arXiv subjects

H. S. Lee

Publications and source records attributed to H. S. Lee.

At least 19 recordsLinked to original sources

arXiv2026

Preventing quart-NaI adhesion in Bridgman growth using ammonium iodide

Adhesion between NaI(Tl) single crystals and the walls of quartz ampoules remains a major limitation for Bridgman growth under sealed conditions, particularly for applications requiring ultra-radiopure scintillators for dark matter searches, where sealed handling is essential. In this study, ammonium iodide (NH4I) was used as an additive to generate HI in situ, thereby suppressing the NaOH-SiO2 reaction that forms adhesive sodium silicate phases. Small-diameter crystals (8 mm) were first grown to determine the NH4I concentration required to eliminate adhesion. The optimized condition was then applied to the growth of a large NaI(Tl) crystal. A crack-free and bubble-free NaI(Tl) crystal with dimensions of 3 inches in diameter by 3 inches in length was successfully grown. The crystal exhibited a light output of 59,000 photons/MeV, which is higher than that of the commercial NaI(Tl) crystals used as references in this study.

physics.ins-det↗

arXiv2026

Development of a 10 mol% Rubidium-doped CsI Crystal for $^{87}$Rb Beta-Spectroscopy and Sterile Neutrino Searches

The third-forbidden non-unique beta-decay of $^{87}$Rb to $^{87}$Sr (Q$_β= 282.275(6)$ keV) has long served as an important benchmark for understanding forbidden beta-decay. To investigate this, we have developed a novel CsI scintillator with a 10 mol% Rb concentration using the Bridgman method. The incorporated $^{87}$Rb serves as an intrinsic radioactive source, enabling a source-in-detector configuration with high detection efficiency and minimal energy loss for low-energy electrons from beta-decay. We investigated both Rb doped and Tl co-doped CsI crystals and characterized their scintillation properties, including light yield, energy resolution, and non-linear response. We report distinct scintillation characteristics for the CsI:Rb and CsI:Tl,Rb crystals, with light yields of $1.38\pm0.01$ and $4.73\pm0.13$ PE/keV, respectively. Using the measured $^{87}$Rb beta-spectrum, we search for a keV-scale sterile neutrino admixture through the characteristic kink-like distortion induced by a heavy neutrino mass eigenstate. This study provides a basis for future sterile neutrino searches using rubidium doped CsI crystal.

physics.ins-det↗

arXiv2026

Temperature-Dependent Performance of NaI(Tl) Crystal with Dual-Channel SiPM Readout for Low-Mass Dark Matter Searches

We report the first temperature-dependent characterization of a NaI(Tl) crystal readout by two silicon photomultipliers (SiPMs) directly coupled to opposite ends of the crystal for rare-event searches. A $6 \text{ mm} \times 6 \text{ mm} \times 13 \text{ mm}$ NaI(Tl) crystal was directly coupled to two SiPMs and characterized in a liquid nitrogen-cooled cryostat over a temperature range of 94$-$293 K. The light yield, energy resolution, and scintillation decay time were measured using $γ$-ray peak from a $^{241}$Am source. After correcting for optical crosstalk contributions, the light yield increased, reaching $17.7 \pm 1.1$ photoelectrons/keV at 238 K, corresponding to a 34.5% enhancement relative to room temperature (293 K). Furthermore, dual-channel configuration effectively suppresses random thermal noise via coincidence triggers, which together with the observed increase in light yield, provides a critical pathway toward lowering the energy threshold for dark matter and coherent elastic neutrino$-$nucleus scattering searches.

physics.ins-det↗

arXiv2026

Probing unexplored spin-dependent dark matter-proton coupling with few-photoelectron threshold in COSINE-100

We report new constraints on the spin-dependent scattering cross section between low-mass dark matter and protons using data collected by the COSINE-100 experiment. By implementing a specialized event selection process using a multi-layer perceptron and robust noise mitigation, this analysis pioneers a detection threshold of 3 and 4 isolated peaks, corresponding to the reconstructed photoelectrons, which are significantly lower than the 8 photoelectron threshold used in previous analyses. In this unstudied few-photoelectron regime, where instrumental noise and phosphorescence are prevalent, we utilize a phenomenological background model to search for the annual modulation signal expected from the Standard Halo Model. No statistically significant annual modulation is observed in our data. We derive new 90% confidence level (C.L.) upper limits for the spin-dependent DM-proton cross section, establishing the world's most stringent constraints in the 1.75-2.25 GeV/c$^2$ mass range. Furthermore, by incorporating the Migdal effect, we extend the experimental sensitivity to the sub-GeV/c$^2$ regime, setting world-leading limits in the 15-58 MeV/c$^2$ range. These results demonstrate the capability of NaI(Tl) target materials to probe previously unexplored regions of the dark matter parameter space.

hep-ex↗

arXiv2026

Femtoscopy Measurement with S$π$RIT TPC in Radioactive BeamHeavy-ion Collisions

Femtoscopy is a powerful tool for exploring the dynamic emitting structure in heavy-ion collisions, while radioactive beam heavy-ion collisions enable the investigation of nuclear matter under extreme isospin conditions. Here, we successfully perform femtoscopy measurements using the S$π$RIT Time Projection Chamber (TPC). A dedicated correction scheme for track merging and splitting is proposed, which is well applicable to rectangular TPCs housed inside dipole magnets and effectively improves the reconstructed correlation functions at small relative momenta. Focusing on the proton-proton (p-p) correlation function in the 270 MeV/u $^{132}\text{Sn}+^{124}\text{Sn}$ system, we successfully apply the track merging and splitting correction; additionally, the TPC angular acceptance exhibits a negligible impact on the correlation function. A systematic uncertainty quantification framework is established. The experimental results of the p-p correlation function confirm the feasibility of the S$π$RIT TPC for femtoscopy measurements and provide technical support for high-precision femtoscopy studies using rectangular TPCs in radioactive beam heavy-ion collisions.

physics.ins-det↗

arXiv2026

A study of neutrinoless double electron capture in $^{40}$Ca from the AMoRE experiment

The search for neutrinoless double electron capture ($0ν\mathrm{2EC}$) provides a sensitive probe of lepton-number violation and the Majorana nature of neutrinos. We investigate the $0ν\mathrm{2EC}$ decay of $^{40}$Ca using cryogenic detectors equipped with metallic magnetic calorimeters in the AMoRE-I experiment. The analysis is based on a physics dataset corresponding to a total exposure of 7.32 kg$\cdot$yr from thirteen $^{40}$Ca$^{100}$MoO$_4$ crystals. No significant excess is observed, and a lower limit on the half-life is obtained as $T^{0ν}_{1/2} > 1.7 \times 10^{22}$ yr at 90$\%$ confidence level. An improved sensitivity is expected for the upcoming AMoRE-II experiment. These results demonstrate the potential of CaMoO$_4$ detectors to explore rare decay processes beyond the primary $^{100}$Mo $0νββ$ search program.

nucl-ex↗

arXiv2026

Large amplification of the isospin-dependence of proton emitting source size in radioactive heavy-ion collisions: a signal of n-p correlation

We report proton-proton correlation function measurements in central $^{132}$Sn+$^{124}$Sn and $^{108}$Sn+$^{112}$Sn collisions at 270 MeV/nucleon. The proton emitting source sizes are extracted for the systems by using femtoscopic imaging technique. The fast dynamic core radius for the neutron-rich system is found to be $2.22 \pm 0.13\ \text{(stat.)} \pm 0.07\ \text{(syst.)}$ fm, which is approximately 24\% larger than that for the neutron-deficient system, $1.74 \pm 0.08\ \text{(stat.)} \pm 0.05\ \text{(syst.)}$ fm. This difference is an order of magnitude larger than the $\sim$3\% difference in the ground-state charge radii of the projectile nuclei. Transport model simulations based on mean-field dynamics cannot reproduce this amplification. The observation reveals a beyond-mean-field mechanism associated to short-range neutron-proton correlations, which dynamically enhance the proton emitting source in the neutron-rich environment. Our results demonstrate that heavy-ion collisions induced by radioactive beam, combined with femtoscopic precision, provide a new hadronic probe of short-range correlation, and that careful treatment of the beyond-mean-field interactions are required in modeling such processes.

nucl-ex↗

arXiv2026

Constraints on sub-GeV dark matter scattering on electrons with COSINE-100

We present results of the search for sub-GeV dark matter interaction with electrons in the NaI(Tl) crystals of the COSINE-100 experiment. The two benchmark scenarios of a heavy and a light vector boson as mediator of the interaction were studied. We found no excess events over the expected background in a data-set of 2.82 years, with a total exposure of 172.9 kg-year. The derived 90% confidence level upper limits exclude a DM-electron scattering cross section above 6.4 $\times$ 10$^{-33}$ cm$^2$ for a DM mass of 0.25 GeV, assuming a light mediator; and above 3.4 $\times$ 10$^{-37}$ cm$^2$ for a 0.4 GeV DM, assuming a heavy mediator, and represent the most stringent constraints for a NaI(Tl) target to date. We also briefly discuss a planned analysis using an annual modulation method below the current 0.7 keV threshold of COSINE-100, down to few photoelectrons yield.

hep-ex↗

arXiv2026

Impact of the in-medium cross section on cluster spectra in ${}^{40,48}\mathrm{Ca}+{}^{58,64}\mathrm{Ni}$ collisions at $56$ and $140$ $\mathbf{\mathrm{MeV}}/\mathrm{\mathbf{nucleon}}$

Although significant efforts have been made to investigate the density dependence of the nuclear symmetry energy, the influence of the in-medium cross section on particle production in transport models is not well constrained. The in-medium cross section reflects the dynamic situation of the medium such as a nontrivial phase space distribution. In this study, we analyze the transverse momentum spectra of $p$, $d$, $t$, ${}^3{\mathrm{He}}$ and $α$ particles emitted near mid-rapidity in central $^{40,48}\mathrm{Ca}$ + $^{58, 64}\mathrm{Ni}$ reactions at $56$ and $140$ $\mathrm{MeV}/\mathrm{nucleon}$. The Antisymmetrized Molecular Dynamics ($\mathrm{AMD}$) model is chosen as the transport model for data comparison. Central events are selected based on charged-particle multiplicity in both the experimental data and AMD calculations after applying an experimental filter. Our results show that the in-medium nucleon-nucleon scattering cross-sections are more strongly reduced at $56$ $\mathrm{MeV}/\mathrm{nucleon}$ than at $140$ $\mathrm{MeV}/\mathrm{nucleon}$ incident energy.

nucl-th↗

arXiv2025

Limits on WIMP dark matter with NaI(Tl) crystals in three years of COSINE-100 data

We report limits on WIMP dark matter derived from three years of data collected by the COSINE-100 experiment with NaI(Tl) crystals, achieving an improved energy threshold of 0.7 keV. This lowered threshold enhances sensitivity in the sub-GeV mass range, extending the reach for direct detection of low-mass dark matter. Although no excess of WIMP-like events was observed, the increased sensitivity enabled a model-insensitive comparison between the expected WIMP signal rate-based on mass limits from our data-and DAMA's reported modulation amplitude. Our findings strongly disfavor the DAMA signal as originating from WIMP interactions, fully excluding DAMA/LIBRA 3$σ$ allowed regions and providing enhanced WIMP mass limits by an order of magnitude in the spin-independent model compared to previous results. In the spin-dependent model, cross-section upper limits were obtained in the mass range [0.1-5.0] GeV/c$^2$, with additional sensitivity to sub-GeV WIMPs through the inclusion of the Migdal effect. These results represent substantial progress in low-mass dark matter exploration and reinforce constraints on the longstanding DAMA claim.

hep-ex↗

arXiv2025

Combined Annual Modulation Dark Matter Search with COSINE-100 and ANAIS-112

The annual modulation signal, claimed to be consistent with dark matter as observed by DAMA/LIBRA in a sodium-iodide based detector, has persisted for over two decades. COSINE-100 and ANAIS-112 were designed to test the claim directly using the same target material. COSINE-100, located at Yangyang Underground Laboratory in South Korea, and ANAIS-112, located at Canfranc Underground Laboratory in Spain, have been taking data since 2016 and 2017, respectively. Each experiment published its respective results independently. In this paper, we present the results of an annual modulation search as a test of the signal observed by DAMA/LIBRA with the first three respective years of data from COSINE-100 and ANAIS-112. Using a Markov Chain Monte Carlo method, we find best fit values for modulation amplitude of $-0.0002 {\pm} 0.0026$ cpd/kg/keV in the 1-6 keV and $0.0021 {\pm} 0.0028$ cpd/kg/keV in the 2-6 keV energy regions. These results are not compatible with DAMA/LIBRA's assertion for their observation of annual modulation at $3.7σ$ and $2.6σ$, respectively. Performing a simple combination of the newly released 6-years datasets from both experiments find values consistent with no modulation at $0.0005 {\pm} 0.0019$ cpd/kg/keV in the 1-6 keV and $0.0027 {\pm} 0.0021$ cpd/kg/keV in the 2-6 keV energy regions with $4.68σ$ and $3.53σ$ respective exclusions of the DAMA/LIBRA signal.

astro-ph.IM↗

arXiv2025

Scintillation characteristics of an undoped CsI crystal at low-temperature for dark matter search

The scintillation characteristics of 1 g undoped CsI crystal were studied by directly coupling two silicon photomultipliers(SiPMs) over a temperature range from room temperature to 86 K. The scintillation decay time and light output were measured using x-ray and gamma-ray peaks from a 109Cd radioactive source. An increase in decay time was observed as the temperature decreased from room temperature to 86 K, ranging from 76 ns to 605 ns. The light output also increased, reaching 26.2 +/- 1.3 photoelectrons per keV electron-equivalent at 86 K. Leveraging the significantly enhanced scintillation light output of the undoped CsI crystal at low temperatures, coupling it with SiPMs results in a promising detector for rare event searches. Both cesium and iodine have an odd number of protons, making them suitable targets for probing dark matter-proton spin-dependent interactions. This study evaluates the sensitivity of the proposed detector to such interactions, incorporating the Migdal effect and assuming 200 kg of undoped CsI crystals for dark matter searches. The results indicate that undoped CsI coupled with SiPM can achieve world-competitive sensitivity for low-mass dark matter detection, particularly in the context of dark matter-proton spin-dependent interactions.

physics.ins-det↗

arXiv2025

COSINE-100 Full Dataset Challenges the Annual Modulation Signal of DAMA/LIBRA

For over 25 years, the DAMA/LIBRA collaboration has claimed to observe an annual modulation signal, suggesting the existence of dark matter interactions. However, no experiment employing different target materials has observed a dark matter signal consistent with their result. To address this puzzle, the COSINE-100 collaboration conducted a model-independent test using sodium iodide crystal detectors, the same target material as DAMA/LIBRA. Analyzing data collected over 6.4 years by the effective mass of 61.3 kg, with improved energy calibration and time-dependent background modeling, we found no evidence of an annual modulation signal, challenging the DAMA/LIBRA result with a confidence level greater than 3$σ$. This finding represents a substantial step toward resolving the long-standing debate surrounding DAMA/LIBRA's dark matter claim, indicating that the observed modulation is unlikely to be caused by dark matter interactions.

hep-ex↗

arXiv2025

Radiopurity measurements of liquid scintillator for the COSINE-100 Upgrade

A new 2,400 L liquid scintillator has been produced for the COSINE-100 Upgrade, which is under construction at Yemilab for the next COSINE dark matter experiment phase. The linear-alkyl-benzene-based scintillator is designed to serve as a veto for NaI(Tl) crystal targets and a separate platform for rare event searches. We measured using a sample consisting of a custom-made 445 mL cylindrical Teflon container equipped with two 3-inch photomultiplier tubes. Analyses show activity levels of $0.091 \pm 0.042$ mBq/kg for $^{238}$U and $0.012 \pm 0.007$ mBq/kg for $^{232}$Th.

physics.ins-det↗

arXiv2025

Upgrading the COSINE-100 Experiment for Enhanced Sensitivity to Low-Mass Dark Matter Detection

The DAMA/LIBRA experiment has reported an annual modulation signal in NaI(Tl) detectors, which has been interpreted as a possible indication of dark matter interactions. However, this claim remains controversial, as several experiments have tested the modulation signal using NaI(Tl) detectors. Among them, the COSINE-100 experiment, specifically designed to test DAMA/LIBRA's claim, observed no significant signal, revealing a more than 3 $σ$ discrepancy with DAMA/LIBRA's results. Here we present COSINE-100U, an upgraded version of the experiment, which aims to expand the search for dark matter interactions by improving light collection efficiency and reducing background noise. The detector, consisting of eight NaI(Tl) crystals with a total mass of 99.1 kg, has been relocated to Yemilab, a new underground facility in Korea, and features direct PMT-coupling technology to enhance sensitivity. These upgrades significantly improve the experiment's ability to probe low-mass dark matter candidates, contributing to the ongoing global effort to clarify the nature of dark matter.

hep-ex↗

arXiv2025

Improved limit on neutrinoless double beta decay of $^{100}$Mo from AMoRE-I

AMoRE searches for the signature of neutrinoless double beta decay of $^{100}$Mo with a 100 kg sample of enriched $^{100}$Mo. Scintillating molybdate crystals coupled with a metallic magnetic calorimeter operate at milli-Kelvin temperatures to measure the energy of electrons emitted in the decay. As a demonstration of the full-scale AMoRE, we conducted AMoRE-I, a pre-experiment with 18 molybdate crystals, at the Yangyang Underground Laboratory for over two years. The exposure was 8.02 kg$\cdot$year (or 3.89 kg$_{\mathrm{^{100}Mo}}\cdot$year) and the total background rate near the Q-value was 0.025 $\pm$ 0.002 counts/keV/kg/year. We observed no indication of $0νββ$ decay and report a new lower limit of the half-life of $^{100}$Mo $0νββ$ decay as $ T^{0ν}_{1/2}>2.9\times10^{24}~\mathrm{yr}$ at 90\% confidence level. The effective Majorana mass limit range is $m_{ββ}<$(210--610) meV using nuclear matrix elements estimated in the framework of different models, including the recent shell model calculations.

nucl-ex↗

arXiv2025

Development of MMC-based lithium molybdate cryogenic calorimeters for AMoRE-II

The AMoRE collaboration searches for neutrinoless double beta decay of $^{100}$Mo using molybdate scintillating crystals via low temperature thermal calorimetric detection. The early phases of the experiment, AMoRE-pilot and AMoRE-I, have demonstrated competitive discovery potential. Presently, the AMoRE-II experiment, featuring a large detector array with about 90 kg of $^{100}$Mo isotope, is under construction. This paper discusses the baseline design and characterization of the lithium molybdate cryogenic calorimeters to be used in the AMoRE-II detector modules. The results from prototype setups that incorporate new housing structures and two different crystal masses (316 g and 517 - 521 g), operated at 10 mK temperature, show energy resolutions (FWHM) of 7.55 - 8.82 keV at the 2.615 MeV $^{208}$Tl $γ$ line, and effective light detection of 0.79 - 0.96 keV/MeV. The simultaneous heat and light detection enables clear separation of alpha particles with a discrimination power of 12.37 - 19.50 at the energy region around $^6$Li(n, $α$)$^3$H with Q-value = 4.785 MeV. Promising detector performances were demonstrated at temperatures as high as 30 mK, which relaxes the temperature constraints for operating the large AMoRE-II array.

physics.ins-det↗

arXiv2024

First Direct Search for Light Dark Matter Using the NEON Experiment at a Nuclear Reactor

We report new results from the Neutrino Elastic Scattering Observation with NaI (NEON) experiment in the search for light dark matter (LDM) using 2,636 kg$\cdot$days of NaI(Tl) exposure. The experiment employs an array of NaI(Tl) crystals with a total mass of 16.7 kg, located 23.7 meters away from a 2.8 GW thermal power nuclear reactor. We investigated LDM produced by the $\textit{invisible decay}$ of dark photons generated by high-flux photons during reactor operation. The energy spectra collected during reactor-on and reactor-off periods were compared within the LDM signal region of $1-10$ keV. No signal consistent with LDM interaction with electrons was observed, allowing us to set 90% confidence level exclusion limits for the dark matter-electron scattering cross-section ($σ_e$) across dark matter masses ranging from 1 keV/c$^2$ to 1 MeV/c$^2$. Our results set a 90% confidence level upper limit of $σ_e = 3.17\times10^{-35}~\mathrm{cm^2}$ for a dark matter mass of 100 keV/c$^2$, marking the best laboratory result in this mass range. Additionally, our search extends the coverage of LDM below 100 keV/c$^2$ first time.

hep-ex↗