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Hikaru Kawamura

Publications and source records attributed to Hikaru Kawamura.

At least 19 recordsLinked to original sources

Magnetic field effects on spin-split band and magnon transport in altermagnets and emergent compensated ferrimagnets

In altermagnets and fully compensated ferrimagnets, not only the electron band but also the magnon band exhibits spin splitting without net magnetization, which enables thermal activation of the magnon spin current. Here, we theoretically investigate magnetic field effects on the magnon properties of these antiferromagnets in the presence of a weak easy-axis anisotropy which makes the collinear states robust against the magnetic field. For the altermagnet and compensated ferrimagnet, we analyze a 2 sublattice order in the $J_1$-$J_2$-$J_2^\prime$ model on the square lattice and a triple-${\bf Q}$ 12-sublattice order in the $J_1$-$J_3$ model on the kagome lattice, respectively, each accompanied by $d$-wave and $s$-wave spin splitting at zero field. It is shown that for positive (negative) magnetic field $H$ whose energy scale is smaller than the anisotropy gap, the up- and down-spin magnon bands are shifted to lower (higher) and higher (lower) energies, respectively, similarly to the Zeeman coupling in electron systems. In the altermagnet, with increasing field, the $d$-wave splitting tends to be deformed into the $s$-wave one, which is reflected as the change in the direction of the spin current generated by thermal gradient. In the compensated ferrimagnet, the $s$-wave nature, i.e., the population imbalance between the up- and down-spin magnons at $H=0$, can induce an asymmetric field dependence of the longitudinal spin and thermal conductivities in a field-sweep process.

cond-mat.str-el

Triple-${\bf Q}$ collinear state with compensated ferrimagnetic nature on frustrated kagome lattice

Spin-selective band splitting without net magnetization and spin-orbit couplings serves for a next-generation spin-current generator, and its typical platforms are altermagnets and compensated ferrimagnets as well, where the existence of a crystal asymmetry or nonequivalent sites is essential. Here, we theoretically demonstrate that such a splitting can be realized in a triple-{\bf Q} 12-sublattice state emerging in a $J_3$-dominant kagome antiferromagnet, without the help of the crystal asymmetry. Reflecting the multi-sublattice nature, a local magnetization reveals a fully compensated ferrimagnetic pattern in units of a triangle plaquette, leading to $s$-wave-type spin splittings in magnon and electron bands. This enables an atiferromagnetic spin Seebeck effect at zero field in insulating systems and filling-controlled polarized states in metallic systems, highlighting the potential of frustrated magnets to realize novel spintronics functionalities.

cond-mat.str-el

Spontaneous chirality selection and nonreciprocal spin wave in breathing-kagome antiferromagnets at zero field

It has been known that the spin-wave dispersion, which is usually symmetric in the momentum space with respect to ${\bf q}=0$, can be asymmetric in the presence of the Dzyaloshinskii-Moriya (DM) interaction and an applied magnetic field. Here, we theoretically demonstrate that in $J_3$-dominant classical Heisenberg antiferromagnets on the breathing kagome lattice, the asymmetric spin-wave dispersion appears in a chiral phase due to non-uniform geometric phases acquired in the spin-wave propagation processes. This points to the emergence of a nonreciprocal spin wave in the absence of both the DM interaction and the magnetic field. Reflecting the asymmetry, positive-spin-chirality and negative-spin-chirality states, either one of which is selected in the low-temperature phase by the symmetry breaking, show different spin-wave dispersions, suggesting that the two energetically-degenerate chiral states can be distinguished by the spin-wave propagation.

cond-mat.str-el

Skyrmion crystal formation and temperature -- magnetic field phase diagram of the frustrated tirangular-lattice Heisenberg magnet with easy-axis masugnetic anisotropy

The nature of the skyrmion-crystal (SkX) formation and various multiple-$q$ phases encompassing the SkX phase are investigated by extensive Monte Carlo simulations on the frustrated $J_1$-$J_3$ triangular-lattice Heisenberg model with the weak easy-axis magnetic anisotropy. Phase diagram in the temperature $T$ vs. magnetic-field $H$ plane are constructed, leading to a rich variety of multiple-$q$ phases. The anisotropy stabilizes the SkX state down to $T=0$ at intermediate fields, while in the lower-field range the SkX state becomes only metastable, and new multiple-$q$ states with a broken $C_3$ symmetry are instead stabilized. Implications to experiments are discussed.

cond-mat.str-el

Zero-field miniature skyrmion crystal and chiral domain state in breathing-kagome antiferromagnets

The stability of a miniature skyrmion crystal (SkX) with only a small number of spins in the magnetic unit cell has been theoretically investigated in $J_1$-$J_3$ antiferromagnets on the breathing kagome lattice with a single-ion anisotropy $D$ at zero field. It is found by means of Monte Carlo simulations that due to the breathing bond-alternation, a zero-field triple-${\bf Q}$ miniature SkX can be stabilized not only in the specific case of $D=0$ [K. Aoyama and H. Kawamura, Phys. Rev. B 105, L100407 (2022)] but also in more general situations with easy-axis ($D<0$) and easy-plane ($D>0$) anisotropies which favor triple-${\bf Q}$ collinear and noncoplanar states, respectively. Since the SkX and anti-SkX each having positive or negative chirality are energetically degenerate, the topological Hall effect of alternative sign is possible at zero field. It is also found that reflecting the chiral degeneracy, the collinear and coplanar phases preempting the SkX phase possess random domain structures consisting of positive- and negative-chirality clusters.

cond-mat.str-el

Hedgehog lattice and field-induced chirality in breathing-pyrochlore Heisenberg antiferromagnets

We theoretically investigate a $J_1$-$J_3$ classical Heisenberg model on the breathing pyrochlore lattice, where the nearest-neighbor (NN) exchange interactions for small and large tetrahedra, $J_1$ and $J_1'$, take different values due to the breathing bond-alternation and $J_3$ is the third NN antiferromagnetic interaction along the bond direction. It is found by means of Monte Carlo simulations that for large $J_3$, a hedgehog lattice, a three-dimensional periodic array of magnetic monopoles and antimonopoles, emerges in the form of a quadruple-${\bf Q}$ state characterized by the ordering vector of ${\bf Q}=(\pm\frac{1}{2},\pm\frac{1}{2},\pm\frac{1}{2})$, being irrespective of the signs of $J_1$ and/or $J_1'$ as long as $J_1\neq J_1'$. It is also found that in an applied magnetic field, there appear six quadruple-${\bf Q}$ states depending on the values of $J_1$ and $J_1'$, among which three phases including the in-field hedgehog-lattice state exhibit nonzero total chirality $\mbox{\boldmath $χ$}^{\rm T}$ associated with the anomalous Hall effect of chirality origin. In the remaining two chiral phases, which are realized in the presence of ferromagnetic $J_1$ and/or $J_1'$, the spin structure is not topologically nontrivial, in spite of the fact that $\mbox{\boldmath $χ$}^{\rm T} \neq 0$. The role of the topological objects of the monopoles in $\mbox{\boldmath $χ$}^{\rm T}$ is also discussed.

cond-mat.str-el

Emergent skyrmion-based chiral order in zero-field Heisenberg antiferromagnets on the breathing kagome lattice

We show that classical Heisenberg antiferromagnets on the breathing kagome lattice can be a platform to realize a zero-field topological order of the scalar spin chirality which can be viewed as a miniature skyrmion crystal (SkX) of discrete form with a small number of spins in its magnetic unit cell. In the model, a third nearest-neighbor (NN) antiferromagnetic interaction along the bond direction $J_3$ and the breathing bond-alternation characterized by the ratio of the NN interaction for large triangles to that for small ones, $J_1'/J_1$, are essential. It is found by means of Monte Carlo simulations that a commensurate triple-${\bf Q}$ state appearing for relatively strong $J_3$ at zero field is the noncoplanar state with the SkX structure in the breathing case of $J_1'/J_1 \neq 1$, while in the uniform case of $J_1'/J_1 =1$, it is a collinear state favored by thermal fluctuations. The origin of this chiral order and experimental implications of our result are also discussed.

cond-mat.str-el

Skyrmion crystal in the RKKY system on the two-dimensional triangular lattice

We study the ordering properties of the isotropic RKKY Heisenberg model on the two-dimensional (2D) triangular lattice by extensive Monte Carlo simulations to get insights into the chiral-degenerate skyrmion crystal (SkX) of metallic magnets. Our Hamiltonian contains only the spin-quadratic RKKY interaction derived from the spherical Fermi surface, containing neither the nesting nor the many-body interaction. The SkX phase is stabilized under applied fields where the frustration associated with the oscillating nature of the RKKY interaction and the emergent many-body interactions generated by thermal fluctuations play important roles. Replica symmetry breaking, reported in our recent study on the 3D RKKY model [Phys. Rev. B 104, 184432 (2021)], turns out to be absent in the present 2D model. Implications to the SkX formation mechanism are discussed.

cond-mat.str-el

Effects of spin-lattice coupling and a magnetic field in classical Heisenberg antiferromagnets on the breathing pyrochlore lattice

We theoretically investigate spin-lattice coupling (SLC) effects on the in-field ordering properties of classical Heisenberg antiferromagnets on the breathing pyrochlore lattice. Here, we use the two possible simplified models describing the effect of local lattice distortions on the spin ordering via the SLC, the bond-phonon and site-phonon models. It is found by means of Monte Carlo simulations that in both models, the $\frac{1}{2}$ plateau shows up in the magnetization curve being relatively robust against the breathing bond-alternation, although magnetic long-range orders (LRO's) are realized only in the site-phonon model. In the bond-phonon model, additional further neighbor interactions are necessary to induce a magnetic LRO. In the site-phonon model, it is also found that in addition to the low-field, middle-field 1/2-plateau, and high-field phases appearing on both the uniform and breathing pyrochlore lattices, various types of unconventional phases which can be viewed as LRO's in units of tetrahedron are induced by the breathing bond-alternation just below the 1/2 plateau and the saturation field. The occurrence of these tetrahedron-based orders could be attributed to the nature characteristic of the breathing pyrochlore lattice, i.e., the existence of the nonequivalent small and large tetrahedra. Experimental implications of our result are also discussed.

cond-mat.str-el

Spin dynamics simulation of the $Z_2$-vortex fluctuations

Motivated by the recent quasi-elastic neutron scattering experiment, we extend the spin-dynamics simulation on the triangular-lattice Heisenberg antiferromagnet, to observe a sharp central peak of its energy width $\sim 0.001J$ ($J$ the exchange coupling) of the $Z_2$-vortex origin, consistently with the experiment.

cond-mat.str-el

Frustration-induced quantum spin liquid behavior in the $s=$1/2 random-bond Heisenberg antiferromagnet on the zigzag chain

Recent studies have revealed that the randomness-induced quantum spin liquid (QSL)-like state is stabilized in certain frustrated quantum magnets in two and three dimensions. In order to clarify the nature of this gapless QSL-like state, we investigate both zero- and finite-temperature properties of the random-bond one-dimensional (1D) $s=12$ Heisenberg model with the competing nearest-neighbor and next-nearest-neighbor antiferromagnetic interactions, $J_1$ and $J_2$, by means of the exact diagonalization, density-matrix renormalization-group and Hams--de Raedt methods. We find that, on increasing the frustration $J_2$, the gapless nonmagnetic state stabilized in the unfrustrated model with $J_2=0$, the {\it unfrustrated\} random-singlet (RS) state, exhibits a phase transition into different gapless nonmagnetic state, the {\it frustrated\} RS state. This frustrated RS state in 1D has properties quite similar to the randomness-induced QSL-like state recently identified in 2D and 3D frustrated magnets exhibiting the $T$-linear low-temperature ($T$) specific heat, while the unfrustrated RS state is more or less specific to the unfrustrated 1D system exhibiting the $\sim 1(\log T)^3$ low-$T$ specific heat. Universal features and the robustness against perturbations of the frustrated RS state are emphasized.

cond-mat.str-el

Replica symmetry breaking in the RKKY skyrmion crystal system

We study the RKKY Heisenberg model on a three-dimensional stacked-triangular lattice under magnetic fields by extensive Monte Carlo simulations to get insight into the chiral-degenerate symmetric skyrmion crystal (SkX) in centrosymmetric metallic magnets. The triple-$q$ SkX state and the double-$q$ states are realized, together with the single-$q$ state. We find an unexpected phenomenon of the replica-symmetry breaking (RSB) well-known in glassy systems, although the Hamiltonian and the ordered state are entirely regular. In the RSB SkX phase, the triple-$q$ SkX state macroscopically coexists with the single-$q$ state, in spite of the fact that these ordered states cannot be transformed via any Hamiltonian-symmetry operation. In the thermodynamic limit, the free energies of these states are degenerate whereas the free-energy barrier between the states diverges, breaking the ergodicity. A similar RSB is observed also in the RSB double-$q$ phase where the double-$q$ state macroscopically coexists with the single-$q$ state. Experimental implications are discussed.

cond-mat.str-el

Hedgehog-lattice spin texture in classical Heisenberg antiferromagnets on the breathing pyrochlore lattice

The hedgehog lattice, a three-dimensional periodic array of magnetic monopoles and antimonopoles, is known to be realized in the presence of the Dzyaloshinskii-Moriya (DM) interaction. Here, we demonstrate by means of Monte Carlo simulations that the hedgehog lattice is induced by not the DM interaction but frustration in classical Heisenberg antiferromagnets on the breathing pyrochlore lattice. In the model, the breathing bond-alternation is characterized by the ratio of the nearest-neighbor (NN) antiferromagnetic exchange interaction for large tetrahedra to that for small ones, J1'/J1. A quadruple-q state with the ordering vector of q=(\pm 1/2,\pm 1/2,\pm 1/2), which is realized for a large third NN antiferromagnetic interaction along the bond direction J3, turns out to become the hedgehog-lattice state in the breathing case of J1'/J1 <1, while in the uniform case of J1'/J1 =1, it is a collinear state favored by thermal fluctuations. It is also found that in a magnetic field, the structure of the (1/2,1/2,1/2) hedgehog lattice is changed from cubic to tetragonal, resulting in a nonzero net spin chirality which in a metalic system, should yield a characteristic topological Hall effect.

cond-mat.str-el

Monte Carlo studies of the spin-chirality decoupling in the three-dimensional Heisenberg spin glass

An extensive equilibrium Monte Carlo simulation is performed on the 3D isotropic Heisenberg SG model with the random nearest-neighbor Gaussian coupling, with particular interest in its chiral-glass (CG) and spin-glass (SG) orderings. For this model, the possibility of the spin-chirality decoupling, {\it i.e.\}, the CG order setting in at a higher temperature than that of the SG order was suggested earlier, but still remains controversial. We simulate the model up to the maximum size (linear dimension) $L=48$ under both periodic and open boundary conditions (BC). In locating the CG and SG transition temperatures $T_{\rm CG}$ and $T_{\rm SG}$ by the $L\rightarrow \infty$ extrapolation, a variety of independent physical quantities under the both BC are computed and utilized to get larger number of degrees of freedom (NDF). Thanks to the large NDF up to NDF=43, we succeed in obtaining stable and accurate estimates of the CG and SG transition temperatures, $T_{\rm CG}=0.142\pm 0.001$ and $T_{\rm SG}=0.131^{+0.001}_{-0.006}$. No sign of the size crossover is observed. For larger $L$, the CG correlation length progressively outgrows the SG correlation length at low temperatures. These results provide strong numerical support for the spin-chirality decoupling. The critical exponents associated with the CG and SG transitions are evaluated by use of the finite-size scaling with the scaling correction. For the CG transition, we get the CG exponents, $ν_{\rm CG}=1.36\pm 0.10$ and $η_{\rm CG}=0.49\pm 0.10$, consistently with the corresponding experimental exponents of canonical SG. Implications to the chirality scenario of experimental SG ordering is discussed.

cond-mat.dis-nn

Monte Carlo study of the critical properties of noncollinear Heisenberg magnets: $O(3)\times O(2)$ universality class

The critical properties of the antiferromagnetic Heisenberg model on the three-dimensional stacked-triangular lattice are studied by means of a large-scale Monte Carlo simulation in order to get insight into the controversial issue of the criticality of the noncollinear magnets with the $O(3)\times O(2)$ symmetry. The maximum size studied is $384^3$, considerably larger than the sizes studied by the previous numerical works on the model. Availability of such large-size data enables us to examine the detailed critical properties including the effect of corrections to the leading scaling. Strong numerical evidence of the continuous nature of the transition is obtained. Our data indicates the existence of significant corrections to the leading scaling. Careful analysis by taking account of the possible corrections yield critical exponents estimates, $α=0.44(3)$, $β=0.26(2)$, $γ=1.03(5)$, $ν=0.52(1)$, $η=0.02(5)$, and the chirality exponents $β_κ=0.40(3)$ and $γ_κ=0.77(6)$, supporting the existence of the $O(3)$ chiral (or $O(3)\times O(2)$) universality class governed by a new `chiral' fixed point. We also obtain an indication that the underlying fixed point is of the focus-type, characterized by the complex-valued correction-to-scaling exponent, $ω=0.1^{+0.4}_{-0.05} + i\ 0.7^{+0.1}_{-0.4}$. The focus-like nature of the chiral fixed point accompanied by the spiral-like renormalization-group (RG) flow is likely to be the origin of the apparently complicated critical behavior. The results are compared and discussed in conjunction with the results of other numerical simulations, several distinct types of RG calculations including the higher-order perturbative massive and massless RG calculations and the nonperturbative functional RG calculation, and the conformal-bootstrap program.

cond-mat.str-el

Multiple-$q$ states of the $J_1$-$J_2$ classical honeycomb-lattice Heisenberg antiferromagnet under magnetic fields

Motivated by the recent theoretical study by Okubo $et \ al$ [Phys. Rev. Lett. ${\bf 108}$, 017206 (2012)] on the possible realization of the frustration-induced $ symmetric$ skyrmion-lattice state in the $J_1$-$J_2$ (or $J_1$-$J_3$) triangular-lattice Heisenberg model without the Dzyaloshinskii-Moriya interaction, we investigate the ordering of the classical $J_1$-$J_2$ honeycomb-lattice Heisenberg antiferromagnet under magnetic fields by means of a Monte Carlo simulation, a mean-field analysis and a low-temperature expansion. The model has been known to have an infinite ring-like degeneracy in the wavevector space in its ground state for $1/6<J_2/J_1<0.5$, in distinction with the triangular-lattice model. As reported by Okumura $et \ al$ [J. Phys. Soc. Jpn. ${\bf 79}$, 114705 (2010)], such a ring-like degeneracy gives rise to exotic spin liquid states in zero field, $e.g$, the "ring-liquid" state and the "pancake-liquid" state. In this paper, we study the in-field ordering properties of the model paying attention to the possible appearance of exotic multiple-$q$ states. Main focus is made on the $J_2/J_1=0.3$ case, where we observe a rich variety of multiple-$q$ states including the single-$q$, double-$q$ and triple-$q$ states. While the skyrmion-lattice triple-$q$ state observed in the triangular-lattice model is not realized, we instead observe an exotic double-$q$ state consisting of meron/antimeron lattice textures.

cond-mat.str-el

Effects of magnetic anisotropy on spin and thermal transports in classical antiferromagnets on the square lattice

Transport properties of the classical antiferromagnetic XXZ model on the square lattice have been theoretically investigated, putting emphasis on how the occurrence of a phase transition is reflected in spin and thermal transports. As is well known, the anisotropy of the exchange interaction $Δ\equiv J_z/J_x$ plays a role to control the universality class of the transition of the model, i.e., either a second-order transition at $T_N$ into a magnetically ordered state or the Kosterlitz-Thouless (KT) transition at $T_{KT}$, which respectively occur for the Ising-type ($Δ>1$) and $XY$-type ($Δ<1$) anisotropies, while for the isotropic Heisenberg case of $Δ=1$, a phase transition does not occur at any finite temperature. It is found by means of the hybrid Monte-Carlo and spin-dynamics simulations that the spin current probes the difference in the ordering properties, while the thermal current does not. For the $XY$-type anisotropy, the longitudinal spin-current conductivity $σ^s_{xx}$ ($=σ^s_{yy}$) exhibits a divergence at $T_{KT}$ of the exponential form, $σ^s_{xx} \propto \exp\big[ B/\sqrt{T/T_{KT}-1 }\, \big]$ with $B={\cal O}(1)$, while for the Ising-type anisotropy, the temperature dependence of $σ^s_{xx}$ is almost monotonic without showing a clear anomaly at $T_{N}$ and such a monotonic behavior is also the case in the Heisenberg-type spin system. The significant enhancement of $σ^s_{xx}$ at $T_{KT}$ is found to be due to the exponential rapid growth of the spin-current-relaxation time toward $T_{KT}$, which can be understood as a manifestation of the topological nature of a vortex whose lifetime is expected to get longer toward $T_{KT}$. Possible experimental platforms for the spin-transport phenomena associated with the KT topological transition are discussed.

cond-mat.str-el

Nature of the randomness-induced quantum spin liquids in two dimensions

The nature of the randomness-induced quantum spin liquid state, the random-singlet state, is investigated in two dimensions (2D) by means of the exact-diagonalization and the Hams-de Raedt methods for several frustrated lattices, e.g., the triangular, the kagome and the J_1-J_2 square lattices. Properties of the ground state, the low-energy excitations and the finite-temperature thermodynamic quantities are investigated. The ground state and the low-lying excited states consist of nearly isolated singlet-dimers, clusters of resonating singlet-dimers, and orphan spins. Low-energy excitations are either singlet-to-triplet excitations, diffusion of orphan spins accompanied by the recombination of nearby singlet-dimers, creation or destruction of resonating singlet-dimers clusters. The latter two excitations give enhanced dynamical `liquid-like' features to the 2D random-singlet state. Comparison is made with the random-singlet state in a 1D chain without frustration, the similarity and the difference between in 1D and in 2D being highlighted. Frustration in a wide sense, not only the geometrical one but also including the one arising from the competition between distinct types of interactions, play an essential role in stabilizing this frustrated random singlet state. Recent experimental situations on both organic and inorganic materials are reviewed and discussed.

cond-mat.str-el