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Hairun Guo

Publications and source records attributed to Hairun Guo.

At least 19 recordsLinked to original sources

Harnessing thermo-optic dynamics for frequency-agile soliton microcombs

Dissipative Kerr soliton microcombs enable compact and scalable frequency comb sources for precision metrology, spectroscopy, communications and coherent LiDAR, where broad and reliable frequency tuning is essential. Thermo-optic response can support thermal locking during soliton operation, enabling resonance tracking and thereby extending the tuning range, albeit modestly. However, it also induces pronounced thermal instability during soliton initiation, hindering reliable access to this extended operating regime and limiting practical deployment in applications requiring frequency agility. Here we show that strong mode coupling reshapes the effective detuning trajectory governing soliton formation, establishing a distinct operating regime in which thermo-optic response is significantly reinforced and constructively harnessed. In this regime, soliton formation proceeds without the thermal instability inherent to conventional operation, enabling robust soliton generation in material platforms previously limited by strong thermal effects. Importantly, the enhanced thermo-optic response strengthens thermal locking during soliton operation, enabling more effective resonance tracking and substantially extending the tuning range. Leveraging this regime in AlGaAs-on-insulator multimode microresonators, we demonstrate soliton generation with a tuning range approaching 100 GHz at a pump power of 32 mW. The same mechanism further enables frequency-agile operation through direct pump-frequency tuning without auxiliary stabilization, allowing massively parallel chirped comb generation with more than 90 channels exhibiting frequency excursions exceeding 10 GHz. These results establish a general operating principle for transforming thermo-optic effects from a limiting factor into an active resource, enabling robust and frequency-agile integrated soliton microcombs.

physics.optics

Mid-infrared-to-ultraviolet supercontinuum generation in low-loss tantalum pentoxide nanophotonic waveguides

Optical frequency combs on photonic integrated platforms are revolutionizing precision metrology, bio-imaging, atomic and molecular sensing, and ultrafast photonics, yet most remain confined to the near-infrared. This restriction prevents access to the ultraviolet, visible, and mid-infrared bands critical for a vast array of quantum, atomic, and molecular systems. The fundamental obstacle has been the lack of a nanophotonic waveguide that simultaneously provides an ultra-broad transparency window, engineered dispersion, ultra-low propagation loss, and a strong Kerr nonlinearity, all while suppressing detrimental two-photon absorption at short wavelengths. Here, we overcome this challenge by exploring tantalum pentoxide for ultra-broadband supercontinuum spanning continuously from the ultraviolet to the mid-infrared, leveraging its broad transparency window (300-8000 nm), a high nonlinear refractive index three times larger than that of silicon nitride, and a wide bandgap that suppresses two-photon absorption. Critically, by using a photolithography assisted chemo-mechanical etching process that avoids a lossy SiO2 upper cladding, we achieve dispersion engineered waveguides with record-low propagation losses of 0.066 dB/cm at telecom wavelengths and 0.43 dB/cm at 780 nm, significantly facilitating the supercontinuum spectral extension into the ultraviolet and the mid-infrared. Pumping these anomalous-dispersion waveguides with femtosecond pulses at 1550 nm yields a gap-free, 3.2-octave supercontinuum spanning from 350 to 3200 nm via a soliton-based dynamics at only 54 pJ pulse energy, representing the broadest comb spectrum on this platform. We further demonstrate a relatively flat spectrum with a -30 dB bandwidth of 1182 nm by engineering normal dispersion, validate the comb coherence via heterodyne detection, and achieve soliton-effect pulse self-compression from 126.7 fs to 19.2 fs.

physics.optics

High-speed mid-infrared single-photon upconversion spectrometer

Sensitive and fast mid-infrared (MIR) spectroscopy is highly attractive in a variety of applications including astronomical observation, pharmaceutical synthesis, and environmental monitoring. However, the performance of conventional MIR spectrometers has long been hindered by the limited sensitivity of narrow-bandgap detectors and/or the deficient brightness of broadband light sources. Here, we devise and implement an ultra-sensitive and broadband MIR upconversion spectrometer, which integrates a supercontinuum source covering 1.5-4.2 $\mu$m based on a silicon nitride nanophotonic waveguide. High-efficiency and low-noise nonlinear frequency upconversion is realized based on coincidence pulsed pumping with spectro-temporal optimization, which enables to leverage silicon detectors for facilitating MIR single-photon spectroscopy at 0.2 photons/nm/pulse. Furthermore, the upconversion-based array spectrometer is manifested with high-speed spectral acquisition rates beyond 200 kHz, which is about ten-fold faster than the state-of-the-art scan rates for FTIR-based spectrometers at a comparable spectral resolution. The achieved features of broadband spectral coverage, single-photon sensitivity, and sub-MHz refreshing rate might open up new possibilities in infrared transient spectral measurements in combustion analysis, high-throughput sorting and reaction tracking, among others.

physics.optics

Single-photon time-stretch infrared spectroscopy

Sensitive mid-infrared (MIR) spectroscopy is highly demanded in various fields ranging from industrial inspection, biomedical diagnosis to astronomical observation. However, the detection sensitivity of conventional MIR spectrometers has been severely limited by excessive noises for existing infrared sensors, which hinders widespread use in photon-scarce scenarios. Here, we devise and implement a broadband MIR single-photon time-stretch spectrometer based on high-fidelity spectral upconversion and time-correlated coincidence counting. Specifically, a nanophotonic supercontinuum illumination covering 2.4-4.2 $\mu$m is nonlinearly converted to the near-infrared band, where low-loss single-mode fiber and high-performance silicon detector can be leveraged to facilitate dispersive operation and sensitive detection, respectively. The arrival time for the dispersed upconversion photons is precisely registered with a low-timing-jitter photon counter, which enables us to obtain a high spectral resolution about 0.5 cm$^{-1}$ under a low-light-level illumination down to 0.14 photons/nm/pulse. In comparison to previous MIR upconversion spectrometers, the presented time-stretch architecture favors single-pixel simplicity and high-throughput acquisition for the single-photon spectral measurement. The achieved MIR spectroscopic features of broadband spectral coverage, sub-wavenumber resolution, single-photon sensitivity, and room-temperature operation would stimulate immediate applications in material and life sciences.

physics.optics

Mid-Infrared Single-Photon Compressive Spectroscopy

Sensitive mid-infrared (MIR) spectroscopy plays an indispensable role in various photon-starved conditions. However, the detection sensitivity of conventional MIR spectrometers is severely limited by excessive noises of the involved infrared sensors, especially for multi-pixel arrays in parallel spectral acquisition. Here, we devise and implement an ultra-sensitive MIR single-pixel spectrometer, which relies on high-fidelity spectral upconversion and wavelength-encoding compressive measurement. Specifically, a MIR nanophotonic supercontinuum from 3.1 to 3.9 $\mu$m is nonlinearly converted to the near-infrared band via synchronous chirped-pulse pumping, which facilitates both the precise spectral mapping and sensitive upconversion detection. The upconverted signal is then spatially dispersed onto a programmable digital micromirror device, before being registered by a single-element silicon detector. Consequently, the spectral information can be deciphered from the correlation between encoded patterns and recorded measurements, which results in a spectral resolution of 0.5 cm$^{-1}$ under an illumination flux down to 0.01 photons/nm/pulse. Moreover, we demonstrate faithful reconstructions at sub-Nyquist sampling rates by using the compressive sensing algorithm, which leads to a 95\% reduction in data acquisition time. The presented single-pixel computational spectrometer features wavelength multiplexing, high throughput, and efficient sampling, which thus paves a new way for sensitive and fast spectroscopic analysis at the single-photon level.

physics.optics

Metrology-grade mid-infrared spectroscopy for multi-dimensional perception

The mid-infrared spectral window is essential for molecular fingerprinting and atmospheric sensing, yet unlocking its full potential is currently constrained by a fundamental instrumental trade-off: existing systems cannot simultaneously deliver broad bandwidth, high photon flux, and metrological frequency fidelity. Here, we resolve this bottleneck by demonstrating a metrology-grade spectroscopic system based on difference frequency generation, driven by widely tunable, near-infrared diode lasers traceable to atomic standards. Our system achieves continuous tunability across the 3-3.7 $\mu$m atmospheric window and delivers output power exceeding 45 mW with an absolute frequency accuracy of 7.2 MHz. We harness this convergence to overcome a critical barrier in integrated photonics, unambiguously identifying and eliminating hydrogen-induced absorption in silicon nitride microresonators to achieve an 88-fold reduction in optical loss. We further reveal multi-phonon absorption in the silica cladding as the fundamental limit to mid-infrared integrated photonics. Finally, we demonstrate the system's versatility through scattering-resilient LiDAR capable of penetrating optically dense fog, and dual-modality sensing that simultaneously retrieves target distance and chemical composition. By unifying the rigor of frequency metrology with the versatility of broadband sensing, this architecture establishes a new paradigm for multi-dimensional perception in complex environments.

physics.optics

Photonic electrometry using a piezoelectric-Pockels microresonator

Facilitated by low-noise laser frequency locking, optical microresonators with the Pockels effect have shown unprecedented high resolutions in sensing electrical field. However, the requirement for tunable and low-noise laser sources considerably increases the cost and the size of the system, thereby limiting the industrial applicability of the microresonator-based technology. Here, we explore the possibility of using a low-cost fixed-frequency semiconductor laser as the pump laser to perform radiofrequency electrometry. A resonant mode in a lithium niobate microresonator is frequency-locked to the laser using the electrooptic effect. This same effect also underlies the radiofrequency electric-field sensing mechanism. Our experimental results show that the electrometry resolution can be maintained at signal frequencies beyond the optical resonance bandwidth and that the signal-to-noise ratio does not change with varied coupling conditions as long as the laser frequency noise is the dominant noise source of the system. In addition, narrowband electrooptic sensitivity enhancement is observed at frequencies of the microresonator's piezoelectric resonances, resulting in a resolution enhancement factor of approximately 3 at signal frequencies around 4 MHz. Our work advances the photonic resonant electrometry technology by studying the bandwidth limitation, and opens the road to the employment of low-cost lasers in high-resolution sensing applications.

physics.optics

1-GHz VIS-to-MIR frequency combs enabled by CMOS-compatible nanophotonic waveguides

A fully stabilized frequency comb is essential for precision metrology and coherent optical synthesis. However, fully-stabilized frequency combs generally require separate stages for supercontinuum generation (SCG) and self-referencing, largely limiting their compactness. Here, enabled by the low-threshold multi-octave supercontinuum generation and concurrent third-harmonic generation in low-loss silicon nitride waveguides, we present a novel approach to a self-referenced frequency comb source at 1 GHz repetition rate spanning from the full visible (VIS) to the mid-infrared (MIR). Our coherent comb is seeded by an all-polarization-maintaining ultrafast fiber laser at 1556 nm, with a pulse duration of 73 fs at 1 GHz repetition rate. With an injected energy of merely 110 pJ, the pulses propagate through dispersion-engineered Si3N4 waveguides, generating supercontinuum spanning over three octaves from 350-3280 nm i.e. 0.76 PHz of coherent bandwidth. Moreover, the on-chip third harmonic generation provides a carrier envelope offset beat note via f-3f with a signal-to-noise ratio of 43 dB. Fueled by the evolving photonic integration providing possibilities of on-chip filtering and photo-detectors, this approach for single-chip self-referencing of high-repetition-rate frequency combs paves the way for ultrabroadband comb sources with unprecedented compactness and field-readiness.

physics.optics

Laser transfer and retrieval via nanophotonic supercontinuum process

The nature of optical metrology is to perform efficient transfer and precise retrieval for lasers and optical signals, which is beneficial for a variety of applications ranging from optical clocking, spectroscopy, to telecommunications and quantum optics. While efforts have been made to promote the detection accuracy of optical frequencies, retrieval on optical waveforms remains on the autocorrelation scheme with limited performances. Here, we demonstrate a novel scheme for optical metrology, particularly on direct retrieval of optical waveform in terms of the field amplitude profile. The scheme is based on massive four-wave-mixings underlying a nanophotonic supercontinuum process, which enables arbitrary transfer of an additive laser to modulational sidebands of the broadened continuum. Detection of the transferred signals is then flexible to be within the whole span of the supercontinuum from visible to the mid-infrared range. We demonstrate such a transfer scheme for both CW lasers and pulsed lasers. For the latter, the temporal amplitude profile of the optical wave can be retrieved, which reveals high-order dynamics of solitary pulses including the self-steepening, self-compression, and the soliton splitting, and shows a remarkable square-fold increase of signal-to-noise ratio in the power spectrum. Our results may contribute to advance optical metrology particularly towards chip scale optical waveform detection, and more fundamentally, they reveal insights of massive ultrafast nonlinear interactions underlying the soliton-based supercontinuum process.

physics.optics

2.7-octave supercontinuum generation spanning from ultraviolet to near-infrared in thin-film lithium niobate waveguides

Supercontinuum generation (SCG) with spectral coverage across the full visible and ultraviolet (UV) ranges is crucial for optical clocks, quantum computing and sensing. However, achieving such SCG in nanophotonic platforms is challenging due to the difficulties in spectrum broadening. Here, Such ultrabroad-bandwidth SCG was demonstrated in thin-film lithium niobate (TFLN) nanophotonic waveguides by dispersion management, without periodic poling for spectral broadening. Anomalous-dispersion waveguides were designed in the telecom band, simultaneously enabling dispersive wave emergence, modal-matched second harmonic generation, and third harmonic generation for spectrum broadening. Moreover, MgO was intentionally doped to mitigate the photorefractive effect of lithium niobate, which frequently results in un-sustained spectrum broadening and in turn limits the accessible SCG coverage. By leveraging photolithography assisted chemo-mechanical etching, low-loss MgO doped TFLN nanophotonic waveguides were fabricated. As a result, thanks to the utilization of the strong second-order and third-order nonlinear processes, gap-free 2.7-octave SCG spanning from 330 nm to 2250 nm was observed by pumping the waveguide with a 1550-nm femtosecond pulsed laser with 0.687 nJ, agreeing well with numerical simulation. This spectral coverage represents the state of the art in TFLN platforms without fine microdomains, and even close to the record in sophisticated chirped periodically poled TFLN waveguides.

physics.optics

A wideband, high-resolution vector spectrum analyzer for integrated photonics

The analysis of optical spectra - emission or absorption -- has been arguably the most powerful approach for discovering and understanding matters. The invention and development of many kinds of spectrometers have equipped us with versatile yet ultra-sensitive diagnostic tools for trace gas detection, isotope analysis, and resolving hyperfine structures of atoms and molecules. With proliferating data and information, urgent and demanding requirements have been placed today on spectrum analysis with ever-increasing spectral bandwidth and frequency resolution. These requirements are especially stringent for broadband laser sources that carry massive information, and for dispersive devices used in information processing systems. In addition, spectrum analyzers are expected to probe the device's phase response where extra information is encoded. Here we demonstrate a novel vector spectrum analyzer (VSA) that is capable of characterizing passive devices and active laser sources in one setup. Such a dual-mode VSA can measure loss, phase response and dispersion properties of passive devices. It also can coherently map a broadband laser spectrum into the RF domain. The VSA features a bandwidth of 55.1 THz (1260 to 1640 nm), frequency resolution of 471 kHz, and dynamic range of 56 dB. Meanwhile, our fiber-based VSA is compact and robust. It requires neither high-speed modulators and photodetectors, nor any active feedback control. Finally, we successfully employ our VSA for applications including characterization of integrated dispersive waveguides, mapping frequency comb spectra, and coherent light detection and ranging (LiDAR). Our VSA presents an innovative approach for device analysis and laser spectroscopy, and can play a critical role in future photonic systems and applications for sensing, communication, imaging, and quantum information processing.

physics.optics

Programmable access to microresonator solitons with modulational sideband heating

Dissipative Kerr solitons formed in high-$Q$ optical microresonators provide a route to miniaturized optical frequency combs that can revolutionize precision measurements, spectroscopy, sensing, and communication. In the last decade, a myriad of integrated material platforms have been extensively studied and developed to create photonic-chip-based soliton combs. However, the photo-thermal effect in integrated optical microresonators has been a major issue preventing simple and reliable soliton generation. Several sophisticated techniques to circumvent the photo-thermal effect have been developed. In addition, instead of the single-soliton state, emerging applications in microwave photonics and frequency metrology prefer multi-soliton states. Here we demonstrate an approach to manage the photo-thermal effect and facilitate soliton generation. The approach is based on a single phase-modulated pump, where the generated blue-detuned sideband synergizes with the carrier and thermally stabilizes the microresonator. We apply this technique and demonstrate deterministic soliton generation of 19.97 GHz repetition rate in an integrated silicon nitride microresonator. Furthermore, we develop a program to automatically address to target $N-$soliton state, in addition to the single-soliton state, with near 100% success rate and as short as 10 s time consumption. Our method is valuable for soliton generation in essentially any platforms even with strong photo-thermal effect, and can promote wider applications of soliton frequency comb systems for microwave photonics, telecommunication and frequency metrology.

physics.optics

Foundry manufacturing of tight-confinement, dispersion-engineered, ultralow-loss silicon nitride photonic integrated circuit

The foundry development of integrated photonics has revolutionized today's optical interconnect and datacenters. Over the last decade, we have witnessed the rising of silicon nitride (Si$_3$N$_4$) integrated photonics, which is currently transferring from laboratory research to foundry manufacturing. The development and transition are triggered by the ultimate need of low optical loss offered by Si$_3$N$_4$, which is beyond the reach of silicon and III-V semiconductors. Combined with modest Kerr nonlinearity, tight optical confinement and dispersion engineering, Si$_3$N$_4$ has today become the leading platform for linear and Kerr nonlinear photonics, and has enabled chip-scale lasers featuring ultralow noise on par with table-top fiber lasers. However, so far all the reported fabrication processes of tight-confinement, dispersion-engineered Si$_3$N$_4$ photonic integrated circuit (PIC) with optical loss down to few dB/m have only been developed on 4-inch or smaller wafers. Yet, to transfer these processes to established CMOS foundries that typically operate 6-inch or even larger wafers, challenges remain. In this work, we demonstrate the first foundry-standard fabrication process of Si$_3$N$_4$ PIC with only 2.6 dB/m loss, thickness above 800 nm, and near 100% fabrication yield on 6-inch wafers. Such thick and ultralow-loss Si$_3$N$_4$ PIC enables low-threshold generation of soliton frequency combs. Merging with advanced heterogeneous integration, active ultralow-loss Si$_3$N$_4$ integrated photonics could pave an avenue to addressing future demands in our increasingly information-driven society.

physics.optics

Optical microcombs in whispering gallery mode crystalline resonators with dispersive intermode interactions

Soliton microcombs have shown great potential in a variety of applications ranging from chip scale frequency metrology to optical communications and photonic data center, in which light coupling among cavity transverse modes, termed as intermode interactions, are long-existing and usually give rise to localized impacts on the soliton state. Of particular interest are whispering gallery mode based crystalline resonators, which with dense mode families, potentially feature interactions of all kind. While effects of narrow-band interactions such as spectral power spikes have been well recognized in crystalline resonators, that of broadband interactions remains unexplored. Here, we demonstrate microcombs with broadband and dispersive intermode interactions, in home-developed magnesium fluoride microresonators with an intrinsic $\mathbf{Q}$-factor approaching 10 billion.In addition to conventional soliton comb generation in the single mode pumping scheme, comb states with broadband spectral tailoring effect have been observed, via an intermode pumping scheme.Remarkably, footprints of both constructive and destructive interference on the comb spectrum have been observed, which as confirmed by simulations, are connected to the dispersive effects of the coupled mode family.Our results not only contribute to the understanding of dissipative soliton dynamics in multi-mode or coupled resonator systems, but also extend the access to stable soliton combs in crystalline microresonators where mode control and dispersion engineering are usually challenging.

physics.optics

Soliton Microcombs in Integrated Chalcogenide Microresonators

Photonic integrated microcombs have enabled advanced applications in optical communication, microwave synthesis, and optical metrology, which in nature unveil an optical dissipative soliton pattern under cavity-enhanced nonlinear processes. The most decisive factor of microcombs lies in the photonic material platforms, where materials with high nonlinearity and in capacity of high-quality chip integration are highly demanded. In this work, we present a home-developed chalcogenide glasses-Ge25Sb10S65 (GeSbS) for the nonlinear photonic integration and for the dissipative soliton microcomb generation. Compared with the current integrated nonlinear platforms, the GeSbS features wider transparency from the visible to 11 um region, stronger nonlinearity, and lower thermo-refractive coefficient, and is CMOS compatible in fabrication. In this platform, we achieve chip-integrated optical microresonators with a quality (Q) factor above 2 x 10^6, and carry out lithographically controlled dispersion engineering. In particular, we demonstrate that both a bright soliton-based microcomb and a dark-pulsed comb are generated in a single microresonator, in its separated fundamental polarized mode families under different dispersion regimes. The overall pumping power is on the ten-milliwatt level, determined by both the high Q-factor and the high material nonlinearity of the microresonator. Our results may contribute to the field of nonlinear photonics with an alternative material platform for highly compact and high-intensity nonlinear interactions, while on the application aspect, contribute to the development of soliton microcombs at low operation power, which is potentially required for monolithically integrated optical frequency combs.

physics.optics

Temporal dissipative structures in optical Kerr resonators with transient loss fluctuation

Dissipative structures are the result of spontaneous symmetry breaking in a dynamic open system, which is induced by either the nonlinear effect or loss fluctuations. While optical temporal dissipative solitons in nonlinear Kerr cavities has been widely studied, they are operated in a red-detuned regime that is non-trivial to access. Here, we demonstrate an emergent dissipative soliton state in optical cavities in the presence of loss fluctuations, which is accessible by self-evolution of the system and is operated in resonance. We numerically investigate both the effect of loss modulation and the effect of saturable absorption, based on a standard dissipative and Kerr-nonlinear microresonator model, and observe stable soliton states in a close-to-zero detuning region. The self-starting soliton state working in resonance is potentially of wide interest, which would not only ease the operation for ultrafast temporal soliton generation, but also imply a high conversion efficiency for soliton micro-combs.

physics.optics

Engineered Raman Lasing in Photonic Integrated Chalcogenide Microresonators

Chalcogenide glass (ChG) is an attractive material for integrated nonlinear photonics due to its wide transparency and high nonlinearity, and its capability of being directly deposited and patterned on Silicon wafer substrates. It has a singular Raman effect among amorphous materials. Yet, the Raman lasing performance in high quality and chip integrated ChG microresonators remains unexplored. Here, we demonstrate an engineered Raman lasing dynamic based on home developed photonic integrated high-Q ChG microresonators. With a quality factor above 10^6, we achieve the record-low lasing threshold 3.25 mW among integrated planar photonic platforms. Both the single-mode Raman lasers and a broadband Raman-Kerr comb are observed and characterized, which is dependent on the dispersion of our flexible photonic platform and engineered via tuning the waveguide geometric size. The tunability of such a chipscale Raman laser is also demonstrated through tuning the pump wavelength and tuning the operating temperature on the chip. This allows for the access of single-mode lasing at arbitrary wavelengths in the range 1615-1755 nm. Our results may contribute to the understanding of rich Raman and Kerr nonlinear interactions in dissipative and nonlinear microresonators, and on application aspect, may pave a way to chip-scale efficient Raman lasers that is highly desired in spectroscopic applications in the infrared.

physics.optics

Dissipative Kerr solitons in a photonic dimer on both sides of exceptional point

Exceptional points are a ubiquitous concept widely present in driven-dissipative coupled systems described by a non-Hermitian Hamiltonian. It is characterized by the degeneracy of the Hamiltonian's eigenvalues and coalescence of corresponding eigenvectors. Recent developments demonstrated that exceptional points can play an important role in photonics. However, to date, exceptional points have been extensively examined in the systems supporting only a few optical modes, thereby leaving the observation of collective (multimode) effects outside of the scope of study. In the present paper, we analyze the role of exceptional points in nonlinear multimode photonics. Specifically, we provide insights into complex nonlinear dynamics arising in a continuous wave-driven pair of strongly coupled nonlinear micro-resonators (i.e. a nonlinear photonic dimer) operating in the multimode regime. Investigating this system, which is known to possess exceptional points, we find two fundamentally different nonlinear regimes of operation corresponding to effective parity-time symmetric and broken parity-time symmetry states. We demonstrate that the photonic dimer can be critically coupled to a bus waveguide, thereby, providing an efficient generation of the dissipative Kerr solitons on both sides of the exceptional point. The parity-time symmetric case, which corresponds to a pair of symmetrically split resonances, has been recently shown to exhibit a variety of emergent phenomena including gear soliton generation, symmetry breaking, and soliton hopping. Dissipative solitons generation in the parity-time symmetry broken case - leading to the dissipation splitting - up to now remains unexplored.

physics.optics