arXiv subjects

Hans J. Hug

Publications and source records attributed to Hans J. Hug.

12 recordsLinked to original sources

arXiv2026

Bias-Engineered Synthetic Antiferromagnets Hosting sub-20 nm Zero-Field Skyrmions at Room Temperature

Synthetic antiferromagnetic skyrmions (SAFsk) are nanoscale, topologically protected spin textures with strong potential for spintronic technologies because of their high stability and the absence of the skyrmion Hall effect. However, robust zero field stabilization remains a central challenge. Here, a synthetic antiferromagnetic (SAF) bias system is introduced as a novel strategy to stabilize both ferromagnetic skyrmions (FMsk) and SAFsk at zero field. Ferromagnetic (FM) and SAF multilayers are designed, fabricated and integrated with the SAF bias system to enable controlled skyrmion stabilization and polarity setting via multilayer design and a preparatory field cycle. Combining quantitative and high-sensitivity magnetic force microscopy (MFM) with micromagnetic modeling, reliable zero field skyrmion formation is demonstrated and sub 20nm SAFsk are directly observed, the smallest SAFsk reported to date. Moreover, the SAF bias system concept introduced here offers a robust and scalable route to bias future skyrmion multilayers, as its compensated nature suppresses domain formation and preserves a uniform exchange field.

cond-mat.mes-hall↗

arXiv2026

Beyond conventional skyrmions in synthetic antiferromagnets

Magnetic skyrmions are topologically protected spin textures that can act as reconfigurable nanoscale information carriers. In synthetic antiferromagnets (SAFs), interlayer exchange coupling offers an additional control parameter beyond the interfacial Dzyaloshinskii-Moriya interaction (DMI) and magnetic anisotropy. Here, we engineer a SAF composed of two chemically distinct ferromagnets (CoB and CoFeB), in which the external magnetic field and interlayer exchange act asymmetrically on the sublattices. The competition of these effects, acting as a resultant effective-field, gives rise to two distinct skyrmion families in different field regimes. In large fields, conventional-polarity skyrmions nucleate, with core antiparallel to the external field, whereas in smaller fields an inverse-polarity skyrmion state emerges as the effective-field reverses sign and almost saturates the CoFeB layers. Return-point memory measurements confirm independent nucleation pathways for the two families. Using element-resolved x-ray magnetometry, correlative magnetic force and Lorentz transmission electron microscopies, and parameter-matched micromagnetic modelling, we show that all textures reside only in the CoFeB layers, which experience a Ruderman-Kittel-Kasuya-Yosida (RKKY) exchange field originating from the CoB layers. This effective-field method provides a robust route to programmable three-dimensional spin textures with controlled polarity in selected layers of a multilayer with potential for applications in skyrmion-based computing and spin-logic architectures.

cond-mat.mes-hall↗

arXiv2025

On Tailoring Structural and Optoelectronic Properties of TiO2 Thin Films Synthesized via 'Room' Temperature High Power Impulse Magnetron Sputtering (HiPIMS)

Titanium dioxide (TiO2) is a key material in optoelectronic and energy conversion technologies, including solar cells and photocatalysis. However, integrating TiO2 into flexible or temperature-sensitive devices requires deposition techniques that avoid high-temperature processing while maintaining control over both phase composition and crystallinity. In this work, we demonstrate the synthesis of nanocrystalline TiO2 thin films using High Power Impulse Magnetron Sputtering (HiPIMS) at nearroom temperature. By systematically varying total pressure and oxygen flow, we achieve tunable anatase to rutile phase ratios and control over crystalline quality, as evidenced by Raman and photoluminescence trends. The observed optical trends in both refractive index and emission are directly linked to the underlying structural evolution, with compositional analysis verifying stoichiometric consistency across all deposition conditions. Our findings establish HiPIMS as a powerful low temperature method for tailoring TiO2 thin films and enabling their application in flexible photovoltaics, photoelectrochemical water splitting, and other energy-related systems.

cond-mat.mtrl-sci↗

arXiv2024

Differential Magnetic Force Microscopy with a Switchable Tip

The separation of physical forces acting on the tip of a magnetic force microscope (MFM) is essential for correct magnetic imaging. Electrostatic forces can be modulated by varying the tip-sample potential and minimized to map the local Kelvin potential. However, distinguishing magnetic forces from van der Waals forces typically requires two measurements with opposite tip magnetizations under otherwise identical measurement conditions. Here, we present an inverted magnetic force microscope where the sample is mounted on a flat cantilever for force sensing, and the magnetic tip is attached to a miniaturized electromagnet that periodically flips the tip magnetization. This setup enables the extraction of magnetic tip-sample interactions from the sidebands occurring at the switching rate in the cantilever oscillation spectrum. Our method achieves the separation of magnetic signals from other force contributions in a single-scan mode. Future iterations of this setup may incorporate membrane, trampoline, or string resonators with ultra-high quality factors, potentially improving measurement sensitivity by up to three orders of magnitude compared to the state-of-the-art MFM systems using cantilevers.

physics.app-ph↗

arXiv2022

Tuning the coexistence regime of incomplete and tubular skyrmions in ferro/ferri/ferromagnetic trilayers

The development of skyrmionic devices requires a suitable tuning of material parameters in order to stabilize skyrmions and control their density. It has been demonstrated recently that different skyrmion types can be simultaneously stabilized at room temperature in heterostructures involving ferromagnets, ferrimagnets and heavy metals, offering a new platform of coding binary information in the type of skyrmion instead of the presence/absence of skyrmions. Here, we tune the energy landscape of the two skyrmion types in such heterostructures by engineering the geometrical and material parameters of the individual layers. We find that a fine adjustment of the ferromagnetic layer thickness and thus its magnetic anisotropy, allows the trilayer system to support either one of the skyrmion types or the coexistence of both and with varying densities.

cond-mat.mtrl-sci↗

arXiv2021

Mapping the Structure of Oxygen-Doped Wurtzite Aluminum Nitride Coatings From Ab Initio Random Structure Search and Experiments

Machine learning is changing how we design and interpret experiments in materials science. In this work, we show how unsupervised learning, combined with ab initio modeling, improves our understanding of structural metastability in multicomponent alloys. We use the example case of Al-O-N alloys where the formation of aluminum vacancies in wurtzite AlN upon the incorporation of substitutional oxygen can be seen as a general mechanism of solids where crystal symmetry is reduced to stabilize defects. The ideal AlN wurtzite crystal structure occupation cannot be matched due to the presence of an aliovalent hetero-element into the structure. The traditional interpretation of the c-lattice shrinkage in sputter-deposited Al-O-N films from X-ray diffraction (XRD) experiments suggests the existence of a solubility limit at 8at.% oxygen content. Here we show that such naive interpretation is misleading. We support XRD data with a machine learning analysis of ab initio simulations and positron annihilation lifetime spectroscopy data, revealing no signs of a possible solubility limit. Instead, the presence of a wide range of non-equilibrium oxygen-rich defective structures emerging at increasing oxygen contents suggests that the formation of grain boundaries is the most plausible mechanism responsible for the lattice shrinkage measured in Al-O-N sputtered films.

cond-mat.mtrl-sci↗

arXiv2017

Halbach arrays at the nanoscale from chiral spin textures

Mallinson's idea that some spin textures in planar magnetic structures could produce an enhancement of the magnetic flux on one side of the plane at the expense of the other gave rise to permanent magnet configurations known as Halbach magnet arrays. Applications range from wiggler magnets in particle accelerators and free electron lasers, to motors, to magnetic levitation trains, but exploiting Halbach arrays in micro- or nanoscale spintronics devices requires solving the problem of fabrication and field metrology below 100 μm size. In this work we show that a Halbach configuration of moments can be obtained over areas as small as 1 x 1 μm^2 in sputtered thin films with Néel-type domain walls of unique domain wall chirality, and we measure their stray field at a controlled probe-sample distance of 12.0 x 0.5 nm. Because here chirality is determined by the interfacial Dyzaloshinkii-Moriya interaction the field attenuation and amplification is an intrinsic property of this film, allowing for flexibility of design based on an appropriate definition of magnetic domains. 100 nm-wide skyrmions illustrate the smallest kind of such structures, for which our measurement of stray magnetic fields and mapping of the spin structure shows they funnel the field toward one specific side of the film given by the sign of the Dyzaloshinkii-Moriya interaction parameter D.

cond-mat.mtrl-sci↗

arXiv2016

Surface single-molecule dynamics controlled by entropy at low temperatures

Configuration transitions of individual molecules and atoms on surfaces are traditionally described with energy barriers and attempt rates using an Arrhenius law. This approach yields consistent energy barrier values, but also attempt rates orders of magnitude below expected oscillation frequencies of particles in the meta-stable state. Moreover, even for identical systems, the measurements can yield values differing from each other by orders of magnitude. Using low temperature scanning tunnelling microscopy (STM) to measure an individual dibutyl-sulfide molecule (DBS) on Au(111), we show that we can avoid these apparent inconsistencies if we account for the relative position of tip apex and molecule with accuracy of a fraction of the molecule size. Altering the tip position on that scale modifies the transition's barrier and attempt rate in a highly correlated fashion, which on account of the relation between the latter and entropy results in a single-molecular enthalpy-entropy compensation. By appropriately positioning the tip apex the STM tip can be used to select the operating point on the compensation line and modify the transition rates. The results highlight the need to consider entropy in transition rates of a single molecule, even at temperatures where entropy effects are usually neglected.

cond-mat.mes-hall↗

arXiv2016

How to measure the local Dzyaloshinskii Moriya Interaction in Skyrmion Thin Film Multilayers

The current driven motion of skyrmions in MnSi and FeGe thinned single crystals could be initiated at current densities of the order of $10^6$ A/m, five orders of magnitude smaller than for magnetic domain walls. The technologically crucial step of replicating these results in thin films has not been successful to date, but the reasons are not clear. Elucidating them requires analyzing system characteristics at scales of few nm where the key Dzyaloshinskii Moriya (DM) interactions vary, and doing so in near application conditions, i.e. oxidation protected systems at room temperature. In this work's magnetic force microscopy (MFM) studies of magnetron sputtered Ir/Co/Pt multilayers we show skyrmions that are smaller than previously observed, are not circularly symmetric, and are pinned to 50 nm wide areas of 75 percent higher than average DM interaction. This finding matches our measurement of Co layer thickness inhomogeneity of the order of $\pm$1.2 atomic monolayers per 0.6 nm layer, and indicates that layer flatness must be controlled with greater precision to preclude skyrmion pinning.

cond-mat.mtrl-sci↗

arXiv2015

Bimodal Magnetic Force Microscopy with Capacitive Tip-Sample Distance Control

A single-passage, bimodal magnetic force microscopy technique optimized for scanning samples with arbitrary topography is discussed. A double phase-locked loop (PLL) system is used to mechanically excite a high quality factor cantilever under vacuum conditions on its first mode and via an oscillatory tip-sample potential on its second mode. The obtained second mode oscillation amplitude is then used as a proxy for the tip-sample distance, and for the control thereof. With appropriate $z$-feedback parameters two data sets reflecting the magnetic tip-sample interaction and the sample topography are simultaneously obtained.

cond-mat.mes-hall↗

arXiv2014

Microscale Motion Control Through Ferromagnetic Films

Actuation and control of motion in micro-mechanical systems are technological challenges, since they are accompanied by mechanical friction and wear, principal and well known sources of device lifetime reduction. In this theoretical work we propose a non-contact motion control technique based on the introduction of a tunable magnetic interaction. The latter is realized by coating two non-touching sliding bodies with ferromagnetic films. The resulting dynamics is determined by shape, size and ordering of magnetic domains arising in the films below the Curie temperature. We demonstrate that the domain behavior can be tailored by acting on handles like ferromagnetic coating preparation, external magnetic fields and the finite distance between the plates. In this way, motion control can be achieved without mechanical contact. Moreover, we discuss how such handles can disclose a variety of sliding regimes. Finally, we propose how to practically implement the proposed model sliding system.

cond-mat.mes-hall↗

arXiv2014

Role of interface coupling inhomogeneity in domain evolution in exchange bias

Models of exchange-bias in thin films have been able to describe various aspects of this technologically relevant effect. Through appropriate choices of free parameters the modelled hysteresis loops adequately match experiment, and typical domain structures can be simulated. However, the use of these parameters, notably the coupling strength between the systems' ferromagnetic (F) and antiferromagnetic (AF) layers, obscures conclusions about their influence on the magnetization reversal processes. Here we develop a 2D phase-field model of the magnetization process in exchange-biased CoO/(Co/Pt)xn that incorporates the 10 nm-resolved measured local biasing characteristics of the antiferromagnet. Just three interrelated parameters set to measured physical quantities of the ferromagnet and the measured density of uncompensated spins thus suffice to match the experiment in microscopic and macroscopic detail. We use the model to study changes in bias and coercivity caused by different distributions of pinned uncompensated spins of the antiferromagnet, in application-relevant situations where domain wall motion dominates the ferromagnetic reversal. We show the excess coercivity can arise solely from inhomogeneity in the density of biasing- and anti-biasing pinned uncompensated spins in the antiferromagnet. Counter to conventional wisdom, irreversible processes in the latter are not essential.

cond-mat.mes-hall↗