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Haiqing Lin

Publications and source records attributed to Haiqing Lin.

At least 19 recordsLinked to original sources

Nonlinear Photonic Tripartite Phase

Anderson localization is usually understood as a transition between extended and localized phases, with criticality confined to a single mobility edge. Recent advances predict that quasiperiodic systems can instead host a finite critical window bounded by mobility edges, in which localized, critical and extended states coexist. Yet both the experimental realization of this regime and whether interactions can provide controlled access to it remain unknown. Here, we realize such a tripartite phase in a nonlinear quasiperiodic photonic lattice and show that Kerr nonlinearity, acting as an effective interaction, enables state-selective access to the critical window. By tracking wavepacket dynamics, we distinguish localized, critical and extended transport regimes and uncover a state-selective response: rather than simply reinforcing localization through self-trapping, weak nonlinearity drives low-energy localized states into the critical window, whereas stronger nonlinearity restores localization. By contrast, critical, extended and high-energy localized states evolve monotonically towards self-trapped behaviour. Our results reveal a state-selective mechanism by which interactions provide controlled access to a pre-existing critical window in quasiperiodic systems.

cond-mat.mes-hall

Spatially and Temporally Resolved Mapping of Contact Electrification on Stand-Alone Ultrathin Glass Materials via Kelvin Probe Force Microscopy

Contact electrification (CE) remains a critical challenge in advanced material technologies where uncontrolled surface charging can compromise manufacturability, reliability, and performance in practical applications. Ultrathin glass with micrometer-scale thickness is a state-of-the-art specialty oxide material for flexible touchscreens in next-generation electronic devices. Here, we visualize and quantify CE-induced surface charges on ultrathin glass using sideband-mode Kelvin probe force microscopy (KPFM). Nanoscale atomic force microscopy (AFM) probes are used to scan and induce triboelectric charges on stand-alone glass surfaces under ultra-pure N$_2$ conditions. Time-dependent measurements reveal that surface charges on a 30~$\mu$m-thick glass sample decay from 4.47~V to 0.37~V over 240~minutes. Furthermore, electrostatic charges are found to exhibit capacitor-like discharging behavior primarily through the bulk material, yielding a long relaxation time constant of approximately 41~minutes. This behavior differs from the lateral surface discharging observed in thermally grown SiO$2$ thin films reported previously. A self-capacitance analytical model is developed to estimate the corresponding surface charge density ($\sigma$), yielding comparable values of 136.26~$\pm$~16.25~$\mu$C/m$^2$ at 30~$\mu$m and 131.44~$\pm$~28.41~$\mu$C/m$^2$ at 100~$\mu$m. Additionally, external bias applied to AFM tips can be used to enhance, suppress, or invert the intrinsic CE response of glass materials.

physics.app-ph

Encoding complex-balanced thermalization in quantum circuits

Non-Markovian dynamics in open quantum systems often invalidates the complex-balanced thermalization framework, hindering predictive control of quantum simulation platforms designed to prepare out-of-equilibrium states at prescribed temperatures. We resolve this bottleneck by engineering reservoir qubits as modular microscopic units coupled to a target quantum system and constructing a quantum-circuit platform that enforces strictly Markovian complex-balanced thermalization. The platform exploits the non-orthogonality of reservoir qubit eigenstates to drive inhomogeneous heating through a modified Kubo-Martin-Schwinger relation, and uses tunable microscopic time-reversibility breaking to generate amplification-dissipation dynamics. We demonstrate two applications: temporally correlated dichromatic emission and Liouvillian exceptional-point-protected quantum synchronization at finite temperatures, displaying predictive control over out-of-equilibrium state preparation.

quant-ph

Post-$GW$ theory and its application to pseudogap in strongly correlated system

The $GW$ approximation is a widely used framework for studying correlated materials, but it struggles with certain limitations, such as its inability to explain pseudogap phenomena. To overcome these problems, we propose a systematic theoretical framework for Green's function corrections and apply it specifically to the $GW$ approximation. In this new theory, the screened potential is reconnected to the physical response function, i.e. the covariant response function proposed in \cite{cGW_2023}, rather than using the RPA formula. We apply our scheme to calculate Green's function, the spectral function, and the charge compressibility in the two-dimensional Hubbard model. Our scheme yields significant qualitative and quantitative improvements over the standard $GW$ method and successfully captures the pseudogap behavior.

cond-mat.str-el

Quantum highway: Observation of minimal and maximal speed limits for few and many-body states

Tracking the time evolution of a quantum state allows one to verify the thermalization rate or the propagation speed of correlations in generic quantum systems. Inspired by the energy-time uncertainty principle, bounds have been demonstrated on the maximal speed at which a quantum state can change, resulting in immediate and practical tasks. Based on a programmable superconducting quantum processor, we test the dynamics of various emulated quantum mechanical systems encompassing single- and many-body states. We show that one can test the known quantum speed limits and that modifying a single Hamiltonian parameter allows the observation of the crossover of the different bounds on the dynamics. We also unveil the observation of minimal quantum speed limits in addition to more common maximal ones, i.e., the lowest rate of change of a unitarily evolved quantum state. Our results establish a comprehensive experimental characterization of quantum speed limits and pave the way for their subsequent study in engineered non-unitary conditions.

quant-ph

Competition between dimerization and vector chirality in the spin-$3/2$ $J_1$-$J_2$ Heisenberg chain with uniaxial single-ion anisotropy

The spin-$3/2$ chain is a versatile prototypical platform for the study of competition between different kinds of magnetic orders, with the objective of obtaining a deeper understanding of the corresponding quantum phase transitions. In this work, we investigate the spin-$3/2$ chain with nearest-neighbor $J_1$, next-nearest-neighbor $J_2$, and uniaxial single-ion anisotropy $D$ terms in the absence of a magnetic field. For positive values of $J_2/J_1$ and $D/J_1$, we find seven different phases in a rich phase diagram. Without frustration $J_2=0$, a gapless Luttinger liquid phase remains stable for all $D>0$. As $J_2$ increases, we observe three phases with distinct dimerized valence bond orders, which show an intricate competition with vector chiral order and incommensurate correlations. For large $J_2$, regions of phase coexistence between the dimerized and vector chiral orders emerge. We present large-scale numerical data for the determination of transition lines, order parameters, and the nature of the phase transitions.

cond-mat.str-el

Exotic d-wave Cooper Pair Bose Metal in two dimensions

The study of non-Fermi liquids sheds light on unconventional phenomena in condensed matter systems that lie beyond the scope of Landau Fermi liquid theory. One intriguing example is the Bose metal, characterized by an uncondensed bosonic ground state. However, constructing a Bose metal phase in two dimensions (2D) remains a significant challenge.} Utilizing constraint path quantum Monte Carlo and functional renormalization group methods on a fermionic system with spin anisotropy in a 2D lattice, we reveal the emergence of a Cooper pair Bose metal (CPBM) phase in a highly anisotropic regime ($\alpha < 0.30$) with wide range of filling, as proposed in [A. E. Feiguin and M. P. A. Fisher, Phys. Rev. Lett. 103, 025303 (2009)]. Our findings exhibit a visible nonzero momentum Bose surface in the Cooper-pair distribution function, accompanied by a distinct signal of $d_{xy}$ correlation between pairs. Our results highlight that spin-dependent anisotropy in the Fermi surface leads to versatile pairing forms. Platforms such as ultracold atoms in optical lattices and recently proposed altermagnets hold promise for realizing this intriguing phase.

cond-mat.supr-con

Diagnosing thermalization dynamics of non-Hermitian quantum systems via GKSL master equations

The application of the eigenstate thermalization hypothesis to non-Hermitian quantum systems has become one of the most important topics in dissipative quantum chaos, recently giving rise to intense debates. The process of thermalization is intricate, involving many time-evolution trajectories in the reduced Hilbert space of the system. By considering two different expansion forms of the density matrices adopted in the biorthogonal and right-state time evolutions, we have derived two versions of the Gorini-Kossakowski-Sudarshan-Lindblad master equations describing the non-Hermitian systems coupled to a bosonic heat bath in thermal equilibrium. By solving the equations, we have identified a sufficient condition for thermalization under both time evolutions, resulting in Boltzmann biorthogonal and right-eigenstate statistics, respectively. This finding implies that the recently proposed biorthogonal random matrix theory needs an appropriate revision. Moreover, we have exemplified the precise dynamics of thermalization and thermodynamic properties with test models.

quant-ph

Non-Hermitian sensing in the absence of exceptional points

Open systems possess unique potentials in high-precision sensing, yet the majority of previous studies rely on the spectral singularities known as exceptional points. Here we theoretically propose and experimentally demonstrate universal non-Hermitian sensing in the absence of exceptional points. The scheme makes use of the intrinsic sensitivity of a non-Hermitian probe to weak external fields, which can be understood as the direct consequence of non-Hermiticity. We confirm the basic mechanism by simulating the sensor-field dynamics using photon interferometry, and, as a concrete example, demonstrate the enhanced sensing of signals encoded in the setting angle of a wave plate. While the sensitivity of the probe is ultimately limited by the measurement noise, we find the non-Hermitian sensor showing superior performance under background noises that cannot be suppressed through repetitive measurements. Our experiment opens the avenue of enhanced sensing without exceptional points, complementing existing efforts aimed at harnessing the unique features of open systems.

quant-ph

Free-standing cubic gauche nitrogen stable at 760 K under ambient pressure

Cubic gauche nitrogen (cg-N) has received wide attention due to its high energy density and environmental friendliness. However, existing synthesis methods for cg-N predominantly rely on the high-pressure techniques, or the utilization of nanoconfined effects using highly toxic and sensitive sodium azide as precursor, which significantly restrict the practical application of cg-N as high energy density materials (HDEM). Here, based on the first-principles simulations, we find that the adsorption of potassium on the cg-N surface exhibits superior stabilization compared to sodium. Then, we chose the safer potassium azide as raw material for synthesizing cg-N. Through plasma-enhanced chemical vapor deposition treatment, the free-standing cg-N was successfully synthesized without the need of high-pressure and nanoconfined effects. Importantly, it demonstrates excellent thermal stability up to 760 K, and then a rapid and intense thermal decomposition occurs, exhibiting typical behaviors of HDEM thermal decomposition. Our work has significantly promoted the practical application of cg-N as HDEM.

cond-mat.mtrl-sci

Density-matrix renormalization group algorithm for non-Hermitian systems

A biorthonormal-block density-matrix renormalization group algorithm is proposed to accurately compute properties of large-scale non-Hermitian many-body systems, in which a renormalized-space partition of the non-Hermitian reduced density matrix is implemented to fulfill the prerequisite for the biorthonormality of the renormalization group (RG) transformation and to optimize the construction of saved Hilbert spaces. A redundancy in saved spaces of the reduced density matrix is exploited to reduce a condition number resulting from the non-unitarity of the left and right transformation matrices, in order to ensure the numerical stability of the RG procedure. The algorithm is successfully applied to an interacting fermionic Su-Schrieffer-Heeger model with nonreciprocal hoppings and staggered complex chemical potential, exhibiting novel many-body phenomena.

cond-mat.str-el

Experimental observation of the Yang-Lee quantum criticality in open systems

The Yang-Lee edge singularity was originally studied from the standpoint of mathematical foundations of phase transitions, and its physical demonstration has been of active interest both theoretically and experimentally. However, the presence of an imaginary magnetic field in the Yang-Lee edge singularity has made it challenging to develop a direct observation of the anomalous scaling with negative scaling dimension associated with this critical phenomenon. We experimentally implement an imaginary magnetic field and demonstrate the Yang-Lee edge singularity through a nonunitary evolution governed by a non-Hermitian Hamiltonian in an open quantum system, where a classical system is mapped to a quantum system via the equivalent canonical partition function. In particular, we directly observe the partition function in our experiment using heralded single photons. The nonunitary quantum criticality is identified with the singularity at an exceptional point. We also demonstrate unconventional scaling laws for the finite-temperature dynamics unique to quantum systems.

cond-mat.stat-mech

Experimental Simulation of Symmetry-Protected Higher-Order Exceptional Points with Single Photons

Exceptional points (EPs) of non-Hermitian (NH) systems have recently attracted increasing attention due to their rich phenomenology and intriguing applications. Compared to the predominantly studied second-order EPs, higher-order EPs have been assumed to play a much less prominent role because they generically require the tuning of more parameters. Here we experimentally simulate two-dimensional topological NH band structures using single-photon interferometry, and observe topologically stable third-order EPs obtained by tuning only two real parameters in the presence of symmetry. In particular, we explore how different symmetries stabilize qualitatively different third-order EPs: the parity-time symmetry leads to a generic cube-root dispersion, while a generalized chiral symmetry implies a square-root dispersion coexisting with a flat band. Additionally, we simulate fourfold degeneracies, composed of the non-defective twofold degeneracies and second-order EPs. Our work reveals the abundant and conceptually richer higher-order EPs protected by symmetries and offers a versatile platform for further research on topological NH systems.

cond-mat.mes-hall

Negative superinflating bipartite fluctuations near exceptional points in $\mathcal{PT}$-symmetric models

We investigate bipartite particle number fluctuations near the rank-$2$ exceptional points (EPs) of $\mathcal{PT}$-symmetric Su-Schrieffer-Heeger models. Beyond a conformal field theory of massless fermions, fluctuations or equivalently compressibility is negative definite and exhibits superinflation in leading order at EPs, due to the defectiveness in the biorthogonal Hilbert space. Associated with the bipartite von Neumann entanglement entropy, a parameter in an anomalous correspondence referencing from a purely non-Hermitian limit helps characterize two inequivalent EP sets. Our work paves the way for understanding the singularity of fluctuations relevant to EPs, more promisingly detectable in experiments.

cond-mat.mes-hall

Theoretical understanding of correlation between magnetic phase transition and the superconducting dome in high-Tc cuprates

Many issues concerning the origin of high-temperature superconductivity (HTS) are still under debate. For example, how the magnetic ordering varies with doping and its relationship with the superconducting temperature; and why the maximal Tc always occurs near the quantum critical point. In this paper, taking hole-doped La2CuO4 as a classical example, we employ the first-principles band structure and total energy calculations and Monte Carlo simulations to explore how the symmetry-breaking magnetic ground state evolves with hole doping and the origin of a dome-shaped superconductivity region in the phase diagram. We demonstrate that the local antiferromagnetic ordering and doping play key roles in determining the electron-phonon coupling, thus Tc. Initially, the La2CuO4 possesses a checkerboard local antiferromagnetic ground state. As the hole doping increases, Tc increases with the increase of the density of states at the Fermi surface. But as the doping increases further, the strength of the antiferromagnetic interaction weakens. At the critical doping level, a magnetic phase transition occurs that reduces the local antiferromagnetism-assisted electron-phonon coupling, thus diminishing the Tc. The superconductivity disappears in the heavily overdoped region when the antiferromagnetic ordering disappears. These observations could account for why cuprates have a dome-shaped superconductivity region in the phase diagram. Our study, thus, contributes to a fundamental understanding of the correlation between doping, local magnetic ordering, and superconductivity of HTS.

cond-mat.supr-con

Moiré Magnetic Exchange Interactions in Twisted Magnets

Besides moiré superlattice, twisting can also generate moiré magnetic exchange interactions (MMEIs) in van der Waals magnets. However, due to the extreme complexity and twist-angle-dependent sensitivity, all existing models fail to capture the MMEIs, preventing the understanding of MMEIs-induced new physics. Here, we develop a microscopic moiré spin Hamiltonian that enables the effective description of MMEIs via a sliding-mapping approach in twisted magnets, as demonstrated in twisted bilayer CrI3. Unexpectedly, we discover that the emergence of MMEIs can create an unprecedented magnetic skyrmion bubble (SkB) with non-conversed helicity, named as moiré-type SkB, representing a unique spin texture solely generated by MMEIs and ready to be detected under the current experimental conditions. Importantly, the size and population of SkBs can be finely controlled by twist angle, a key step for skyrmion-based quantum computing and information storage. Furthermore, we reveal that the MMEIs can be effectively manipulated by the substrate-induced interfacial Dzyaloshinskii-Moriya interaction, modulating the twist-angle-dependent magnetic phase diagram, which solves the outstanding disagreements between prior theories and experiments and verifies our theory.

cond-mat.mtrl-sci

Linear Response Functions Respecting Ward-Takahashi Identity and Fluctuation-Dissipation Theorem within $GW$ Approximation

The calculation of response functions in correlated electronic systems is one of the most important problems in the condensed matter physics. To obtain a physical response function, preserving both the Ward-Takahashi identity and the fluctuation-dissipation theorem are crucial. Here we propose a self-consistent many body method within the GW framework to calculate the response functions based on the fluctuation-dissipation theorem, which also satisfies the Ward-Takahashi identity. The validity of this methodology is demonstrated on the two-dimensional one-band Hubbard model, where both the Ward-Takahashi identity and fluctuation-dissipation theorem are verified numerically. Moreover, comparing to the accurate spin susceptibility of the determinantal Monte Carlo approach, the results obtained from our method are quite satisfactory and the computational cost are greatly reduced.

cond-mat.str-el

Quantum phase diagram for two species hardcore bosons in one-dimensional optical lattices with the resonantly driven Rabi frequency

We propose an experimental realization of the time-periodically modulated Rabi frequency and suggest density-dependent hoppings of two species hardcore bosons in a one-dimensional optical lattice. Distinct from the previous work [Phys. Rev. Research {\bf 2}, 013275 (2020)], we study effects in the first resonance region. In the effective Hamiltonian, the intra-species hopping occurs only if the density discrepancy of the other species on these sites is zero, while the inter-species one is allowed once the relevant density discrepancy becomes nonzero. At integer-$1$ filling, the quantum phase diagram of the effective Hamiltonian is determined by the perturbation analysis together with numerical calculations. We find that in the limit of dominant $J_{1}$, the system becomes a double-degenerate dimerized state, with spontaneously breaking the translation symmetry. The interplay of $J_{0}$, $J_{1}$ and the fixed ${\bar U}=1$ leads to three BKT transition lines and a tricritical BKT point. Exact transition lines are obtained by the level spectroscopic technique. Besides, general physical properties, including the charge gap, neutral gap, superfluid density and dimerization strength, are investigated as well.

cond-mat.quant-gas