arXiv subjects

H. Okamoto

Publications and source records attributed to H. Okamoto.

32 records · Page 2Linked to original sources

arXiv2014

Terahertz radiation imaging of ferroelectric domain topology in room-temperature organic supramolecular ferroelectrics

We demonstrate a new method to detect ferroelectric domains in inside and surface regions of organic ferroelectrics by mapping out two orthogonally polarized terahertz waves radiated from the crystal upon the irradiation of near-infrared femtosecond laser pulses. We used polarization dependence of the effective depths radiating the terahertz waves, which originate from the optical anisotropy in the terahertz frequency region. This allows us to distinguish ferroelectric domains in the inside and surface regions of the crystals. We applied this method to a room-temperature organic supramolecular ferroelectric crystal, 1:1 salt of 5,5'-dimethyl-2,2'-bipyridine and deuterated iodanilic acid. A single domain covering almost all the area of an as-grown crystal ($\sim$600 $μ$m $\times$ 800 $μ$m) is discerned in the inside region, while complicated multi-domain in size of $\sim$ 200 $μ$m is observed in the surface region. By applying external electric field along the 2c-b axis (ferroelectric polarization direction), the polarization switching proceeds with successive propagations of uncharged (neutral) and quasi-one-dimensional 180$^\circ$ domain walls (DWs) along the b-axis ($\perp$ 2c-b axis). This results in the formation of another uncharged and two-dimensional 180$\circ$ DW parallel to the (100) plane, which covers all the area of the crystal. We discuss the usefulness of the present terahertz radiation imaging technique and ferroelectric DW dynamics in terms of anisotropic stacking of hydrogen-bonded chains.

cond-mat.mtrl-sci↗

arXiv2014

Elliptically polarized terahertz radiation from a chiral oxide

Polarization control of terahertz wave is a challenging subject in terahertz science and technology. Here, we report a simple method to control polarization state of the terahertz wave in terahertz generation process. At room temperature, terahertz radiation from a noncentrosymmetric and chiral oxide, sillenite Bi$_{12}$GeO$_{20}$, is observed by the irradiation of linearly polarized femtosecond laser pulses at 800 nm. The polarization state of the emitted terahertz wave is found to be elliptic with an ellipticity of $\sim$0.37$\pm$0.10. Furthermore, the ellipticity was altered to a nearly zero ($\sim$0.01$\pm$0.01) by changing the polarization of the incident linearly polarized femtosecond laser pulses. Such a terahertz radiation characteristic is attributable to variation of the polarization state of the emitted terahertz waves, which is induced by retardation due to the velocity mismatch between the incident femtosecond laser pulse and generated terahertz wave and by the polarization tilting due to the optical activity at 800 nm.

cond-mat.mtrl-sci↗

arXiv2014

Terahertz radiation by optical rectification in a hydrogen-bonded organic molecular ferroelectric crystal, 2-phenylmalondialdehyde

Terahertz radiation by optical rectification has been observed at room temperature in a hydrogen-bonded organic molecular ferroelectric crystal, 2-phenyl malondialdehyde (PhMDA). The radiated electromagnetic wave consisted of a single-cycle terahertz pulse with a temporal width of $\sim$ 0.5 ps. The terahertz radiation amplitude divided by the sample thickness in PhMDA was nearly equivalent to that in a typical terahertz wave emitter ZnTe. This is attributable to a long coherence length in the range of 130 $\sim$ 800 $μ$m for the terahertz radiation from PhMDA. We also discussed the possibility of PhMDA as a terahertz wave emitter in terms of the phase-matching condition.

cond-mat.mtrl-sci↗

arXiv2014

Visualization of ferroelectric domains in boracite using emission of terahertz radiation

We report on the emission of terahertz radiation by irradiation of femtosecond laser pulses in non-centrosymmetric paraelectric and ferroelectric phases of Co$_3$B$_7$O$_{13}$I boracite. The Generation of the terahertz waves in both phases is caused by optical rectification via a second-order nonlinear optical effect. In the ferroelectric phase, we successfully visualized ferroelectric domains by analyzing the polarization state of the terahertz wave radiated from the crystal. In a large area of the crystal ($\sim$ 500 $\times$ 500 $μ$m$^2$), the observed polarization vector of the radiated terahertz wave was tilted from directions of spontaneous polarization, i.e., [100]$_{\rm cub}$, [010]$_{\rm cub}$, and [001]$_{\rm cub}$ in cubic setting, which can be explained by the presence of a ferroelectric 90$^\circ$ domain wall of the (101)$_{\rm cub}$ plane.

cond-mat.mtrl-sci↗

arXiv2014

Terahertz radiation induced by coherent phonon generation via impulsive stimulated Raman scattering in paratellurite

We report on the observation of terahertz radiation in a non-centrosymmetric insulating oxide, paratellurite ($α$-TeO$_2$) by irradiation of a femtosecond laser pulse at room temperature. In the power spectrum of the terahertz radiation, an intensity fringe pattern with a period of $\sim$ 0.25 THz shows up below 3 THz. It can be reproduced by taking into account the effective generation length for the terahertz radiation with a poor phase-matching condition. In addition, a temporal oscillation component appears in the radiated terahertz wave with a frequency of $\sim$ 3.71 THz, which is in good agreement with the center frequency of the Raman active longitudinal optical (LO) $E$ mode. On the basis of comprehensive polarized optical and Raman spectroscopic studies, we explain the generation mechanism of the temporal oscillation component in terms of the coherent phonon generation via impulsive stimulated Raman scattering.

cond-mat.mtrl-sci↗

arXiv2014

Two-mode squeezing in an electromechanical resonator

The widespread availability of quantum entanglement with photons, in the guise of two-mode squeezed states, can be attributed to the phenomenon of parametric down-conversion. A reinterpretation of this effect with macroscopic mechanical objects can offer a route towards a purely mechanical entanglement and the unique possibility of probing the quantum mechanical nature of our everyday classical world. In spite of this prospect, mechanical two-mode squeezed states have remained elusive due to the inability to recreate the nonlinear interaction at the heart of this phenomenon in the mechanical domain. To address this we have developed a parametric down-converter, in a mechanical resonator integrated with electrical functionality, which enables mechanical nonlinearities to be dynamically engineered to emulate the parametric down-conversion interaction. In this configuration, phonons are simultaneously generated in pairs in two macroscopic vibration modes which results in the amplification of their motion. In parallel, mechanical two-mode squeezed states are also created which exhibit fluctuations far below the thermal level of their constituent modes as well as harbouring correlations between the modes that become almost perfect as their amplification is increased. This remarkable observation of correlations between two massive phonon ensembles paves the way towards an entangled macroscopic mechanical system at the single phonon level.

cond-mat.mes-hall↗

arXiv2012

Deconstructing the Hubbard Hamiltonian by Ultrafast Quantum Modulation Spectroscopy in Solid-state Mott Insulators

Most available theories for correlated electron transport are based on the Hubbard Hamiltonian. In this effective theory, renormalized hopping and interaction parameters only implicitly incorporate the coupling of correlated charge carriers to microscopic degrees of freedom. Unfortunately, no spectroscopy can individually probe such renormalizations, limiting the applicability of Hubbard models. We show here that the role of each individual degree of freedom can be made explicit by using a new experimental technique, which we term 'quantum modulation spectroscopy' and we demonstrate here in the one-dimensional Mott insulator ET-F2TCNQ. We explore the role on the charge hopping of two localized molecular modes, which we drive with a mid infrared optical pulse. Sidebands appear in the modulated optical spectrum, and their linshape is fitted with a model based on the dynamic Hubbard Hamiltonian. A striking asymmetry between the renormalization of doublons and holons is revealed. The concept of quantum modulation spectroscopy can be used to systematically deconstruct Hubbard Hamiltonians in many materials, exposing the role of any mode, electronic or magnetic, that can be driven to large amplitude with a light field.

cond-mat.str-el↗

arXiv2012

Performance of a 250L liquid Argon TPC for sub-GeV charged particle identification

We have constructed a liquid Argon TPC detector with fiducial mass of 150 kg as a part of the R&D program of the next generation neutrino and nucleon decay detector. This paper describes a study of particle identification performance of the detector using well-defined charged particles (pions, kaons, and protons) with momentum of ~800 MeV/$c$ obtained at J-PARC K1.1BR beamline.

physics.ins-det↗

arXiv2011

A tagged low-momentum kaon test-beam exposure with a 250L LAr TPC (J-PARC T32)

At the beginning of 2010, we presented at the J-PARC PAC an R$&$D program towards large (100 kton scale) liquid argon TPCs, suitable to investigate, in conjunction with the J-PARC neutrino beam, the possibility of CP violation in the neutrino sector and to search for nucleon decay. As a first step we proposed a test experiment to identify and measure charged kaons, including their decays, in liquid argon. The detector, a 250L LAr TPC, is exposed to charged kaons, in a momentum range of 540-800 MeV/c, in the K1.1BR beamline of the J-PARC slow extraction facility. This is especially important to estimate efficiency and background for nucleon decay searches in the charged kaon mode ($p \rightarrow \barν K^+$, etc.), where the kaon momentum is expected to be in the few hundred MeV/c range. A prototype setup has been exposed in the K1.1BR beamline in the fall of 2010. This paper describes the capabilities of the beamline, the construction and setting up of the detector prototype, along with some preliminary results.

physics.ins-det↗

arXiv2007

Controllable Coupling between Flux Qubit and Nanomechanical Resonator by Magnetic Field

We propose an active mechanism for coupling the quantized mode of a nanomechanical resonator to the persistent current in the loop of a superconducting Josephson junction (or phase slip) flux qubit. This coupling is independently controlled by an external coupling magnetic field. The whole system forms a novel solid-state cavity quantum electrodynamics (QED) architecture in the strong coupling limit. This architecture can be used to demonstrate quantum optics phenomena and coherently manipulate the qubit for quantum information processing. The coupling mechanism is applicable for more generalized situations where the superconducting Josephson junction system is a multi-level system.We also address the practical issues concerning experimental realization.

cond-mat.mes-hall↗

arXiv2005

Fine structure and magneto-optics of exciton, trion, and charged biexciton states in single InAs quantum dots emitting at 1.3 um

We present a detailed investigation into the optical characteristics of individual InAs quantum dots (QDs) grown by metalorganic chemical vapor deposition, with low temperature emission in the telecoms window around 1300 nm. Using micro-photoluminescence (PL) spectroscopy we have identified neutral, positively charged, and negatively charged exciton and biexciton states. Temperature-dependent measurements reveal dot-charging effects due to differences in carrier diffusivity. We observe a pronounced linearly polarized splitting of the neutral exciton and biexciton lines (~250 ueV) resulting from asymmetry in the QD structure. This asymmetry also causes a mixing of the excited trion states which is manifested in the fine structure and polarization of the charged biexciton emission; from this data we obtain values for the ratio between the anisotropic and isotropic electron-hole exchange energies of (Delta1)/(Delta0)= 0.2--0.5. Magneto-PL spectroscopy has been used to investigate the diamagnetic response and Zeeman splitting of the various exciton complexes. We find a significant variation in g-factor between the exciton, the positive biexciton, and the negative biexciton; this is also attributed to anisotropy effects and the difference in lateral extent of the electron and hole wavefunctions.

cond-mat.mes-hall↗

arXiv2005

Charged exciton emission at 1.3 $μ$m from single InAs quantum dots grown by metalorganic chemical vapor deposition

We have studied the emission properties of self-organized InAs quantum dots (QDs) grown in an InGaAs quantum well by metalorganic chemical vapor deposition. Low-temperature photoluminescence spectroscopy shows emission from single QDs around 1300 nm; we clearly observe the formation of neutral and charged exciton and biexciton states, and we obtain a biexciton binding energy of 3.1 meV. The dots exhibit an s-p shell splitting of approximately 100 meV, indicating strong confinement.

cond-mat.mes-hall↗

arXiv2004

Charge dynamics of Ca_{2-x}Na_{x}CuO_{2}Cl_{2} as a correlated electron system with the ideal tetragonal lattice

We report the reflectivity and the resistivity measurement of Ca_{2-x}Na_{x}CuO_{2}Cl_{2} (CNCOC), which has a single-CuO2-plane lattice with no orthorhombic distortion. The doping dependence of the in-plane optical conductivity spectra for CNCOC is qualitatively the same to those of other cuprates, but a slight difference between CNCOC and LSCO, i.e., the absence of the 1.5 eV peak in CNCOC, can be attributed to the smaller charge-stripe instability in CNCOC. The temperature dependence of the optical onductivity spectra of CNCOC has been analyzed both by the two-component model (Drude+Lorentzian) and by the one-component model (extended-Drude analysis). The latter analysis gives a universal trend of the scattering rate Gamma(omega) with doping. It was also found that Gamma(omega) shows a saturation behavior at high frequencies, whose origin is the same as that of resistivity saturation at high temperatures.

cond-mat.supr-con↗

arXiv2004

Oxygen and Cation Ordered Perovskite, Ba2Y2Mn4O11

A three-step route has been developed for the synthesis of a new oxygen-ordered double perovskite, BaYMn2O5.5 or Ba2Y2Mn4O11. (i) The A-site cation ordered perovskite, BaYMn2O5+d, is first synthesized at d ~ 0 by an oxygen-getter-controlled low-O2-pressure encapsulation technique utilizing FeO as the getter for excess oxygen. (ii) The as-synthesized, oxygen-deficient BaYMn2O5.0 phase is then readily oxygenated to the d ~ 1 level by means of 1-atm-O2 annealing at low temperatures. (iii) By annealing this fully-oxygenated BaYMn2O6.0 in flowing N2 gas at moderate temperatures the new intermediate-oxygen-content oxide, BaYMn2O5.5 or Ba2Y2Mn4O11, is finally obtained. From thermogravimetric observation it is seen that the final oxygen depletion from d ~ 1.0 to 0.5 occurs in a single sharp step about 600 C, implying that the oxygen stoichiometry of BaYMn2O5+d is not continuously tunable within 0.5 < d < 1.0. For BaYMn2O5.5 synchrotron x-ray diffraction analysis reveals an orthorhombic crystal lattice and a long-range ordering of the excess oxygen atoms in the YO0.5 layer. The magnetic behavior of BaYMn2O5.5 (with a ferromagnetic transition at ~ 133 K) is found different from those previously reported for the known phases, BaYMn2O5.0 and BaYMn2O6.0.

cond-mat.str-el↗