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Hayden Binger

Publications and source records attributed to Hayden Binger.

3 recordsLinked to original sources

A Fourier-Space Approach to Physics-Informed Magnetization Reconstruction from Nitrogen-Vacancy Measurements

Reconstructing magnetization textures from nitrogen-vacancy (NV) magnetometry stray-field measurements is a challenging, fundamentally ill-posed inverse problem, further complicated by the unknown effective distance between sensor and magnetic material. Here we show that incorporating a micromagnetic energy functional directly into the inversion filters out unphysical, high-energy configurations, while Fourier-space upward continuation of the stray field allows us to simultaneously fit the distance. Applied to measurements of the van der Waals ferromagnet Fe$_{3-x}$GaTe$_2$, it recovers an effective distance estimate of approximately 81nm and low-energy configurations that reproduce the observed field. More broadly, embedding physics directly into the reconstruction turns ill-posed magnetic inverse problems into transparent, interpretable reconstructions, with applicability well beyond NV magnetometry.

cond-mat.mes-hall

Machine Learning-Assisted Nano-imaging and Spectroscopy of Phase Coexistence in a Wide-Bandgap Semiconductor

Wide bandgap semiconductors with high room temperature mobilities are promising materials for high-power electronics. Stannate films provide wide bandgaps and optical transparency, although electron-phonon scattering can limit mobilities. In SrSnO3, epitaxial strain engineering stabilizes a high-mobility tetragonal phase at room temperature, resulting in a threefold increase in electron mobility among doped films. However, strain relaxation in thicker films leads to nanotextured coexistence of tetragonal and orthorhombic phases with unclear implications for optoelectronic performance. The observed nanoscale phase coexistence demands nano-spectroscopy to supply spatial resolution beyond conventional, diffraction-limited microscopy. With nano-infrared spectroscopy, we provide a comprehensive analysis of phase coexistence in SrSnO3 over a broad energy range, distinguishing inhomogeneous phonon and plasma responses arising from structural and electronic domains. We establish Nanoscale Imaging and Spectroscopy with Machine-learning Assistance (NISMA) to map nanotextured phases and quantify their distinct optical responses through a robust quantitative analysis, which can be applied to a broad array of complex oxide materials.

cond-mat.mtrl-sci

Interfacial strong coupling and negative dispersion of propagating polaritons in freestanding oxide membranes

Membranes of complex oxides like perovskite SrTiO3 extend the multi-functional promise of oxide electronics into the nanoscale regime of two-dimensional materials. Here we demonstrate that free-standing oxide membranes supply a reconfigurable platform for nano-photonics based on propagating surface phonon polaritons. We apply infrared near-field imaging and -spectroscopy enabled by a tunable ultrafast laser to study pristine nano-thick SrTiO3 membranes prepared by hybrid molecular beam epitaxy. As predicted by coupled mode theory, we find that strong coupling of interfacial polaritons realizes symmetric and antisymmetric hybridized modes with simultaneously tunable negative and positive group velocities. By resolving reflection of these propagating modes from membrane edges, defects, and substrate structures, we quantify their dispersion with position-resolved nano-spectroscopy. Remarkably, we find polariton negative dispersion is both robust and tunable through choice of membrane dielectric environment and thickness and propose a novel design for in-plane Veselago lensing harnessing this control. Our work lays the foundation for tunable transformation optics at the nanoscale using polaritons in a wide range of freestanding complex oxide membranes.

cond-mat.mes-hall