arXiv subjects

Hiroshi Okamoto

Publications and source records attributed to Hiroshi Okamoto.

25 records · Page 2Linked to original sources

arXiv2015

A quantum mechanical scheme to reduce radiation damage in electron microscopy

We show that radiation damage to unstained biological specimens is not an intractable problem in electron microscopy. When a structural hypothesis of a specimen is available, quantum mechanical principles allow us to verify the hypothesis with a very low electron dose. Realization of such a concept requires precise control of the electron wave front. Based on a diffractive electron optical implementation, we demonstrate the feasibility of this new method by both experimental and numerical investigations.

quant-ph↗

arXiv2015

A quantum interface to charged particles in a vacuum

A superconducting qubit device suitable for interacting with a flying electron has recently been proposed [H. Okamoto and Y. Nagatani, Appl. Phys. Lett. \textbf{104}, 062604 (2014)]. Either a clockwise or counter clockwise directed loop of half magnetic flux quantum encodes a qubit, which naturally interacts with any single charged particle with arbitrary kinetic energy. Here, the device's properties, sources of errors and possible applications are studied in detail. In particular, applications include detection of a charged particle without applying a force to it. Furthermore, quantum states can be transferred between an array of the proposed devices and the charged particle.

quant-ph↗

arXiv2014

Measurement errors in entanglement-assisted electron microscopy

The major resolution-limiting factor in cryoelectron microscopy of unstained biological specimens is radiation damage by the very electrons that are used to probe the specimen structure. To address this problem, an electron microscopy scheme that employs quantum entanglement to enable phase measurement precision beyond the standard quantum limit has recently been proposed {[}Phys. Rev. A \textbf{85}, 043810{]}. Here we identify and examine in detail measurement errors that will arise in the scheme. An emphasis is given to considerations concerning inelastic scattering events because in general schemes assisted with quantum entanglement are known to be highly vulnerable to lossy processes. We find that the amount of error due both to elastic and inelastic scattering processes are acceptable provided that the electron beam geometry is properly designed.

quant-ph↗

arXiv2013

Entanglement-assisted electron microscopy based on a flux qubit

A notorious problem in high-resolution biological electron microscopy is radiation damage to the specimen caused by probe electrons. Hence, acquisition of data with minimal number of electrons is of critical importance. Quantum approaches may represent the only way to improve the resolution in this context, but all proposed schemes to date demand delicate control of the electron beam in highly unconventional electron optics. Here we propose a scheme that involves a flux qubit based on a radio-frequency superconducting quantum interference device (rf-SQUID), inserted in essentially a conventional transmission electron microscope. The scheme significantly improves the prospect of realizing a quantum-enhanced electron microscope for radiation-sensitive specimens.

quant-ph↗

arXiv2011

Possible use of a Cooper-pair box for low-dose electron microscopy

A transmission electron microscope that takes advantage of superconducting quantum circuitry is proposed. The microscope is designed to improve image contrast of radiation-sensitive weak phase objects, in particular biological specimens. The objective in this setting is to measure the phase shift of the probe electron wave to a precision $Δθ$ within the number of electrons $N$ that does not destroy the specimen. In conventional electron microscopy $Δθ$ scales as $\sim 1/N^{1/2}$, which falls short of the Heisenberg limit $\sim 1/N$. To approach the latter by using quantum entanglement, we propose a design that involves a Cooper pair box placed on the surface of an electrostatic electron mirror in the microscope. Significant improvement could be attained if inelastic scattering processes are sufficiently delocalized.

quant-ph↗

arXiv2007

Ultrafast Photoinduced Formation of Metallic State in a Perovskite-type Manganite with Short Range Charge and Orbital Order

Femtosecond reflection spectroscopy was performed on a perovskite-type manganite, Gd0.55Sr0.45MnO3, with the short-range charge and orbital order (CO/OO). Immediately after the photoirradiation, a large increase of the reflectivity was detected in the mid-infrared region. The optical conductivity spectrum under photoirradiation obtained from the Kramers-Kronig analyses of the reflectivity changes demonstrates a formation of a metallic state. This suggests that ferromagnetic spin arrangements occur within the time resolution (ca. 200 fs) through the double exchange interaction, resulting in an ultrafast CO/OO to FM switching.

cond-mat.str-el↗

arXiv2002

Angle-resolved photoemission study of MX-chain compound [Ni(chxn)$_2$Br]Br$_2$

We report on the results of angle-resolved photoemission experiments on a quasi-one-dimensional $MX$-chain compound [Ni(chxn)$_2$Br]Br$_2$ (chxn = 1$R$,2$R$-cyclohexanediamine), a one-dimensional Heisenberg system with $S=1/2$ and $J \sim 3600$ K, which shows a gigantic non-linear optical effect. A "band" having about 500 meV energy dispersion is found in the first half of the Brillouin zone $(0\le kb/π<1/2)$, but disappears at $kb / π\sim 1/2$. Two dispersive features, expected from the spin-charge separation, as have been observed in other quasi-one-dimensional systems like Sr$_2$CuO$_3$, are not detected. These characteristic features are well reproduced by the $d$-$p$ chain model calculations with a small charge-transfer energy $Δ$ compared with that of one-dimensional Cu-O based compounds. We propose that this smaller $Δ$ is the origin of the absence of clear spin- and charge-separation in the photoemission spectra and strong non-linear optical effect in [Ni(chxn)$_2$Br]Br$_2$.

cond-mat.str-el↗