arXiv subjects

Hiroshi Okamoto

Publications and source records attributed to Hiroshi Okamoto.

At least 19 recordsLinked to original sources

arXiv2026

High-harmonic generation during ultrafast melting of a Mott insulating state

Solids in an intense laser field show high-harmonic generation (HHG), which can provide information on carrier dynamics and band structures in weakly correlated systems. In strongly correlated systems, a laser field can induce a transition between the various electronic phases formed by the entanglement of charge, spin, and orbital degrees of freedom via carrier generation. The HHG accompanying this process can reflect information on the nonequilibrium electronic-state dynamics along the oscillating field-an aspect that remains unresolved to date. Here, we show that an intense mid-infrared (MIR) pulse induces melting of a Mott-insulator state in a one-dimensional cuprate, Sr2CuO3, the evolution of which leaves a trace in the HH spectra. When the electric-field amplitude exceeds 6 MV/cm, carriers are efficiently generated and each harmonic frequency decreases from odd multiples of the MIR frequency. Dynamical mean-field theory (DMFT) presents a possibility that these redshifts originate from a series of electronic-structure reconstructions in each electric-field cycle during the melting of the Mott-insulator state, which modifies the radiation phase from carrier recombination cycle-by-cycle. This phenomenon is negligible in rigid-band systems. This experimental-theoretical study suggests that HH spectroscopy has the potential to obtain information on the cycle-by-cycle dynamics of nonequilibrium transitions in correlated materials.

cond-mat.str-el↗

arXiv2026

Low-dose Image Recognition with Quantum Computational Electron Microscopy

We show that quantum computational imaging is advantageous in the setting of low-dose electron microscopy of beam-sensitive specimens. Two qudits placed near the electron beam enable full transfer of quantum information between the electron microscope and a quantum computer in the proposed scheme, providing the specimen is a phase object. We present a quantum algorithm that identifies the correct image among n candidate images, where n is larger than the effective dimension of the Hilbert space of the imaging electron.

quant-ph↗

arXiv2025

Piezoelectric Transition in a Nonpyroelectric Gyroidal Metal-Organic Framework

Among the thirty-two crystallographic point groups, 432 is the only one that lacks an inversion center but does not exhibit piezoelectricity. A gyroidal structure belongs to point group 432 and shows characteristic physical properties attributed to its distinctive strong isotropic network. Here, we investigate a gyroidal cobalt oxalate metal-organic framework (MOF) with disordered orientations of SO4 tetrahedra. Synchrotron X-ray diffraction experiments using a single crystal reveal a cubic-to-cubic structural phase transition at TS = 120 K. This transition involves a change in the point group from nonpiezoelectric 432 to piezoelectric 23. The symmetry change arises from the ordering of distorted SO4 molecules, leading to a three-dimensional helical arrangement of electric dipole moments. Furthermore, pyroelectric current measurements using polycrystalline pellet samples reveal that electric polarization emerges below TS depending on the magnitude of the pelletizing pressure, demonstrating piezoelectricity. The gyroidal MOF offers an opportunity to explore unique dielectric properties induced by the helical ordering of molecules and structural flexibility.

cond-mat.mtrl-sci↗

arXiv2024

Walk model that continuously generates Brownian walks to Lévy walks depending on destination attractiveness

The Lévy walk, a type of random walk characterized by linear step lengths that follow a power-law distribution, is observed in the migratory behaviors of various organisms, ranging from bacteria to humans. Notably, Lévy walks with power exponents close to two, also known as Cauchy walks, are frequently observed, though their underlying causes remain elusive. This study proposes a walk model in which agents move toward a destination in multi-dimensional space and their movement strategy is parameterized by the extent to which they pursue the shortest path to the destination. This parameter is taken to represent the attractiveness of the destination to the agents. Our findings reveal that if the destination is very attractive, agents intensively search the area around it using Brownian walks, whereas if the destination is unattractive, they explore a distant region away from the point using Lévy walks with power exponents less than two. In the case where agents are unable to determine whether the destination is attractive or unattractive, Cauchy walks emerge. The Cauchy walker searches the region with a probability inversely proportional to the distance from the destination. This suggests that it preferentially searches the area close to the destination, while concurrently having the potential to extend the search area much further. Our model, which can change the search method and search area depending on the attractiveness of the destination, has the potential to be utilized for exploring the parameter space of optimization problems.

cs.MA↗

arXiv2023

Universal Quantum Electron Microscopy: A Small-Scale Quantum Computing Application with Provable Advantage

We propose a simple design of a quantum electron microscope that ``queries'' a beam-sensitive phase object, such as a biological specimen, as part of quantum computation. Lower quantum query complexity, not the time complexity, of a quantum algorithm means less specimen damage, which translates to more data extracted from the specimen. Hence small-scale quantum computing offers provable quantum advantage in this context. A possible application of the proposed microscope is the Grover search for a true structure, out of a set of candidate structures.

quant-ph↗

arXiv2023

Melting of excitonic insulator phase by an intense terahertz pulse in Ta$_2$NiSe$_5$

In this study, the optical response to a terahertz pulse was investigated in the transition metal chalcogenide Ta$_2$NiSe$_5$, a candidate excitonic insulator. First, by irradiating a terahertz pulse with a relatively weak electric field (0.3 MV/cm), the spectral changes in reflectivity near the absorption edge due to third-order optical nonlinearity were measured and the absorption peak characteristic of the excitonic phase just below the interband transition was identified. Next, by irradiating a strong terahertz pulse with a strong electric field of 1.65 MV/cm, the absorption of the excitonic phase was found to be reduced, and a Drude-like response appeared in the mid-infrared region. These responses can be interpreted as carrier generation by exciton dissociation induced by the electric field, resulting in the partial melting of the excitonic phase and metallization. The presence of a distinct threshold electric field for carrier generation indicates exciton dissociation via quantum-tunnelling processes. The spectral change due to metallization by the electric field is significantly different from that due to the strong optical excitation across the gap, which can be explained by the different melting mechanisms of the excitonic phase in the two types of excitations.

cond-mat.str-el↗

arXiv2023

Testing the Power-Law Hypothesis of the Inter-Conflict Interval

The severity of war, measured by battle deaths, follows a power-law distribution. Here, we demonstrate that power law also holds in the temporal aspects of interstate conflicts. A critical quantity is the inter-conflict interval (ICI), the interval between the end of a conflict in a dyad and the start of the subsequent conflict in the same dyad. Using elaborate statistical tests, we confirmed that the ICI samples compiled from the history of interstate conflicts from 1816 to 2014 followed a power-law distribution. We propose an information-theoretic model to account for the power-law properties of ICIs. The model predicts that a series of ICIs in each dyad is independently generated from an identical power-law distribution. This was confirmed by statistical examination of the autocorrelation of the ICI series. Our findings help us understand the nature of wars between normal states, the significance of which has increased since the Russian invasion of Ukraine in 2022.

physics.soc-ph↗

arXiv2023

Inverse square Levy walk emerging universally in goal-oriented tasks

The Levy walk in which the frequency of occurrence of step lengths follows a power-law distribution, can be observed in the migratory behavior of organisms at various levels. Levy walks with power exponents close to 2 are observed, and the reasons are unclear. This study aims to propose a model that universally generates inverse square Levy walks (called Cauchy walks) and to identify the conditions under which Cauchy walks appear. We demonstrate that Cauchy walks emerge universally in goal-oriented tasks. We use the term "goal-oriented" when the goal is clear, but this can be achieved in different ways, which cannot be uniquely determined. We performed a simulation in which an agent observed the data generated from a probability distribution in a two-dimensional space and successively estimated the central coordinates of that probability distribution. The agent has a model of probability distribution as a hypothesis for data-generating distribution and can modify the model such that each time a data point is observed, thereby increasing the estimated probability of occurrence of the observed data. To achieve this, the center coordinates of the model must be moved closer to those of the observed data. However, in the case of a two-dimensional space, arbitrariness arises in the direction of correction of the center; this task is goal oriented. We analyze two cases: a strategy that allocates the amount of modification randomly in the x- and y-directions, and a strategy that determines allocation such that movement is minimized. The results reveal that when a random strategy is used, the Cauchy walk appears. When the minimum strategy is used, the Brownian walk appears. The presence or absence of the constraint of minimizing the amount of movement may be a factor that causes the difference between Brownian and Levy walks.

cond-mat.stat-mech↗

arXiv2022

TEM at Millikelvin Temperatures: Observing and Utilizing Superconducting Qubits

We present a case for developing a millikelvin-temperature transmission electron microscope (TEM). We start by reviewing known reasons for such development, then present new possibilities that have been opened up by recent progress in superconducting quantum circuitry, and finally report on our ongoing experimental effort. Specifically, we first review possibilities to observe a quantum mechanically superposed electromagnetic field around a superconducting qubit. This is followed by a new idea on TEM observation of microwave photons in an unusual quantum state in a resonator. We then proceed to review potential applications of these phenomena, which include low dose electron microscopy beyond the standard quantum limit. Finally, anticipated engineering challenges, as well as the authors' current ongoing experimental effort towards building a millikelvin TEM are described. In addition, we provide a brief introduction to superconducting circuitry in the Appendix for the interested reader who is not familiar with the subject.

quant-ph↗

arXiv2022

Resilient quantum electron microscopy

We investigate the fundamental limit of biological quantum electron microscopy, which is designed to go beyond the shot noise limit. Inelastic scattering is expected to be the main obstacle in this setting, especially for thick specimens of actual biological interest. Here we describe a measurement procedure that, in principle, significantly neutralizes the effect of inelastic scattering.

quant-ph↗

arXiv2020

Lévy walks derived from a Bayesian decision-making model in non-stationary environments

Lévy walks are found in the migratory behaviour patterns of various organisms, and the reason for this phenomenon has been much discussed. We use simulations to demonstrate that learning causes the changes in confidence level during decision-making in non-stationary environments, and results in Lévy-walk-like patterns. One inference algorithm involving confidence is Bayesian inference. We propose an algorithm that introduces the effects of learning and forgetting into Bayesian inference, and simulate an imitation game in which two decision-making agents incorporating the algorithm estimate each other's internal models from their opponent's observational data. For forgetting without learning, agent confidence levels remained low due to a lack of information on the counterpart and Brownian walks occurred for a wide range of forgetting rates. Conversely, when learning was introduced, high confidence levels occasionally occurred even at high forgetting rates, and Brownian walks universally became Lévy walks through a mixture of high- and low-confidence states.

cs.AI↗

arXiv2019

Modular decomposition of Markov chain: detecting hierarchical organization of pervasive communities

In network science, a group of nodes connected with each other at higher probability than with those outside the group is referred to as a community. From the perspective that individual communities are associated with functional modules constituting complex systems described by networks, discovering communities is primarily important for understanding overall functions of these systems. Much effort has been devoted to developing methods to detect communities in networks since the early days of network science. Nevertheless, the method to reveal key characteristics of communities in real-world network remains to be established. Here we formulate decomposition of a random walk spreading over the entire network into local modules as proxy for communities. This formulation will reveal the pervasive structure of communities and their hierarchical organization, which are the hallmarks of real-world networks but are out of reach of most existing methods.

physics.soc-ph↗

arXiv2019

A charge model as an effective model of one-dimensional Hubbard and extended Hubbard systems: its application to linear optical spectrum calculations in large systems based upon many-body Wannier functions

We propose an effective model called the "charge model", for the half-filled one-dimensional Hubbard and extended Hubbard models. In this model, spin-charge separation, which has been justified from an infinite on-site repulsion ($U$) in the strict sense, is compatible with charge fluctuations. Our analyses based on the many-body Wannier functions succeeded in determining the optical conductivity spectra in large systems. The obtained spectra reproduce the spectra for the original models well even in the intermediate $U$ region of $U=5-10T$, with $T$ being the nearest-neighbor electron hopping energy. These results indicate that the spin-charge separation works fairly well in this intermediate $U$ region against the usual expectation and that the charge model is an effective model that applies to actual quasi-one-dimensional materials classified as strongly correlated electron systems.

cond-mat.str-el↗

arXiv2018

Strong terahertz radiation via rapid polarization reduction in photoinduced ionic-to-neutral transition of tetrathiafulvalene-p-chloranil

Terahertz lights are usually generated through the optical rectification process within a femtosecond laser pulse in non-centrosymmetric materials. Here, we report a new generation mechanism of terahertz lights based upon a photoinduced phase transition (PIPT), in which an electronic structure is rapidly changed by a photoirradiation. When a ferroelectric organic molecular compound, tetrathiafulvalene-p-chloranil, is excited by a femtosecond laser pulse, the ionic-to-neutral transition is driven and simultaneously a strong terahertz radiation is produced. By analyzing the terahertz electric-field waveforms and their dependence on the polarization direction of the incident laser pulse, we demonstrate that the terahertz radiation originates from the ultrafast decrease of the spontaneous polarization in the photoinduced ionic-to-neutral transition. The efficiency of the observed terahertz radiation via the PIPT mechanism is found to be much higher than that via the optical rectification in the same material and in a typical terahertz emitter, ZnTe.

cond-mat.mtrl-sci↗

arXiv2018

A full-vortex flux qubit for charged particle optics

We introduce a design of a superconducting flux qubit capable of holding a full magnetic flux quantum $ϕ_{0}$, which arguably is an essential property for applications in charged particle optics. The qubit comprises a row of $N$ constituent qubits, which hold a fractional magnetic flux quantum $ϕ_{0}/N$. Insights from physics of the transverse-field Ising chain reveal that properly designed interaction between these constituent qubits enables their collective behavior while also maintaining the overall quantumness.

quant-ph↗

arXiv2018

Terahertz radiation by subpicosecond spin-polarized photocurrent originating from Dirac electrons in a Rashba-type polar semiconductor

The spin-splitting energy bands induced by the relativistic spin-orbit interaction in solids provide a new opportunity to manipulate the spin-polarized electrons on the sub-picosecond time scale. Here, we report one such example in a bulk Rashba-type polar semiconductor BiTeBr. Strong terahertz electromagnetic waves are emitted after the resonant excitation of the interband transition between the Rashba-type spin-splitting energy bands with a femtosecond laser pulse circularly polarized. The phase of the emitted terahertz waves is reversed by switching the circular polarization. This suggests that the observed terahertz radiation originates from the subpicosecond spin-polarized photocurrents, which are generated by the asymmetric depopulation of the Dirac state. Our result provides a new way for the current-induced terahertz radiation and its phase control by the circular polarization of incident light without external electric fields.

cond-mat.str-el↗

arXiv2018

Separation of Charge Instability and Lattice Symmetry Breaking in an Organic Ferroelectric

We investigate the charge and lattice states in a quasi-one-dimensional organic ferroelectric material, TTF-QCl$_{4}$, under pressures of up to 35 kbar by nuclear quadrupole resonance experiments. The results reveal a global pressure-temperature phase diagram, which spans the electronic and ionic regimes of ferroelectric transitions, which have so far been studied separately, in a single material. The revealed phase diagram clearly shows that the charge-transfer instability and the lattice symmetry breaking, which coincide in the electronic ferroelectric regime at low pressures, bifurcate at a certain pressure, leading to the conventional ferroelectric regime. The present results reveal that the crossover from electronic to ionic ferroelectricity occurs through the separation of charge and lattice instabilities.

cond-mat.mtrl-sci↗

arXiv2017

Biological implications of possible unattainability of comprehensive, molecular-resolution, real-time, volume imaging of the living cell

Despite the impressive advances in biological imaging, no imaging modality today generates, in a comprehensive manner, high-resolution images of crowded molecules working deep inside the living cell in real time. In this paper, instead of tackling this engineering problem in the hope of solving it, we ask a converse question: What if such imaging is \emph{fundamentally} impossible? We argue that certain decoherence processes could be suppressed because the internal workings of the cell are not being closely "observed" in the quantum mechanical sense, as implied by the assumed impossibility of imaging. It is certainly true that the "wet and warm" living cell should not exhibit quantum behavior merely because of the lack of observation. Despite this, we plow ahead to see what \emph{might} result from such absence of the outward flow of information. We suggest that chaotic dynamics in the cell could be quantum mechanically suppressed --- a known phenomenon in quantum chaology, which is potentially resistant to various mechanisms for the emergence of classicality. We also consider places where experimental evidence for/against such a possibility may be sought.

physics.bio-ph↗