arXiv subjects

H. Ding

Publications and source records attributed to H. Ding.

At least 163 records · Page 9Linked to original sources

arXiv2011

Strong nodeless pairing on separate electron Fermi surface sheets in (Tl, K)Fe$_{1.78}$Se$_2$ probed by ARPES

We performed a high-resolution angle-resolved photoemission spectroscopy study of the Tl$_{0.63}$K$_{0.37}$Fe$_{1.78}$Se$_2$ superconductor ($T_c=29$ K). We show the existence of two electronlike bands at the M$(π, 0)$ point which cross the Fermi level at similar Fermi wave vectors to form nearly circular electronlike Fermi surface pockets. We observe a nearly isotropic $\sim$ 8.5 meV superconducting gap ($Δ/k_BT_c\sim 7$) on these Fermi surfaces. Our analysis of the band structure around the Brillouin zone centre reveals two additional electronlike Fermi surfaces: a very small one and a larger one with $k_F$ comparable to the FS pockets at M. Interestingly, a SC gap with a magnitude of $\sim$ 8 meV also develops along the latter FS. Our observations are consistent with the s-wave strong coupling scenario.

cond-mat.supr-con↗

arXiv2011

Universality of superconducting gaps in overdoped Ba0.3K0.7Fe2As2 observed by angle-resolved photoemission spectroscopy

We have performed angle-resolved photoemission spectroscopy on the overdoped Ba$_{0.3}$K$_{0.7}$Fe$_2$As$_2$ superconductor ($T_c$ = 22 K). We demonstrate that the superconducting (SC) gap on each Fermi surface (FS) is nearly isotropic whereas the gap value varies from 4.4 to 7.9 meV on different FSs. By comparing with under- and optimally-doped Ba$_{1-x}$K$_x$Fe$_2$As$_2$, we find that the gap value on each FS nearly scales with $T_c$ over a wide doping range (0.25 $\textyen leq$ $x$ $\textyen leq$ 0.7). Although the FS volume and the SC gap magnitude are strongly doping dependent, the multiple nodeless gaps can be commonly fitted by a single gap function assuming pairing up to the second-nearest-neighbor, suggesting the universality of the short-range pairing states with the $s_{\yenpm}$-wave symmetry.

cond-mat.supr-con↗

arXiv2010

Absence of holelike Fermi surface in superconducting K0.8Fe1.7Se2 revealed by ARPES

We have performed an angle-resolved photoemission spectroscopy study of the new iron-based superconductor K0.8Fe1.7Se2 (Tc ~ 30 K). Clear band dispersion is observed with the overall bandwidth renormalized by a factor of 2.5 compared to our local density approximation calculations, indicating relatively strong correlation effects. Only an electronlike band crosses the Fermi energy, forming a nearly circular Fermi surface (FS) at M (π, 0). The holelike band at Γ sinks ~ 90 meV below the Fermi energy, with an indirect band gap of 30 meV to the bottom of the electronlike band. The observed FS topology in this superconductor favors (π, π) inter-FS scattering between the electronlike FSs at the M points, in sharp contrast with other iron-based superconductors which favor (π, 0) inter-FS scattering between holelike and electronlike FSs.

cond-mat.supr-con↗

arXiv2010

Observation of novel interference patterns in Bi2-xFexTe3+d by Fourier transform scanning tunneling spectroscopy

In topological insulators (TI), strong spin-orbit coupling results in non-trivial scattering processes of the surface states, whose effects include suppressed back scattering1, 2, 3, 4 weak anti-localization5, 6 and the possibility of an exotic Kondo effect that mimics graphene7. Introducing time reversal breaking perturbations and establishing long-range magnetic order has been theorized to lead to the formation of quantized magnetoelectric phenomena8, fractionalized charge excitations, and the appearance of quantum wire states9. A key, elusive, step in exploring these and other novel electronic phases is the experimental observation of charge backscattering due to spin-flip processes at the surface of a magnetically-doped TI. Here we utilize Fourier transform scanning tunneling spectroscopy (FT-STS) to probe the surface of a magnetically doped TI, Bi2-xFexTe3+d. Our measurements show the appearance of a hitherto unobserved channel of electronic backscattering along surface q-vector Γκ. By combining FT-STS with angle-resolved photoemission data, we identify the momentum space origins of the observed q-vectors, which on comparison to a model calculation are enhanced by spin-flip scattering. Our findings present compelling evidence for the first spatial and momentum resolved measurements of magnetic impurity induced backscattering in a prototypical TI.

cond-mat.mtrl-sci↗

arXiv2010

Fermiology of Sr4V2O6Fe2As2: Quasi-Nested Fe vs Mott-Insulating V Orbitals

We have performed an angle-resolved photoemission spectroscopy study of a new iron-based superconductor Sr4V2O6Fe2As2. While V 3d orbitals are found to be in a Mott insulator state and show an incoherent peak at ~ 1 eV below the Fermi level, the dispersive Fe 3d bands form several hole- and electron-like Fermi surfaces (FSs), some of which are quasi-nested by the (pi, 0) wave vector. This differs from the local density approximation (LDA) calculations, which predict non-nested FSs for this material. However, LDA+U with a large effective Hubbard energy U on V 3d electrons can reproduce the experimental observation reasonably well. The observed fermiology in superconducting Sr4V2O6Fe2As2 strongly supports that (pi, 0) interband scattering between quasi-nested FSs is indispensable to superconductivity in pnictides.

cond-mat.supr-con↗

arXiv2010

Electron-Hole Asymmetry in Superconductivity of Pnictides Originated from the Observed Rigid Chemical Potential Shift

We have performed a systematic photoemission study of the chemical potential shift as a function of carrier doping in a pnictide system based on BaFe$_2$As$_2$. The experimentally determined chemical potential shift is consistent with the prediction of a rigid band shift picture by the renormalized first-principle band calculations. This leads to an electron-hole asymmetry (EHA) in the Fermi surface (FS) nesting condition due to different effective masses for different FS sheets, which can be calculated from the Lindhard function of susceptibility. This built-in EHA from the band structure, which matches well with observed asymmetric superconducting domes in the phase diagram, strongly supports FS near-nesting driven superconductivity in the iron pnictides.

cond-mat.supr-con↗

arXiv2009

Observation of Dirac Cone Electronic Dispersion in BaFe2As2

We performed an angle-resolved photoemission spectroscopy study of BaFe2As2, which is the parent compound of the so-called 122 phase of the iron-pnictide high-temperature superconductors. We reveal the existence of a Dirac cone in the electronic structure of this material below the spin-density-wave temperature, which is responsible for small spots of high photoemission intensity at the Fermi level. Our analysis suggests that the cone is slightly anisotropic and its apex is located very near the Fermi level, leading to tiny Fermi surface pockets. Moreover, the bands forming the cone show an anisotropic leading edge gap away from the cone that suggests a nodal spin-density-wave description.

cond-mat.supr-con↗

arXiv2009

Angle-Resolved Photoemission Spectroscopy of Iron-Chalcogenide Superconductor Fe1.03Te0.7Se0.3 : Strong-Coupling Superconductivity and Universality of Inter-Band Scattering

We have performed high-resolution angle-resolved photoemission spectroscopy of iron-chalcogenide superconductor Fe1.03Te0.7Se0.3 (Tc = 13 K) to investigate the electronic structure relevant to superconductivity. We observed a hole- and an electron-like Fermi surfaces at the Brillouin zone center and corner, respectively, which are nearly nested by the Q~(pi, pi) wave vector. We do not find evidence for the nesting instability with Q~(pi+delta, 0) reminiscent of the antiferromagnetic order in the parent compound Fe1+yTe. We have observed an isotropic superconducting gap along the hole-like Fermi surface with the gap size Delta of ~4 meV (2Delta/kBTc~7), demonstrating the strong-coupling nature of the superconductivity. The observed similarity of low-energy electronic excitations between iron-chalcogenide and iron-arsenide superconductors strongly suggests that common interactions which involve Q~(pi, pi) scattering are responsible for the superconducting pairing.

cond-mat.supr-con↗

arXiv2009

Fermi surface nesting induced strong pairing in iron-based superconductors

The discovery of high-temperature superconductivity in iron pnictides raised the possibility of an unconventional superconducting mechanism in multiband materials. The observation of Fermi-surface(FS)-dependent nodeless superconducting gaps suggested that inter-FS interactions may play a crucial role in superconducting pairing. In the optimally hole-doped Ba$_{0.6}$K$_{0.4}$Fe$_2$As$_2$, the pairing strength is enhanced simultaneously (2$Δ$/Tc$\sim$7) on the nearly nested FS pockets, i.e. the inner holelike ($α$) FS and the two hybridized electronlike FSs, while the pairing remains weak (2$Δ$/Tc$\sim$3.6) in the poorly-nested outer hole-like ($β$) FS. Here we report that in the electron-doped BaFe$_{1.85}$Co$_{0.15}$As$_2$ the FS nesting condition switches from the $α$ to the $β$ FS due to the opposite size changes for hole- and electron-like FSs upon electron doping. The strong pairing strength (2$Δ$/Tc$\sim$6) is also found to switch to the nested $β$ FS, indicating an intimate connection between FS nesting and superconducting pairing, and strongly supporting the inter-FS pairing mechanism in the iron-based superconductors.

cond-mat.supr-con↗

arXiv2009

Superconducting gap symmetry of Ba0.6K0.4Fe2As2 studied by angle-resolved photoemission spectroscopy

We have performed high-resolution angle-resolved photoemission spectroscopy on the optimally-doped Ba$_{0.6}$K$_{0.4}$Fe$_2$As$_2$ compound and determined the accurate momentum dependence of the superconducting (SC) gap in four Fermi-surface sheets including a newly discovered outer electron pocket at the M point. The SC gap on this pocket is nearly isotropic and its magnitude is comparable ($Δ$ $\sim$ 11 meV) to that of the inner electron and hole pockets ($\sim$12 meV), although it is substantially larger than that of the outer hole pocket ($\sim$6 meV). The Fermi-surface dependence of the SC gap value is basically consistent with $Δ$($k$) = $Δ$$_0$cos$k_x$cos$k_y$ formula expected for the extended s-wave symmetry. The observed finite deviation from the simple formula suggests the importance of multi-orbital effects.

cond-mat.supr-con↗

arXiv2009

Electronic structure of heavily electron-doped BaFe$_{1.7}$Co$_{0.3}$As$_2$ studied by angle-resolved photoemission

We have performed high-resolution angle-resolved photoemission spectroscopy on heavily electron-doped non-superconducting (SC) BaFe$_{1.7}$Co$_{0.3}$As$_2$. We find that the two hole Fermi surface pockets at the zone center observed in the hole-doped superconducting Ba$_{0.6}$K$_{0.4}$Fe$_2$As$_2$ are absent or very small in this compound, while the two electron pockets at the M point significantly expand due to electron doping by the Co substitution. Comparison of the Fermi surface between non-SC and SC samples indicates that the coexistence of hole and electron pockets connected via the antiferromagnetic wave vector is essential in realizing the mechanism of superconductivity in the iron-based superconductors.

cond-mat.supr-con↗

arXiv2008

Electronic structure of optimally doped pnictide Ba$_{0.6}$K$_{0.4}$Fe$_2$As$_2$: a comprehensive ARPES investigation

We have conducted a comprehensive angle-resolved photoemission study on the normal state electronic structure of the Fe-based superconductor Ba$_{0.6}$K$_{0.4}$Fe$_2$As$_2$. We have identified four dispersive bands which cross the Fermi level and form two hole-like Fermi surfaces around $Γ$ and two electron-like Fermi surfaces around M. There are two nearly nested Fermi surface pockets connected by an antiferromagnetic ($π$, $π$) wavevector. The observed Fermi surfaces show small $k_z$ dispersion and a total volume consistent with Luttinger theorem. Compared to band structure calculations, the overall bandwidth is reduced by a factor of 2. However, many low energy dispersions display stronger mass renormalization by a factor of $\sim$ 4, indicating possible orbital (energy) dependent correlation effects. Using an effective tight banding model, we fitted the band structure and the Fermi surfaces to obtain band parameters reliable for theoretical modeling and calculations of the important physical quantities, such as the specific heat coefficient.

cond-mat.supr-con↗

arXiv2008

Band Structure and Fermi Surface of an Extremely Overdoped Iron-Based Superconductor KFe2As2

We have performed high-resolution angle-resolved photoemission spectroscopy on heavily overdoped KFe_2As_2 (transition temperature (Tc = 3 K). We observed several renormalized bands near the Fermi level with a renormalization factor of 2-4. While the Fermi surface (FS) around the Brillouin-zone center is qualitatively similar to that of optimally-doped Ba_{1-x}K_xFe_2As_2 (x = 0.4; Tc = 37 K), the FS topology around the zone corner (M point) is markedly different: the two electron FS pockets are completely absent due to excess of hole doping. This result indicates that the electronic states around the M point play an important role in the high-Tc superconductivity of Ba$_{1-x}$K$_x$Fe$_2$As$_2$ and suggests that the interband scattering via the antiferromagnetic wave vector essentially controls the Tc value in the overdoped region.

cond-mat.supr-con↗

arXiv2008

Observation of an Orbital Selective Electron-Mode Coupling in Fe-Based High-$T_c$ Superconductors

We have performed an angle-resolved photoemission spectroscopy study of the new superconductor Ba$_{0.6}$K$_{0.4}$Fe$_2$As$_2$ in the low energy range. We report the observation of an anomaly around 25 meV in the dispersion of superconducting Ba$_{0.6}$K$_{0.4}$Fe$_2$As$_2$ samples that nearly vanishes above $T_c$. The energy scale of the related mode (13$\pm$2 meV) and its strong dependence on orbital and temperature indicates that it is unlikely related to phonons. Moreover, the momentum locations of the kink can be connected by the antiferromagnetic wavevector. Our results point towards an unconventional electronic origin of the mode and the superconducting pairing in the Fe-based superconductors, and strongly support the anti-phase s-wave pairing symmetry.

cond-mat.supr-con↗

arXiv2008

Observation of a novel orbital selective Mott transition in Ca$_{1.8}$Sr$_{0.2}$RuO$_4$

Electrons in a simple correlated system behave either as itinerant charge carriers or as localized moments. However, there is growing evidence for the coexistence of itinerant electrons and local moments in transition metals with nearly degenerate $d$-orbitals. It demands one or more selective electron orbitals undergo the Mott transition while the others remain itinerant. Here we report the first observation of such an orbital selective Mott transition (OSMT) in Ca$_{1.8}$Sr$_{0.2}$RuO$_4$ by angle-resolved photoemission spectroscopy (ARPES). While we observed two sets of dispersing bands and Fermi surface associated with the doubly-degenerate $d_{yz}$ and $d_{zx}$ orbitals, the Fermi surface associated with the wider $d_{xy}$ band is missing, a consequence of selective Mott localization. Our theoretical calculations demonstrate that this novel OSMT is mainly driven by the combined effects of interorbital carrier transfer, superlattice potential, and orbital degeneracy, whereas the bandwidth difference plays a less important role.

cond-mat.str-el↗

arXiv2008

Coexistence of competing orders with two energy gaps in real and momentum space in high-Tc superconductor Bi2Sr2-xLaxCuO6+delta

The superconducting phase of the high-Tc cuprates has been thought to be described by a single d-wave pairing order parameter. Recently, there has been growing evidence suggesting that another form of order, possibly inherited from the pseudogap phase above Tc, may coexist with superconductivity in the underdoped regime. Through a combined study of scanning tunneling microscopy and angle-resolved photoemission spectroscopy, we report the observation of two distinct gaps (a small-gap and a large-gap) that coexist both in real space and in the anti-nodal region of momentum space in the superconducting phase of Bi2Sr2-xLaxCuO6+delta. We show that the small-gap is associated with superconductivity. The large-gap persists to temperatures above the transition temperature Tc and is found to be linked to short-range charge ordering. Remarkably, we find a strong, short-ranged correlation between the local small- and large- gap magnitudes suggesting that the superconductivity and charge ordering are affected by similar physical processes.

cond-mat.str-el↗

arXiv2008

Observation of Fermi-surface-dependent nodeless superconducting gaps in Ba0.6K0.4Fe2As2

The recent discovery of superconductivity in iron-arsenic compounds below a transition temperature (Tc) as high as 55K ended the monopoly of copper oxides (cuprates) in the family of high-Tc superconductors. A critical issue in understanding this new superconductor, as in the case of cuprates, is the nature, in particular the symmetry and orbital dependence, of the superconducting gap. There are conflicting experimental results, mostly from indirect measurements of the low energy excitation gap, ranging from one gap to two gaps, from line nodes to nodeless gap function in momentum space. Here we report a direct observation of the superconducting gap, including its momentum, temperature, and Fermi surface (FS) dependence in Ba0.6K0.4Fe2As2 (Tc = 37 K) using angle-resolved photoelectron spectroscopy. We find two superconducting gaps with different values: a large gap (~ 12 meV) on the two small hole-like and electron-like FS sheets, and a small gap (~ 6 meV) on the large hole-like FS. Both gaps, closing simultaneously at the bulk Tc, are nodeless and nearly isotropic around their respective FS sheets. The isotropic pairing interactions are strongly orbital dependent, as the ratio 2Delta/kBTc switches from weak to strong coupling on different bands. The same and surprisingly large superconducting gap due to strong pairing on the two small FS, which are connected by the (pi, 0) spin-density-wave vector in the parent compound, strongly suggests that the pairing mechanism originates from the inter-band interactions between these two nested FS sheets.

cond-mat.supr-con↗

arXiv2008

A distinct bosonic mode in an electron-doped high-transition-temperature superconductor

Despite recent advances in understanding high-transition-temperature (high-T c) superconductors, there is no consensus on the origin of the superconducting 'glue': that is, the mediator that binds electrons into superconducting pairs. The main contenders are lattice vibrations (phonons) and spin-excitations with the additional possibility of pairing without mediators. In conventional superconductors, phonon-mediated pairing was unequivocally established by data from tunnelling experiments. Proponents of phonons as the high-T c glue were therefore encouraged by the recent scanning tunnelling microscopy experiments on hole-doped Bi2Sr2CaCu2O8-delta (BSCCO) that reveal an oxygen lattice vibrational mode whose energy is anticorrelated with the superconducting gap energy scale. Here we report high-resolution scanning tunnelling microscopy measurements of the electron-doped high-T c superconductor Pr0.88LaCe0.12CuO4 (PLCCO) (T c = 24 K) that reveal a bosonic excitation (mode) at energies of 10.5 plus/minus 2.5 meV. This energy is consistent with both spin-excitations in PLCCO measured by inelastic neutron scattering (resonance mode) and a low-energy acoustic phonon mode, but differs substantially from the oxygen vibrational mode identified in BSCCO. Our analysis of the variation of the local mode energy and intensity with the local gap energy scale indicates an electronic origin of the mode consistent with spin-excitations rather than phonons.

cond-mat.supr-con↗