arXiv subjects

Hilbert v. Löhneysen

Publications and source records attributed to Hilbert v. Löhneysen.

At least 19 recordsLinked to original sources

arXiv2020

Terahertz Conductivity of Heavy-fermion Systems from Time-resolved Spectroscopy

The Drude model describes the free-electron conduction in simple metals, governed by the freedom that the mobile electrons have within the material. In strongly correlated systems, however, a significant deviation of the optical conductivity from the simple metallic Drude behavior is observed. Here, we investigate the optical conductivity of the heavy-fermion system CeCu$_{\mathrm{6-x}}$Au$_{\mathrm{x}}$, using time-resolved, phase-sensitive terahertz spectroscopy. Terahertz electric field creates two types of excitations in heavy-fermion materials: First, the intraband excitations that leave the heavy quasiparticles intact. Second, the resonant interband transitions between the heavy and light parts of the hybridized conduction band that break the Kondo singlet. We find that the Kondo-singlet breaking interband transitions do not create a Drude peak, while the Kondo-retaining intraband excitations yield the expected Drude response; thus, making it possible to separate these two fundamentally different correlated contributions to the optical conductivity.

cond-mat.str-el↗

arXiv2018

Tuning anti-Klein to Klein tunneling in bilayer graphene

We show that in gapped bilayer graphene, quasiparticle tunneling and the corresponding Berry phase can be controlled such that it exhibits features of single layer graphene such as Klein tunneling. The Berry phase is detected by a high-quality Fabry-Pérot interferometer based on bilayer graphene. By raising the Fermi energy of the charge carriers, we find that the Berry phase can be continuously tuned from $2π$ down to $0.68π$ in gapped bilayer graphene, in contrast to the constant Berry phase of $2π$ in pristine bilayer graphene. Particularly, we observe a Berry phase of $π$, the standard value for single layer graphene. As the Berry phase decreases, the corresponding transmission probability of charge carriers at normal incidence clearly demonstrates a transition from anti-Klein tunneling to nearly perfect Klein tunneling.

cond-mat.mes-hall↗

arXiv2017

Evolution of the partially frustrated magnetic order in CePd$_{1-x}$Ni$_x$Al

We report on a single-crystal neutron diffraction study of the evolution of the antiferromagnetic order in the heavy-fermion compound CePd$_{1-x}$Ni$_x$Al which exhibits partial geometric frustration due to its distorted Kagomé structure. The magnetic structure is found to be unchanged with a propagation vector $Q_\mathrm{AF} \approx (0.5~0~0.35)$ for all Ni concentrations $x$ up to $x_c \approx 0.14$. Upon approaching the quantum critical concentration $x_c$, the ordered moment vanishes linearly with Néel temperature $T_{\rm N}$, in good agreement with CePdAl under hydrostatic pressure. For all Ni concentrations, substantial short-range magnetic correlations are observed above $T_{\rm N}$ as a result of frustration.

cond-mat.str-el↗

arXiv2017

Two-band superconductivity of bulk and surface states in Ag thin films on Nb

We use epitaxial strain to shift the energy of the two-dimensional Ag(111) surface states of Ag islands on Nb(110) substrates, allowing to spatially tune the bottom of the surface-state band $E_{\rm SS}$ through the Fermi level $E_{\rm F}$. Bulk and surface-state contributions to the Ag(111) local density of states (LDOS) can be separated with scanning tunneling spectroscopy. For thick islands ($\approx$\, 20 nm), the Ag surface states are decoupled from the Ag bulk states via orthogonality, and the superconductive gap induced by proximity to Nb is due to bulk states only. However, for thin islands (3-4 nm), surface-state electrons develop superconducting correlations as identified by a complete energy gap in the LDOS when $E_{\rm F}$ is smaller than but close to $E_{\rm F}$. The induced superconductivity in this case is of two-band nature and appears to occur when the surface-state wave function reaches down to the Ag/Nb interface.

cond-mat.supr-con↗

arXiv2016

Entropy evolution in the magnetic phases of partially frustrated CePdAl

In the heavy-fermion metal CePdAl long-range antiferromagnetic order coexists with geometric frustration of one third of the Ce moments. At low temperatures the Kondo effect tends to screen the frustrated moments. We use magnetic fields $B$ to suppress the Kondo screening and study the magnetic phase diagram and the evolution of the entropy with $B$ employing thermodynamic probes. We estimate the frustration by introducing a definition of the frustration parameter based on the enhanced entropy, a fundamental feature of frustrated systems. In the field range where the Kondo screening is suppressed the liberated moments tend to maximize the magnetic entropy and strongly enhance the frustration. Based on our experiments, this field range may be a promising candidate to search for a quantum spin liquid.

cond-mat.str-el↗

arXiv2016

Signature of frustrated moments in quantum critical CePd$_{1-x}$Ni$_x$Al

CePdAl with Ce $4f$ moments forming a distorted kagomé network is one of the scarce materials exhibiting Kondo physics and magnetic frustration simultaneously. As a result, antiferromagnetic (AF) order setting in at $T_{\mathrm{N}} = 2.7$~K encompasses only two thirds of the Ce moments. We report measurements of the specific heat, $C$, and the magnetic Grüneisen parameter, $Γ_{\rm mag}$, on single crystals of CePd$_{1-x}$Ni$_x$Al with $x\leq 0.16$ at temperatures down to 0.05~K and magnetic fields $B$ up to $8$~T. Field-induced quantum criticality for various concentrations is observed with the critical field decreasing to zero at $x_c\approx 0.15$. Remarkably, two-dimensional (2D) AF quantum criticality of Hertz-Millis-Moriya type arises for $x=0.05$ and $x=0.1$ at the suppression of 3D magnetic order. Furthermore, $Γ_{\rm mag}(B)$ shows an additional contribution near $2.5$~T for all concentrations which is ascribed to correlations of the frustrated one third of Ce moments.

cond-mat.str-el↗

arXiv2016

Signature of f-electron conductance in $α$-Ce single-atom contacts

Cerium is a fascinating element exhibiting, with its different phases, long-range magnetic order and superconductivity in bulk form. The coupling of the 4f electron to sd conduction electrons and to the lattice is responsible for unique structural and electronic properties like the isostructural first-order solid-solid transition from the cubic $γ$ phase to the cubic $α$ phase, which is accompanied by a huge volume collapse of 14 %. While the $γ- α$ phase transition has been investigated for decades, experiments aiming at disentangling the 4f contribution to the electric conductance of the different phases have not been performed. Here we report on the strongly enhanced conductance of single-atom Ce contacts. By controlling the content of $α$-Ce employing different rates of cooling, we find a strong correlation between the fraction of $α$-Ce and the magnitude of the last conductance plateau before the contact breaks. We attribute the enhanced conductance of $α$-Ce to the additional contribution of the 4f level.

cond-mat.mtrl-sci↗

arXiv2016

Switching of a large anomalous Hall effect between metamagnetic phases of a non-collinear antiferromagnet

The anomalous Hall effect (AHE), which in long-range ordered ferromagnets appears as a voltage transverse to the current and usually is proportional to the magnetization, often is believed to be of negligible size in antiferromagnets due to their low uniform magnetization. However, recent experiments and theory have demonstrated that certain antiferromagnets with a non-collinear arrangement of magnetic moments exhibit a sizeable spontaneous AHE at zero field due to a non-vanishing Berry curvature arising from the quantum mechanical phase of the electron's wave functions. Here we show that antiferromagnetic Mn5Si3 single crystals exibit a large AHE which is strongly anisotropic and shows multiple transitions with sign changes at different magnetic fields due to field-induced rearrangements of the magnetic structure despite only tiny variations of the total magnetization. The presence of multiple non-collinear magnetic phases offers the unique possiblity to explore the details of the AHE and the sensitivity of the Hall effect on the details of the magnetic texture.

cond-mat.mtrl-sci↗

arXiv2016

CePdAl - a Kondo lattice with partial frustration

Magnetic frustration, which is well-defined in insulating systems with localized magnetic moments, yields exotic ground states like spin ices, spin glasses, or spin liquids. In metals magnetic frustration is less well defined because of the incipient delocalization of magnetic moments by the interaction with conduction electrons, viz., the Kondo effect. Hence, the Kondo effect and magnetic frustration are antithetic phenomena. Here we present experimental data of electrical resistivity, magnetization, specific heat and neutron diffraction on CePdAl, which is one of the rare examples of a geometrically frustrated Kondo lattice, demonstrating that the combination of Kondo effect and magnetic frustration leads to an unusual ground state.

cond-mat.str-el↗

arXiv2016

Fermi surface reconstruction in FeSe under high pressure

We report Shubnikov-de Haas (SdH) oscillation measurements on FeSe under high pressure up to $P$ = 16.1 kbar. We find a sudden change in SdH oscillations at the onset of the pressure-induced antiferromagnetism at $P$ $\sim$ 8 kbar. We argue that this change can be attributed to a reconstruction of the Fermi surface by the antiferromagnetic order. The negative d$T_c$/d$P$ observed in a range between $P$ $\sim$ 8 and 12 kbar may be explained by the reduction in the density of states due to the reconstruction. The ratio of the transition temperature to the effective Fermi energy remains high under high pressure: $k_BT_c/E_F$ $\sim$ 0.1 even at $P$ = 16.1 kbar.

cond-mat.supr-con↗

arXiv2015

Quantum criticality in AFe2As2 with A = K, Rb, and Cs suppresses superconductivity

Superconductors close to quantum phase transitions often exhibit a simultaneous increase of electronic correlations and superconducting transition temperatures. Typical examples are given by the recently discovered iron-based superconductors. We investigated the band-specific quasiparticle masses of AFe2As2 single crystals with A = K, Rb, and Cs and determined their pressure dependence. The evolution of electronic correlations could be tracked as a function of volume and hole doping. The results indicate that with increasing alkali-metal ion radius a quantum critical point is approached. The critical fluctuations responsible for the enhancement of the quasiparticle masses appear to suppress the superconductivity.

cond-mat.supr-con↗

arXiv2015

Pressure-induced antiferromagnetic transition and phase diagram in FeSe

We report measurements of resistance and ac magnetic susceptibility on FeSe single crystals under high pressure up to 27.2 kbar. The structural phase transition is quickly suppressed with pressure, and the associated anomaly is not seen above $\sim$18 kbar. The superconducting transition temperature evolves nonmonotonically with pressure, showing a minimum at $\sim12$ kbar. We find another anomaly at 21.2 K at 11.6 kbar. This anomaly most likely corresponds to the antiferromagnetic phase transition found in $μ$SR measurements [M. Bendele \textit{et al.}, Phys. Rev. Lett. \textbf{104}, 087003 (2010)]. The antiferromagnetic and superconducting transition temperatures both increase with pressure up to $\sim25$ kbar and then level off. The width of the superconducting transition anomalously broadens in the pressure range where the antiferromagnetism coexists.

cond-mat.supr-con↗

arXiv2014

Anomalous Fermi surface in FeSe seen by Shubnikov-de Haas oscillation measurements

We have observed Shubnikov-de Haas oscillations in FeSe. The Fermi surface deviates significantly from predictions of band-structure calculations and most likely consists of one electron and one hole thin cylinder. The carrier density is in the order of 0.01 carriers/ Fe, an order-of-magnitude smaller than predicted. Effective Fermi energies as small as 3.6 meV are estimated. These findings call for elaborate theoretical investigations incorporating both electronic correlations and orbital ordering.

cond-mat.supr-con↗

arXiv2014

Magnetotransport in ferromagnetic Mn5Ge3, Mn5Ge3C0.8, and Mn5Si3C0.8 thin films

The electrical resistivity, anisotropic magnetoresistance (AMR), and anomalous Hall effect of ferromagnetic Mn5Ge3, Mn5Ge3C0.8, and Mn5Si3C0.8 thin films has been investigated. The data show a behavior characteristic for a ferromagnetic metal, with a linear increase of the anomalous Hall coefficient with Curie temperature. While for ferromagnetic Mn5Si3C0.8 the normal Hall coefficient R0 and the AMR ratio are independent of temperature, these parameters strongly increase with temperature for the germanide films. This difference is attributed to the different hybridization of electronic states in the materials due different lattice parameters and different atomic configurations (Ge vs. Si metalloid). The concomitant sign change of R0 and the AMR ratio with temperature observed for the germanide films is discussed in a two-current model indicating an electron-like minority-spin transport at low temperatures.

cond-mat.mes-hall↗

arXiv2013

Anomalous Microwave Surface Resistance of CeCu6

We present surface resistance measurements of the archetypical heavy-fermion compound CeCu6 for frequencies between 3.7 and 18 GHz and temperatures from 1.2 to 6 K. The measurements were performed with superconducting stripline resonators that allow simultaneous measurements at multiple frequencies. The surface resistance of CeCu6 exhibits a pronounced decrease below 3 K, in consistence with dc resistivity. The low-temperature frequency dependence of the surface resistance follows a power law with exponent 2/3. While for conventional metals this would be consistent with the anomalous skin effect, we discuss the present situation of a heavy-fermion metal, where this frequency dependence might instead stem from the influence of electronic correlations.

cond-mat.str-el↗

arXiv2013

Two-dimensional simulations of temperature and current-density distribution in electromigrated structures

We report on the application of a feedback-controlled electromigration technique for the formation of nanometer-sized gaps in mesoscopic gold wires and rings. The effect of current density and temperature, linked via Joule heating, on the resulting gap size is investigated. Experimentally, a good thermal coupling to the substrate turned out to be crucial to reach electrode spacings below 10 nm and to avoid overall melting of the nanostructures. This finding is supported by numerical calculations of the current-density and temperature profiles for structure layouts subjected to electromigration. The numerical method can be used for optimizing the layout so as to predetermine the location where electromigation leads to the formation of a gap.

cond-mat.mes-hall↗

arXiv2011

Controlled fabrication of single-walled carbon nanotube electrodes by electron-beam-induced oxidation

The fabrication of metallic single-walled carbon nanotube electrodes separated by gaps of typically 20nm width by electron-beam-induced oxidation is studied within an active device configuration. The tube conductance is measured continuously during the process. The experiment provides a statistical evaluation of gap sizes as well as the electron dose needed for gap formation. Also, the ability to precisely cut many carbon nanotubes in parallel is demonstrated.

cond-mat.mes-hall↗

arXiv2010

Pressure versus concentration tuning of the superconductivity in Ba(Fe(1-x)Cox)2As2

In the iron arsenide compound BaFe2As2, superconductivity can be induced either by a variation of its chemical composition, e.g., by replacing Fe with Co, or by a reduction of the unit-cell volume through the application of hydrostatic pressure p. In contrast to chemical substitutions, pressure is expected to introduce no additional disorder into the lattice. We compare the two routes to superconductivity by measuring the p dependence of the superconducting transition temperature Tc of Ba(Fe(1-x)Cox)2As2 single crystals with different Co content x. We find that Tc(p) of underdoped and overdoped samples increases and decreases, respectively, tracking quantitatively the Tc(x) dependence. To clarify to which extent the superconductivity relies on distinct structural features we analyze the crystal structure as a function of x and compare the results with that of BaFe2As2 under pressure.

cond-mat.supr-con↗