnetism. Understanding quantum many-body systems is thus one of the central goals of modern sciences. Here we demonstrate an experimental approach towards this goal by utilizing an ultracold Rydberg gas generated with a broadband picosecond laser pulse. We follow the ultrafast evolution of its electronic coherence by time-domain Ramsey interferometry with attosecond precision. The observed electronic coherence shows an ultrafast oscillation with a period of 1 femtosecond, whose phase shift on the attosecond timescale is consistent with many-body correlations among Rydberg atoms beyond mean-field approximations. This coherent and ultrafast many-body dynamics is actively controlled by tuning the orbital size and population of the Rydberg state, as well as the mean atomic distance. Our approach will offer a versatile platform to observe and manipulate non-equilibrium dynamics of quantum many-body systems on the ultrafast timescale.

physics.atom-ph↗

Time-domain Ramsey interferometry with interacting Rydberg atoms

We theoretically investigate the dynamics of a gas of strongly interacting Rydberg atoms subject to a time-domain Ramsey interferometry protocol. The many-body dynamics is governed by an Ising-type Hamiltonian with long range interactions of tunable strength. We analyze and model the contrast degradation and phase accumulation of the Ramsey signal and identify scaling laws for varying interrogation times, ensemble densities, and ensemble dimensionalities.

cond-mat.quant-gas↗

Two holes in a two-dimensional quantum antiferromagnet: A variational study based on entangled-plaquette states

We show that the entangled-plaquette variational ansatz can be adapted to study the two-dimensional $t-J$ model in the presence of two mobile holes. Specifically, we focus on a square lattice comprising up to $N=256$ sites in the parameter range $0.4\leq J/ t\leq2.0$. Ground state energies are obtained via the optimization of a wave function in which the weight of a given configuration is expressed in terms of variational coefficients associated with square and linear entangled plaquettes. Our estimates are in excellent agreement with exact results available for the $N=16$ lattice. By extending our study to considerably larger systems we find, based on the analysis of the long distance tail of the probability of finding two holes at spatial separation $r$, and on our computed two-hole binding energies, the existence of a two-hole bound state for all the values of $J/t$ explored here. It is estimated that d-wave binding of the two holes does not occur for $J/t<J_c/t\simeq 0.19$.

cond-mat.str-el↗

Effective Theory and Breakdown of Conformal Symmetry in a Long-Range Quantum Chain

We deal with the problem of studying the effective theories and the symmetries of long-range models around critical points. We focus in particular on the Kitaev chain with long-range pairings decaying with distance as power-law with exponent $α$. This is a quadratic solvable model, yet displaying non-trivial quantum phase transitions. By renormalization group approach we derive first the effective theory close to the critical line at positive chemical potential. This is the sum of two terms: a Dirac action $S_D$, found in the short-range Ising universality class, and a CS breaking term $S_{AN}$. While $S_D$ originates from low-energy excitations, $S_{AN}$ derives from the higher energy modes where singularities develop, due to the long-range nature of the model. At criticality $S_{AN}$ flows to zero if $α> 2$, while if $α< 2$ it dominates and determines the breakdown of the CS. Out of criticality $S_{AN}$ breaks, in the considered approximation, the effective Lorentz invariance (ELI) for every finite $α$. As $α$ increases, such ELI breakdown becomes less and less pronounced and in the short-range limit $α\to \infty$ the ELI is restored. To test the validity of the effective theory, we compared the two-fermion static correlations and the von Neumann entropy obtained from them with the ones calculated on the lattice, finding agreement. From the effective theory one can also see that new phases emerge for $α< 1$. Finally we show that at every finite $α$ the critical exponents are the same as for the short-range ($α\to \infty$) model. At variance, for the critical line with negative chemical potential, only $S_{AN}$ ($S_D$) is present for $1 < α< 2$ (for $α> 2$). Close to this line, where the minimum of the spectrum coincides with the momentum where singularities develop, the critical exponents change exactly where CS is broken.

cond-mat.str-el↗

Cavity polaritons with Rydberg blockade and long-range interactions

We study interactions between polaritons, arising when photons strongly couple to collective excitations in an array of two-level atoms trapped in an optical lattice inside a cavity. We consider two types of interactions between atoms: Dipolar forces and atomic saturability, which ranges from hard-core repulsion to Rydberg blockade. We show that, in spite of the underlying repulsion in the subsystem of atomic excitations, saturability induces a broadband bunching of photons for two-polariton scattering states. We interpret this bunching as a result of interference, and trace it back to the mismatch of the quantization volumes for atomic excitations and photons. We examine also bound bipolaritonic states: These include states created by dipolar forces, as well as a gap bipolariton, which forms solely due to saturability effects in the atomic transition. Both types of bound states exhibit strong bunching in the photonic component. We discuss the dependence of bunching on experimentally relevant parameters.

quant-ph↗

Event-Driven Monte Carlo: exact dynamics at all time-scales for discrete-variable models

We present an algorithm for the simulation of the exact real-time dynamics of classical many-body systems with discrete energy levels. In the same spirit of kinetic Monte Carlo methods, a stochastic solution of the master equation is found, with no need to define any other phase-space construction. However, unlike existing methods, the present algorithm does not assume any particular statistical distribution to perform moves or to advance the time, and thus is a unique tool for the numerical exploration of fast and ultra-fast dynamical regimes. By decomposing the problem in a set of two-level subsystems, we find a natural variable step size, that is well defined from the normalization condition of the transition probabilities between the levels. We successfully test the algorithm with known exact solutions for non-equilibrium dynamics and equilibrium thermodynamical properties of Ising-spin models in one and two dimensions, and compare to standard implementations of kinetic Monte Carlo methods. The present algorithm is directly applicable to the study of the real time dynamics of a large class of classical markovian chains, and particularly to short-time situations where the exact evolution is relevant.

cond-mat.stat-mech↗

Superglass phase of interaction-blockaded gases on a triangular lattice

We investigate the quantum phases of monodispersed bosonic gases confined to a triangular lattice and interacting via a class of soft-shoulder potentials. The latter correspond to soft-core potentials with an additional hard-core onsite interaction. Using exact quantum Monte Carlo simulations, we show that the low temperature phases for weak and strong interactions following a temperature quench are a homogeneous superfluid and a glass, respectively. The latter is an insulating phase characterized by inhomogeneity in the density distribution and structural disorder. Remarkably, we find that for intermediate interaction strengths a {\it superglass} occurs in an extended region of the phase diagram, where glassy behavior coexists with a sizable finite superfluid fraction. This glass phase is obtained in the absence of geometrical frustration or external disorder and is a result of the competition of quantum fluctuations and cluster formation in the corresponding classical ground state. For high enough temperature, the glass and superglass turn into a floating stripe solid and a supersolid, respectively. Given the simplicity and generality of the model, these phases should be directly relevant for state-of-the-art experiments with Rydberg-dressed atoms in optical lattices.

cond-mat.quant-gas↗

Long-range Ising and Kitaev Models: Phases, Correlations and Edge Modes

We analyze the quantum phases, correlation functions and edge modes for a class of spin-1/2 and fermionic models related to the 1D Ising chain in the presence of a transverse field. These models are the Ising chain with anti-ferromagnetic long-range interactions that decay with distance $r$ as $1/r^α$, as well as a related class of fermionic Hamiltonians that generalise the Kitaev chain, where both the hopping and pairing terms are long-range and their relative strength can be varied. For these models, we provide the phase diagram for all exponents $α$, based on an analysis of the entanglement entropy, the decay of correlation functions, and the edge modes in the case of open chains. We demonstrate that violations of the area law can occur for $α\lesssim1$, while connected correlation functions can decay with a hybrid exponential and power-law behaviour, with a power that is $α$-dependent. Interestingly, for the fermionic models we provide an exact analytical derivation for the decay of the correlation functions at every $α$. Along the critical lines, for all models breaking of conformal symmetry is argued at low enough $α$. For the fermionic models we show that the edge modes, massless for $α\gtrsim 1$, can acquire a mass for $α< 1$. The mass of these modes can be tuned by varying the relative strength of the kinetic and pairing terms in the Hamiltonian. Interestingly, for the Ising chain a similar edge localization appears for the first and second excited states on the paramagnetic side of the phase diagram, where edge modes are not expected. We argue that, at least for the fermionic chains, these massive states correspond to the appearance of new phases, notably approached via quantum phase transitions without mass gap closure. Finally, we discuss the possibility to detect some of these effects in experiments with cold trapped ions.

cond-mat.str-el↗

Broadband photon-photon interactions mediated by cold atoms in a photonic crystal fiber

We demonstrate theoretically that photon-photon attraction can be engineered in the continuum of scattering states for pairs of photons propagating in a hollow-core photonic crystal fiber filled with cold atoms. The atoms are regularly spaced in an optical lattice configuration and the photons are resonantly tuned to an internal atomic transition. We show that the hard-core repulsion resulting from saturation of the atomic transitions induces bunching in the photonic component of the collective atom-photon modes (polaritons). Bunching is obtained in a frequency range as large as tens of GHz, and can be controlled by the inter-atomic separation. We provide a fully analytical explanation for this phenomenon by proving that correlations result from a mismatch of the quantization volumes for atomic excitations and photons in the continuum. Even stronger correlations can be observed for in-gap two-polariton bound states. Our theoretical results use parameters relevant for current experiments with Rb atoms excited on the D2-line.

quant-ph↗

Tuneable defect interactions and supersolidity in dipolar quantum gases on a lattice potential

Point defects in self-assembled crystals, such as vacancies and interstitials, attract each other and form stable clusters. This leads to a phase separation between perfect crystalline structures and defect conglomerates at low temperatures. We propose a method that allows one to tune the effective interactions between point defects from attractive to repulsive by means of external periodic fields. In the quantum regime, this allows one to engineer strongly-correlated many-body phases. We exemplify the microscopic mechanism by considering dipolar quantum gases of ground state polar molecules and weakly bound molecules of strongly magnetic atoms trapped in a weak optical lattice in a two-dimensional configuration. By tuning the lattice depth, defect interactions turn repulsive, which allows us to deterministically design a novel supersolid phase in the continuum limit.

cond-mat.quant-gas↗

Monodisperse cluster crystals: classical and quantum dynamics

We study the phases and dynamics of a gas of monodisperse particles interacting via soft-core potentials in two spatial dimensions, which is of interest for soft-matter colloidal systems and quantum atomic gases. Using exact theoretical methods, we demonstrate that the equilibrium low-temperature classical phase simultaneously breaks continuous translational symmetry and dynamic space-time homogeneity, whose absence is usually associated with out-of-equilibrium glassy phenomena. This results in an exotic self-assembled cluster crystal with coexisting liquid-like long-time dynamical properties, which corresponds to a classical analog of supersolid behavior. We demonstrate that the effects of quantum fluctuations and bosonic statistics on cluster-glassy crystals are separate and competing: zero-point motion tends to destabilize crystalline order, which can be restored by bosonic statistics.

cond-mat.soft↗

Cavity enhanced transport of excitons

We show that exciton-type transport in certain materials can be dramatically modified by their inclusion in an optical cavity: the modification of the electromagnetic vacuum mode structure introduced by the cavity leads to transport via delocalized polariton modes rather than through tunneling processes in the material itself. This can help overcome exponential suppression of transmission properties as a function of the system size in the case of disorder and other imperfections. We exemplify massive improvement of transmission for excitonic wave-packets through a cavity, as well as enhancement of steady-state exciton currents under incoherent pumping. These results may have implications for experiments of exciton transport in disordered organic materials. We propose that the basic phenomena can be observed in quantum simulators made of Rydberg atoms, cold molecules in optical lattices, as well as in experiments with trapped ions.

quant-ph↗

Coherent coupling of molecular resonators with a micro-cavity mode

The optical hybridization of the electronic states in strongly coupled molecule-cavity systems have revealed unique properties such as lasing, room temperature polariton condensation, and the modification of excited electronic landscapes involved in molecular isomerization. Here we show that molecular vibrational modes of the electronic ground state can also be coherently coupled with a micro-cavity mode at room temperature, given the low vibrational thermal occupation factors associated with molecular vibrations, and the collective coupling of a large ensemble of molecules immersed within the cavity mode volume. This enables the enhancement of the collective Rabi-exchange rate with respect to the single oscillator coupling strength. The possibility of inducing large shifts in the vibrational frequency of selected molecular bonds should have immediate consequences for chemistry.

quant-ph↗

Kitaev chains with long-range pairing

We propose and analyze a generalization of the Kitaev chain for fermions with long-range $p$-wave pairing, which decays with distance as a power-law with exponent $α$. Using the integrability of the model, we demonstrate the existence of two types of gapped regimes, where correlation functions decay exponentially at short range and algebraically at long range ($α> 1$) or purely algebraically ($α< 1$). Most interestingly, along the critical lines, long-range pairing is found to break conformal symmetry for sufficiently small $α$. This is accompanied by a violation of the area law for the entanglement entropy in large parts of the phase diagram in the presence of a gap, and can be detected via the dynamics of entanglement following a quench. Some of these features may be relevant for current experiments with cold atomic ions.

cond-mat.str-el↗

Hybrid cavity mechanics with doped systems

We investigate the dynamics of a mechanical resonator in which is embedded an ensemble of two-level systems interacting with an optical cavity field. We show that this hybrid approach to optomechanics allows for enhanced effective interactions between the mechanics and the cavity field, leading for instance to ground state cooling of the mechanics, even in regimes, like the unresolved sideband regime, in which standard radiation pressure cooling would be inefficient.

quant-ph↗