arXiv subjects

H. Eisaki

Publications and source records attributed to H. Eisaki.

At least 217 records · Page 12Linked to original sources

arXiv2004

Normal State Spectral Lineshapes of Nodal Quasiparticles in Single Layer Bi2201 Superconductor

A detailed study of the normal state photoemission lineshapes and quasiparticle dispersion for the single layer Bi$_2$Sr$_{2-x}$La$_x$CuO$_{6+δ}$ (Bi2201) superconductor is presented. We report the first experimental evidence of a double peak structure and a dip of spectral intensity in the energy distribution curves (EDCs) along the nodal direction. The double peak structure is well identified in the normal state, up to ten times the critical temperature. As a result of the same self-energy effect, a strong mass renormalization of the quasiparticle dispersion, i.e. kink, and an increase of the quasiparticle lifetime in the normal state are also observed. Our results provide unambiguous evidence on the existence of bosonic excitation in the normal state, and support a picture where nodal quasiparticles are strongly coupled to the lattice.

cond-mat.supr-con↗

arXiv2004

Marginal Fermi liquid analysis of 300 K reflectance of Bi2Sr2CaCu2O8+x

We use 300 K reflectance data to investigate the normal-state electrodynamics of the high temperature superconductor Bi$_{2}$Sr$_{2}$CaCu$_{2}$O$_{8+δ}$ over a wide range of doping levels. The data show that at this temperature the free carriers are coupled to a continuous spectrum of fluctuations. Assuming the Marginal Fermi Liquid (MFL) form as a first approximation for the fluctuation spectrum, the doping-dependent coupling constant $λ(p)$ can be estimated directly from the slope of the reflectance spectrum. We find that $λ(p)$ decreases smoothly with the hole doping level, from underdoped samples with $ p=0.103$ ($T_c = 67$ K) where $λ(p)= 0.93$ to overdoped samples with $p=0.226$, ($T_c= 60$ K) where $λ(p)= 0.53$. An analysis of the intercept and curvature of the reflectance spectrum shows deviations from the MFL spectrum symmetrically placed at the optimal doping point $p=0.16$. The Kubo formula for the conductivity gives a better fit to the experiments with the MFL spectrum up to 2000 cm$^{-1}$ and with an additional Drude component or an additional Lorentz component up to 7000 cm$^{-1}$. By comparing three different model fits we conclude that the MFL channel is necessary for a good fit to the reflectance data. Finally, we note that the monotonic variation of the reflectance slope with doping provides us with an independent measure of the doping level for the Bi-2212 system.

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arXiv2004

Mutual Experimental and Theoretical Validation of Bulk Photoemission Spectra of Sr1-xCaxVO3

We report high-resolution high-energy photoemission spectra together with parameter-free LDA+DMFT (local density approximation + dynamical mean-field theory) results for Sr1-xCaxVO3, a prototype 3d1 system. In contrast to earlier investigations the bulk spectra are found to be insensitive to x. The good agreement between experiment and theory confirms the bulk-sensitivity of the high-energy photoemission spectra.

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arXiv2004

Superconducting order parameter in heavily overdoped $Bi_2 Sr_2 Ca Cu_2 O_{8+δ}$: a global quantitative analysis

A systematic analysis of the complex lineshape at $(π,0)$ of heavily overdoped Bi$_2$Sr$_2$CaCu$_2$O$_{8+δ}$ is presented. We show that a coherent component in the quasi-particle excitation is correlated with the superfluid density throughout the entire doping range and suggest it is a direct measure of the order parameter of high temperature superconductors.

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arXiv2004

Asymmetries in the electron-hole pair dynamics and strong Mott pseudogap effect in the phase diagram of cuprates

Electron behavior in doped Mott systems continues to be a major unsolved problem in quantum many-electron physics. A central issue in understanding the universal Mott behavior in a variety of complex systems is to understand the nature of their electron-hole pair excitation modes. Using high resolution resonant inelastic x-ray scattering (RIXS) we resolve the momentum dependence of electron-hole pair excitations in two major classes of doped copper oxides which reveals a Mott pseudogap over the full Brillouin zone and over the entire phase diagram. The pair bandwidth and zone-boundary pair velocity renormalize on either sides of the phase diagram at very different rates indicating strong particle-hole doping asymmetries observed for the first time.

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arXiv2004

Coupling Of The B1g Phonon To The Anti-Nodal Electronic States of Bi2Sr2Ca0.92Y0.08Cu2O(8+delta)

Angle-resolved photoemission spectroscopy (ARPES) on optimally doped Bi2Sr2Ca0.92Y0.08Cu2O(8+delta) uncovers a coupling of the electronic bands to a 40 meV mode in an extended k-space region away from the nodal direction, leading to a new interpretation of the strong renormalization of the electronic structure seen in Bi2212. Phenomenological agreements with neutron and Raman experiments suggest that this mode is the B1g oxygen bond-buckling phonon. A theoretical calculation based on this assignment reproduces the electronic renormalization seen in the data.

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arXiv2004

Destruction of antinodal state coherence via `checkerboard' charge ordering in strongly underdoped superconducting BSCCO-2212

Microscopy (STM). At all dopings, the low energy density-of-states modulations are analyzed according to a simple model of quasiparticle interference and found to be consistent with Fermi-arc superconductivity. The superconducting coherence-peaks, ubiquitous in near-optimal tunneling spectra, are destroyed with strong underdoping and a new spectral type appears. Exclusively in regions exhibiting this new spectrum, we find local `checkerboard' charge-order with wavevector Q=(2pi/4.5a,0);(0,2pi/4.5a)+15%. Surprisingly, this order coexists harmoniously with the the low energy

cond-mat.supr-con↗

arXiv2004

Homogenous nodal superconductivity coexisting with inhomogeneous charge order in strongly underdoped Bi-2212

We use novel STM techniques in concert to study the doping dependence of electronic structure in Bi-2212. At all dopings, the low energy states are relatively homogenous except for dispersive density-of-states modulations whose properties are used to elucidate the momentum-space characteristics of quasi-particles. The superconductive coherence-peaks, ubiquitous in near-optimal tunneling spectra, are destroyed with strong underdoping. A new spectral type, likely characteristic of the zero temperature pseudogap regime, appears in these samples. Exclusively in regions exhibiting this new spectrum, we find a quasi periodic modulations in dI/dV as well as in topograph with Q(2pi/4.5a,0) and (0,2pi/4.5a)+-15%. This is consistent with the existence of a local charge density modulation at these wave vectors. Surprisingly, this state coexists harmoniously with the low energy nodal quasi-particles. We discuss the relevance of these findings to the cuprate phase diagram and to the relationship between the pseudogap and superconductivity.

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arXiv2004

Site-Dilution in quasi one-dimensional antiferromagnet Sr2(Cu1-xPdx)O3: reduction of Neel Temperature and spatial distribution of ordered moment sizes

We investigate the Neel temperature of Sr2CuO3 as a function of the site dilution at the Cu (S=1/2) sites with Pd (S=0), utilizing the muon spin relaxation (muSR) technique. The Neel temperature, which is Tn=5.4K for the undoped system, becomes significantly reduced for less than one percent of doping Pd, giving a support for the previous proposal for the good one-dimensionality. The Pd concentration dependence of the Neel temperature is compared with a recent theoretical study (S. Eggert, I. Affleck and M.D.P. Horton, Phys. Rev. Lett. 89, 47202 (2002)) of weakly coupled one-dimensional antiferromagnetic chains of S=1/2 spins, and a quantitative agreement is found. The inhomogeneity of the ordered moment sizes is characterized by the muSR time spectra. We propose a model that the ordered moment size recovers away from the dopant S=0 sites with a recovery length of ξ= 150-200 sites. The origin of the finite recovery length ξfor the gapless S=1/2 antiferromagnetic chain is compared to the estimate based on the effective staggered magnetic field from the neighboring chains.

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arXiv2004

The Dichotomy between Nodal and Antinodal Quasiparticles in Underdoped (La$_{2-x}$Sr$_x$)CuO$_4$ Superconductors

High resolution angle-resolved photoemission measurements on underdoped (La$_{2-x}$Sr$_x$)CuO$_4$ system show that, at energies below 70 meV, the quasiparticle peak is well defined around the ($π$/2,$π$/2) nodal region and disappears rather abruptly when the momentum is changed from the nodal point to the ($π$,0) antinodal point along the underlying ``Fermi surface''. It indicates that there is an extra low energy scattering mechanism acting upon the antinodal quasiparticles. We propose that this mechanism is the scattering of quasiparticles across the nearly parallel segments of the Fermi surface near the antinodes.

cond-mat.str-el↗

arXiv2004

Thermodynamic and transport properties of underdoped cuprates from ARPES data

he relationship between photoemission spectra of high-$T_{\textrm{c}}$ cuprates and their thermodynamic and transport properties are discussed. The doping dependence of the expected quasi-particle density at the Fermi level ($E_\mathrm{F}$) are compared with the electronic specific heat coefficient $γ$ and that of the spectral weight at $E_\mathrm{F}$ with the in-plane and out-of-plane superfluid density. We have estimated the electrical resistivity of underdoped cuprates from the momentum distribution curve (MDC) at $E_\mathrm{F}$ in the nodal direction. The temperature dependence of the MDC width is also consistent with that of the electrical resistivity.

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arXiv2003

Effect of chemical inhomogeneity in the bismuth-based copper oxide superconductors

We examine the effect on the superconducting transition temperature (Tc) of chemical inhomogeneities in Bi2201 and Bi2212 single crystals. Cation disorder at the Sr crystallographic site is inherent in these materials and strongly affects the value of Tc. Partial substitution of Sr by Ln (Ln = La, Pr, Nd, Sm, Eu, Gd, and Bi) in Bi_{2}Sr_{1.6}Ln_{0.4}CuO_{6} results in a monotonic decrease of Tc with increasing ionic radius mismatch. By minimizing Sr site disorder at the expense of Ca site disorder, we demonstrate that the Tc of Bi2212 can be increased to 96 K. Based on these results we discuss the effects of chemical inhomogeneity in other bulk high-temperature superconductors.

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arXiv2003

Effects of next-nearest-neighbor hopping $t^{\prime}$ on the electronic structure of cuprates

Photoemission spectra of underdoped and lightly-doped Bi$_{2-z}$Pb$_z$Sr$_2$Ca$_{1-x}${\it R}$_{x}$Cu$_2$O$_{8+y}$ ($R=$ Pr, Er) (BSCCO) have been measured and compared with those of La$_{2-x}$Sr$_x$CuO$_4$ (LSCO). The lower-Hubbard band of the insulating BSCCO, like Ca$_2$CuO$_2$Cl$_2$, shows a stronger dispersion than La$_2$CuO$_4$ from ${\bf k}\sim$($π/2,π/2$) to $\sim$($π,0$). The flat band at ${\bf k}\sim$($π,0$) is found generally deeper in BSCCO. These observations together with the Fermi-surface shapes and the chemical potential shifts indicate that the next-nearest-neighbor hopping $|t^{\prime}|$ of the single-band model is larger in BSCCO than in LSCO and that $|t^{\prime}|$ rather than the super-exchange $J$ influences the pseudogap energy scale.

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arXiv2003

Genuine Electronic States of Vanadium Perovskites Revealed by High-Energy Photoemission

Bulk-sensitive high-resolution photoemission was carried out on a prototype 3d1 metallic Sr1-xCaxVO3. In a strong contrast to so far reported results, the bulk spectral functions are revealed to be insensitive to x. The conservation of the density of states at the Fermi level in spite of the electron correlation is clarified by the successful suppression and deconvolution of the surface contribution. Our study has demonstrated the importance of high-energy and high-resolution photoemission spectroscopy for revealing detailed bulk electronic states of transition metal oxides.

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arXiv2003

Fully Gapped Single-Particle Excitations in the Lightly Doped Cuprates

The low-energy excitations of the lightly doped cuprates were studied by angle-resolved photoemission spectroscopy. A finite gap was measured over the entire Brillouin zone, including along the d_{x^2 - y^2} nodal line. This effect was observed to be generic to the normal states of numerous cuprates, including hole-doped La_{2-x}Sr_{x}CuO_{4} and Ca_{2-x}Na_{x}CuO_{2}Cl_{2} and electron-doped Nd_{2-x}Ce_{x}CuO_{4}. In all compounds, the gap appears to close with increasing carrier doping. We consider various scenarios to explain our results, including the possible effects of chemical disorder, electronic inhomogeneity, and a competing phase.

cond-mat.supr-con↗

arXiv2003

Powerlaw optical conductivity with a constant phase angle in high Tc superconductors

In certain materials with strong electron correlations a quantum phase transition (QPT) at zero temperature can occur, in the proximity of which a quantum critical state of matter has been anticipated. This possibility has recently attracted much attention because the response of such a state of matter is expected to follow universal patterns defined by the quantum mechanical nature of the fluctuations. Forementioned universality manifests itself through power-law behaviours of the response functions. Candidates are found both in heavy fermion systems and in the cuprate high Tc superconductors. Although there are indications for quantum criticality in the cuprate superconductors, the reality and the physical nature of such a QPT are still under debate. Here we identify a universal behaviour of the phase angle of the frequency dependent conductivity that is characteristic of the quantum critical region. We demonstrate that the experimentally measured phase angle agrees precisely with the exponent of the optical conductivity. This points towards a QPT in the cuprates close to optimal doping, although of an unconventional kind.

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arXiv2003

Nodal metallic behavior of lightly-doped La$_{2-x}$Sr$_x$CuO$_4$

Lightly-doped La$_{2-x}$Sr$_x$CuO$_4$ in the so-called "insulating" spin-glass/diagonal-stripe phase has been studied by angle-resolved photoemission spectroscopy. A quasi-particle (QP) peak crossing the Fermi level has been observed in the node direction of the d-wave superconducting gap, forming an "arc" of Fermi surface consistent with the recently observed metallic transport behavior at high temperatures of lightly-doped materials. The spectral weight of the nodal QP smoothly increases with hole doping, corresponding to the $n \sim x$ behavior of the carrier number in the underdoped and lightly-doped regions.

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arXiv2003

Sliding conduction by the quasi one-dimensional charge-ordered state in Sr$_{14-x}$Ca$_x$Cu$_{24}$O$_{41}$

Nonlinear conduction (NLC) of the two-leg spin ladder, Sr$_{14-x}$Ca$_x$Cu$_{24}$O$_{41}$, was investigated for the $x$=0, 1 and 12 materials . Although insulating materials ($x$=0 and 1) exibited the NLC both in the ladder- and rung directions, the NLC in the ladder direction of the $x$=0-material was found to be very special. We considered this to be due to the sliding motion of the charge ordered state, which was responsible for the resonance at microwave frequencies. We discussed possible candidates for the charge ordered state responsible for the NLC, including Wigner crystal in quasi one dimension (4$k_F$-CDW).

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