arXiv subjects

H. S. J. van der Zant

Publications and source records attributed to H. S. J. van der Zant.

At least 55 records · Page 3Linked to original sources

arXiv2009

Carbon nanotubes as ultra-high quality factor mechanical resonators

We have observed the transversal vibration mode of suspended carbon nanotubes at millikelvin temperatures by measuring the single-electron tunneling current. The suspended nanotubes are actuated contact-free by the radio frequency electric field of a nearby antenna; the mechanical resonance is detected in the time-averaged current through the nanotube. Sharp, gate-tuneable resonances due to the bending mode of the nanotube are observed, combining resonance frequencies of up to ν_0 = 350 MHz with quality factors above Q = 10^5, much higher than previously reported results on suspended carbon nanotube resonators. The measured magnitude and temperature dependence of the Q-factor shows a remarkable agreement with the intrinsic damping predicted for a suspended carbon nanotube. By adjusting the RF power on the antenna, we find that the nanotube resonator can easily be driven into the non-linear regime.

cond-mat.mes-hall↗

arXiv2009

Efficient readout of micromechanical resonator arrays in ambient conditions

We present a method for efficient spectral readout of mechanical resonator arrays in dissipative environments. Magnetomotive drive and detection is used to drive double clamped resonators in the nonlinear regime. Resonators with almost identical resonance frequencies can be tracked individually by sweeping the drive power. Measurements are performed at room temperature and atmospheric pressure. These conditions enable application in high throughput resonant sensor arrays.

physics.ins-det↗

arXiv2009

Pumping of vibrational excitations in a Coulomb blockaded suspended carbon nanotube

Low-temperature transport spectroscopy measurements on a suspended few-hole carbon nanotube quantum dot are presented, showing a gate-dependent harmonic excitation spectrum which, strikingly, occurs in the Coulomb blockade regime. The quantized excitation energy corresponds to the scale expected for longitudinal vibrations of the nanotube. The electronic transport processes are identified as cotunnel-assisted sequential tunneling, resulting from non-equilibrium occupation of the mechanical mode. They appear only above a high-bias threshold at the scale of electronic nanotube excitations. We discuss models for the pumping process that explain the enhancement of the non-equilibrium occupation and show that it is connected to a subtle interplay between electronic and vibrational degrees of freedom.

cond-mat.mes-hall↗

arXiv2008

Self-detecting gate-tunable nanotube paddle resonators

We have fabricated suspended metal paddle resonators with carbon nanotubes functioning as self-detecting torsional springs. We observe gate-tunable resonances, that either tune to higher or to lower frequencies when increasing the dc voltage on the back-gate. We attribute the former modes to flexural vibrations of the paddle resonator, while the latter ones are identified as torsional vibrations. Compared to top-down silicon fabricated paddle resonators, nanotube springs have smaller torsional spring constants and provide a larger frequency tunability.

cond-mat.mes-hall↗

arXiv2008

Lithographic mechanical break junctions for single-molecule measurements in vacuum: possibilities and limitations

We have investigated electrical transport through the molecular model systems benzenedithiol, benzenediamine, hexanedithiol and hexanediamine. Conductance histograms under different experimental conditions indicate that measurements using mechanically controllable break junctions in vacuum are limited by the surface density of molecules at the contact. Hexanedithiol histograms typically exhibit a broad peak around 7 * 10^{-4} G_0. In contrast to recent results on STM-based break junctions in solution we find that the spread in single-molecule conductance is not reduced by amino anchoring groups. Histograms of hexanediamine exhibit a very wide peak around 4 * 10^{-4} G_0. For both benzenedithiol and benzenediamine we observe a large variability in low-bias conductance. We attribute these features to the slow breaking of the lithographic mechanically controllable break junctions and the absence of a solvent that may enable molecular readsorption after bond breaking. Nevertheless, we have been able to acquire reproducible current-voltage characteristics of benzenediamine and benzenedithiol using a statistical measurement approach. Benzenedithiol measurements yield a conductance gap of about 0.9 V at room temperature and 0.6 V at 77 K. In contrast, the current-voltage characteristics of benzenediamine-junctions typically display conductance gaps of about 0.9 V at both temperatures.

cond-mat.mes-hall↗

arXiv2007

Self-breaking in planar few-atom Au constrictions for nm-spaced electrodes

We present results on electromigrated Au nanojunctions broken near the conductance quantum $77.5 μ$S. At room temperature we find that wires, initially narrowed by an actively-controlled electromigration technique down to a few conductance quanta, continue to narrow after removing the applied voltage. Separate electrodes form as mobile gold atoms continuously reconfigure the constriction. We find, from results obtained on over 300 samples, no evidence for gold cluster formation in junctions broken without an applied voltage, implying that gold clusters may be avoided by using this self-breaking technique.

cond-mat.mtrl-sci↗

arXiv2006

Electron transport through single Mn12 molecular magnets

We report transport measurements through a single-molecule magnet, the Mn12 derivative [Mn12O12(O2C-C6H4-SAc)16(H2O)4], in a single-molecule transistor geometry. Thiol groups connect the molecule to gold electrodes that are fabricated by electromigration. Striking observations are regions of complete current suppression and excitations of negative differential conductance on the energy scale of the anisotropy barrier of the molecule. Transport calculations, taking into account the high-spin ground state and magnetic excitations of the molecule, reveal a blocking mechanism of the current involving non-degenerate spin multiplets.

cond-mat.mes-hall↗

arXiv2006

In-Chain Tunneling Through Charge-Density Wave Nanoconstrictions and Break-Junctions

We have fabricated longitudinal nanoconstrictions in the charge-density wave conductor (CDW) NbSe$_{3}$ using a focused ion beam and using a mechanically controlled break-junction technique. Conductance peaks are observed below the T$_{P1}$$=145 $K and T$_{P2}$$=59 $K CDW transitions, which correspond closely with previous values of the full CDW gaps $2Δ_{1}$ and $2Δ_{2}$ obtained from photo-emission. These results can be explained by assuming CDW-CDW tunneling in the presence of an energy gap corrugation $ε_{2}$ comparable to $Δ_{2}$, which eliminates expected peak at $Δ_{1}+Δ_{2}$. The nanometer length-scales our experiments imply indicate that an alternative explanation based on tunneling through back-to-back CDW-normal junctions is unlikely.

cond-mat.str-el↗

arXiv2005

The Kondo Effect in the Presence of Magnetic Impurities

We measure transport through gold grain quantum dots fabricated using electromigration, with magnetic impurities in the leads. A Kondo interaction is observed between dot and leads, but the presence of magnetic impurities results in a gate-dependent zero-bias conductance peak that is split due to an RKKY interaction between the spin of the dot and the static spins of the impurities. A magnetic field restores the single Kondo peak in the case of an antiferromagnetic RKKY interaction. This system provides a new platform to study Kondo and RKKY interactions in metals at the level of a single spin.

cond-mat.mes-hall↗

arXiv2005

Tunneling in suspended carbon nanotubes assisted by longitudinal phonons

Current-voltage characteristics of suspended single-wall carbon nanotube quantum dots show a series of steps equally spaced in voltage. The energy scale of this harmonic, low-energy excitation spectrum is consistent with that of the longitudinal low-k phonon mode (stretching mode) in the nanotube. Agreement is found with a Franck-Condon-based model in which the phonon-assisted tunneling process is modeled as a coupling of electronic levels to underdamped quantum harmonic oscillators. Comparison with this model indicates a rather strong electron-phonon coupling factor of order unity.

cond-mat.mes-hall↗

arXiv2004

Electronic excitation spectrum of metallic carbon nanotubes

We have studied the discrete electronic spectrum of closed metallic nanotube quantum dots. At low temperatures, the stability diagrams show a very regular four-fold pattern that allows for the determination of the electron addition and excitation energies. The measured nanotube spectra are in excellent agreement with theoretical predictions based on the nanotube band structure. Our results permit the complete identification of the electron quantum states in nanotube quantum dots.

cond-mat.mes-hall↗

arXiv2004

Electronic Transport Spectroscopy of Carbon Nanotubes in a Magnetic Field

We report magnetic field spectroscopy measurements in carbon nanotube quantum dots exhibiting four-fold shell structure in the energy level spectrum. The magnetic field induces a large splitting between the two orbital states of each shell, demonstrating their opposite magnetic moment and determining transitions in the spin and orbital configuration of the quantum dot ground state. We use inelastic cotunneling spectroscopy to accurately resolve the spin and orbital contributions to the magnetic moment. A small coupling is found between orbitals with opposite magnetic moment leading to anticrossing behavior at zero field.

cond-mat.mes-hall↗

arXiv2004

One-dimensional conduction in Charge-Density Wave nanowires

We report a systematic study of the transport properties of coupled one-dimensional metallic chains as a function of the number of parallel chains. When the number of parallel chains is less than 2000, the transport properties show power-law behavior on temperature and voltage, characteristic for one-dimensional systems.

cond-mat.str-el↗

arXiv2003

Crossover from 2-dimensional to 1-dimensional collective pinning in NbSe3

We have fabricated NbSe$_3$ structures with widths comparable to the Fukuyama-Lee-Rice phase-coherence length. For samples already in the 2-dimensional pinning limit, we observe a crossover from 2-dimensional to 1-dimensional collective pinning when the crystal width is less than 1.6 $μ$m, corresponding to the phase-coherence length in this direction. Our results show that surface pinning is negligible in our samples, and provide a means to probe the dynamics of single domains giving access to a new regime in charge-density wave physics.

cond-mat.str-el↗

arXiv2003

Carbon Nanotubes as Nanoelectromechanical Systems

We theoretically study the interplay between electrical and mechanical properties of suspended, doubly clamped carbon nanotubes in which charging effects dominate. In this geometry, the capacitance between the nanotube and the gate(s) depends on the distance between them. This dependence modifies the usual Coulomb models and we show that it needs to be incorporated to capture the physics of the problem correctly. We find that the tube position changes in discrete steps every time an electron tunnels onto it. Edges of Coulomb diamonds acquire a (small) curvature. We also show that bistability in the tube position occurs and that tunneling of an electron onto the tube drastically modifies the quantized eigenmodes of the tube. Experimental verification of these predictions is possible in suspended tubes of sub-micron length.

cond-mat.mes-hall↗

arXiv2001

Luttinger-liquid-like behavior in bulk crystals of the quasi-one-dimensional conductor NbSe$_3$

CDW/Normal metal/CDW junctions and nanoconstrictions in crystals of the quasi-one-dimensional conductor NbSe$_3$ are manufactured using a focused-ion-beam. It is found that the low-temperature conduction of these structures changes dramatically and loses the features of the charge-density-wave transition. Instead, a dielectric phase is developed. Up to 6-order power-law variations of the conduction as a function of both temperature and electric field can be observed for this new phase. The transition from quasi-one-dimensional behavior to one-dimensional behavior is associated with destruction of the three-dimensional order of the charge-density waves by fluctuations. It results in a recovery of the Luttinger-liquid properties of metallic chains, like it takes place in sliding Luttinger liquid phase.

cond-mat.str-el↗

arXiv2001

Negative Resistance and Local Charge-Density-Wave Dynamics

Charge-density-wave dynamics is studied on a submicron length scale in NbSe_3 and o-TaS_3. Regions of negative absolute resistance are observed in the CDW sliding regime at sufficiently low temperatures. The origin of the negative resistance is attributed to the different forces that the deformed CDW and quasi-particles feel: the force on the CDW is merely caused by a difference of the electric potentials, while the quasi-particle current is governed by a difference of the electrochemical potentials.

cond-mat.str-el↗

arXiv1999

Tunable Charge Density Wave Transport in a Current-Effect Transistor

The collective charge density wave (CDW) conduction is modulated by a transverse single-particle current in a transistor-like device. Nonequilibrium conditions in this geometry lead to an exponential reduction of the depinning threshold, allowing the CDWs to slide for much lower bias fields. The results are in excellent agreement with a recently proposed dynamical model in which ''wrinkles'' in the CDW wavefronts are ''ironed'' by the transverse current. The experiment might have important implications for other driven periodic media, such as moving vortex lattices or ''striped phases'' in high-Tc superconductors.

cond-mat.str-el↗