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Herbert Schoeller

Publications and source records attributed to Herbert Schoeller.

At least 55 records · Page 3Linked to original sources

Real-time renormalization group in frequency space: A 2-loop analysis of the nonequilibrium anisotropic Kondo model at finite magnetic field

We apply a recently developed nonequilibrium real-time renormalization group method in frequency space to describe nonlinear quantum transport through a small fermionic quantum system coupled weakly to several reservoirs via spin and/or orbital fluctuations. We provide an analytic and well-controlled procedure to solve the RG equations in the weak-coupling regime. Within a 2-loop analysis, we derive analytic formulas for the nonlinear conductance and the kernel determining the time evolution of the reduced density matrix. Most importantly, we present a consistent formalism how the RG flow is cut off by relaxation and dephasing rates, which is necessary to calculate the precise line shape at resonances. We apply the general formalism to the nonequilibrium anisotropic Kondo model at finite magnetic field. We consider the weak-coupling regime, where the maximum of voltage and bare magnetic field is larger than the Kondo-temperature. In this regime, we calculate the nonlinear conductance, the magnetic susceptibility, the renormalized spin relaxation and dephasing rates, and the renormalized g-factor. All quantities are considered up to the first logarithmic contributions at resonance. Up to a redefinition of the Kondo temperature, we confirm previous results for the conductance and the magnetic susceptibility in the isotropic case. In addition, we present a consistent calculation of the line shape at the resonances, including the determination which rate cuts off the logarithmic divergence. Furthermore, we calculate the rates and the renormalized g-factor in nonequilibrium beyond leading order, being quantities characterizing the exponential decay of the time evolution of the magnetization. For all quantities we analyse also the anisotropic case and find interesting nonequilibrium effects at resonance.

cond-mat.mes-hall↗

A perturbative nonequilibrium renormalization group method for dissipative quantum mechanics: Real-time RG in frequency space (RTRG-FS)

We study a generic problem of dissipative quantum mechanics, a small local quantum system with discrete states coupled in an arbitrary way (i.e. not necessarily linear) to several infinitely large particle or heat reservoirs. For both bosonic or fermionic reservoirs we develop a quantum field-theoretical diagrammatic formulation in Liouville space by expanding systematically in the reservoir-system coupling and integrating out the reservoir degrees of freedom. As a result we obtain a kinetic equation for the reduced density matrix of the quantum system. Based on this formalism, we present a formally exact perturbative renormalization group (RG) method from which the kernel of this kinetic equation can be calculated. It is demonstrated how the nonequilibrium stationary state (induced by several reservoirs kept at different chemical potentials or temperatures), arbitrary observables such as the transport current, and the time evolution into the stationary state can be calculated. Most importantly, we show how RG equations for the relaxation and dephasing rates can be derived and how they cut off generically the RG flow of the vertices. The method is based on a previously derived real-time RG technique but formulated here in Laplace space and generalized to arbitrary reservoir-system couplings. Furthermore, for fermionic reservoirs with flat density of states, we make use of a recently introduced cutoff scheme on the imaginary frequency axis which has several technical advantages. We demonstrate the method by applying it to the nonequilibrium isotropic Kondo model in 1-loop. We present a systematic way to solve the RG equations analytically in the weak-coupling limit and provide an outlook of the applicability to the strong-coupling case.

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Real-time renormalization group and cutoff scales in nonequilibrium applied to an arbitrary quantum dot in the Coulomb blockade regime

We apply the real-time renormalization group (RG) in nonequilibrium to an arbitrary quantum dot in the Coulomb blockade regime. Within one-loop RG-equations, we include self-consistently the kernel governing the dynamics of the reduced density matrix of the dot. As a result, we find that relaxation and dephasing rates generically cut off the RG flow. In addition, we include all other cutoff scales defined by temperature, energy excitations, frequency, and voltage. We apply the formalism to transport through single molecular magnets, realized by the fully anisotropic Kondo model (with three different exchange couplings J_x, J_y, and J_z) in a magnetic field h_z. We calculate the differential conductance as function of bias voltage V and discuss a quantum phase transition which can be tuned by changing the sign of J_x J_y J_z via the anisotropy parameters. Finally, we calculate the noise S(Omega) at finite frequency Omega for the isotropic Kondo model and find that the dephasing rate determines the height of the shoulders in dS(Ω)/d Omega near Omega=V.

cond-mat.str-el↗

Nonequilibrium functional renormalization group for interacting quantum systems

We propose a nonequilibrium version of functional renormalization within the Keldysh formalism by introducing a complex valued flow parameter in the Fermi or Bose functions of each reservoir. Our cutoff scheme provides a unified approach to equilibrium and nonequilibrium situations. We apply it to nonequilibrium transport through an interacting quantum wire coupled to two reservoirs and show that the nonequilibrium occupation induces new power law exponents for the conductance.

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Temperature induced phase averaging in one-dimensional mesoscopic systems

We analyse phase averaging in one-dimensional interacting mesoscopic systems with several barriers and show that for incommensurate positions an independent average over several phases can be induced by finite temperature. For three strong barriers with conductances G_i and mutual distances larger than the thermal length, we obtain G ~ sqrt{G_1 G_2 G_3} for the total conductance G. For an interacting wire, this implies power laws in G(T) with novel exponents, which we propose as an experimental fingerprint to distinguish temperature induced phase averaging from dephasing.

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Fingerprints of the Magnetic Polaron in Nonequilibrium Electron Transport through a Quantum Wire Coupled to a Ferromagnetic Spin Chain

We study nonequilibrium quantum transport through a mesoscopic wire coupled via local exchange to a ferromagnetic spin chain. Using the Keldysh formalism in the self-consistent Born approximation, we identify fingerprints of the magnetic polaron state formed by hybridization of electronic and magnon states. Because of its low decoherence rate, we find coherent transport signals. Both elastic and inelastic peaks of the differential conductance are discussed as a function of external magnetic fields, the polarization of the leads and the electronic level spacing of the wire.

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Magnon transport and spin current switching through quantum dots

We study the nonequilibrium spin current through a quantum dot consisting of two localized spin-1/2 coupled to two ferromagnetic insulators. The influence of an intra-dot magnetic field and exchange coupling, different dot-reservoir coupling configurations, and the influence of magnon chemical potential differences vs. magnetic field gradients onto the spin current are examined. We discuss various spin switching mechanisms and find that, in contrast to electronic transport, the spin current is very sensitive to the specific coupling configuration and band edges. In particular, we identify 1- and 2-magnon transport processes which can lead to resonances and antiresonances for the spin current.

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Designable electron transport features in one-dimensional arrays of metallic nanoparticles: Monte Carlo study of the relation between shape and transport

We study the current and shot noise in a linear array of metallic nanoparticles taking explicitly into consideration their discrete electronic spectra. Phonon assisted tunneling and dissipative effects on single nanoparticles are incorporated as well. The capacitance matrix which determines the classical Coulomb interaction within the capacitance model is calculated numerically from a realistic geometry. A Monte Carlo algorithm which self-adapts to the size of the system allows us to simulate the single-electron transport properties within a semiclassical framework. We present several effects that are related to the geometry and the one-electron level spacing like e.g. a negative differential conductance (NDC) effect. Consequently these effects are designable by the choice of the size and arrangement of the nanoparticles.

cond-mat.mes-hall↗

Nonperturbative analysis of coupled quantum dots in a phonon bath

Transport through coupled quantum dots in a phonon bath is studied using the recently developed real-time renormalization-group method. Thereby, the problem can be treated beyond perturbation theory regarding the complete interaction. A reliable solution for the stationary tunnel current is obtained for the case of moderately strong couplings of the dots to the leads and to the phonon bath. Any other parameter is arbitrary, and the complete electron-phonon interaction is taken into account. Experimental results are quantitatively reproduced by taking into account a finite extension of the wavefunctions within the dots. Its dependence on the energy difference between the dots is derived.

cond-mat.mes-hall↗

Spin accumulation in ferromagnetic single-electron transistors in the cotunneling regime

We propose a new method of direct detection of spin accumulation, which overcomes problems of previous measurement schemes. A spin dependent current in a single-electron transistor with ferromagnetic electrodes leads to spin accumulation on the metallic island. The resulting spin-splitting of the electrochemical potentials of the island, because of an additional shift by the charging energy, can be detected from the spacing between two resonances in the current-voltage characteristics. The results were obtained in the framework of a real-time diagrammatic approach which allows to study higher order (co-)tunneling processes in the strong nonequlibrium situation.

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Quantum Phase Transition in a Multi-Level Dot

We discuss electronic transport through a lateral quantum dot close to the singlet-triplet degeneracy in the case of a single conduction channel per lead. By applying the Numerical Renormalization Group, we obtain rigorous results for the linear conductance and the density of states. A new quantum phase transition of the Kosterlitz-Thouless type is found, with an exponentially small energy scale $T^*$ close to the degeneracy point. Below $T^*$, the conductance is strongly suppressed, corresponding to a universal dip in the density of states. This explains recent transport measurements.

cond-mat.mes-hall↗

Non-Linear Transport through a Molecular Nanojunction

We present a simple model of electrical transport through a metal-molecule-metal nanojunction that includes charging effects as well as aspects of the electronic structure of the molecule. The interplay of a large charging energy and an asymmetry of the metal-molecule coupling can lead to various effects in non-linear electrical transport. In particular, strong negative differential conductance is observed under certain conditions.

cond-mat.mes-hall↗

Interference and interaction effects in multi-level quantum dots

Using renormalization group techniques, we study spectral and transport properties of a spinless interacting quantum dot consisting of two levels coupled to metallic reservoirs. For strong Coulomb repulsion $U$ and an applied Aharonov-Bohm phase $ϕ$, we find a large direct tunnel splitting $|Δ|\sim (Γ/π)|\cos(ϕ/2)|\ln(U/ω_c)$ between the levels of the order of the level broadening $Γ$. As a consequence we discover a many-body resonance in the spectral density that can be measured via the absorption power. Furthermore, for $ϕ=π$, we show that the system can be tuned into an effective Anderson model with spin-dependent tunneling.

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Kondo Correlations and the Fano Effect in Closed AB-Interferometers

We study the Fano-Kondo effect in a closed Aharonov-Bohm (AB) interferometer which contains a single-level quantum dot and predict a frequency doubling of the AB oscillations as a signature of Kondo-correlated states. Using Keldysh formalism, Friedel sum rule and Numerical Renormalization Group, we calculate the exact zero-temperature linear conductance $G$ as a function of AB phase $ϕ$ and level position $ε$. In the unitary limit, $G(ϕ)$ reaches its maximum $2e^2/h$ at $ϕ=π/2$. We find a Fano-suppressed Kondo plateau for $G(ε)$ similar to recent experiments.

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Influence of nano-mechanical properties on single electron tunneling: A vibrating Single-Electron Transistor

We describe single electron tunneling through molecular structures under the influence of nano-mechanical excitations. We develop a full quantum mechanical model, which includes charging effects and dissipation, and apply it to the vibrating C$_{60}$ single electron transistor experiment by Park {\em et al.} {[Nature {\bf 407}, 57 (2000)].} We find good agreement and argue vibrations to be essential to molecular electronic systems. We propose a mechanism to realize negative differential conductance using local bosonic excitations.

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Real-Time-RG Analysis of the Dynamics of the Spin-Boson Model

Using a real-time renormalization group method we determine the complete dynamics of the spin-boson model with ohmic dissipation for coupling strengths $α\lesssim 0.1-0.2$. We calculate the relaxation and dephasing time, the static susceptibility and correlation functions. Our results are consistent with quantum Monte Carlo simulations and the Shiba relation. We present for the first time reliable results for finite cutoff and finite bias in a regime where perturbation theory in $α$ or in tunneling breaks down. Furthermore, an unambigious comparism to results from the Kondo model is achieved.

cond-mat.stat-mech↗

Orbital and spin Kondo effects in a double quantum dot

Motivated by recent experiments, in which the Kondo effect has been observed for the first time in a double quantum-dot structure, we study electron transport through a system consisting of two ultrasmall, capacitively-coupled dots with large level spacing and charging energy. Due to strong interdot Coulomb correlations, the Kondo effect has two possible sources, the spin and orbital degeneracies, and it is maximized when both occur simultaneously. The large number of tunable parameters allows a range of manipulations of the Kondo physics -- in particular, the Kondo effect in each dot is sensitive to changes in the state of the other dot. For a thorough account of the system dynamics, the linear and nonlinear conductance is calculated in perturbative and non-perturbative approaches. In addition, the temperature dependence of the resonant peak heights is evaluated in the framework of a renormalization group analysis.

cond-mat.mes-hall↗

Spin dynamics of Mn12-acetate in the thermally-activated tunneling regime: ac-susceptibility and magnetization relaxation

In this work, we study the spin dynamics of Mn12-acetate molecules in the regime of thermally assisted tunneling. In particular, we describe the system in the presence of a strong transverse magnetic field. Similar to recent experiments, the relaxation time/rate is found to display a series of resonances; their Lorentzian shape is found to stem from the tunneling. The dynamic susceptibility $χ(w)$ is calculated starting from the microscopic Hamiltonian and the resonant structure manifests itself also in $χ(w)$. Similar to recent results reported on another molecular magnet, Fe8, we find oscillations of the relaxation rate as a function of the transverse magnetic field when the field is directed along a hard axis of the molecules. This phenomenon is attributed to the interference of the geometrical or Berry phase. We propose susceptibility experiments to be carried out for strong transverse magnetic fields to study of these oscillations and for a better resolution of the sharp satellite peaks in the relaxation rates.

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