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Hairun Guo

Publications and source records attributed to Hairun Guo.

At least 37 records · Page 2Linked to original sources

Emergent Nonlinear Phenomena in a Driven Dissipative Photonic Dimer

Emergent phenomena are ubiquitous in nature and refer to spatial, temporal, or spatiotemporal pattern formation in complex nonlinear systems driven out of equilibrium that is not contained in the microscopic descriptions at the single-particle level. Examples range from novel phases of matter in both quantum and classical many-body systems, to galaxy formation or neural dynamics. Two characteristic phenomena are length scales that exceed the characteristic interaction length and spontaneous symmetry breaking. Recent advances in integrated photonics indicate that the study of emergent phenomena is possible in complex coupled nonlinear optical systems. Here we demonstrate that out-of-equilibrium driving of a strongly coupled ("dimer") pair of photonic integrated Kerr microresonators, which at the "single-particle" (i.e. individual resonator) level generate well understood dissipative Kerr solitons, exhibit emergent nonlinear phenomena. By exploring the dimer phase diagram, we find unexpected and therefore unpredicted regimes of soliton hopping, spontaneous symmetry breaking, and periodically emerging (in)commensurate dispersive waves. These phenomena are not included in the single-particle description and related to the parametric frequency conversion between hybridized supermodes. Moreover, by controlling supermode hybridization electrically, we achieve wide tunability of spectral interference patterns between dimer solitons and dispersive waves. Our findings provide the first critical step towards the study of emergent nonlinear phenomena in soliton networks and multimode lattices.

nlin.PS↗

Nanophotonic soliton-based microwave synthesizers

Microwave photonic technologies, which upshift the carrier into the optical domain to facilitate the generation and processing of ultrawide-band electronic signals at vastly reduced fractional bandwidths, have the potential to achieve superior performance compared to conventional electronics for targeted functions. For microwave photonic applications such as filters, coherent radars, subnoise detection, optical communications and low-noise microwave generation, frequency combs are key building blocks. By virtue of soliton microcombs, frequency combs can now be built using CMOS compatible photonic integrated circuits, operated with low power and noise, and have already been employed in system-level demonstrations. Yet, currently developed photonic integrated microcombs all operate with repetition rates significantly beyond those that conventional electronics can detect and process, compounding their use in microwave photonics. Here we demonstrate integrated soliton microcombs operating in two widely employed microwave bands, X- and K-band. These devices can produce more than 300 comb lines within the 3-dB-bandwidth, and generate microwave signals featuring phase noise levels below 105 dBc/Hz (140 dBc/Hz) at 10 kHz (1 MHz) offset frequency, comparable to modern electronic microwave synthesizers. In addition, the soliton pulse stream can be injection-locked to a microwave signal, enabling actuator-free repetition rate stabilization, tuning and microwave spectral purification, at power levels compatible with silicon-based lasers (<150 mW). Our results establish photonic integrated soliton microcombs as viable integrated low-noise microwave synthesizers. Further, the low repetition rates are critical for future dense WDM channel generation schemes, and can significantly reduce the system complexity of photonic integrated frequency synthesizers and atomic clocks.

physics.optics↗

Dynamics of soliton crystals in optical microresonators

Dissipative Kerr solitons in optical microresonators provide a unifying framework for nonlinear optical physics with photonic-integrated technologies and have recently been employed in a wide range of applications from coherent communications to astrophysical spectrometer calibration. Dissipative Kerr solitons can form a rich variety of stable states, ranging from breathers to multiple-soliton formations, among which, the recently discovered soliton crystals stand out. They represent temporally-ordered ensembles of soliton pulses, which can be regularly arranged by a modulation of the continuous-wave intracavity driving field. To date, however, the dynamics of soliton crystals remains mainly unexplored. Moreover, the vast majority of the reported crystals contained defects - missing or shifted pulses, breaking the symmetry of these states, and no procedure to avoid such defects was suggested. Here we explore the dynamical properties of soliton crystals and discover that often-neglected chaotic operating regimes of the driven optical microresonator are the key to their understanding. In contrast to prior work, we prove the viability of deterministic generation of $\mathrm{perfect}$ soliton crystal states, which correspond to a stable, defect-free lattice of optical pulses inside the cavity. We discover the existence of critical pump power, below which the stochastic process of soliton excitation suddenly becomes deterministic enabling faultless, device-independent access to perfect soliton crystals. Furthermore, we demonstrate the switching of soliton crystal states and prove that it is also tightly linked to the pump power and is only possible in the regime of transient chaos. Finally, we report a number of other dynamical phenomena experimentally observed in soliton crystals including the formation of breathers, transitions between soliton crystals, their melting, and recrystallization.

physics.optics↗

Nanophotonic supercontinuum based mid-infrared dual-comb spectroscopy

High resolution and fast detection of molecular vibrational absorption is important for organic synthesis, pharmaceutical process and environmental monitoring, and is enabled by mid-infrared (mid-IR) laser frequency combs via dual-comb spectroscopy. Here, we demonstrate a novel and highly simplified approach to broadband mid-IR dual-comb spectroscopy via supercontinuum generation, achieved using unprecedented nanophotonic dispersion engineering that allows for flat-envelope, ultra-broadband mid-IR comb spectra. The mid-IR dual-comb has an instantaneous bandwidth covering the functional group region from 2800-3600 1/cm, comprising more than 100,000 comb lines, enabling parallel gas-phase detection with a high sensitivity, spectral resolution, and speed. In addition to the traditional functional groups, their isotopologues are also resolved in the supercontinuum based dual-comb spectroscopy. Our approach combines well established fiber laser combs, digital coherent data averaging, and integrated nonlinear photonics, each in itself a state-of-the-art technology, signalling the emergence of mid-IR dual-comb spectroscopy for use outside of the protected laboratory environment.

physics.optics↗

Spectral purification of microwave signals with disciplined dissipative Kerr solitons

Continuous-wave-driven Kerr nonlinear microresonators give rise to self-organization in terms of dissipative Kerr solitons, which constitute optical frequency combs that can be used to generate low-noise microwave signals. Here, by applying either amplitude or phase modulation to the driving laser we create an intracavity potential trap, to discipline the repetition rate of the solitons. We demonstrate that this effect gives rise to a novel spectral purification mechanism of the external microwave signal frequency, leading to reduced phase noise of the output signal. We experimentally observe that the microwave signal generated from disciplined solitons follows the external drive at long time scales, but exhibits an unexpected suppression of the fast timing jitter. Counter-intuitively, this filtering takes place for frequencies that are substantially lower than the cavity decay rate. As a result, while the long-time-scale stability of the Kerr frequency comb repetition rate is improved by more than 4 orders of magnitude as a result of locking to the external microwave signal, the soliton stream shows a reduction of the phase noise by 30 dB at offset frequencies above 10 kHz.

physics.app-ph↗

Detuning-dependent Properties and Dispersion-induced Instabilities of Temporal Dissipative Kerr Solitons in Optical Microresonators

Temporal-dissipative Kerr solitons are self-localized light pulses sustained in driven nonlinear optical resonators. Their realization in microresonators has enabled compact sources of coherent optical frequency combs as well as the study of dissipative solitons. A key parameter of their dynamics is the effective-detuning of the pump laser to the thermally- and Kerr-shifted cavity resonance. Together with the free spectral range and dispersion, it governs the soliton-pulse duration, as predicted by an approximate analytical solution of the Lugiato-Lefever equation. Yet, a precise experimental verification of this relation was lacking so far. Here, by measuring and controlling the effective-detuning, we establish a new way of stabilizing solitons in microresonators and demonstrate that the measured relation linking soliton width and detuning deviates by less than 1 % from the approximate expression, validating its excellent predictive power. Furthermore, a detuning-dependent enhancement of specific comb lines is revealed, due to linear couplings between mode-families. They cause deviations from the predicted comb power evolution, and induce a detuning-dependent soliton recoil that modifies the pulse repetition-rate, explaining its unexpected dependence on laser-detuning. Finally, we observe that detuning-dependent mode-crossings can destabilize the soliton, leading to an unpredicted soliton breathing regime (oscillations of the pulse) that occurs in a normally-stable regime. Our results test the approximate analytical solutions with an unprecedented degree of accuracy and provide new insights into dissipative-soliton dynamics.

physics.optics↗

Electrically pumped photonic integrated soliton microcomb

Optical frequency combs have revolutionized frequency metrology and timekeeping, and can be used in a wide range of optical technologies. Advances are under way that allow dramatic miniaturization of optical frequency combs using Kerr nonlinear optical microresonators, where broadband and coherent optical frequency combs can be generated from a continuous wave laser. Such `microcombs', provide a broad bandwidth with low power consumption, unprecedented form factor, wafer scale fabrication compatibility. For future high volume applications, integration and electrical pumping of soliton microcombs is essential. To date, however, microcombs still rely on optical pumping by bulk external laser modules that provide the required coherence, frequency agility and power levels for soliton formation. Electrically-driven, chip-integrated microcombs are inhibited by the high threshold power for soliton formation, typically exceeding the power of integrated silicon based lasers, and the required frequency agility for soliton initiation. Recent advances in high-Q Si3N4 microresonators suggest that electrically driven soliton microcombs are possible. Here we demonstrate an electrically-driven, chip-integrated soliton microcomb by coupling an indium phosphide (III-V) multiple-longitudinal-mode laser diode chip to a high-Q Si3N4 photonic integrated microresonator. We observe that self-injection locking of the laser diode to the microresonator, which is accompanied by a x1000 fold narrowing of the laser linewidth, can simultaneously initiate the formation of dissipative Kerr solitons. By tuning the current, we observe a transition from modulation instability, breather solitons to single soliton states. The system requires less than 1 Watt of electrical power, operates at electronically-detectable sub-100 GHz mode spacing and can fit in a volume of ca. 1cm3.

physics.optics↗

Ultralow-power chip-based soliton microcombs for photonic integration

The generation of dissipative Kerr solitons in optical microresonators has provided a route to compact frequency combs of high repetition rate, which have already been employed for optical frequency synthesizers, ultrafast ranging, coherent telecommunication and dual-comb spectroscopy. Silicon nitride (Si$_3$N$_4$) microresonators are promising for photonic integrated soliton microcombs. Yet to date, soliton formation in Si$_3$N$_4$ microresonators at electronically detectable repetition rates, typically less than 100 GHz, is hindered by the requirement of external power amplifiers, due to the low quality ($Q$) factors, as well as by thermal effects which necessitate the use of frequency agile lasers to access the soliton state. These requirements complicate future photonic integration, heterogeneous or hybrid, of soliton microcomb devices based on Si$_3$N$_4$ microresonators with other active or passive components. Here, using the photonic Damascene reflow process, we demonstrate ultralow-power single soliton formation in high-Q ($Q_0>15\times10^6$) Si$_3$N$_4$ microresonators with 9.8 mW input power (6.2 mW in the waveguide) for devices of electronically detectable, 99 GHz repetition rate. We show that solitons can be accessed via simple, slow laser piezo tuning, in many resonances in the same sample. These power levels are compatible with current silicon-photonics-based lasers for full photonic integration of soliton microcombs, at repetition rates suitable for applications such as ultrafast ranging and coherent communication. Our results show the technological readiness of Si$_3$N$_4$ optical waveguides for future all-on-chip soliton microcomb devices.

physics.optics↗

Highly efficient 4 micron light generation through fs-fiber laser driven supercontinuum in Si$_3$N$_4$ waveguides

Directly accessing the middle infrared, the molecular functional group spectral region, via supercontinuum generation processes based on turn-key fiber lasers offers the undeniable advantage of simplicity and robustness. Recently, the assessment of the coherence of the mid-IR dispersive wave in silicon nitride waveguides, pumped at telecom wavelength, established an important first step towards mid-IR frequency comb generation based on such compact systems. Yet, the spectral reach and efficiency still fall short for practical implementation. Here, we experimentally demonstrate for the first time to our knowledge, that fs-fiber laser driven systems based on large-cross section silicon nitride waveguides can reach, with powers sufficient to drive dual-comb spectroscopy, the important greenhouse gases spectral region near 4 micron, typically accessed through different frequency generation or more complex approaches. We show, from a 2 micron femtosecond fiber laser, up to 30% power conversion and milliwatt-level output powers, proving that such sources are suitable candidate for compact, chip-integrated spectroscopic and sensing applications.

physics.optics↗

Double inverse nanotapers for efficient light coupling to integrated photonic devices

Efficient light coupling into integrated photonic devices is of key importance to a wide variety of applications. "Inverse nanotapers" are widely used, in which the waveguide width is reduced to match an incident mode. Here, we demonstrate novel, "double inverse" tapers, in which we taper both the waveguide height, as well as the width. We demonstrate that in comparison to regular inverse tapers, the double inverse tapers have excellent polarization-independent coupling. In addition, the optimum coupling is achieved with much larger taper dimension, enabling the use of photolithography instead of electron beam lithography, relevant for applications at near-IR and visible wavelengths. The low coupling loss makes them particularly suitable for nonlinear photonics, e.g. supercontinuum and soliton micro-comb generation.

physics.app-ph↗

Mid-infrared frequency comb generation with silicon nitride nano-photonic waveguides

Mid-infrared optical frequency combs are of significant interest for molecular spectroscopy due to the large absorption of molecular vibrational modes on one hand, and the ability to implement superior comb-based spectroscopic modalities with increased speed, sensitivity and precision on the other hand. Substantial advances in mid-infrared frequency comb generation have been made in recent years based on nonlinear frequency conversion, microresonator Kerr frequency combs, quantum cascade lasers and mode locking regimes. Here we demonstrate a simple, yet effective method for the direct generation of mid-infrared optical frequency combs in the region from ${2.5-4~μ{\rm m}}$, i.e. ${2500-4000~{\rm cm}^{-1}}$ covering a large fraction of the functional group region, directly from a conventional and compact erbium-fiber-based femtosecond laser in the telecommunication band (i.e. ${1.55~μ{\rm m}}$). The wavelength conversion is based on dispersive wave generation within the supercontinuum process in large-cross-section and dispersion-engineered silicon nitride (${\rm Si_3N_4}$) waveguides. The long-wavelength dispersive wave, with its position lithographically determined, performs as a mid-infrared frequency comb, whose coherence is demonstrated via optical heterodyne measurements. Such a simple and versatile approach to mid-infrared frequency comb generation is suitable for spectroscopic applications in the first mid-infrared atmospheric window. Moreover, the compactness and simplicity of the approach have the potential to realize compact dual-comb spectrometers. The generated combs have a fine teeth-spacing, making them also suitable for gas phase analysis.

physics.optics↗

Inter-mode breather solitons in optical microresonators

The observation of temporal dissipative Kerr solitons in optical microresonators provides, on the applied side, compact sources of coherent optical frequency combs that have already been applied in coherent communications, dual comb spectroscopy and metrology. On a fundamental level, it enables the study of soliton physics in driven nonlinear cavities. Microresonators are commonly multimode and, as a result, inter-mode interactions inherently occur among mode families - a condition referred to as "avoided mode crossings". Avoided mode crossings can cause soliton decay, but can also modify the soliton spectrum, leading to e.g. the formation of dispersive wave and inducing a spectral recoil. Yet, to date, the entailing temporal soliton dynamics from inter-mode interactions has rarely been studied, but is critical to understand regimes of soliton-stability. Here we report the discovery of an inter-mode breather soliton. Such breathing dynamics occurs within a laser detuning range where conventionally stationary dissipative solitons are expected. We demonstrate experimentally the phenomenon in two microresonator platforms (crystalline magnesium fluoride and photonic chip-based silicon nitride microresonators), and theoretically describe the dynamics based on a pair of coupled Lugiato-Lefever equations. We demonstrate experimentally that the breathing is associated with a periodic energy exchange between the soliton and another optical mode family. We further show that inter-mode interactions can be modeled by a response function acting on dissipative solitons. The observation of breathing dynamics in the conventionally stable soliton regime is critical to applications, ranging from low-noise microwave generation, frequency synthesis to spectroscopy. On a fundamental level, our results provide new understandings of the rich dissipative soliton dynamics in multimode nonlinear cavities.

physics.optics↗

Octave-spanning dissipative Kerr soliton frequency combs in $Si_3N_4$ microresonators

Octave-spanning, self-referenced frequency combs are applied in diverse fields ranging from precision metrology to astrophysical spectrometer calibration. In the past decade, Kerr frequency comb generators have emerged as alternative scheme offering chip-scale integration, high repetition rate and bandwidths that are only limited by group velocity dispersion. The recent observation of Kerr frequency combs operating in the dissipative Kerr soliton (DKS) regime, along with dispersive wave formation, has provided the means for fully coherent, broadband Kerr frequency comb generation with engineered spectral envelope. Here, by carefully optimizing the photonic Damascene fabrication process, and dispersion engineering of $\mathrm{Si_{3}N_{4}}$ microresonators with $1\,\mathrm{THz}$ free spectral range, we achieve bandwidths exceeding one octave at low powers ($\mathcal{O}(100\,\mathrm{mW})$) for pump lasers residing in the telecom C-band ($1.55\,\mathrm{μm}$), as well as for the first time in the O-band ($1.3\,\mathrm{μm}$). Equally important, we find that for THz repetition rate comb states, conventional criteria applied to identify DKS comb states fail. Investigating the coherence of generated, octave-spanning Kerr comb states we unambiguously identify DKS states using a response measurement. This allows to demonstrate octave-spanning DKS comb states at both pump laser wavelengths of $1.3\mathrm{\,μm}$ and $1.55\,\mathrm{μm}$ including the broadest DKS state generated to date, spanning more than $200\,\mathrm{THz}$ of optical bandwidth. Octave spanning DKS frequency combs can form essential building blocks for metrology or spectroscopy, and their operation at $1.3\mathrm{\,μm}$ enables applications in life sciences such as Kerr comb based optical coherence tomography or dual comb coherent antistokes Raman scattering.

physics.optics↗

Breathing dissipative solitons in optical microresonators

Dissipative solitons are self-localized structures resulting from a double balance between dispersion and nonlinearity as well as dissipation and a driving force. They occur in a wide variety of fields ranging from optics, hydrodynamics to chemistry and biology. Recently, significant interest has focused on their temporal realization in driven optical microresonators, known as dissipative Kerr solitons. They provide access to coherent, chip-scale optical frequency combs, which have already been employed in optical metrology, data communication and spectroscopy. Such Kerr resonator systems can exhibit numerous localized intracavity patterns and provide rich insights into nonlinear dynamics. A particular class of solutions consists of breathing dissipative solitons, representing pulses with oscillating amplitude and duration, for which no comprehensive understanding has been presented to date. Here, we observe and study single and multiple breathing dissipative solitons in two different microresonator platforms: crystalline $\mathrm{MgF_2}$ resonator and $\mathrm{Si_3N_4}$ integrated microring. We report a deterministic route to access the breathing state, which allowed for a detailed exploration of the breathing dynamics. In particular, we establish the link between the breathing frequency and two system control parameters - effective pump laser detuning and pump power. Using a fast detection, we present a direct observation of the spatiotemporal dynamics of individual solitons, revealing irregular oscillations and switching. An understanding of breathing solitons is not only of fundamental interest concerning nonlinear systems close to critical transition, but also relevant for applications to prevent breather-induced instabilities in soliton-based frequency combs.

physics.optics↗

Frequency Comb Assisted Broadband Precision Spectroscopy with Cascaded Diode Lasers

Frequency comb assisted diode laser spectroscopy, employing both the accuracy of an optical frequency comb and the broad wavelength tuning range of a tunable diode laser, has been widely used in many applications. In this letter we present a novel method using cascaded frequency agile diode lasers, which allows extending the measurement bandwidth to 37.4 THz (1355 to 1630 nm) at MHz resolution with scanning speeds above 1 THz/s. It is demonstrated as a useful tool to characterize a broadband spectrum for molecular spectroscopy and in particular it enables to characterize the dispersion of integrated microresonators up to the fourth order.

physics.optics↗

Higher order mode suppression in high-Q anomalous dispersion SiN microresonators for temporal dissipative Kerr soliton formation

High-Q silicon nitride (SiN) microresonators enable optical Kerr frequency comb generation on a photonic chip and have recently been shown to support fully coherent combs based on temporal dissipative Kerr soliton formation. For bright soliton formation it is necessary to operate SiN waveguides in the multimode regime so as to produce anomalous group velocity dispersion. This can lead to local disturbances of the dispersion due to avoided crossings caused by coupling between different mode families, and therefore prevent the soliton formation. Here we demonstrate that a single mode "filtering" section inside high-Q resonators enables to efficiently suppress avoided crossings, while preserving high quality factors (Q~10^6). We demonstrate the approach by single soliton formation in SiN resonators with filtering section.

physics.optics↗

Raman induced soliton self-frequency shift in microresonator Kerr frequency combs

The formation of temporal dissipative solitons in continuous wave laser driven microresonators enables the generation of coherent, broadband and spectrally smooth optical frequency combs as well as femtosecond pulses with compact form factor. Here we report for the first time on the observation of a Raman-induced soliton self-frequency shift for a microresonator soliton. The Raman effect manifests itself in amorphous SiN microresonator based single soliton states by a spectrum that is hyperbolic secant in shape, but whose center is spectrally red-shifted (i.e. offset) from the continuous wave pump laser. The Raman induced spectral red-shift is found to be tunable via the pump laser detuning and grows linearly with peak power. The shift is theoretically described by the first order shock term of the material's Raman response, and we infer a Raman shock time of 20 fs for amorphous SiN. Moreover, we observe that the Raman induced frequency shift can lead to a cancellation or overcompensation of the soliton recoil caused by the formation of a (coherent) dispersive wave. The observations are in excellent agreement with numerical simulations based on the Lugiato-Lefever equation (LLE) with a Raman shock term. Our results contribute to the understanding of Kerr frequency combs in the soliton regime, enable to substantially improve the accuracy of modeling and are relevant to the fundamental timing jitter of microresonator solitons.

physics.optics↗

Mid-IR femtosecond frequency conversion by soliton-probe collision in phase-mismatched quadratic nonlinear crystals

We show numerically that ultrashort self-defocusing temporal solitons colliding with a weak pulsed probe in the near-IR can convert the probe to the mid-IR. A near-perfect conversion efficiency is possible for a high effective soliton order. The near-IR self-defocusing soliton can form in a quadratic nonlinear crystal (beta-barium borate) in the normal dispersion regime due to cascaded (phase-mismatched) second-harmonic generation, and the mid-IR converted wave is formed in the anomalous dispersion regime between $λ=2.2-2.4~μ\rm m$ as a resonant dispersive wave. This process relies on non-degenerate four-wave mixing mediated by an effective negative cross-phase modulation term caused by cascaded soliton-probe sum-frequency generation.

physics.optics↗