arXiv subjects

Hiroaki Shishido

Publications and source records attributed to Hiroaki Shishido.

At least 19 recordsLinked to original sources

arXiv2026

Emergence of Chiral Helimagnetic Order in Chromium-intercalated Tantalum Disulfide CrTa$_3$S$_6$ Powders with Controlled Intercalation

We report a highly sensitive change in magnetic properties of a chiral Cr-intercalated transition-metal dichalcogenide Cr$_{x}$Ta$_{3}$S$_{6}$. Magnetization curves and small-angle neutron scattering data revealed that the powder samples exhibit chiral helimagnetism with a Cr intercalation quantity $x$ below 0.996, while they show ferromagnetism above 1.000. The emergence and temperature-dependent evolution of the helimagnetic period are argued in terms of sample dimensions of powders and microfabricated crystals.

cond-mat.mtrl-sci↗

arXiv2025

Experimental Studies on Spatial Resolution of a Delay-Line Current-Biased Kinetic-Inductance Detector

A current-biased kinetic inductance detector (CB-KID) is a novel superconducting detector to construct a neutron transmission imaging system. The characteristics of a superconducting neutron detector have been systematically studied to improve spatial resolution of our CB-KID neutron detector. In this study, we investigated the distribution of spatial resolutions under different operating conditions and examined the homogeneity of spatial resolutions in the detector in detail. We used a commercial standard Gd Siemens-star pattern as a conventional method to estimate the spatial resolution, and a lab-made 10B-dot array intended to examine detailed profiles on a distribution of spatial resolutions. We found that discrepancy in propagation velocities in the detector affected the uniformity of the spatial resolutions in neutron imaging. We analyzed the ellipsoidal line profiles along the circumferences of several different test circles in the Siemens-star image to find a distribution of spatial resolutions. Note that we succeeded in controlling the detector temperature precisely enough to realize stable propagation velocities of the signals in the detector to achieve the best spatial resolution with a delay-line CB-KID technique.

physics.ins-det↗

arXiv2024

Superconductivity in Ternary Germanite TaAl$_{x}$Ge$_{2-x}$ with a C40 chiral structure

We report a new family of chiral intermetallic superconductors TaAl$_{x}$Ge$_{2-x}$. The mother compound TaGe$_2$ has a C40-type chiral hexagonal crystal structure with a pair of enantiomorphic space groups of $P6{_2}22$ and $P6{_4}22$. By substituting Ge with Al, TaAl$_{x}$Ge$_{2-x}$ polycrystals with the C40 structure were synthesized with Al substitution $x$ from 0 to 0.8. Magnetic susceptibility, magnetization curves and electrical resistivity revealed that TaAl$_{x}$Ge$_{2-x}$ with $x$ of 0.2 to 0.4 was a type-II superconductor with a superconducting transition temperature $T_{\rm c}$ of 2.0 to 2.2 K. The superconductivity disappeared or was largely suppressed at $x$ less than 0.2 and more than 0.4, although all the measurements were performed at temperatures above 1.8 K. An emergence of superconductivity is discussed in terms of the lattice constants changes with the Al substitution.

cond-mat.supr-con↗

arXiv2024

Chirality-Induced Selectivity of Phonon Angular Momenta in Chiral Quartz Crystals

A generation, propagation, and transfer of phonon angular momenta are examined on thermal transport in chiral insulative and diamagnetic crystals of $α$-quartz. We found that thermally-driven phonons carry chirality-dependent angular momenta in the quartz crystals and they could be extracted from the quartz as a spin signal. Namely, chirality-induced selectivity of phonon angular momenta is realized in the chiral quartz. We argue that chiral phonons available in chiral materials could be a key element in triggering or enhancing chirality-induced spin selectivity with robust spin polarization and long-range spin transport found in various chiral materials.

cond-mat.mtrl-sci↗

arXiv2023

Orientation mapping of YbSn$_3$ single crystals based on Bragg-dip analysis using a delay-line superconducting sensor

Recent progress in high-power pulsed neutron sources has stimulated the development of the Bragg-dip and Bragg-edge analysis methods using a two-dimensional neutron detector with high temporal resolution to resolve the neutron energy by the time-of-flight method. The delay-line current-biased kinetic-inductance detector (CB-KID) is a two-dimensional superconducting sensor with a high temporal resolution and multi-hit capability. We demonstrate that the delay-line CB-KID with a $^{10}$B neutron conversion layer can be applied to high-spatial-resolution neutron transmission imaging and spectroscopy up to 100\,eV. Dip structures in the transmission spectrum induced by Bragg diffraction and nuclear resonance absorption in YbSn$_3$ single crystals. We successfully drew the orientation mapping of YbSn$_3$ crystals based on the analysis of observed Bragg-dip positions in the transmission spectrum.

physics.app-ph↗

arXiv2023

Spin polarization gate device based on the chirality-induced spin selectivity and robust nonlocal spin polarization

Nonlocal spin polarization phenomena are thoroughly investigated in the devices made of chiral metallic single crystals of CrNb$_3$S$_6$ and NbSi$_2$ as well as of polycrystalline NbSi$_2$. We demonstrate that simultaneous injection of charge currents in the opposite ends of the device with the nonlocal setup induces the switching behavior of spin polarization in a controllable manner. Such a nonlocal spin polarization appears regardless of the difference in the materials and device dimensions, implying that the current injection in the nonlocal configuration splits spin-dependent chemical potentials throughout the chiral crystal even though the current is injected into only a part of the crystal. We show that the proposed model of the spin dependent chemical potentials explains the experimental data successfully. The nonlocal double-injection device may offer significant potential to control the spin polarization to large areas because of the nature of long-range nonlocal spin polarization in chiral materials.

cond-mat.mtrl-sci↗

arXiv2022

Chirality-selected crystal growth and spin polarization over centimeters of transition metal disilicide crystals

We performed a chirality-controlled crystal growth of transition metal disilicide NbSi$_{2}$ and TaSi$_{2}$ by using a laser-diode-heated floating zone (LDFZ) method. The crystal chirality was evaluated in the crystals of centimeters in length by performing single crystal X-ray diffraction as well as probing a spin polarization originating from chirality-induced spin selectivity (CISS) effect. The crystals of right-handed NbSi$_{2}$ and of left-handed TaSi$_{2}$ were obtained in the conventional LDFZ crystal growth, while the left-handed NbSi$_{2}$ and right-handed TaSi$_{2}$ crystals were grown by the LDFZ method with the composition-gradient feed rods. The spin polarization via the CISS was observed over centimeters in the NbSi$_{2}$ single crystals and the sign of the CISS signals was dependent on the chirality of crystals. The correlation between the crystal chirality and CISS signals indicates that the CISS measurements work as a non-destructive method for chirality determination even in centimeter-long specimens.

cond-mat.mtrl-sci↗

arXiv2021

Detection of chirality-induced spin polarization over millimeters in polycrystalline bulk samples of chiral disilicides NbSi$_2$ and TaSi$_2$

We report that spin polarization occurs over millimeters in polycrystalline bulk samples of chiral disilicide NbSi$_2$ and TaSi$_2$. As previously demonstrated in the experiments using single crystals of NbSi$_2$ and TaSi$_2$, electrical transport measurements allow detection of direct and inverse signals associated with the chirality-induced spin polarization even in the chiral polycrystals. The spin polarization signals also appear in nonlocal measurements, in which charge current flows only in the area millimeters away from the detection electrode. These data mean that the spin polarization phenomena occur regardless of the presence of crystalline grains in the polycrystals, indicating a robustness and resilience of the chirality-induced spin polarization. On the basis of the experimental data, we found that the sum rule holds for the spin transport signals. A distribution of handedness over the samples was determined on average in the polycrystals. While the mechanism of preserving the spin polarization over millimeters remains to be clarified, the present study may open up prospects of spin control and manipulation over macroscopic length scales using chiral materials.

cond-mat.mtrl-sci↗

arXiv2021

High Spatial Resolution Neutron Transmission Imaging Using a Superconducting Two-Dimensional Detector

Neutron imaging is one of the most powerful tools for nondestructive inspection owing to the unique characteristics of neutron beams, such as high permeability for many heavy metals, high sensitivity for certain light elements, and isotope selectivity owing to a specific nuclear reaction between an isotope and neutrons. In this study, we employed a superconducting detector, current-biased kinetic-inductance detector (CB-KID) for neutron imaging using a pulsed neutron source. We employed the delay-line method, and high spatial resolution imaging with only four reading channels was achieved. We also performed wavelength-resolved neutron imaging by the time-of-flight method for the pulsed neutron source. We obtained the neutron transmission images of a Gd-Al alloy sample, inside which single crystals of GdAl3 were grown, using the delay-line CB-KID. Single crystals were well imaged, in both shapes and distributions, throughout the Al-Gd alloy. We identified Gd nuclei via neutron transmissions that exhibited characteristic suppression above the neutron wavelength of 0.03 nm. In addition, the ^{155}Gd resonance dip, a dip structure of the transmission caused by the nuclear reaction between an isotope and neutrons, was observed even when the number of events was summed over a limited area of 15 X 12 um^2. Gd selective imaging was performed using the resonance dip of ^{155}Gd, and it showed clear Gd distribution even with a limited neutron wavelength range of 1 pm.

physics.app-ph↗

arXiv2021

Practical tests of neutron transmission imaging with a superconducting kinetic-inductance sensor

Samples were examined using a superconducting (Nb) neutron imaging system employing a delay-line technique which in previous studies was shown to have high spatial resolution. We found excellent correspondence between neutron transmission and scanning electron microscope (SEM) images of Gd islands with sizes between 15 and 130 micrometer which were thermally-sprayed onto a Si substrate. Neutron transmission images could be used to identify tiny voids in a thermally-sprayed continuous Gd2O3 film on a Si substrate which could not be seen in SEM images. We also found that neutron transmission images revealed pattern formations, mosaic features and co-existing dendritic phases in Wood's metal samples with constituent elements Bi, Pb, Sn and Cd. These results demonstrate the merits of the current-biased kinetic inductance detector (CB-KID) system for practical studies in materials science. Moreover, we found that operating the detector at a more optimal temperature (7.9 K) appreciably improved the effective detection efficiency when compared to previous studies conducted at 4 K. This is because the effective size of hot-spots in the superconducting meanderline planes increases with temperature, which makes particle detections more likely.

cond-mat.supr-con↗

arXiv2021

Thin Film Growth of Heavy Fermion Chiral Magnet YbNi3Al9

We grew thin films of a heavy fermion chiral magnet YbNi$_3$Al$_9$ by using molecular beam epitaxy. They were grown on $c$-plane sapphire substrates under ultra-high vacuum while maintaining a deposition rate at a stoichiometric ratio among Yb, Ni, and Al. The resulting thin films contain epitaxial grains with a $c$ axis parallel to the substrate surface: The YbNi$_3$Al$_9$ $c$ axis is parallel to the sapphire $b$ or $a$ axis. The temperature dependence of the resistivity exhibits a typical feature of a dense Kondo system with a broad shoulder structure at $\sim$40\,K, as well as a kink as a signature of the chiral helimagnetic ordering at 3.6\,K. These features are consistent with those previously observed in bulk samples. The shift in the kink associated with the field-induced phase transition is found in the magnetoresistance curves under a magnetic field applied in the direction perpendicular to the $c$-axis. The magnetic phase diagram well reproduces that for the bulk crystals, implying that the chiral soliton lattice phase arises under magnetic fields, even in thin films.

cond-mat.str-el↗

arXiv2020

Homogeneity of neutron transmission imaging over a large sensitive area with a four-channel superconducting detector

We previously proposed a method to detect neutrons by using a current-biased kinetic inductance detector (CB-KID), where neutrons are converted into charged particles using a 10B conversion layer. The charged particles are detected based on local changes in kinetic inductance of X and Y superconducting meanderlines under a modest DC bias current. The system uses a delay-line method to locate the positions of neutron-10B reactions by acquiring the four arrival timestamps of signals that propagate from hot spots created by a passing charged particle to the end electrodes of the meanderlines. Unlike conventional multi-pixel imaging systems, the CB-KID system performs high spatial resolution imaging over a 15 mm x 15 mm sensitive area using only four channel readouts. Given the large sensitive area, it is important to check the spatial homogeneity and linearity of detected neutron positions when imaging with CB-KID. To this end we imaged a pattern of 10B dot absorbers with a precise dot pitch to investigate the spatial homogeneity of the detector. We confirmed the spatial homogeneity of detected dot positions based on the distribution of measured dot pitches across the sensitive area of the detector. We demonstrate potential applications of the system by taking a clear transmission image of tiny metallic screws and nuts and a ladybug. The image was useful for characterizing the ladybug noninvasively. Detection efficiencies were low when the detector was operated at 4 K, so we plan to explore raising the operating temperature towards the critical temperature of the detector as a means to improve counting rates.

physics.ins-det↗

arXiv2019

Energy-resolved neutron imaging with high spatial resolution using a superconducting delay-line kinetic inductance detector

Neutron imaging is one of the key technologies for non-destructive transmission testing. Recent progress in the development of intensive neutron sources allows us to perform energy-resolved neutron imaging with high spatial resolution. Substantial efforts have been devoted to developing a high spatial and temporal resolution neutron imager. We have been developing a neutron imager aiming at conducting high spatial and temporal resolution imaging based on a delay-line neutron detector, called the current-biased kinetic-inductance detector, with a conversion layer $^{10}$B. The detector allowed us to obtain a neutron transmission image with four signal readout lines. Herein, we expanded the sensor active area, and improved the spatial resolution of the detector. We examined the capability of high spatial resolution neutron imaging over the sensor active area of 15 $\times$ 15 mm$^2$ for various samples, including biological and metal ones. We also demonstrated an energy-resolved neutron image in which stainless-steel specimens were discriminating of other specimens with the aid of the Bragg edge transmission.

physics.app-ph↗

arXiv2019

Search for the field-induced magnetic instability around the upper critical field of superconductivity in H || c in CeCoIn5

We present nuclear spin-lattice relaxation rate (1/T1) at the Co site and ac-susceptibility results in the normal and superconducting (SC) states of CeCoIn5 for H || c near the SC upper critical field Hc2 above 0.1 K. At 4.2 T, 1/T1 rapidly decreases below the SC transition temperature, consistent with the previous reports. Although the field dependence of 1/T1T at 0.1 K shows a peak at 5.2 T above Hc2, the temperature dependence of 1/T1T at 5.2 T is independent of temperature below 0.2 K, showing a Fermi-liquid behavior. In addition, we found no NMR-spectrum broadening by the appearance of internal fields around Hc2 at 0.1 K. We could not detect any field-induced magnetic instability around Hc2 down to 0.1 K although the remarkable non-Fermi-liquid behavior towards Hc2 was observed in various physical quantities.

cond-mat.str-el↗

arXiv2018

Anomalous change in the de Haas-van Alphen oscillations of CeCoIn$_5$ at ultra-low temperatures

We have performed de Haas-van Alphen (dHvA) measurements of the heavy-fermion superconductor CeCoIn$_5$ down to 2 mK above the upper critical field. We find that the dHvA amplitudes show an anomalous suppression, concomitantly with a shift of the dHvA frequency, below the transition temperature $T_{\rm n}=20$ mK. We suggest that the change is owing to magnetic breakdown caused by a field-induced antiferromagnetic (AFM) state emerging below $T_{\rm n}$, revealing the origin of the field-induced quantum critical point (QCP) in CeCoIn$_5$. The field dependence of $T_{\rm n}$ is found to be very weak for 7--10 T, implying that an enhancement of AFM order by suppressing the critical spin fluctuations near the AFM QCP competes with the field suppression effect on the AFM phase. We suggest that the appearance of a field-induced AFM phase is a generic feature of unconventional superconductors, which emerge near an AFM QCP, including CeCoIn$_5$, CeRhIn$_5$, and high-$T_{\rm c}$ cuprates.

cond-mat.str-el↗

arXiv2017

Magnetic and superconducting properties of the heavy-fermion CeCoIn5 epitaxial film probed by nuclear quadrupole resonance

Since the progress in the fabrication techniques of thin-films of exotic materials such as strongly correlated heavy-fermion compounds, microscopic studies of the magnetic and electronic properties inside the films have been needed. Herein, we report the first observation of 115In nuclear quadrupole resonance (NQR) in an epitaxial film of the heavy-fermion superconductor CeCoIn5, for which the microscopic field gradient within the unit cell as well as magnetic and superconducting properties at zero field are evaluated. We find that the nuclear spin-lattice relaxation rate in the film is in excellent agreement with that of bulk crystals, whereas the NQR spectra show noticeable shifts and significant broadening indicating a change in the electric-field distribution inside the film. The analysis implies a displacement of In layers in the film, which however does not affect the magnetic fluctuations and superconducting pairing. This implies that inhomogeneity of the electronic field gradient in the film sample causes no pair breaking effect.

cond-mat.supr-con↗

arXiv2015

The interface between heavy fermions and normal electrons investigated by spatially-resolved nuclear magnetic resonance

We have studied the superlattices with alternating block layers (BLs) of heavy-fermion superconductor CeCoIn5 and conventional-metal YbCoIn5 by site-selective nuclear magnetic resonance(NMR) spectroscopy, which uniquely offers spatially-resolved dynamical magnetic information. We find that the presence of antiferromagnetic fluctuations is confined to the Ce-BLs, indicating that magnetic degrees of freedom of f-electrons are quenched inside the Yb-BLs. Contrary to simple expectations that the two-dimensionalization enhances fluctuations, we observe that antiferromagnetic fluctuations are rapidly suppressed with decreasing Ce-BL thickness. Moreover, the suppression is more prominent near the interfaces between the BLs. These results imply significant effects of local inversion-symmetry breaking at the interfaces.

cond-mat.str-el↗

arXiv2013

Terahertz Conductivity of the Heavy-Fermion State in CeCoIn5

The optical properties of thin films of the heavy-fermion compound CeCoIn5, which were deposited by molecular beam epitaxy onto MgF2 substrates, have been studied at frequencies 7 to 45 cm^{-1} (corresponding to 0.2 to 1.3 THz) and temperatures 2 to 300 K. We observe an electrodynamic behavior which is typical for heavy fermions, namely Drude-like conductivity with a relaxation rate at rather low frequencies. This relaxation rate increases almost linearly with temperature up to at least 30 K. The coherent heavy-fermion state, characterized by an increase of the effective mass, continuously evolves upon cooling and is not fully developed for temperatures as low as 5 K.

cond-mat.str-el↗