arXiv subjects

H. Ishiyama

Publications and source records attributed to H. Ishiyama.

8 recordsLinked to original sources

arXiv2026

New Ground State in ${}^{149}$La Removes Two-Neutron-Separation-Energy Anomaly in Lanthanum Isotopes

Nuclear mass is a key indicator of how the nuclear shell structure evolves. The recent mass measurement study of neutron-rich lanthanum isotopes [A. Jaries, $et~al$., Phys. Rev. Lett. {\bf 134}, 042501(2025)] reveals the presence of a distinct prominence in their two-neutron separation energies. However, its presence has been called into question based on the results of another mass determination [B. Liu, Ph.D. thesis, University of Notre Dame (2025)]. In this letter, we report an effort to clarify these contradictory results through the use of the simultaneous mass-lifetime measurement of the neutron-rich lanthanum isotope ${}^{149}$La using a multi-reflection time-of-flight mass spectrograph combined with a $β$-TOF detector. The peak corresponding to a $β$-decaying state was observed in the time-of-flight spectra at a position of $221(6)~{\rm keV/c^2}$ lighter than the reported ${}^{149}$La mass in A. Jaries, $et~al$., but our measured result is in excellent agreement with the mass value reported in B. Liu. We have concluded that this peak is the ground state of ${}^{149}$La. With this, the previously reported distinct prominence in the two-neutron separation energies disappears, while a new kink structure, similar to that in the cerium isotopes, appears. Comparison with theoretical models suggests that a nuclear shape transition from octupole deformation to another type of deformation occurs around $N=91$ and is likely the cause of this kink structure.

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arXiv2026

High-Precision Mass Measurements of Proton-Rich Rh, Pd, Cd isotopes in the vicinity of 100Sn and Impact on X-Ray Burst and Supernova Nucleosynthesis

Using the ZeroDegree multi-reflection time-of-flight mass spectrograph of the CRISMASS project at RIKEN Radioactive Isotope Beam Factory, we performed high-precision mass measurements of proton-rich nuclei near the doubly magic nucleus 100Sn, achieving uncertainties on the order of 10 keV. The masses of 91Rh, 92Pd, and 96Cd were determined for the first time with high precision, and the accuracy of several additional masses was substantially improved. Incorporating the new data into X-ray burst simulations significantly reduces the abundance uncertainties in the $A$ = 90-100 region, shifting the reaction flow toward $A$ = 90 production and suppressing the synthesis of heavier nuclei. Further investigation of the $νp$-process indicates that 99Rh plays a significant role in the reaction flow within the mass region studied. These high-precision mass measurements refine the mass surface near 100Sn and provide critical constraints on models of proton-rich nucleosynthesis.

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arXiv2025

Precision mass measurements around ${}^{84}$Mo rule out ZrNb cycle formation in the rapid proton-capture process at type I X-ray bursts

The rapid proton-capture ($rp$-) process is one of the primary, explosive thermonuclear burning processes that drive type I X-ray bursts. A possible termination of the $rp$-process at around ${}^{84}$Mo was previously suggested by the formation of a ZrNb cycle. We report here precision mass measurements at around ${}^{84}$Mo, which have concluded the possibility of the cycle. The experiment was conducted using the multi-reflection time-of-flight spectrograph at RIKEN RI Beam Factory, and the masses of ${}^{79}$Y, ${}^{83}$Nb, ${}^{84}$Mo, ${}^{88}$Ru, and an isomer in ${}^{78}$Y were measured. For ${}^{84}$Mo, and ${}^{88}$Ru, and the isomeric state of ${}^{78}$Y, their masses are experimentally determined for the first time with uncertainties of $δm \approx 20~{\rm keV/c^2}$. The mass precision of ${}^{79}$Y and ${}^{83}$Nb is improved to $13~{\rm keV/c^2}$ and $9.6~{\rm keV/c^2}$, respectively. The new $α$-separation energy of ${}^{84}$Mo, 1.434(83) MeV, unambiguously rules out the possibility of forming the ZrNb cycle. The X-ray burst simulation with the new masses shows that our measurements effectively remove the large final abundance uncertainties in the $A=80-90$ mass region. The new mass values improve the prediction power for the composition of the nuclear ashes in X-ray bursts.

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arXiv2022

A new study of the $N=32$ and $N=34$ shell gap for Ti and V by the first high-precision MRTOF mass measurements at BigRIPS-SLOWRI

The atomic masses of $^{55}$Sc, $^{56,58}$Ti, and $^{56-59}$V have been determined using the high-precision multi-reflection time-of-flight technique. The radioisotopes have been produced at RIKEN's RIBF facility and delivered to the novel designed gas cell and multi-reflection system (ZD MRTOF), which has been recently commissioned downstream of the ZeroDegree spectrometer following the BigRIPS separator. For $^{56,58}$Ti and $^{56-59}$V the mass uncertainties have been reduced down to the order of $10\,\mathrm{keV}$, shedding new light on the $N=34$ shell effect in Ti and V isotopes by the first high-precision mass measurements of the critical species $^{58}$Ti and $^{59}$V. With the new precision achieved, we reveal the non-existence of the $N=34$ empirical two-neutron shell gaps for Ti and V, and the enhanced energy gap above the occupied $νp_{3/2}$ orbit is identified as a feature unique to Ca. We perform new Monte Carlo shell model calculations including the $νd_{5/2}$ and $νg_{9/2}$ orbits and compare the results with conventional shell model calculations, which exclude the $νg_{9/2}$ and the $νd_{5/2}$ orbits. The comparison indicates that the shell gap reduction in Ti is related to a partial occupation of the higher orbitals for the outer two valence neutrons at $N=34$.

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arXiv2022

The new MRTOF mass spectrograph following the ZeroDegree spectrometer at RIKEN's RIBF facility

A newly assembled multi-reflection time-of-flight mass spectrograph (MRTOF-MS) at RIKEN's RIBF facility became operational for the first time in spring 2020; further modifications and performance tests using stable ions were completed in early 2021. By using a pulsed-drift-tube technique to modify the ions' kinetic energy in a wide range, we directly characterize the dispersion function of the system for use in a new procedure for optimizing the voltages applied to the electrostatic mirrors. Thus far, a mass resolving power of $R_m > 1\,000\,000$ is reached within a total time-of-flight of only $12.5\,\mathrm{ms}$, making the spectrometer capable of studying short-lived nuclei possessing low-lying isomers. Detailed information about the setup and measurement procedure is reported, and an alternative in-MRTOF ion selection scheme to remove molecular contaminants in the absence of a dedicated deflection device is introduced. The setup underwent an initial on-line commissioning at the BigRIPS facility at the end of 2020, where more than 70 nuclear masses have been measured. A summary of the commissioning experiments and results from a test of mass accuracy will be presented.

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arXiv2021

Alpha-decay-correlated mass measurement of 206,207Ra using an $α$-TOF detector equipped MRTOF-MS system

The atomic masses of the isotopes $^{206,207}$Ra have been measured via decay-correlated mass spectroscopy using a multi-reflection time-of-flight mass spectrograph equipped with an $α$-TOF detector. The Ra isotopes were produced as fusion-evaporation products in the $^{51}$V+$^{159}$Tb reaction system and delivered by the gas-filled recoil ion separator GARIS-II at RIKEN. The $α$-TOF detector provides for high-accuracy mass measurements by correlating time-of-flight signals with subsequent $α$-decay events. The masses of $^{206}$Ra and $^{207g,m}$Ra were directly measured using a multi-reflection time-of-flight mass spectrograph equipped with an $α$-TOF detector. A mass excess of ME = 3538(15) keV/c$^2$ and an excitation energy of E$_{\rm ex}$ = 552(42) keV were determined. The $α$-decay branching ratio of $^{207m}$Ra, b$α$ = 0.26(20), was directly determined from decay-correlated time-of-flight signals, and the reduced alpha width of $^{207m}$Ra was calculated to be $δ^2$ = 50+62-41 keV from the branching ratio. The spin-parity of $^{207m}$Ra was confirmed to be $J^π$ = 13/2$^-$ from decay correlated mass measurement results.

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arXiv2021

First high-precision direct determination of the atomic mass of a superheavy nuclide

We present the first direct measurement of the atomic mass of a superheavy nuclide. Atoms of $^{257}$Db ($Z$=105) were produced online at the RIKEN Nishina Center for Accelerator-Based Science using the fusion-evaporation reaction $^{208}$Pb($^{51}$V, 2n)$^{257}$Db. The gas-filled recoil ion separator GARIS-II was used to suppress both the unreacted primary beam and some transfer products, prior to delivering the energetic beam of $^{257}$Db ions to a helium gas-filled ion stopping cell wherein they were thermalized. Thermalized $^{257}$Db$^{3+}$ ions were then transferred to a multi-reflection time-of-flight mass spectrograph for mass analysis. An alpha particle detector embedded in the ion time-of-flight detector allowed disambiguation of the rare $^{257}$Db$^{3+}$ time-of-flight detection events from background by means of correlation with characteristic $α$-decays. The extreme sensitivity of this technique allowed a precision atomic mass determination from 11 events. The mass excess was determined to be $100\,063(231)_\textrm{stat}(132)_\textrm{sys}$~keV/c$^2$. Comparing to several mass models, we show the technique can be used to unambiguously determine the atomic number as $Z$=105 and should allow similar evaluations for heavier species in future work.

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arXiv2012

Development of a resonant laser ionization gas cell for high-energy, short-lived nuclei

A new laser ion source configuration based on resonant photoionization in a gas cell has been developed at RIBF RIKEN. This system is intended for the future PArasitic RI-beam production by Laser Ion-Source (PALIS) project which will be installed at RIKEN's fragment separator, BigRIPS. A novel implementation of differential pumping, in combination with a sextupole ion beam guide (SPIG), has been developed. A few small scroll pumps create a pressure difference from 1000 hPa - 10^-3 Pa within a geometry drastically miniaturized compared to conventional systems. This system can utilize a large exit hole for fast evacuation times, minimizing the decay loss for short-lived nuclei during extraction from a buffer gas cell, while sufficient gas cell pressure is maintained for stopping high energy RI-beams. In spite of the motion in a dense pressure gradient, the photo-ionized ions inside the gas cell are ejected with an assisting force gas jet and successfully transported to a high-vacuum region via SPIG followed by a quadrupole mass separator. Observed behaviors agree with the results of gas flow and Monte Carlo simulations.

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